David Borlaug, Robert Rice, Bahram Jalali
We report evidence of beam cleanup during stimulated Raman scattering in silicon. An amplified near-diffraction-limited Stokes beam is obtained from a severely aberrated pump beam.
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We experimentally study the competition between Kerr beam self-cleaning and Raman beam cleanup in a multimode air-silica microstructure optical fiber. Kerr beam self-cleaning of the pump is observed for a certain range of input powers only. Raman Stokes beam generation and cleanup lead to both depletion and degradation of beam quality for the pump. The interplay of modal four-wave mixing and Raman scattering in the infrared domain lead to the generation of a multimode supercontinuum ranging from 500 nm up to 1800 nm.
We report on the generation of a Raman cascade spanning the wavelength range of 523 to 1750 nm wavelength range, in a standard telecommunication graded-index multimode optical fiber. Despite the highly multimode nature of the pump, the Raman peaks are generated in specific modes of the fiber, confirming substantial beam cleanup during the stimulated Raman scattering process.
Continuous-wave Raman amplification in silicon waveguides with negative electrical power dissipation is reported. It is shown that a p-n junction can simultaneously achieve carrier sweep-out leading to net continuous-wave gain, and electrical power generation. The approach is also applicable to silicon Raman lasers and other third-order nonlinear optical devices.
We demonstrate for the first time a mid infrared silicon Raman amplifier. Amplification of 12 dB is reported for a signal at 3.39 micron wavelength. The active medium was a 2.5 cm long silicon sample that was pumped with 5ns pulses at 2.88 micron. The absence of the nonlinear losses which severely limit the performance of silicon Raman devices in the near infrared combined with unsurpassed crystal quality, high thermal conductivity render silicon a very attractive Raman medium. Such a technology can potentially extend silicon photonics application beyond data communication in the near infrared…
We present the design and anticipated performance of an optically pumped monolithic all-silicon mid-IR (MIR) Raman laser. For the proposed 3.15 um cw laser design pumped at a 2.71 um pump wavelength, we estimate a threshold pump power of < 10 mW and an estimated output laser linewidth of <50 MHz. This design may pave the road toward demonstration of the first mid-IR silicon Raman laser.
We demonstrate the first low-noise mid-IR frequency comb source using a silicon microresonator. Our observation of strong Raman scattering lines in the generated comb suggests that Raman and four-wave mixing interactions play a role in assisting the transition to the low-noise state. In addition, we characterize, the intracavity comb generation dynamics using an integrated PIN diode, which takes advantage of the inherent three-photon absorption process in silicon.
Stimulated Raman scattering is a well-known nonlinear process that can be harnessed to produce optical gain in a wide variety of media. This effect has been used to produce the first silicon-based lasers and high-gain amplifiers. Interestingly, the Raman effect can also produce intensity-dependent nonlinear loss through a corollary process known as inverse Raman scattering (IRS). Here, we demonstrate IRS in silicon--a process that is substantially modified by the presence of optically-generated free carriers--achieving attenuation levels >15 dB with a pump intensity of 4 GW/cm^2. Ironically, w…
We experimentally show that the self-phase modulation of picosecond pump pulses, induced by both the optical Kerr effect and free-carrier refraction, has a detrimental effect on the maximum on-off Raman gain achievable in silicon on insulator nanowaveguides, causing it to saturate. A simple calculation of the Raman gain coefficient from the measured broadened output pump spectra perfectly matches the saturated behavior of the amplified Raman signal observed experimentally at different input pump powers.
Enhancement of optical response with high-index dielectric nanoparticles is attributed to the excitation of their Mie-type magnetic and electric resonances. Here we study Raman scattering from crystalline silicon nanoparticles and reveal that magnetic dipole modes have much stronger effect on the scattering than electric modes of the same order. We demonstrate experimentally a 140-fold enhancement of Raman signal from individual silicon spherical nanoparticles at the magnetic dipole resonance. Our results confirm the importance of the optically-induced magnetic response of subwavelength dielec…
We report the observations of spontaneous Raman scattering in silicon photonic crystal waveguides. Continuous-wave measurements of Stokes emission for both wavelength and power dependence is reported in single line-defect waveguides in hexagonal lattice photonic crystal silicon membranes. By utilizing the Bragg gap edge dispersion of the TM-like mode for pump enhancement and the TE-like fundamental mode-onset for Stokes enhancement, the Stokes emission was observed to increase by up to five times in the region of slow group velocity. The results show explicit nonlinear enhancement in a silicon…
We demonstrate the dynamics of stimulated Raman scattering in designed high-Q/Vm silicon photonic band gap nanocavities through the coupled-mode theory framework towards optically-pumped silicon lasing. The interplay of other chi(3) effects such as two-photon absorption and optical Kerr, related free-carrier dynamics, thermal effects, as well as linear losses such as cavity radiation and linear material absorption are included and investigated numerically. Our results clarify the relative contributions and evolution of the mechanisms, and demonstrate the lasing and shutdown thresholds. Our stu…
Stokes microcombs in silicon nitride microresonators
本文首次在正常色散氮化硅微环谐振腔中观测到斯托克斯微梳，揭示了克尔与拉曼非线性相互作用机制，实现了两种梳态的可控切换，并通过数值模型验证了拉曼诱导 platicon 形成，为新型光子器件奠定基础。
Silicon Nitride Microresonator Raman Lasers
研究利用氮化硅微谐振器实现高效拉曼激光，通过优化光学模式与硅氧化物包层重叠，抑制非线性竞争效应，实现低阈值激光输出，并展示宽频调谐能力。
The realization of ultrahigh quality (Q) resonators regardless of the underpinning material platforms has been a ceaseless pursuit, because the high Q resonators provide an extreme environment of storage of light to enable observations of many unconventional nonlinear optical phenomenon with high efficiencies. Here, we demonstrate an ultra-high Q factor (7.1*10^6) microresonator on the 4H-silicon-carbide-on-insulator (4H-SiCOI) platform in which both \c{hi}^(2) and \c{hi}^(3) nonlinear processes of high efficiencies have been generated. Broadband frequency conversions, including second-, third…
We propose a new type of waveguide optical amplifier. The device consists of collinearly propagating pump and amplified Stokes beams with periodic imaging of the Stokes beam due to the Talbot effect. The application of this device as an Image preamplifier for Mid Wave Infrared (MWIR) remote sensing is discussed and its performance is described. Silicon is the preferred material for this application in MWIR due to its excellent transmission properties, high thermal conductivity, high damage threshold and the mature fabrication technology. In these devices, the Raman amplification process also i…
As the silicon industry continues to push the limits of device dimensions, tools such as Raman spectroscopy are ideal to analyze and characterize the doped silicon channels. The effect of inter-valence band transitions on the zone center optical phonon in heavily p-type doped silicon is studied by Raman spectroscopy for a wide range of excitation wavelengths extending from the red (632.8 nm) into the ultra-violet (325 nm). The asymmetry in the one-phonon Raman lineshape is attributed to a Fano interference involving the overlap of a continuum of electronic excitations with a discrete phonon st…
We numerically study the mechanisms of frequency comb generation in the mid-infrared spectral region from cw pumped silicon microring resonators. Coherent soliton comb generation may be obtained even for a pump with zero linear cavity detuning, through suitable control of the effective lifetime of free-carriers from multiphoton absorption, which introduces a nonlinear cavity detuning via free-carrier dispersion. Conditions for optimal octave spanning Raman comb generation are also described.
Electronic Raman scattering in silicon glass
针对硅玻璃中无序诱导的光发射现象，本文提出其机制为电子拉曼散射，而非声子辅助间接跃迁，并揭示禁带内 Urbach 桥态与纳米限域光子动量匹配的关键作用。
Resonantly enhanced Raman scattering in dielectric nanostructures has been recently proven to be an effcient tool for developing nanothermometry and experimental determination of their mode- composition. In this paper, we develop a rigorous analytical theory based on the Green's function approach to calculate the Raman emission from crystalline high-index dielectric nanoparticles. As an example, we consider silicon nanoparticles which have a strong Raman response due to active optical phonon modes. We relate enhancement of Raman signal emission to Purcell effect due to the excitation of Mie mo…
We show that fluctuations of Raman amplified pulses, in the presence of a noisy pump, follow extreme value statistics, and provide mathematical insight into the origin of this perplexing behavior.
We investigate for the first time the enhancement of the stimulated Raman scattering in slow-light Silicon-on-Insulator (SOI) photonic crystal line defect waveguides. By applying the Bloch-Floquet formalism to the guided modes in a planar photonic crystal, we develop a formalism that relates the intensity of the down-shifted Stokes signal to the pump intensity and the modal group velocities. The formalism is then applied to two prospective schemes for enhanced stimulated Raman generation in slow-light photonic crystal waveguides. The results demonstrate a maximum factor of 10^4 (66,000) enhanc…
Hybrid Nonlinear Effects in Photonic Integrated Circuits
本研究利用两种材料的混合光学非线性，在熔融石英包层氮化硅微谐振腔中实现了拉曼散射与Kerr频率梳的联合产生，为集成光子器件的多功能化与高效非线性电路提供了新途径。
Precise measurement of the refractive index of stable silicon isotopes $^{28}$Si, $^{29}$Si, $^{30}$Si single crystals with enrichments above 99.9 at.% and a silicon single crystal $^{nat}$Si of natural isotopic composition is performed with the Fourier-transform interference refractometry method from 1.06 to more than 80 mkm with 0.1 cm$^{-1}$ resolution and accuracy of $2 \times 10^{-5} ... 1 \times 10^{-4}$. The oxygen and carbon concentrations in all crystals are within $5 \times 10^{15}$ cm$^{-3}$ and the content of metal impurities is $10^{-5} ... 10^{-6}$ at.%. The peculiar changes of t…
L-shape probability distributions are extremely non-Gaussian distributions that have been surprisingly successful in describing the frequency of occurrence of extreme events, ranging from stock market crashes and natural disasters, the structure of biological systems, fractals, and optical rogue waves. In this paper, we show that fluctuations in stimulated Raman scattering in silicon, as well as in coherent anti-Stokes Raman scattering, can follow extreme value statistics and provide mathematical insight into the origin of this behavior. As an example of the experimental observations, we find …
Surface-enhanced coherent anti-Stokes Raman scattering (SE-CARS) takes advantage of surface plasmon resonances supported on metallic nanostructures to amplify the coherent Raman response of target molecules. While these metallic antennas have found significant success in SE-CARS studies, photo-induced morphological changes to the nanoantenna under ultrafast excitation introduce significant hurdles in terms of stability and reproducilibty. These hurdles need to be overcome in order to establish SE-CARS as a reliable tool for rapid biomolecular sensing. Here we address this challenge by performi…
Efficient Raman lasing and Raman-Kerr interaction in an integrated silicon carbide platform
本文在集成碳化硅平台首次实现效率超50%的拉曼激光，通过调谐微腔使斯托克斯共振对准增益谱，阈值低至2.5 mW，并展示拉曼-克尔相互作用拓宽微梳光谱。
Coherent electronic Raman excitation of valley-orbit split states of phosphorus dopants in silicon
本研究通过相干光学激发实现了硅中磷受体谷-轨道分裂态的电子拉曼跃迁，并揭示了载流子密度对波包特性的影响及非共振激发条件下的跃迁机制。
We demonstrated fabrication of black silicon with slanted nanocone array on both planar and 3D micro and meso scale structures produced by a high-throughput lithography-free oblique-angle plasma etching process. Nanocones with gradual change in height were created on the same piece of silicon. The relation between the slanted angle of nanocones and incident angle of directional plasma is experimentally investigated. In order to demonstrate the monolithic integration of nanostructures on micro and meso scale non-planar surfaces, nanocone forest is fabricated on non-planar silicon surfaces in va…
Stimulated Raman Scattering in Nonlinear Silicon Nanophotonic Waveguides: Theory and Applications in Photonic Integrated Circuits
本文综述受激拉曼散射的基本理论、在硅基光子集成电路中的应用与增强途径，并梳理近十年关键实验演示，以克服硅间接能带导致的高效光源难题。
Deep UV Silicon Polaritonic Metasurfaces for Enhancing Biomolecule Autofluorescence and Two-Dimensional Material Double-Resonance Raman Scattering
本文提出一种基于极化激元共振的稳健硅超表面，通过Kerker型空腔设计实现二维半导体双共振拉曼散射分析和生物分子自发荧光增强，为深紫外光谱学和纳米材料研究提供稳定可扩展的平台。
Revealing hidden non-radiative (dark) of resonant nanostructures using optical methods such as dark-field spectroscopy often becomes a sophisticated problem due to a weak coupling of these modes with a far-field radiation, whereas methods of dark-modes spectroscopy, e.g. cathodoluminescence or elastic energy losses, are not always convenient in use. Here, we suggest an approach for experimental determining the mode structure of a nanoresonator basing on utilizing intrinsic incoherent Raman scattering. We theoretically predict the efficiency of this approach and realize it experimentally for si…
The laser cooling of vibrational states of solids has been achieved through photoluminescence in rare-earth elements, optical forces in optomechanics, and the Brillouin scattering light-sound interaction. The net cooling of solids through spontaneous Raman scattering, and laser refrigeration of indirect band gap semiconductors, both remain unsolved challenges. Here, we analytically show that photonic density of states (DoS) engineering can address the two fundamental requirements for achieving spontaneous Raman cooling: suppressing the dominance of Stokes (heating) transitions, and the enhance…
We demonstrate cavity-enhanced Raman emission from a single atomic defect in a solid. Our platform is a single silicon-vacancy center in diamond coupled with a monolithic diamond photonic crystal cavity. The cavity enables an unprecedented frequency tuning range of the Raman emission (100 GHz) that significantly exceeds the spectral inhomogeneity of silicon-vacancy centers in diamond nanostructures. We also show that the cavity selectively suppresses the phonon-induced spontaneous emission that degrades the efficiency of Raman photon generation. Our results pave the way towards photon-mediated…
Hybrid Dielectric-Graphene SERS Metasurfaces for Antibody Sensing
本文提出一种介电硅超表面与功能化石墨烯结合的混合SERS平台，利用Mie共振和PBASE功能化实现催乳素及SARS-CoV-2抗体的低功率无标记选择性检测，并通过拉曼应变与掺杂分析验证分子区分能力。
The temperature dependence of the asymmetry between Stokes and anti-Stokes Raman scattering can be exploited for self-calibrating, optically-based thermometry. In the context of cavity optomechanics, we observe the cavity-enhanced scattering of light interacting with the standing-wave drumhead modes of a silicon nitride membrane mechanical resonator. The ratio of the amplitude of Stokes to anti-Stokes scattered light is used to measure temperatures of optically-cooled mechanical modes down to the level of a few vibrational quanta. We demonstrate that the Raman-ratio technique is able to measur…
Control of light emission of quantum emitters coupled to silicon nanoantenna using cylindrical vector beams
本文研究利用圆柱矢量光束的偏振和形状，结合硅纳米环天线，在空间上同时控制Eu3+离子的电偶极和磁偶极发射，并通过实验与数值模拟验证了激发近场和发射LDOS的协同调控作用。
Disordered optical media are an emerging class of materials capable of strongly scattering light. Their study is relevant to investigate transport phenomena and for applications in imaging, sensing and energy storage. While such materials can be used to generate coherent light, their directional emission is typically hampered by their very multiple scattering nature. Here, we tune the out-of-plane directionality of coherent Raman light scattered by a fractal network of silicon nanowires. By visualizing Rayleigh scattering, photoluminescence and weakly localized Raman light from the random netw…
Although ultrafast laser materials processing has advanced at a breakneck pace over the last two decades, most applications have been developed with laser pulses at near-IR or visible wavelengths. Recent progress in mid-infrared (MIR) femtosecond laser source development may create novel capabilities for material processing. This is because, at high intensities required for such processing, wavelength tuning to longer wavelengths opens the pathway to a special regime of laser-solid interactions. Under these conditions, due to the $λ^2$ scaling, the ponderomotive energy of laser-driven electron…
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