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arXiv 1001.2804cond-mat.supr-concond-mat.mtrl-sci
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CaFe2As2单晶的顺磁自旋关联

Paramagnetic Spin Correlations in CaFe2As2 Single Crystals

S. O. Diallo, D. K. Pratt, R. M. Fernandes, W. Tian, J. L. Zarestky, M. Lumsden, T. G. Perring, C. L. Broholm, N. Ni, S. L. Bud'ko, P. C. Canfield, H. -F. Li, D… 展开作者

S. O. Diallo, D. K. Pratt, R. M. Fernandes, W. Tian, J. L. Zarestky, M. Lumsden, T. G. Perring, C. L. Broholm, N. Ni, S. L. Bud'ko, P. C. Canfield, H. -F. Li, D. Vaknin, A. Kreyssig, A. I. Goldman, R. J. McQueeney

摘要:

用中子非弹性散射方法研究了CaFe_2As_2(T_N=172 K)顺磁相在180 K(~ 1.05 T_N)至300 K(~1.8 T_N)的磁关联。尽管磁有序的一阶性质,但强,但短程反铁磁(AFM)的相关性清楚地观察到。这些相关性,其中包括准弹性散射集中在波矢量Q_{AFM}的低温AFM结构,观察到的最高测量温度为300 K和高能量转移(E> 60毫电子伏)。散射的L依赖性意味着相当弱的层间耦合在tetravec方向对应于近二维波动(ab)平面。铁层内的自旋相关长度被发现是各向异性的,与底层的AFM条纹结构的波动一致。类似的钴掺杂的超导BaFe 2As 2化合物,这些实验功能可以充分再现的散射模型,描述了短程各向异性自旋相关与过阻尼自旋动力学。

英文摘要:

Magnetic correlations in the paramagnetic phase of CaFe2As2 (T_N=172 K) have been examined by means of inelastic neutron scattering from 180 K (~ 1.05 T_N) up to 300 K (~1.8 T_N). Despite the first-order nature of the magnetic ordering, strong but short-range antiferromagnetic (AFM) correlations are clearly observed. These correlations, which consist of quasi-elastic scattering centered at the wavevector Q_{AFM} of the low-temperature AFM structure, are observed up to the highest measured temperature of 300 K and at high energy transfer (E> 60 meV). The L dependence of the scattering implies rather weak interlayer coupling in the tetragonal c-direction corresponding to nearly two-dimensional fluctuations in the (ab) plane. The spin correlation lengths within the Fe layer are found to be anisotropic, consistent with underlying fluctuations of the AFM stripe structure. Similar to the cobalt doped superconducting BaFe2As2 compounds, these experimental features can be adequately reproduced by a scattering model that describes short-range anisotropic spin correlations with overdamped spin dynamics.

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