Ramandeep S. Johal
A pair of two-level systems initially prepared in different thermal states and coupled to an external reversible work source, do not in general reach a common temperature at the end of a unitary work extraction process. We define an effective temperature for the final nonequilibrium but passive state of the bipartite quantum system and analyse its properties.
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We consider quantum heat engines that operate between nonequilibrium stationary reservoirs. We evaluate their maximum efficiency from the positivity of the entropy production and show that it can be expressed in terms of an effective temperature that depends on the nature of the reservoirs. We further compute the efficiency at maximum power for different kinds of engineered reservoirs and derive a nonequilibrium generalization of the Clausius statement of the second law.
Using information entropy formalism, we consider a one-dimensional system with heat flux and extend the meaning of equilibrium variables to non equilibrium scenarios when classical local equilibrium approach is not applicable; this is particularly important for the performance evaluation of modern thermal systems and microdevices, which usually operate in extreme situations. The extended non equilibrium entropy, temperature, thermal conductivity and heat capacity have been analyzed as functions of the local energy density (kinetic temperature) and heat flux.
In a generalized framework for the Landauer erasure protocol, we study bounds on the heat dissipated in typical nonequilibrium quantum processes. In contrast to thermodynamic processes, quantum fluctuations are not suppressed in the nonequilibrium regime and cannot be ignored, making such processes difficult to understand and treat. Here we derive an emergent fluctuation relation that virtually guarantees the average heat produced to be dissipated into the reservoir either when the system or reservoir is large (or both) or when the temperature is high. The implication of our result is that for…
The thermodynamic properties of quantum heat engines are stochastic owing to the presence of thermal and quantum fluctuations. We here experimentally investigate the efficiency and nonequilibrium entropy production statistics of a spin-1/2 quantum Otto cycle. We first study the correlations between work and heat within a cycle by extracting their joint distribution for different driving times. We show that near perfect anticorrelation, corresponding to the tight-coupling condition, can be achieved. In this limit, the reconstructed efficiency distribution is peaked at the macroscopic efficiency…
Quantum many-body systems out of equilibrium can host intriguing phenomena such as transitions to exotic dynamical states. Although this emergent behaviour can be observed in experiments, its potential for technological applications is largely unexplored. Here, we investigate the impact of collective effects on quantum engines that extract mechanical work from a many-body system. Using an opto-mechanical cavity setup with an interacting atomic gas as a working fluid, we demonstrate theoretically that such engines produce work under periodic driving. The stationary cycle of the working fluid fe…
We show that finite system-reservoir coupling imposes a distinct quantum limit on the performance of a non-equilibrium quantum heat engine. Even in the absence of quantum friction along the isentropic strokes, finite system-reservoir coupling induces correlations that result in the generation of coherence between the energy eigenstates of the working system. This coherence acts to hamper the engine's power output, as well as the efficiency with which it can convert heat into useful work, and cannot be captured by a standard Born-Markov analysis of the system-reservoir interactions.
We investigate the heat transport in a nonequilibrium spin-boson model, where a two level system bridging two harmonic reservoirs at different temperatures, by employing a unitary transformation along with a resolvent operator expansion technique. Analytical expressions of the heat current and the thermal conductance of this model are obtained. Compared with the performances of other methods, namely, the nonequilibrium Green's function method and the equation of motion formulation, our approach provides a reasonable description of heat transfer properties of the nonequilibrium spin-boson model…
We propose a machine learning approach based on artificial neural network to gain faster insights on the role of geometric contributions to the nonequilibrium fluctuations of an adiabatically temperature-driven quantum heat engine coupled to a cavity. Using the artificial neural network we have explored the interplay between bunched and antibunched photon exchange statistics for different engine parameters. We report that beyond a pivotal cavity temperature, the Fano factor oscillates between giant and low values as a function of phase difference between the driving protocols. We further obser…
We analyze the efficiency of thermal engines (either quantum or classical) working with a single heat reservoir like atmosphere. The engine first gets an energy intake, which can be done in arbitrary non-equilibrium way e.g. combustion of fuel. Then the engine performs the work and returns to the initial state. We distinguish two general classes of engines where the working body first equilibrates within itself and then performs the work (ergodic engine) or when it performs the work before equilibrating (non-ergodic engine). We show that in both cases the second law of thermodynamics limits th…
We take the perspective of open quantum systems and examine from their nonequilibrium dynamics the conditions when the physical quantities, their relations and the laws of thermodynamics become well defined and viable for quantum many body systems. We first describe how an open system nonequilibrium dynamics (ONEq) approach is different from the closed combined system + environment in a global thermal state (CGTs) setup. Only after the open system equilibrates will it be amenable to conventional thermodynamics descriptions, thus quantum thermodynamics (QTD) comes at the end rather than assumed…
Thermal rectification and heat amplification are investigated in a nonequilibrium V-type three-level system with quantum interference. By applying the Redfield master equation combined with full counting statistics, we analyze the steady state heat transport. The noise-induced interference is found to be able to rectify the heat current, which paves a new way to design quantum thermal rectifier. Within the three-reservoir setup, the heat amplification is clearly identified far-from equilibrium, which is in absence of the negative differential thermal conductance.
We investigate full counting statistics of quantum heat transfer in a collective-qubit system, constructed by multi-qubits interacting with two thermal baths. The nonequilibrium polaron-transformed Redfield approach embedded with an auxiliary counting field is applied to obtain the steady state heat current and fluctuations, which enables us to study the impact of the qubit-bath interaction in a wide regime. The heat current, current noise and skewness are all found to clearly unify the limiting results in the weak and strong couplings, respectively. Moreover, the superradiant heat transfer is…
We study the quantum geometric heat flux in the nonequilibrium spin-boson model. By adopting the noninteracting-blip approximation that is able to accommodate the strong system-bath coupling, we show that there exists a nonzero geometric heat flux only when the two-level system is nondegenerate. Moreover, the pumping, no pumping, and dynamic control of geometric heat flux are discussed in detail, compared to the results with Redfield weak-coupling approximation. In particular, the geometric energy transfer induced by modulation of two system-bath couplings is identified, which is exclusive to …
We study the nonequilibrium steady state (NESS) in a quantum system in contact with two heat baths at different temperatures. We use a time-independent perturbative expansion with respect to the coupling with the two heat baths to obtain the density matrix for the NESS. In particular, we show an explicit representation of the density matrix for the reflection symmetric and weakly nonequilibrium case. We also calculate the expectation value of the energy current and show that the Kubo formula holds in this case.
Quantum heat transfer is analyzed in nonequilibrium two-qubits systems by applying the nonequilibrium polaron-transformed Redfield equation combined with full counting statistics. Steady state heat currents with weak and strong qubit-bath couplings are clearly unified. Within the two-terminal setup, the negative differential thermal conductance is unraveled with strong qubit-bath coupling and finite qubit splitting energy. The partially strong spin-boson interaction is sufficient to show the negative differential thermal conductance. Based on the three-terminal setup, that two-qubits are asymm…
We study the stochastic energetic exchanges in quantum heat engines. Due to microreversibility, these obey a fluctuation relation, called the heat engine fluctuation relation, which implies the Carnot bound: no machine can have an efficiency larger than Carnot's efficiency. The stochastic thermodynamics of a quantum heat engine (including the joint statistics of heat and work and the statistics of efficiency) is illustrated by means of an optimal two-qubit heat engine, where each qubit is coupled to a thermal bath and a two-qubit gate determines energy exchanges between the two qubits. We disc…
We investigate quantum heat transfer and thermal management in the nonequilibrium qubit-phonon hybrid system by applying the quantum master equation embedded with phononic coherent state. We obtain the steady state heat flow by tuning the arbitrary qubit-phonon coupling strength, which particularly exhibits the power-law scaling behavior and the turnover behavior in the weak and strong coupling regimes, respectively. Moreover, we analyze the negative differential thermal conductance and thermal rectification, which becomes profound with weak qubit-phonon interaction and large temperature bias.…
Counter-rotating-wave terms (CRWTs) are traditionally viewed to be crucial in open small quantum systems with strong system-bath dissipation. Here by exemplifying in a nonequilibrium qubit-phonon hybrid model, we show that CRWTs can play the significant role in quantum heat transfer even with weak system-bath dissipation. By using coherent phonon states, we obtain the quantum master equation with heat exchange rates contributed by rotating-wave-terms (RWTs) and CRWTs, respectively. We find that including only RWTs, steady state heat current and current fluctuations will be significantly suppre…
We investigate the nonequilibrium quantum heat transfer in a triangle-coupled spin-boson system within a three-terminal setup. By including the nonequilibrium noninteracting blip approximation approach combined with the full counting statistics, we analytically obtain the steady state populations and heat currents. The negative differential thermal conductance and giant heat amplification factor are clearly observed at strong qubit-bath coupling. %and the heat amplification is dramatically suppressed in the moderate coupling regime. Moreover, the strong interaction between the gating qubit and…
Thermodynamics of one and two-qubit nonequilibrium heat engines running between squeezed thermal reservoirs
本研究针对与压缩热库作用的单、双量子比特有限时间Otto热机展开热力学分析，探究压缩度与量子相干性的相互作用，发现双量子比特热机功率更高，且可通过调节压缩参数切换热机/制冷模式。
To study the full counting statistics of quantum heat transfer in a driven nonequilibrium spin-boson model, we develop a generalized nonequilibrium polaron-transformed Redfield equation with an auxiliary counting field. This enables us to study the impact of qubit-bath coupling ranging from weak to strong regimes. Without external modulations, we observe maximal values of both steady state heat flux and noise power at moderate coupling regimes, below which we find those two transport quantities are enhanced by the finite qubit energy bias. With external modulations, the geometric-phase-induced…
Temperature-heat uncertainty relation in nonequilibrium quantum thermometry
本文提出非平衡量子测温中的温度-热量不确定关系，将热量分解为轨迹热量和关联热量，证明二者均是提升温度估计精度的资源，并建立信息论与热力学的联系。
Quantum thermal transport and two-photon statistics serve as two representative nonequilibrium features in circuit quantum electrodynamics systems. Here, we investigate quantum heat flow and two-photon correlation function at steady-state in a composite qubit-resonator model, where one qubit shows both transverse and longitudinal couplings to a single-mode optical resonator. With weak qubit-resonator interaction, we unravel two microscopic transport pictures, i.e., cotunneling and cyclic heat exchange processes, corresponding to transverse and longitudinal couplings respectively. At strong qub…
Nonequilibrium thermodynamics and power generation in open quantum optomechanical systems
针对非平衡开放量子腔—原子系统难以建立量子发动机热力学解释的问题，本文提出基于持续耗散热流的能量平衡框架，并在弱、强光力学耦合极限下分析时间晶体发动机的功率、效率与亚稳态。
Results on heat current, entropy production rate and entanglement are reported for a quantum system coupled to two different temperature heat reservoirs. By applying a temperature gradient, different quantum states can be found with exactly the same amount of entanglement but different purity degrees and heat currents. Furthermore, a nonequilibrium enhancement-suppression transition behavior of the entanglement is identified.
We suggest a generalisation of the expression of the nonequilibrium density matrix obtained by Hershfield's method for the cases where both heat and charge steady state currents are present in a quantum open system. The finite-size quantum system, connected to two temperature and particle reservoirs, is driven out of equilibrium by the presence of both a temperature gradient and a chemical potential gradient between the two reservoirs. We show that the NE density matrix is given by a generalised Gibbs-like ensemble, and is in full agreement with the general results of the McLennan-Zubarev none…
In this work, we extend the recently established system-bath entanglement theorem (SBET) [J. Chem. Phys. 152, 034102 (2020)] to the nonequilibrium scenario, in which an arbitrary system couples to multiple Gaussian baths environments at different temperatures. While the existing SBET connects the entangled system-bath response functions to those of local systems, the extended theory is concerned with the nonequilibrium steady-state quantum transport current through molecular junctions. The new theory is established on the basis of the generalized Langevin equation, with a close relation to non…
Laser technology has developed and accelerated photo-induced nonequilibrium physics from both scientific and engineering viewpoints. The Floquet engineering, i.e., controlling material properties and functionalities by time-periodic drives, is a forefront of quantum physics of light-matter interaction, but limited to ideal dissipationless systems. For the Floquet engineering extended to a variety of materials, it is vital to understand the quantum states emerging in a balance of the periodic drive and energy dissipation. Here we derive the general description for nonequilibrium steady states (…
We develop an efficient machine learning protocol to predict the noise-induced coherence from the nonequilibrium fluctuations of photon exchange statistics in a quantum heat engine. The engine is a four-level quantum system coupled to a unimodal quantum cavity. The nonequilibrium fluctuations correspond to the work done during the photon exchange process between the four-level system and the cavity mode. We specifically evaluate the mean, variance, skewness, and kurtosis for a range of engine parameters using a full counting statistical approach combined with a quantum master equation techniqu…
We consider open quantum systems weakly coupled to a heat reservoir and driven by arbitrary time-dependent parameters. We derive exact microscopic expressions for the nonequilibrium entropy production and entropy production rate, valid arbitrarily far from equilibrium. By using the two-point energy measurement statistics for system and reservoir, we further obtain a quantum generalization of the integrated fluctuation theorem put forward by Seifert [PRL 95, 040602 (2005)].
We explore the quantum metrology in an optical molecular system coupled to two environments with different temperatures, using a quantum master equation beyond secular approximation. We discover that the steady-state coherence originating from and sustained by the nonequilibrium condition can enhance quantum metrology. We also study the quantitative measures of the nonequilibrium condition in terms of the curl flux, heat current and entropy production at the steady state. They are found to grow with temperature difference. However, an apparent paradox arises considering the contrary behaviors …
We observe the continuous emission of photons into a waveguide from a superconducting qubit without the application of an external drive. To explain this observation, we build a two-bath model where the qubit couples simultaneously to a cold bath (the waveguide) and a hot bath (a secondary environment). Our results show that the thermal-photon occupation of the hot bath is up to 0.14 photons, 35 times larger than the cold waveguide, leading to nonequilibrium heat transport with a power of up to 132 zW, as estimated from the qubit emission spectrum. By adding more isolation between the sample o…
We investigate the quantum thermal transistor effect in nonequilibrium three-level systems by applying the polaron transformed Redfield equation combined with full counting statistics. The steady state heat currents are obtained via this unified approach over a wide region of system-bath coupling, and can be analytically reduced to the Redfield and nonequilibrium noninteracting blip approximation results in the weak and strong coupling limits, respectively. A giant heat amplification phenomenon emerges in the strong system-bath coupling limit, where transitions mediated by the middle thermal b…
Understanding heat transfer between a quantum system and its environment is of undisputed importance if reliable quantum devices are to be constructed. Here, we investigate the heat transfer between system and bath in non-Markovian open systems in the process of adiabatic speedup. Using the quantum state diffusion equation method, the heat current, energy current, and power are calculated during free evolution and under external control of the system. While the heat current increases with increasing system-bath coupling strength and bath temperature, it can be restricted by the non-Markovian n…
Anomalous Heat Transfer in Nonequilibrium Quantum Systems
本文从量子信息视角分类了非平衡量子系统中异常热传输的机制，揭示初始相关性、系统内相互作用和温度不均匀性是导致异常热传输的资源，为开发高效量子自主热机提供指导。
Quantum heat transport in nonequilibrium anisotropic Dicke model
研究非平衡各向异性迪克模型中量子热传输特性，揭示各向异性光子-量子比特相互作用对稳态热流调控的影响，发现强耦合下热流受抑制，中等耦合下热流增强，且量子比特数量增加会放大热流特征。
Continuing our work on the nature and existence of fluctuation-dissipation relations (FDR) in linear and nonlinear open quantum systems [1-3], here we consider such relations when a linear system is in a nonequilibrium steady state (NESS). With the model of two-oscillators (considered as a short harmonic chain with the two ends) each connected to a thermal bath of different temperatures we find that when the chain is fully relaxed due to interaction with the baths, the relation that connects the noise kernel and the imaginary part of the dissipation kernel of the chain in one bath does not ass…
Nonequilibrium quantum heat transport between structured environments
本文运用运动层级方程技术分析自旋-玻色子模型中的非平衡热传输，发现耦合谐振子对在有效谱密度中引入局域间隙，导致弱耦合下热流剧烈改变且稳态电流受抑制，揭示了通过定制热环境谱性质控制纳米尺度热传输的新机制。
We investigate the particle and heat transport in quantum junctions with the geometry of star graphs. The system is in a nonequilibrium steady state, characterized by the different temperatures and chemical potentials of the heat reservoirs connected to the edges of the graph. We explore the Landauer-Buettiker state and its orbit under parity and time reversal transformations. Both particle number and total energy are conserved in these states. However the heat and chemical potential energy are in general not separately conserved, which gives origin to a basic process of energy transmutation a…
We study a quantum absorption refrigerator, in which a target qubit is cooled by two machine qubits in a nonequilibrium steady state. It is realized by a strong internal coupling in the two-qubit fridge and a vanishing tripartite interaction among the whole system. The coherence of a \emph{machine virtual qubit} is investigated as quantumness of the fridge. A necessary condition for cooling shows that the quantum coherence is beneficial to the nonequilibrium fridge, while it is detrimental as far as the maximum coefficient of performance (COP) and the COP at maximum power are concerned. Here, …
Experimental nonequilibrium memory erasure beyond Landauer's bound
本研究通过实验展示了非平衡记忆擦除超越兰道尔界限的可能性，利用非线性势场动态塑造实现了低能耗的完全记忆擦除。
The concept of thermal machines has evolved from the canonical steam engine to the recently proposed nanoscopic quantum systems as working fluids. The latter obey quantum open system dynamics and frequently operate in non-equilibrium conditions. However, the role of this dynamics in the overall performance of quantum heat engines remains an open problem. Here, we analyse and optimize the efficiency and power output of two-stage quantum heat engines fuelled by non-equilibrium steady states. In a charging first stage, the quantum working fluid consisting of a qutrit or two coupled qubits is conn…
In this paper, we show that a nonequilibrium steady state (NESS) exists at late times in open quantum systems with weak nonlinearity by following its nonequilibrium dynamics with a perturbative analysis. Here we consider an oscillator chain containing three-types of anharmonicity in the Fermi-Pasta-Ulam-Tsingou (FPUT) model: cubic $α$- and quartic $β$-type nearest-oscillator interactions and the on-site (pinned) Klein-Gordon (KG) quartic self-interaction. Assuming weak nonlinearity, we introduce a stochastic influence action approach to the problem and obtain the energy flow in different junct…
A general theory of photon-mediated energy and momentum transfer in N-body planar systems out of thermal equilibrium is introduced. It is based on the combination of the scattering theory and the fluctuational-electrodynamics approach in many-body systems. By making a Landauer-like formulation of the heat transfer problem, explicit formulas for the energy transmission coefficients between two distinct slabs as well as the self-coupling coefficients are derived and expressed in terms of the reflection and transmission coefficients of the single bodies. We also show how to calculate local equili…
We consider a quantum harmonic oscillator coupled to a general nonequilibrium environment. We show that the decoherence factor can be expressed in terms of a measurable effective temperature, defined via a generalized fluctuation-dissipation relation. We further propose a simple experimental scheme to determine the time-dependent effective temperature in a linear Paul trap with engineered reservoirs. Our formalism allows quantitative description of nonequilibrium decoherence in the presence of an arbitrary number of non-Markovian noise sources in a unified manner.
We study transport of noninteracting fermions through a periodically driven quantum point contact (QPC) connecting two tight-binding chains. Initially, each chain is prepared in its own equilibrium state, generally with a bias in chemical potentials and temperatures. We examine the heating rate (or, alternatively, energy increase per cycle) in the nonequilibrium time-periodic steady state established after initial transient dynamics. We find that the heating rate vanishes identically when the driving frequency exceeds the bandwidth of the chain. We first establish this fact for a particular ty…
Quantum thermodynamics in nonequilibrium
本文提出非平衡量子热力学框架，通过结合量子相干性理论与热力学定律，揭示了熵平衡关系及非平衡条件下热力学熵的定义，阐明了量子相干性在热力学中的核心作用。
We introduce a functional perturbative method for treating weakly nonlinear systems coupled with a quantum field bath. We demonstrate using this method to obtain the covariance matrix elements and the correlation functions of a quantum anharmonic oscillator interacting with a heat bath. We identify a fluctuation-dissipation relation based on the nonequilibrium dynamics of this nonlinear open quantum system. To establish its connection with dynamical equilibration, we further examine the energy flows between the anharmonic oscillator and the bath field. The vanishing of the net flow {is an indi…
Genuinely two-dimensional robust crosscurrents -- which flow against the natural direction of heat flux -- have been missing since the discovery of their one-dimensional counterpart. We provide a setup to realize them on a cubic three-dimensional (3D) lattice hosting a Hofstadter model coupled to two heat baths with different temperatures. We show that these currents exhibit dissipative robustness: they are stable against the presence of impurities and tilting of the gauge field in certain nonequilibrium configurations. Moreover, we find protected boundary currents with genuinely 3D robustness…
Controlling Nonequilibrium Bose-Einstein Condensation with Engineered Environments
针对非平衡玻色凝聚的逆控制问题，提出超导电路中的玻色凝聚器与基于线性规划的理论，实现目标凝聚构型及转变点的工程化。
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