We demonstrate a multi-spectral polarization sensitive mid-infrared dots-in-a-well (DWELL) photodetector utilizing surface-plasmonic resonant elements, with tailorable frequency response and polarization selectivity. The resonant responsivity of the surface-plasmon detector shows an enhancement of up to 5 times that of an unpatterned control detector. As the plasmonic resonator involves only surface patterning of the top metal contact, this method is independent of light-absorbing material and can easily be integrated with current focal plane array processing for imaging applications.
Here, we study the possibility of selective high-harmonic generation (HHG) based on the concept of charge transfer plasmons (CTP) in bridged nanoparticle assemblies. By choosing plasmonic dimer nanoantenna, as a fundamental member of nanoclusters family, and bridging the gap space between the proximal nanoparticles with an optothermally controllable substance, we selectively produced two different harmonics at different states of the functional bridge. To this end, the conductive connection between the nanoparticles is mediated with Ge2Sb2Te5 (GST), which inherently has opposite optical and el…
Selective configuration control of plasmonic nanostructures using either top-down or bottom-up approaches has remained challenging in the field of active plasmonics. We demonstrate the realization of DNA-assembled reconfigurable plasmonic metamolecules, which can respond to a wide range of pH changes in a programmable manner. This programmability allows for selective reconfiguration of different plasmonic metamolecule species coexisting in solution through simple pH tuning. This approach enables discrimination of chiral plasmonic quasi-enantiomers and arbitrary tuning of chiroptical effects wi…
The study of spin-orbit coupling (SOC) of light is crucial to explore the light-matter interactions in sub-wavelength nanostructures with broken symmetries. In noncentrosymmetric photonic crystals, the SOC results in the splitting of the otherwise degenerate energy bands. Herein, we explore the SOC in a noncentrosymmetric plasmonic crystal, both theoretically and experimentally. Cathodoluminescence (CL) spectroscopy combined with the numerically calculated photonic band structure reveals an energy band splitting that is ascribed to the broken symmetries in the noncentrosymmetric plasmonic crys…
In recent years, the hybridization of hyperbolic van der Waals heterostructures with plasmonic two-dimensional nano-materials is one of the interesting research areas at THz frequencies due to the coupled features of the hybrid structure. This article investigates the propagation of tunable surface phonon-plasmon polaritons in grounded hybrid graphene-hexagonal Boron Nitride (hBN) heterostructures. An analytical model is presented for the proposed structure, by applying the boundary conditions for the electromagnetic components in the various regions, to derive an exact dispersion relation. Th…
This article presents the design of two dual-band graphene-based absorbers for terahertz frequencies. The absorbers are composed of two-dimensional (2D)arrays of ribbons and disks printed on a ground plane backed dielectric spacer. The design is based on the excitation of a specific plasmon polariton of the graphene patterned array at each resonance band. An analytical circuit model is used to derive closed-form relations for the geometrical parameters of the absorber and graphene parameters. The graphene patterned array appears as a surface admittance made of an infinite parallel array of ser…
On-chip manipulating and controlling the temporal and spatial evolution of light is of crucial importance for information processing in future planar integrated nanophotonics. The spin and orbital angular momentum of light, which can be treated independently in classical macroscopic geometrical optics, appear to be coupled on subwavelength scales. We use spin-orbit interactions in a plasmonic achiral nano-coupler to unidirectionally excite surface plasmon polariton modes propagating in seamlessly integrated plasmonic slot waveguides. The spin-dependent flow of light in the proposed nanophotoni…
Extreme mid-infrared field enhancement and anapoles in high-index plasmonic metamaterials
School of Physics and Astronomy, University of Birmingham（伯明翰大学物理与天文学学院）；NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge（剑桥大学卡文迪许实验室纳米光子学中心）
Plasmonic metamaterials can be used to enhance mid-infrared sensors and detectors for immunosensing applications. The major challenge is to integrate these technologies in low-cost, compact, and promising platforms. In this study, as an emerging approach, we utilized toroidal resonant plasmonic metasurfaces to develop an ultrasensitive label-free analytical platform for the detection of specific antibiotics in the mid-IR regime. Taking advantage of unique sensitivity of robustly squeezed electromagnetic fields in toroidal meta-atoms, we validated that our proposed technique based on toroidal m…
Plasmonic sensing in the infrared region employs the direct interaction of the vibrational fingerprints of molecules with the plasmonic resonances, creating surface-enhanced sensing platforms that are superior than the traditional spectroscopy. However, the standard noble metals used for plasmonic resonances suffer from high radiative losses as well as fabrication challenges, such as tuning the spectral resonance positions into mid- to far-infrared regions, and the compatibility issue with the existing complementary metal-oxide-semiconductor (CMOS) manufacturing platform. Here, we demonstrate …
In this work, we use a site-selective functionalization strategy to decorate plasmonic nanopores with one or more fluorescent dyes. Using an easy and robust fabrication method, we manage to build single plasmonic rings on top of dielectric nanotubes with different inner diameters. The modulation of the dimension of the nanopores allows us to both tailor their field confinement and their Purcell Factor in the visible spectral range. In order to investigate how the changes in geometry influence the fluorescence emission efficiency, thiol-conjugated dyes are anchored on the plasmonic ring, thus f…
Waveguide-integrated plasmonics is a growing field with many innovative concepts and demonstrated devices in the visible and near-infrared. Here, we extend this body of work to the mid-infrared for the application of surface-enhanced infrared absorption (SEIRA), a spectroscopic method to probe molecular vibrations in small volumes and thin films. Built atop a silicon-on-insulator (SOI) waveguide platform, two key plasmonic structures useful for SEIRA are examined using computational modeling: gold nanorods and coaxial nanoapertures. We find resonance dips of 80% in near diffraction-limited are…
Nanomaterials capable of confining light are desirable for enhancing spectroscopies such as Raman scattering, infrared absorption, and nonlinear optical processes. Plasmonic superlattices have shown the ability to host collective resonances in the mid-infrared, but require stringent fabrication processes to create well-ordered structures. Here, we demonstrate how short-range-ordered Au nanoparticle multilayers on a mirror, self-assembled by a sub-nm molecular spacer, support collective plasmon-polariton resonances in the visible and infrared, continuously tunable beyond 11 $μ$m by simply varyi…
Controlling the propagation and polarization vectors in linear and nonlinear optical spectroscopy enables to probe the anisotropy of optical responses providing structural symmetry selective contrast in optical imaging. Here we present a novel tilted antenna-tip approach to control the optical vector-field by breaking the axial symmetry of the nano-probe in tip-enhanced near-field microscopy. This gives rise to a localized plasmonic antenna effect with significantly enhanced optical field vectors with control of both \textit{in-plane} and \textit{out-of-plane} components. We use the resulting …
The ability to control and modify infrared excitations in condensed matter is of both fundamental and application interests. Here we explore a system supporting low-energy excitations, in particular, mid-infrared localized plasmon modes and phonon polaritons that are tuned to be strongly coupled. We study the coupled modes by using far-field infrared spectroscopy, state-of-the-art monochromated electron energy-loss spectroscopy, numerical simulations and analytical modeling. We demonstrate that the electron probe facilitates a precise characterization of polaritons constituting the coupled sys…
The nature of light-matter interaction is governed by the spatial-temporal structures of a light field and material wavefunctions. The emergence of the light beam with transverse phase vortex, or equivalently orbital angular momentum (OAM) has been providing intriguing possibilities to induce unconventional optical transitions beyond the framework of the electric dipole interaction. The uniqueness stems from the OAM transfer from light to material, as demonstrated using the bound electron of a single trapped ion. However, many aspects of the vortex light-matter interaction are still unexplored…
We theoretically investigate the plasmonic properties of mid-infrared graphene-based metamaterials and apply deep learning of a neural network for the inverse design. These artificial structures have square periodic arrays of graphene plasmonic resonators deposited on dielectric thin films. Optical spectra vary significantly with changes in structural parameters. Our numerical results are in accordance with previous experiments. Then, the theoretical approach is employed to generate data for training and testing deep neural networks. By merging the pre-trained neural network with the inverse n…
Mid-infrared edge-enhanced imaging via angle-selective nonlinear filtering
East China Normal University（华东师范大学）；Chongqing Institute of East China Normal University（华东师范大学重庆研究院）；Shanxi University（山西大学）；Shanghai Research Center for Quantum Sciences（上海量子科学研究中心）
Plasmonic-cavity Modulator for the Mid-IR with a Semi-transparent and Nonlinear Heavily-doped Semiconductor Mirror
Istituto Italiano di Tecnologia（意大利理工学院）；Istituto di Fotonica e Nanotecnologie, Consiglio Nazionale delle Ricerche（国家研究委员会光子和纳米技术研究所）；University of Luxembourg（卢森堡大学）；Institute for Advanced Studies, University of Luxembourg Campus Belval（卢森堡大学贝尔瓦尔校区高等研究院）；Centre de Nanosciences et de Nanotechnologies (C2N), CNRS UMR 9001, Universit´e Paris-Saclay（巴黎萨克雷大学CNRS 9001联合实验室纳米科学与纳米技术中心）
