We use time-resolved charge detection techniques to investigate single-electron tunneling in semiconductor quantum dots. The ability to detect individual charges in real-time makes it possible to count electrons one-by-one as they pass through the structure. The setup can thus be used as a high-precision current meter for measuring ultra-low currents, with resolution several orders of magnitude better than that of conventional current meters.
In addition to measuring the average current, the counting procedure also makes it possible to investigate correlations between charge carriers. In quantum dots, we find that the strong Coulomb interaction makes electrons try to avoid each other. This leads to electron anti-bunching, giving stronger correlations and reduced noise compared to a current carried by statistically independent electrons.
The charge detector is implemented by monitoring changes in conductance in a near-by capacitively coupled quantum point contact. We find that the quantum point contact not only serves as a detector but also causes a back-action onto the measured device. Electron scattering in the quantum point contact leads to emission of microwave radiation. The radiation is found to induce an electronic transition between two quantum dots, similar to the absorption of light in real atoms and molecules. Using a charge detector to probe the electron transitions, we can relate a single-electron tunneling event to the absorption of a single photon. Moreover, since the energy levels of the double quantum dot can be tuned by external gate voltages, we use the device as a frequency-selective single-photon detector operating at microwave energies.
Destructive interference of single-electron tunneling between three quantum dots can trap an electron in a coherent superposition of charge on two of the dots. Coupling to external charges causes decoherence of this superposition, and in the presence of a large bias voltage each decoherence event transfers a certain number of electrons through the device. We calculate the counting statistics of the transferred charges, finding a crossover from sub-Poissonian to super-Poissonian statistics with increasing ratio of tunnel and decoherence rates.
We examine the full counting statistics of electron transport through double quantum dots coupled in series, with particular attention being paid to the unique features originating from level renormalization. It is clearly illustrated that the energy renormalization gives rise to a dynamic charge blockade mechanism, which eventually results in super-Poissonian noise. Coupling of the double dots to an external heat bath leads to dephasing and relaxation mechanisms, which are demonstrated to suppress the noise in a unique way.
We theoretically consider charge transport through two quantum dots coupled in series. The corresponding full counting statistics for noninteracting electrons is investigated in the limits of sequential and coherent tunneling by means of a master equation approach and a density matrix formalism, respectively. We clearly demonstrate the effect of quantum coherence on the zero-frequency cumulants of the transport process, focusing on noise and skewness. Moreover, we establish the continuous transition from the coherent to the incoherent tunneling limit in all cumulants of the transport process a…
We investigate the zero-frequency shot noise of electronic tunneling through a single quantum dot (SQD) and coherently coupled quantum dots (CQD) taking into account the Coulomb interaction. Within Hartree-Fock approximation, the analytical expressions of current and zero-frequency shot noise are self-consistently derived in the framework of full counting statistics for the both systems. We demonstrate that the correction term of zero-frequency shot noise induced by the intradot Coulomb interaction is almost negligible compared to the noninteracting shot noise in a SQD, while in a CQD the inte…
We investigate the effects of Coulomb interaction on charge transfer through a quantum dot attached to a normal and a superconducting lead. While for voltages much larger than the gap we recover the usual result for normal conductors, for voltages much smaller than the gap superconducting correlations lead to a drastically different behavior. Especially, the usual charge doubling in the normal case is reflected in the occurence of quartets due to the onsite interaction.
Graphene is considered to be a promising material for future electronics. The envisaged transistor applications often rely on precision cutting of graphene sheets with nanometer accuracy. In this letter we demonstrate graphene-based quantum dots created by using atomic force microscopy (AFM) with tip-assisted electrochemical etching. This lithography technique provides resolution of about 20 nm, which can probably be further improved by employing sharper tips and better humidity control. The behavior of our smallest dots in magnetic field has allowed us to identify the charge neutrality point …
Time-dependent driving influences the quantum and thermodynamic fluctuations of a system, changing the familiar physical picture of electronic noise which is an important source of information the about microscopic mechanism of quantum transport. Giving access to all cumulants of the current, the full counting statistics (FCS) is the powerful theoretical method to study fluctuations in nonequilibrium quantum systems. In this paper, we propose the application of FCS to consider periodic driven junctions. The combination of Floquet theory for time dynamics and nonequilibrium counting-field Green…
We measure telegraph noise of current fluctuations in an electrostatically defined quantum dot in bilayer graphene by real-time detection of single electron tunneling with a capacitively coupled neighboring quantum dot. Suppression of the second and third cumulant (related to shot noise) in a tunable graphene quantum dot is demonstrated experimentally. With this method we demonstrate the ability to measure very low current and noise levels. Furthermore, we use this method to investigate the first spin excited state, an essential prerequisite to measure spin relaxation.
We develop a conceptually simple scheme based on a master-equation approach to evaluate the full-counting statistics (FCS) of elastic and inelastic off-resonant tunneling (cotunneling) in quantum dots (QDs) and molecules. We demonstrate the method by showing that it reproduces known results for the FCS and shot noise in the cotunneling regime. For a QD with an excited state, we obtain an analytic expression for the cumulant generating function (CGF) taking into account elastic and inelastic cotunneling. From the CGF we find that the shot noise above the inelastic threshold in the cotunneling r…
We examine the full counting statistics of quantum dots, which display super-Poissonian shot noise. By an extension to a generic situation with many excited states we identify the underlying transport process. The statistics is a sum of independent Poissonian processes of bunches of different sizes, which leads to the enhanced noise. The obtained results could be useful to determine transport characteristics in molecules and large quantum dots, since the noise (and higher cumulants) allow to identify the internal level structure, which is not visible in the average current.
A fundamental question in quantum transport is how quantum coherence influences charge transfer through nanostructures. We address this issue for linear triple quantum dots by comparison of a Lindblad density matrix description with a Pauli rate equation approach and analyze the corresponding zero-frequency counting statistics for coherent and sequential charge tunneling, respectively. The impact of decaying coherences of the density matrix due to dephasing is also studied. Our findings reveal that the sensitivity to coherence shown by shot noise and skewness, in particular in the limit of lar…
Measurements of single electron tunneling through a quantum dot using a quantum point contact as charge detector have been performed for very long time traces with very large event counts. This large statistical basis is used for a detailed examination of the counting statistics for varying symmetry of the quantum dot system. From the measured statistics we extract high order cumulants describing the distribution. Oscillations of the high order cumulants are observed when varying the symmetry. We compare this behavior to the observed oscillation in time dependence and show that the variation o…
We analyze the spin-resolved full counting statistics of electron transfer through an ultrasmall quantum dot coupled to metallic electrodes. Modelling the setup by the Anderson Hamiltonian, we explicitly take into account the onsite Coulomb repulsion $U$. We calculate the cumulant generating function for the probability to transfer a certain number of electrons with a preselected spin orientation during a fixed time interval. With the cumulant generating function at hand we are then able to calculate the spin current correlations which are of outmost importance in the emerging field of spintro…
The electronic energy levels and optical transitions of a semiconductor quantum dot are subject to dynamics within the solid-state environment. In particular, fluctuating electric fields due to nearby charge traps or other quantum dots shift the transition frequencies via the Stark effect. The environment dynamics are mapped directly onto the fluorescence under resonant excitation and diminish the prospects of quantum dots as sources of indistinguishable photons in optical quantum computing. Here, we present an analysis of resonance fluorescence fluctuations based on photon counting statistics…
We measure current by counting single electrons tunneling through an InAs nanowire quantum dot. The charge detector is realized by fabricating a quantum point contact in close vicinity to the nanowire. The results based on electron counting compare well to a direct measurements of the quantum dot current, when taking the finite bandwidth of the detector into account. The ability to detect single electrons also opens up possibilities for manipulating and detecting individual spins in nanowire quantum dots.
We use a configuration-interaction approach and Fermi golden rule to investigate electron-phonon interaction in realistic multi-electron quantum dots. Lifetimes are computed in the low-density, highly correlated regime. We report numerical evidence that electron-electron interaction generally leads to reduced decay rates of excited electronic states in weakly confined quantum dots, where carrier relaxation is dominated by the interaction with longitudinal acoustic phonons.
The observed intermittent light emission from colloidal semiconductor nanocrystals has long been associated with Auger recombination assisted quenching. We test this view by observing transient emission dynamics of CdSe/CdS/ZnS semiconductor nanocrystals using time-resolved photon counting. The size and intensity dependence of the observed decay dynamics are inconsistent with the those expected from Auger processes. Moreover, the data suggests that in the `off' state the quantum dot cycles in a three-step process: photoexcitation, rapid trapping and subsequent slow nonradiative decay.
Nanowire double quantum dots occupied by an even number of electrons are investigated in the context of energy level structure revealed by electric dipole spin resonance measurements. We use numerically exact configuration interaction approach up to 6 electrons for systems tuned to Pauli spin blockade regime. We point out the differences between the spectra of systems with two and a greater number of electrons. For two-electrons the unequal length of the dots results in a different effective $g$-factors in the dots as observed by the recent experiments. For an increased number of electrons the…
We show that quantum dots and quantum wires are formed underneath metal electrodes deposited on a planar semiconductor heterostructure containing a quantum well. The confinement is due to the self-focusing mechanism of an electron wave packet interacting with the charge induced on the metal surface. Induced quantum wires guide the transfer of electrons along metal paths and induced quantum dots store the electrons in specific locations of the nanostructure. Induced dots and wires can be useful for devices operating on the electron spin.
Using a microscopic model for stochastic transport through a single quantum dot that is modified by the Coulomb interaction of environmental (weakly coupled) quantum dots, we derive generic properties of the full counting statistics for multi-stable Markovian transport systems. We study the temporal crossover from multi-modal to broad uni-modal distributions depending on the initial mixture, the long-term asymptotics and the divergence of the cumulants in the limit of a large number of transport branches. Our findings demonstrate that the counting statistics of a single resonant level may be u…
We study a two-level quantum dot embedded in a phonon bath and irradiated by a time-dependent ac field and develope a method that allows us to extract simultaneously the full counting statistics of the electronic tunneling and relaxation (by phononic emission) events as well as their correlation. We find that the quantum noise of both the transmitted electrons and the emitted phonons can be controlled by the manipulation of external parameters such as the driving field intensity or the bias voltage.
Density-functional theory is used to study the electronic structure of quantum dots in a magnetic field. New series of magic numbers are found for the total angular momentum of electrons. The empirical formula for the plateau width is obtained. The effect of a charged impurity on the electronic structure of a quantum dot has been studied.
In this paper we analyse the electronic properties of Dirac electrons in finite-size ribbons and in circular and hexagonal quantum dots made of graphene.
The effects of spin-orbit (SO) coupling arising from the confinement potential in single and two vertically-coupled quantum dots have been investigated. Our work indicates that a dot containing a single electron shows the lifting of the degeneracy of dipole-allowed transitions at B=0 due to the SO coupling which disappears for a dot containing two electrons. For coupled dots with one electron in each dot, the optical spectra is not affected by the coupling and is the same as the dot containing one electron. However, for the case of two coupled dots where one partner dot has two interacting ele…
A classical hydrodynamic approach is used to calculate the magnetoplasma excitations of two vertically coupled electron dots. The electrons are confined by different parabolic potentials in which case Kohn's theorem is no longer valid. The equilibrium density profiles of the electrons in both dots are calculated as function of the interdot distance. We find that for unequal confinements of the two dots the electron density in one of the dots becomes ring-like. The electron densities are then used to obtain the magnetoplasma frequencies. The oscillator strengths are calculated, and we find that…
Two tunnel-coupled few-electron quantum dots were fabricated in a GaAs/AlGaAs quantum well. The absolute number of electrons in each dot could be determined from finite bias Coulomb blockade measurements and gate voltage scans of the dots, and allows the number of electrons to be controlled down to zero. The Zeeman energy of several electronic states in one of the dots was measured with an in-plane magnetic field, and the g-factor of the states was found to be no different than that of electrons in bulk GaAs. Tunnel-coupling between dots is demonstrated, and the tunneling strength was estimate…
We propose a fast optically induced two-qubit \textsc{c-phase} gate between two resident spins in a pair of coupled quantum dots. An excited bound state which extends over the two dots provides an effective electron-electron exchange interaction. The gate is made possible by the electron-hole exchange interaction, which isolates a single transition in the system. When combined with appropriate single qubit rotations, this gate generates an entangled state of the two spins.
We investigate charge dynamics in a two-electron double quantum dot. The quantum dot is manipulated by using a time-dependent external voltage that induces charge oscillations between the dots. We study the dependence of the charge dynamics on the external magnetic field and on the periodicity of the external potential. We find that for suitable parameter values, it is possible to induce both one-electron and two-electron oscillations between the dots.
We theoretically analyze the effect of electron-electron interactions on Aharonov-Bohm (AB) current oscillations in ring-shaped systems with metallic quantum dots pierced by external magnetic field. We demonstrate that electron-electron interactions suppress the amplitude of AB oscillations $I_{AB}$ at all temperatures down to T=0 and formulate quantitative predictions which can be verified in future experiments. We argue that the main physical reason for such interaction-induced suppression of $I_{AB}$ is electron dephasing while Coulomb blockade effects remain insignificant in the case of me…
Kinetics of polarized photoluminescence of the negatively charged InP quantum dots in weak magnetic field is studied experimentally. Effect of both the nuclear spin fluctuations and the dynamical nuclear polarization on the electron spin orientation is observed.
We report the computer-automated tuning of gate-defined semiconductor double quantum dots in GaAs heterostructures. We benchmark the algorithm by creating three double quantum dots inside a linear array of four quantum dots. The algorithm sets the correct gate voltages for all the gates to tune the double quantum dots into the single-electron regime. The algorithm only requires (1) prior knowledge of the gate design and (2) the pinch-off value of the single gate $T$ that is shared by all the quantum dots. This work significantly alleviates the user effort required to tune multiple quantum dot …
We demonstrate electrical control of Si:P double dots in which the potential is defined by nanoscale phosphorus doped regions. Each dot contains approximately 600 phosphorus atoms and has a diameter close to 30 nm. On application of a differential bias across the dots, electron transfer is observed, using single electron transistors in both dc- and rf-mode as charge detectors. With the possibility to scale the dots down to few and even single atoms these results open the way to a new class of precision-doped quantum dots in silicon.
The low-lying eigenstates of a system of two electrons confined within a two-dimensional quantum dot with a hard polygonal boundary are obtained by means of exact diagonalization. The transition from a weakly correlated charge distribution for small dots to a strongly correlated "Wigner molecule" for large dots is studied, and the behaviour at the crossover is determined. In sufficiently large dots, a recently proposed mapping to an effective charge-spin model is investigated, and is found to produce the correct ordering of the energy levels and to give a good first approximation to the size o…
We investigate the effect of electron-electron interactions on Aharonov-Bohm (AB) current oscillations in nanorings formed by a chain of metallic quantum dots. We demonstrate that electron-electron interactions cause electron dephasing thereby suppressing the amplitude of AB oscillations at all temperatures down to T=0. The crossover between thermal and quantum dephasing is found to be controlled by the ring perimeter. Our predictions can be directly tested in future experiments.
We study the effect of electron-electron interaction on the conductance of open quantum dots. We find that Coulomb interactions (i) do not affect the ensemble averaged conductance <G> if time-reversal symmetry has been broken by a magnetic field, (ii) enhance weak localization and weak anti-localization corrections to <G> in the absence of a magnetic field, (iii) increase conductance fluctuations, and (iv) enhance the effect of short trajectories on the conductivity of quantum dot.
We investigate the effects of point charge defects on the single particle electronic structure, emission energies, fine structure splitting and oscillator strengths of excitonic transitions in strained In$_{0.6}$Ga$_{0.4}$As/GaAs and strain-free GaAs/Al$_{0.3}$Ga$_{0.7}$As quantum dots. We find that the charged defects significantly modify the single particle electronic structure and excitonic spectra in both strained and strain-free structures. However, the excitonic fine structure splitting, polarization anisotropy and polarization direction in strained quantum dots remain nearly unaffected,…
We discuss the properties of few electrons and electron-hole pairs confined in coupled semiconductor quantum dots, with emphasis on correlation effects and the role of tunneling. We shall discuss, in particular, exact diagonalization results for biexciton binding energy, electron-hole localization, magnetic-field induced Wigner molecules, and spin ordering.
Reliable detection of single electron tunneling in quantum dots (QD) is paramount to use this category of device for quantum information processing. Here, we report charge sensing in a degenerately phosphorus-doped silicon QD by means of a capacitively coupled single-electron tunneling device made of the same material. Besides accurate counting of tunneling events in the QD, we demonstrate that this architecture can be operated to reveal asymmetries in the transport characteristic of the QD. Indeed, the observation of gate voltage shifts in the detector's response as the QD bias is changed is …
In order to fully characterize the noise associated with electron transport, with its severe consequences for solid-state quantum information systems, the theory of full counting statistics has been developed. It accounts for correlation effects associated with the statistics and effects of entanglement, but it remains a non-trivial task to account for interaction effects. In this article we present two examples: we describe electron transport through quantum dots with strong charging effects beyond perturbation theory in the tunneling, and we analyze current fluctuations in a diffusive intera…
We derive a complete expression for the interaction correction to the $I-V$ curve of two connected in series metallic quantum dots. For strongly asymmetric dots in a wide range of parameters this interaction correction depends logarithmically on voltage and temperature.
We studied experimentally the dynamics of the exchange interaction between two antiparallel electron spins in a so-called metastable double quantum dot where coupling to the electron reservoirs can be ignored. We demonstrate that the level of control of such a double dot is higher than in conventional double dots. In particular, it allows to couple coherently two electron spins in an efficient manner following a scheme initially proposed by Loss and DiVincenzo. The present study demonstrates that metastable quantum dots are a possible route to increase the number of coherently coupled quantum …
The electronic spin precession in semiconductor dots is strongly affected by the spin-orbit coupling. We present a theory of the electronic spin resonance at low magnetic fields that predicts a strong dependence on the dot occupation, the magnetic field and the spin-orbit coupling strength. Coulomb interaction effects are also taken into account in a numerical approach.
We use numerically exact Chebyshev expansion and kernel polynomial methods to study transport through circular graphene quantum dots in the framework of a tight-binding honeycomb lattice model. Our focus lies on the regime where individual modes of the electrostatically defined dot dominate the charge carrier dynamics. In particular, we discuss the scattering of an injected Dirac electron wave packet for a single quantum dot, electron confinement in the dot, the optical excitation of dot-bound modes, and the propagation of an electronic excitation along a linear array of dots.
We present an experimental study of electron-electron exchange interaction in self-assembled CdTe/ZnTe quantum dots based on the photoluminescence measurements. The character and strength of this interaction are obtained by simultaneous observation of various recombination channels of a doubly negatively charged exciton, including previously unrecognized emission lines related to the electron-singlet configuration in the final state. A typical value of the electron singlet-triplet splitting, which corresponds to the exchange integral of electron-electron interaction, has been determined as 20.…
We study and compare two analytic models of graphene quantum dots for calculating charge relaxation times due to electron-phonon interaction. Recently, charge relaxation processes in graphene quantum dots have been probed experimentally and here we provide a theoretical estimate of relaxations times. By comparing a model with pure edge confinement to a model with electrostatic confinement, we find that the latter features much larger relaxation times. Interestingly, relaxation times in electrostatically defined quantum dots are predicted to exceed the experimentally observed lower bound of ~10…
Measuring single-electron charge is one of the most fundamental quantum technologies. Charge sensing, which is an ingredient for the measurement of single spins or single photons, has been already developed for semiconductor gate-defined quantum dots, leading to intensive studies on the physics and the applications of single-electron charge, single-electron spin and photon-electron quantum interface. However, the technology has not yet been realized for self-assembled quantum dots despite their fascinating quantum transport phenomena and outstanding optical functionalities. In this paper, we r…
Few-electron quantum dots are investigated in the regime of strong tunneling to the leads. Inelastic cotunneling is used to measure the two-electron singlet-triplet splitting above and below a magnetic field driven singlet-triplet transition. Evidence for a non-equilibrium two-electron singlet-triplet Kondo effect is presented. Cotunneling allows orbital correlations and parameters characterizing entanglement of the two-electron singlet ground state to be extracted from dc transport.
We present a study of the electronic structure of two laterally coupled gaussian quantum dots filled with two particles. The exact diagonalization method has been used in order to inspect the spatial correlations and examine the particular spin singlet-triplet configurations for different coupling degrees between quantum dots. The outcome of our research shows this structure to have highly modifiable properties promoting it as an interesting quantum device, showing the possible use of this states as a quantum bit gate.
We evaluate the Lande g factor of electrons in quantum dots (QDs) fabricated from GaAs quantum well (QW) structures of different well width. We first determine the Lande electron g factor of the QWs through resistive detection of electron spin resonance and compare it to the enhanced electron g factor determined from analysis of the magneto-transport. Next, we form laterally defined quantum dots using these quantum wells and extract the electron g factor from analysis of the cotunneling and Kondo effect within the quantum dots. We conclude that the Lande electron g factor of the quantum dot is…
Spin relaxation of electrons doped in InP quantum dots was studied by means of luminescence pump-probe and Hanle measurements. Optical pumping makes spins of doped electrons to be oriented in parallel to the helicity of the circularly polarized excitation. The luminescence pump-probe showed the spin orientation of the doped electrons decay on a millisecond time-scale. Hanle measurement clarified the spin dephasing relaxation time of doped electrons is 1.7 ns which is explained by the frozen fluctuation of nuclear spins.
This thesis describes capacitance and tunneling experiments performed on two-dimensional electron gas (2DEG) and quantum dot systems. It develops a system of equations that allow determination, by means of capacitance measurements, of the electronic density of states, the electron density, and the chemical potential in a 2DEG. The thesis describes the use of these techniques in the observation of a magnetic field induced energy gap to tunneling in the 2DEG and the single electron addition spectrum in arrays of quantum dots.
Charge-based quantum computation can be attained through reliable control of single electrons in lead-less quantum systems. Single-charge transitions in electrically-isolated double quantum dots (DQD) realised in phosphorus-doped silicon can be detected via capacitively coupled single-electron tunnelling devices. By means of time-resolved measurements of the detector's conductance, we investigate the dots' occupancy statistics in temperature. We observe a significant reduction of the effective electron temperature in the DQD as compared to the temperature in the detector's leads. This sets pro…
In the hot electron regime, electron-electron scattering strongly modifies not only the shot noise but also the full counting statistics. We employ a method based on a stochastic path integral to calculate the counting statistics of two systems in which noise in the hot electron regime has been experimentally measured. We give an analytical expression for the counting statistics of a chaotic cavity and find that heating due to electron-electron scattering renders the distribution of transmitted charge symmetric in the shot noise limit. We also discuss the frequency dispersion of the third orde…
We here propose a mechanism to teleport electrons between quantum dots through the transformation of a virtual bright exciton into a dark exciton. This mechanism relies on the interactions of two composite bosons: a pair of electrons with opposite spins, trapped in two dots and an electron-hole pair in a free exciton coupled to an unabsorbed pump pulse, which makes it ``bright'' but virtual. This bright exciton first turns ``dark'' by dropping its electron and stealing the trapped electron with opposite spin through an exchange Coulomb process with the trapped pair. In a second step, the dark …
We report the fabrication and measurement of one-electron single and double quantum dots with fast tunnel rates in a Si/SiGe heterostructure. Achieving fast tunnel rates in few-electron dots can be challenging, in part due to the large electron effective mass in Si. Using charge sensing, we identify signatures of tunnel rates in and out of the dot that are fast or slow compared to the measurement rate. Such signatures provide a means to calibrate the absolute electron number and verify single electron occupation. Pulsed gate voltage measurements are used to validate the approach.
We present a detailed theoretical investigation of the effect of Coulomb interactions on electron transport through quantum dots and double barrier structures connected to a voltage source via an arbitrary linear impedance. Combining real time path integral techniques with the scattering matrix approach we derive the effective action and evaluate the current-voltage characteristics of quantum dots at sufficiently large conductances. Our analysis reveals a reach variety of different regimes which we specify in details for the case of chaotic quantum dots. At sufficiently low energies the intera…
The authors report that anisotropic confining potentials in laterally-coupled semiconductor quantum dots (QDs) have large impacts in optical transitions and energies of inter-shell collective electronic excitations. The observed anisotropies are revealed by inelastic light scattering as a function of the in-plane direction of light polarization and can be finely controlled by modifying the geometrical shape of the QDs. These experiments show that the tuning of the QD confinement potential offers a powerful method to manipulate electronic states and far-infrared inter-shell optical transitions …
We theoretically investigate correlated electron-hole states in vertically coupled quantum dots. Employing a prototypical double-dot confinement and a configuration-interaction description for the electron-hole states, it is shown that the few-particle ground state undergoes transitions between different quantum states as a function of the interdot distance, resulting in unexpected spatial correlations among carriers and in electron-hole localization. Such transitions provide a direct manifestations of inter- and intradot correlations, which can be directly monitored in experiments.
