While the phase of a coherent light field can be precisely known, the phase of the individual photons that create this field, considered individually, cannot. Phase changes within single-photon wave packets, however, have observable effects. In fact, actively controlling the phase of individual photons has been identified as a powerful resource for quantum communication protocols. Here we demonstrate the arbitrary phase control of a single photon. The phase modulation is applied without affecting the photon's amplitude profile and is verified via a two-photon quantum interference measurement, which can result in the fermionic spatial behaviour of photon pairs. Combined with previously demonstrated control of a single photon's amplitude, frequency, and polarisation, the fully deterministic phase shaping presented here allows for the complete control of single-photon wave packets.
We present a general theoretical description of the temporal shaping of narrowband noncollinear type-I down-converted photons using a spectral phase filter with a symmetric phase distribution. By manipulating the spectral phase of the signal or idler photon, we demonstrate control of the correlation time and shape of the two-photon wave function with modulation frequency and modulation depth of the phase distribution.
Complete control over the properties of light up to the level of single photons is an invaluable tool for quantum information science and fundamental studies of light-matter interaction. The crucial prerequisite is the ability to create a spatio-temporal distribution of single-photon electromagnetic field with the desired characteristics, i.e. to shape a photon by design. Despite the ever-growing demand for tuneable single-photon sources, there is a lack of practical, efficient and scalable methods for photon shaping. Here we put forward a novel generic method that enables lossless shaping of …
We propose a method to produce pure single photons with an arbitrary designed temporal shape in a heralded, lossless and scalable way. As the indispensable resource, the method uses pairs of time-energy entangled photons. To accomplish the shaping, one photon of a pair undergoes temporal modulation according to the desired shape. Subsequent frequency-resolving detection of the photon heralds its entangled counterpart in a pure quantum state with a temporal shape non-locally affected by the modulation. We found conditions for the shape of the heralded photon to reproduce the modulation function…
We demonstrate experimentally the tunable control of the joint spectrum, i.e. waveform and degree of frequency correlations, of paired photons generated in spontaneous parametric downconversion. This control is mediated by the spatial shape of the pump beam in a type-I noncollinear configuration. We discuss the applicability of this technique to other sources of frequency entangled photons, such as electromagnetically induced Raman transitions.
Inherent loss is always to be avoided in generating single photons or biphotons, but interestingly it provides opportunities for manipulating the photon wave packet. In this paper we show how inherent loss in parametric down-conversion can be employed to tailor the wave packets of single photons and biphotons. As an example, we propose a scheme to realize a single photon in a single cycle using inherent loss. Our work has potential applications in quantum communication, quantum computation, and quantum interface.
Thorough control of the optical mode of a single photon is essential for quantum information applications. We present a comprehensive experimental and theoretical study of a light-matter interface based on cavity quantum electrodynamics. We identify key parameters like the phases of the involved light fields and demonstrate absolute, flexible, and accurate control of the time-dependent complex-valued wave function of a single photon over several orders of magnitude. This capability will be an important tool for the development of distributed quantum systems with multiple components that intera…
We describe a technique for generating pulses of light with controllable photon numbers, propagation direction, timing, and pulse shapes. The technique is based on preparation of an atomic ensemble in a state with a desired number of atomic spin excitations, which is later converted into a photon pulse. Spatio-temporal control over the pulses is obtained by exploiting long-lived coherent memory for photon states and electromagnetically induced transparency (EIT) in an optically dense atomic medium. Using photon counting experiments we observe generation and shaping of few-photon sub-Poissonian…
We present a scheme for engineering the joint spectrum of photon pairs created via spontaneous parametric down conversion. Our method relies on customizing the poling configuration of a quasi-phase-matched crystal. We use simulated annealing to find an optimized poling configuration which allows almost arbitrary shaping of the crystal's phase-matching function. This has direct application in the creation of pure single photons---currently one of the most important goals of single-photon quantum optics. We describe the general algorithm and provide code, written in C++, that outputs an optimize…
We construct an effective Hamiltonian of interacting bosons, based on scattered radiation off vibrational modes of designed molecular architectures. Making use of the infinite yet countable set of spatial modes representing the scattering of light, we obtain a variable photon-photon interaction in this basis. The effective Hamiltonian hermiticity is controlled by a geometric factor set by the overlaps of spatial modes. Using this mapping, we relate intensity measurements of the light to correlation functions of the interacting bosons evolving according to the effective Hamiltonian, rendering l…
We develop quantum-optical input-output theory for resonators with arbitrary coupling strength, and for input fields whose spectrum can be wider than the cavity free-spectral range, while ensuring that the field-operator commutator relations in space-time variables are correct. The cavity-field commutator exhibits a series of space-time echoes, representing causal connections of certain space-time points by light propagation. We apply the theory to two-photon wave-packet shaping by cavity reflection, which displays a remarkable illustration of dispersion cancellation. We also show that the the…
It is a long-standing goal to generate robust deterministic states of light with unique quantum properties, such as squeezing, sub-Poissonian statistics and entanglement. It is of interest to consider whether such quantum states of light could be generated by exploiting interactions with free electrons, going beyond their already ubiquitous use in generating classical light. This question is motivated by developments in electron microscopy, which present a new platform for manipulating photons through their interaction with quantum free electrons. Here, we explore the shaping of photon statist…
We propose a method of arbitrarily shaping and scaling the temporal intensity correlations of an optical signal locally, avoiding periodic correlations. We demonstrate our approach experimentally using stochastic intensity modulation. We also analyze and simulate shaping both temporal correlations and photon statistics that are fully specified by the user. We show that within the confines of monotony and convexity, the temporal correlations are independent of photon statistics and can take any shape.
Semiconductor quantum dots embedded in optical cavities are promising on-demand sources of single photons. Here, we theoretically study single photon emission from an optically driven two-photon Raman transition between the biexciton and the ground state of a quantum dot. The advantage of this process is that it allows all-optical control of the properties of the emitted single photon with a laser pulse. However, with the presence of other decay channels and excitation-induced quantum interference, on-demand emission of the single Raman photon is generally difficult to achieve. Here we show th…
We experimentally demonstrate spectral broadening and shaping of exponentially-decaying nanosecond pulses via nonlinear mixing with a phase-modulated pump in a periodically-poled lithium niobate (PPLN) waveguide. A strong, 1550~nm pulse is imprinted with a temporal phase and used to upconvert a weak 980 nm pulse to 600 nm while simultaneously broadening the spectrum to that of a Lorentzian pulse up to 10 times shorter. While the current experimental demonstration is for spectral shaping, we also provide a numerical study showing the feasibility of subsequent spectral phase correction to achiev…
Free-space quantum key distribution is gaining increasing interest as a leading platform for long range quantum communication. However, the sensitivity of quantum correlations to scattering induced by turbulent atmospheric links limits the performance of such systems. Recently, methods for compensating the scattering of entangled photons have been demonstrated, allowing for real-time optimization of their quantum correlations. In this Letter, we demonstrate the use of wavefront shaping for compensating the scattering of non-collinear and non-degenerate entangled photons. These results demonstr…
We propose an efficient way to generate optical analogs of both even and odd Schrodinger cat states (SCSs) with high fidelity, large amplitude and reasonable generation rate. The resource consumed are a single-mode squeezed vacuum state (SMSV) and possibly a single photon or nothing. We report the generation of even (odd) SCS with amplitude 4.2, fidelity higher than 0.99 and reasonable generation rate by subtraction of 30(31) photons from SMSV by ideal photon number detection. In the case of inefficient detectors, maintaining SCS size and its fidelity at the same level as in the case of ideal …
Quantum technologies hold great promise for revolutionizing photonic applications such as cryptography. Yet their implementation in real-world scenarios is held back, mostly due to sensitivity of quantum light to scattering. Recent developments in optimizing the shape of single photons introduce new ways to control quantum light. Nevertheless, shaping single photons in real-time remains a challenge due to the weak associated signals, which are too noisy for optimization processes. Here, we overcome this challenge and control scattering of entangled photons by shaping the classical laser beam t…
We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a coherent ultrashort pulse. To observe the shaping we perform sum-frequency generation (SFG) with an ultrahigh flux of entangled photons. At the appropriate conditions, SFG performs as a coincidence detector with an ultrashort response time (~100 fs), enabling a direct observation of the two-photon wavefunction. This property also enables us to demonstrate backg…
Uniting Quantum Processing Nodes of Cavity-coupled Ions with Rare-earth Quantum Repeaters Using Single-photon Pulse Shaping Based on Atomic Frequency Comb
Time synchronization and phase shaping of single photons both play fundamental roles in quantum information applications that rely on multi-photon quantum interference. Phase shaping typically requires separate modulators with extra insertion losses. Here, we develop a all-optical built-in phase modulator for single photons using a quantum memory. The fast phase modulation of a single photon in both step and linear manner are verified by observing the efficient quantum-memory-assisted Hong-Ou-Mandel interference between two single photons, where the anti-coalescence effect of bosonic photon pa…
We propose a scheme for the ultrafast control of the emitter-field coupling rate in cavity quantum electrodynamics. This is achieved by the control of the vacuum field seen by the emitter through a modulation of the optical modes in a coupled-cavity structure. The scheme allows the on/off switching of the coupling rate without perturbing the emitter and without introducing frequency chirps on the emitted photons. It can be used to control the shape of single-photon pulses for high-fidelity quantum state transfer, to control Rabi oscillations and as a gain-modulation method in lasers. We discus…
We demonstrate the control of entanglement of a single photon between several spatial modes propagating through a strongly scattering medium. Measurement of the scattering matrix allows the wavefront of the photon to be shaped to compensate the distortions induced by multiple scattering events. The photon can thus be directed coherently to a single or multi-mode output. Using this approach we show how entanglement across different modes can be manipulated despite the enormous wavefront disturbance caused by the scattering medium.
In this work, we experimentally manipulate the spectrum and phase of a biphoton wave packet in a two-dimensional frequency space. The spectrum is shaped by adjusting the temperature of the crystal, and the phase is controlled by tilting the dispersive glass plate. The manipulating effects are confirmed by measuring the two-photon spectral intensity (TSI) and the Hong-Ou-Mandel (HOM) interference patterns. Unlike the previous independent manipulation schemes, here we perform joint manipulation on the biphoton spectrum. The technique in this work paves the way for arbitrary shaping of a multi-ph…
Dynamic coupling of cavities to a quantum network is of major interest to distributed quantum information processing schemes based on cavity quantum electrodynamics. This can be achieved by active tuning a mediating atom-cavity system. In particular, we consider the dynamic coupling between two coupled cavities, each interacting with a two-level atom, realized by tuning one of the atoms. One atom-field system can be controlled to become maximally and minimally coupled with its counterpart, allowing high fidelity excitation confinement, Q-switching and reversible state transport. As an applicat…
High-dimensional entanglement is a valuable resource for quantum communication, and photon pairs entangled in orbital angular momentum are commonly used for encoding high-dimensional quantum states. However, methods for preparation of maximally entangled states of arbitrary dimensionality are still lacking, and currently used approaches essentially rely on filtering and entanglement concentration. Here we experimentally realize a method for generation of high-dimensional maximally entangled OAM states of photon pairs which does not require any of these procedures. Moreover, the prepared state …
Scattering by atmospheric turbulence is one of the main challenges in creating long free-space optical links, and specifically links of entangled photons. Classical compensation methods are hard to apply to entangled photons, due to inherently low signal to noise ratios and the fragility of entanglement. We have recently shown that we can use the bright laser beam that pumps spontaneous parametric down conversion to control the spatial correlations between entangled photons for compensating their scattering. In this work, we apply the pump-shaping technique to compensate for scrambling of corr…
Temporal metamaterials empower novel forms of wave manipulation with direct applications to quantum state transformations. In this work, we investigate vacuum amplification effects in anisotropic temporal boundaries. Our results theoretically demonstrate that the anisotropy of the temporal boundary provides control over the angular distribution of the generated photons. We analyze several single and multi-layered configurations of anisotropic temporal boundaries, each with a distinct vacuum amplification effect. Examples include the inhibition of photon production along specific directions, re…
We investigate the spectral properties of the biphoton state from the cascade emissions of cold atomic ensembles, which composes of a telecommunication photon (signal) followed by an infrared one (idler) via four-wave mixing.\ With adiabatic conditions for Gaussian driving pulses of width $τ$, the spectrum of the biphoton state has the form of a Gaussian that conserves signal and idler photon energies within $\hbar/τ$ modulated by a Lorentzian with a superradiant linewidth.\ Multiplexing the atomic ensembles with frequency-shifted cascade emissions, we may manipulate and shape the spectrum of …
We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor, modulated in amplitude and/or phase, and detected in coincidence by sum-frequency generation. First, we present a Fourier optical analysis of the optical setup yielding an analytic expression for the resulting field distribution at the exit plane of the shaping apparatus. We then introduce amplitude and/or phase shaping and present results which can only be obt…
The ability to engineer the properties of quantum optical states is essential for quantum information processing applications. Here, we demonstrate tunable control of spatial correlations between photon pairs produced by spontaneous parametric down-conversion. By shaping the spatial pump beam profile in a type-I collinear configuration, we tailor the spatial structure of coincidences between photon pairs entangled in high dimensions, without effect on intensity. The results highlight fundamental aspects of spatial coherence and hold potential for the development of quantum technologies based o…
Temporal modulation of the quantum vacuum through fast motion of a neutral body or fast changes of its optical properties is known to promote virtual into real photons, the so-called dynamical Casimir effect. Empowering modulation protocols with spatial control could enable to shape the spectral, spatial, spin, and entanglement properties of the emitted photon pairs. Space-time quantum metasurfaces have been proposed as a platform to realize this physics via modulation of their optical properties. Here, we report the mechanical analog of this phenomenon by considering systems whose lattice str…
We show that inducing sidebands in the emission of a single emitter into a one dimensional waveguide, together with a dissipative re-pumping process, a photon field is cooled down to a squeezed vacuum. Our method does not require to be in the strong coupling regime, works with a continuum of propagating field modes and it may lead to sources of tunable multimode squeezed light in circuit QED systems.
Single-photon pairs created in the nonlinear process of spontaneous parametric downconversion form the backbone of fundamental and applied experimental quantum information science. Many applications benefit from careful spectral shaping of the single-photon wave-packets. In this paper we tailor the joint spectral wave-function of downconverted photons by modulating the nonlinearity of a poled crystal without affecting the phase-matching conditions. We designed a crystal with a Gaussian nonlinearity profile and confirmed successful wave-packet shaping by two-photon interference experiments. We …
We explore the effects of ultrafast shaped pulses for two-level systems that do not have a single photon resonance by developing a multiphoton density-matrix approach. We take advantage of the fact that the dynamics of the intermediate virtual states are absent within our laser pulse timescales. Under these conditions, the multiphoton results are similar to the single photon and that it is possible to extend the single photon coherent control ideas to develop multiphoton coherent control.
Photon pair entangled in high dimensional orbital angular momentum (OAM) degree of freedom (DOF) has been widely regarded as a possible source in improving the capacity of quantum information processing. The need for the generation of a high dimensional maximally entangled state in the OAM DOF is therefore much desired. In this work, we demonstrate a simple method to generate a broader and flatter OAM spectrum, i.e. a larger spiral bandwidth (SB), of entangled photon pairs generated through spontaneous parametric down-conversion by modifying the pump beam profile. By investigating both experim…
We theoretically investigate the spectral property of a biphoton state from multiplexed thermal atomic ensembles. This biphoton state originates from the cascade emissions, which can be generated by two weak pump fields under four-wave mixing condition. Under this condition, a signal photon from the upper transition, chosen in a telecommunication bandwidth, can be generated along with a correlated idler photon from the lower infrared transition. We can spectrally shape the biphoton state by multiplexing the atomic ensembles with frequency-shifted emissions, where the entropy of entanglement ca…
Quantum entanglement is an integral part of quantum optics and has been exploited in areas such as computation, cryptography and metrology. The entanglement between photons can be present in various degrees of freedom (DOFs), and even the simplest bi-partite systems can occupy a large Hilbert space. Therefore, it is desirable to exploit this multi-dimensional space for various quantum applications by fully controlling the properties of the entangled photons in multiple DOFs. While current entangled-photon sources are capable of generating entanglement in one or more DOFs, there is currently a …
Using a realistic quantum master equation we show that the resonance fluorescence spectra of a two-level artificial atom (quantum dot) can be tuned by adjusting its photonic local density of states via biasing of one or more graphene monolayers. The structured photon reservoir is included using a photon Green function theory which fully accounts for the loss and dispersion. The field-driven Mollow triplet spectrum can be actively controlled by the graphene bias in the THz frequency regime. We also consider the effect of a dielectric support environment, and multiple graphene layers, on the emi…
We report two schemes to generate perfect anisotropy in the photoelectron angular distribution of a randomly oriented ensemble of polyatomic molecules. In order to exert full control over the anisotropy of photoelectron emission, we exploit interferences between single-photon pathways and a manifold of resonantly-enhanced two-photon pathways. These are shown to outperform non-sequential $(ω,2ω)$ bichromatic phase control for the example of CHFClBr molecules. We are able to optimize pulses that yield anisotropic photoelectron emission thanks to a very efficient calculation of photoelectron mome…
Single-photon states, which carry quantum information and coherently interact with quantum systems, are vital to the realization of all-optical engineered quantum networks. In this paper we derive the analytical form of the output field state for a large class of quantum finite-level systems driven by single-photon input field states using a transfer function approach. Single-photon pulse shaping via coherent feedback is also studied.
Fundamental quantum electrodynamical (QED) processes such as spontaneous emission and electron-photon scattering encompass a wealth of phenomena that form one of the cornerstones of modern science and technology. Conventionally, calculations in QED and in other field theories assume that incoming particles are single-momentum states. The possibility that coherent superposition states, i.e. "shaped wavepackets", will alter the result of fundamental scattering processes is thereby neglected, and is instead assumed to sum to an incoherent (statistical) distribution in the incoming momentum. Here,…
We present an experiment demonstrating high-resolution coherent control of a four-level atomic system in a closed (diamond) type configuration. A femtosecond frequency comb is used to establish phase coherence between a pair of two-photon transitions in cold Rb atoms. By controlling the spectral phase of the frequency comb we demonstrate the optical phase sensitive response of the diamond system. The high-resolution state selectivity of the comb is used to demonstrate the importance of the signs of dipole moment matrix elements in this type of closed-loop excitation. Finally, the pulse shape i…
Two-photon time-frequency entanglement is a valuable resource in quantum information. Resolving the wavepacket of ultrashort pulsed single-photons, however, is a challenge. Here, we demonstrate remote spectral shaping of single photon states and probe the coherence properties of two-photon quantum correlations in the time-frequency domain, using engineered parametric down-conversion (PDC) and a quantum pulse gate (QPG) in nonlinear waveguides. Through tailoring the joint spectral amplitude function of our PDC source we control the temporal mode structure between the generated photon pairs and …
We employ pulse shaping to abate single-qubit gate errors arising from the weak anharmonicity of transmon superconducting qubits. By applying shaped pulses to both quadratures of rotation, a phase error induced by the presence of higher levels is corrected. Using a derivative of the control on the quadrature channel, we are able to remove the effect of the anharmonic levels for multiple qubits coupled to a microwave resonator. Randomized benchmarking is used to quantify the average error per gate, achieving a minimum of 0.007+/-0.005 using 4 ns-wide pulse.
