High-dimensional entanglement is a valuable resource for quantum communication, and photon pairs entangled in orbital angular momentum are commonly used for encoding high-dimensional quantum states. However, methods for preparation of maximally entangled states of arbitrary dimensionality are still lacking, and currently used approaches essentially rely on filtering and entanglement concentration. Here we experimentally realize a method for generation of high-dimensional maximally entangled OAM states of photon pairs which does not require any of these procedures. Moreover, the prepared state is restricted to the subspace of the specified dimensionality, thus requiring minimal postselection.
The ability to engineer the properties of quantum optical states is essential for quantum information processing applications. Here, we demonstrate tunable control of spatial correlations between photon pairs produced by spontaneous parametric down-conversion. By shaping the spatial pump beam profile in a type-I collinear configuration, we tailor the spatial structure of coincidences between photon pairs entangled in high dimensions, without effect on intensity. The results highlight fundamental aspects of spatial coherence and hold potential for the development of quantum technologies based o…
Free-space quantum key distribution is gaining increasing interest as a leading platform for long range quantum communication. However, the sensitivity of quantum correlations to scattering induced by turbulent atmospheric links limits the performance of such systems. Recently, methods for compensating the scattering of entangled photons have been demonstrated, allowing for real-time optimization of their quantum correlations. In this Letter, we demonstrate the use of wavefront shaping for compensating the scattering of non-collinear and non-degenerate entangled photons. These results demonstr…
We vary the time-frequency mode structure of ultrafast pulse-pumped modulational instability (MI) twin beams in an argon-filled hollow-core kagomé-style PCF by adjusting the pressure, pump pulse chirp, fiber length and parametric gain. Compared to solid-core systems, the pressure dependent dispersion landscape brings increased flexibility to the tailoring of frequency correlations and we demonstrate that the pump pulse chirp can be used to tune the joint spectrum of femtosecond-pumped sources. We also characterize the resulting mode content, not only by measuring the multimode second-order cor…
Scattering by atmospheric turbulence is one of the main challenges in creating long free-space optical links, and specifically links of entangled photons. Classical compensation methods are hard to apply to entangled photons, due to inherently low signal to noise ratios and the fragility of entanglement. We have recently shown that we can use the bright laser beam that pumps spontaneous parametric down conversion to control the spatial correlations between entangled photons for compensating their scattering. In this work, we apply the pump-shaping technique to compensate for scrambling of corr…
Photon pair entangled in high dimensional orbital angular momentum (OAM) degree of freedom (DOF) has been widely regarded as a possible source in improving the capacity of quantum information processing. The need for the generation of a high dimensional maximally entangled state in the OAM DOF is therefore much desired. In this work, we demonstrate a simple method to generate a broader and flatter OAM spectrum, i.e. a larger spiral bandwidth (SB), of entangled photon pairs generated through spontaneous parametric down-conversion by modifying the pump beam profile. By investigating both experim…
We report on studying the dynamic evolution of orbital angular momentum (OAM) carrying light in sum frequency generation (SFG). Dynamic evolution of the SFG beam is studied in different cases, in which the two pump beams are either a single OAM mode or OAM superposition mode. For the cases when the two pumps are both in superposition mode, two kinds of spatial patterns and evolution behaviors are observed, one set of spatial pattern is non-diffractive and unchanged with propagating. In addition, SFG of two pump beams with opposite OAM will evolve into a kind of quasi-Gaussian mode. These obser…
In this work we present a simple method to reconstruct the complex spectral wavefunction of a biphoton, and hence gain complete information about the spectral and temporal properties of a photon pair. The technique, which relies on quantum interference, is applicable to biphoton states produced with a monochromatic pump when a shift of the pump frequency produces a shift in the relative frequencies contributing to the biphoton. We demonstrate an example of such a situation in type-II parametric down-conversion (SPDC) allowing arbitrary paraxial spatial pump and detection modes. Moreover, our t…
The temporal-mode (TM) basis is a prime candidate to perform high-dimensional quantum encoding. Quantum frequency conversion has been employed as a tool to perform tomographic analysis and manipulation of ultrafast states of quantum light necessary to implement a TM-based encoding protocol. While demultiplexing of such states of light has been demonstrated in the Quantum Pulse Gate (QPG), a multiplexing device is needed to complete an experimental framework for TM encoding. In this work we demonstrate the reverse process of the QPG. A dispersion-engineered difference frequency generation in no…
Walk-off effects, originating from the difference between the group and phase velocities, limit the efficiency of nonlinear optical interactions. While transverse walk-off can be eliminated by proper medium engineering, longitudinal walk-off is harder to avoid. In particular, ultrafast twin- beam generation via pulsed parametric down-conversion (PDC) and four-wave mixing (FWM) is only possible in short crystals or fibres or in double-path schemes. Here we show that in high-gain PDC, one can overcome the destructive role of both effects and even turn them into useful tools for shaping the emiss…
We study the quantum correlations induced by spontaneous parametric down-conversion (SPDC) of a frequency comb. We derive a theoretical method to find the output state corresponding to a pump with an arbitrary spectral profile. After applying it to the relevant example of a spectrally chirped pump, we run an optimization algorithm to numerically find the pump profiles maximizing some target functions. These include the number of independently squeezed modes and the variances of nullifiers defining cluster states used in many continuous-variable quantum information protocols. To assess the adva…
In this article, we employ multimode radiation of a synchronously pumped optical parametric oscillator (SPOPO) to build a cluster state through a conversion on the base of quantum memory cell. We demonstrate that by choosing an appropriate driving field we can ensure the effective writing of the only one supermode from the entire set of the SPOPO squeezed supermodes. Further, by changing the driving field profile at the readout, we convert the time profile of the retrieved signal while maintaining its quantum state. We demonstrate the possibilities of using the presented scheme by the example …
Optical vortex beams are profiled as helical wavefronts with a phase singularity carrying an orbital angular momentum (OAM) associated with their spatial distribution. The transverse intensity distribution of a conventional optical vortex has a strong dependence on the carried topological charge. However, perfect optical vortex (POV) beams have their transverse intensity distribution independent of their charge. Such `size-invariant' POV beams have found exciting applications in optical manipulation, imaging and communication. In this article, we investigate the use of POV modes in the efficie…
Quantum entanglement is an integral part of quantum optics and has been exploited in areas such as computation, cryptography and metrology. The entanglement between photons can be present in various degrees of freedom (DOFs), and even the simplest bi-partite systems can occupy a large Hilbert space. Therefore, it is desirable to exploit this multi-dimensional space for various quantum applications by fully controlling the properties of the entangled photons in multiple DOFs. While current entangled-photon sources are capable of generating entanglement in one or more DOFs, there is currently a …
We theoretically investigate the spectral property of a biphoton state from multiplexed thermal atomic ensembles. This biphoton state originates from the cascade emissions, which can be generated by two weak pump fields under four-wave mixing condition. Under this condition, a signal photon from the upper transition, chosen in a telecommunication bandwidth, can be generated along with a correlated idler photon from the lower infrared transition. We can spectrally shape the biphoton state by multiplexing the atomic ensembles with frequency-shifted emissions, where the entropy of entanglement ca…
The capacity of optical communication channels can be increased by space division multiplexing in structured optical fibers. Radial core optical fibers allows for the propagation of twisted light--eigenmodes of orbital angular momentum, which have attracted considerable attention for high-dimensional quantum information. Here we study the generation of entangled photons that are tailor-made for coupling into ring core optical fibers. We show that the coupling of photon pairs produced by parametric down-conversion can be increased by close to a factor of three by pumping the non-linear crystal …
The ability to manipulate and measure the time-frequency structure of quantum light is useful for information processing and metrology. Measuring this structure is also important when developing quantum light sources with high modal purity that can interfere with other independent sources. Here, we present and experimentally demonstrate a scheme based on intensity interferometry to measure the joint spectral mode of photon pairs produced by spontaneous parametric down-conversion. We observe correlations in the spectral phase of the photons due to chirp in the pump. We show that our scheme can …
Anyons, particles displaying a fractional exchange statistics intermediate between bosons and fermions, play a central role in the fractional quantum Hall effect and various spin lattice models, and have been proposed for topological quantum computing schemes due to their resilience to noise. Here we use parametric down-conversion in an integrated semiconductor chip to generate biphoton states simulating anyonic particle statistics, in a reconfigurable manner. Our scheme exploits the frequency entanglement of the photon pairs, which is directly controlled through the spatial shaping of the pum…
High-dimensional quantum information processing promises capabilities beyond the current state of the art, but addressing individual information-carrying modes presents a significant experimental challenge. Here we demonstrate effective high-dimensional operations in the time-frequency domain of non-classical light. We generate heralded photons with tailored temporal-mode structures through ultrafast pulse shaping of a parametric downconversion pump. We then implement a quantum pulse gate, enabled by dispersion-engineered sum-frequency generation, to project onto programmable temporal modes, r…
Air-stable bright entangled photon-pair source from graphene-encapsulated van der Waals ferroelectric NbOI2
Agency for Science, Technology and Research (A*STAR)（科学技术研究局）；Australian National University（澳大利亚国立大学）；Institute of Materials Research and Engineering (IMRE)（材料研究与工程学院）；School of Engineering, College of Engineering, Computing and Cybernetics, the Australian National University（澳大利亚国立大学工程、计算与网络科学学院）；Centre for Quantum Technologies (CQT), National University of Singapore (NUS)（新加坡国立大学量子技术中心）
When building a parametric downconversion photon-pair source with spectrally separable photons, e.g. for making high-purity heralded single photons, two practical issues must be accounted for: the design of the experiment, and its characterization. To address experiment design, we study the impact on spectral separability of realistic (sech shaped and chirped) pump fields, realistic nonlinear crystals with fabrication imperfections, and undesirable PDC generation far from the central PMF peak coming from nonlinearity shaping methods. To address experiment characterization, we study the effect …
