A laser can be understood as thermodynamic engine converting heat to a coherent single mode field close to Carnot efficiency. From this perspective spectral shaping of the excitation light generates a higher effective temperature on the pump than on the gain transition. Here, using a toy model of a quantum well structure with two suitably designed tunnel-coupled wells kept at different temperature, we study a laser operated on an actual spatial temperature gradient between pump and gain region. We predict gain and narrow band laser emission for a sufficient temperature gradient and resonator quality. Lasing appears concurrent with amplified heat flow and points to a new form of stimulated solid state cooling. Such a mechanism could raise the operating temperature limit of quantum cascade lasers by substituting phonon emission driven injection, which generates intrinsic heat, by an extended model with phonon absorption steps.
We explore coherent control of stimulated Raman scattering in the nonimpulsive regime. Optical pulse shaping of the coherent pump field leads to control over the stimulated Raman output. A model of the control mechanism is investigated.
We present a microscopic theory describing the stimulated scattering of intersubband polariton excitations in a microcavity-embedded two-dimensional electron gas. In particular, we consider the polariton scattering induced by the spontaneous emission of optical phonons. Our theory demonstrates the possibility of final-state stimulation for the scattering of such composite excitations, accounting for the deviations from perfect bosonicity occurring at high excitation densities. By using realistic parameters for a GaAs semiconductor system, we predict how to achieve a quantum degenerate regime, …
We present a microscopic laser model for many atoms coupled to a single cavity mode, including the light forces resulting from atom-field momentum exchange. Within a semiclassical description, we solve the equations for atomic motion and internal dynamics to obtain analytic expressions for the optical potential and friction force seen by each atom. When optical gain is maximum at frequencies where the light field extracts kinetic energy from the atomic motion, the dynamics combines optical lasing and motional cooling. From the corresponding momentum diffusion coefficient we predict sub-Doppler…
An almost ideal thresholdless laser can be realized in the strong-coupling regime of light-matter interaction, with Poissonian fluctuations of the field at all pumping powers and all intensities of the field. This ideal scenario is thwarted by quantum nonlinearities when crossing from the linear to the stimulated emission regime, resulting in a universal jump in the second order coherence, which measurement could however be used to establish a standard of lasing in strong coupling.
A cold atomic gas with an inverted population on a transition coupled to a field mode of an optical resonator constitutes a generic model of a laser. For quasi-continuous operation, external pumping, trapping and cooling of the atoms is required to confine them in order to achieve enough gain inside the resonator. As inverted atoms are high-field seekers in blue detuned light fields, tuning the cavity mode to the blue side of the atomic gain transition allows for combining lasing with stimulated cavity cooling and dipole trapping of the atoms at the antinodes of the laser field. We study such …
Taming quantum dynamical processes is the key to novel applications of quantum physics, e.g. in quantum information science. The control of light-matter interactions at the single-atom and single-photon level can be achieved in cavity quantum electrodynamics, in particular in the regime of strong coupling where atom and cavity form a single entity. In the optical domain, this requires permanent trapping and cooling of an atom in a micro-cavity. We have now realized three-dimensional cavity cooling and trapping for an orthogonal arrangement of cooling laser, trap laser and cavity vacuum. This l…
We study the laser cooling of a mechanical oscillator through the coupling with a dissipative three-level system. Under a background temperature beyond the Lamb-Dicke regime, we extend the standard cooling analysis by separately studying the classical motion and the quantum dynamics of the oscillator. In Ladder-system cooling, the cooling rate degrades by orders of magnitude at large classical motion. This phenomenon causes a critical transition of the final temperature at a hot background. In stark contrast, electromagnetic-induced-transparency (EIT) cooling with a $Λ$-system produces signifi…
For a superconducting qubit driven to perform Rabi oscillations and coupled to a slow electromagnetic or nano-mechanical oscillator we describe previously unexplored quantum optics effects. When the Rabi frequency is tuned to resonance with the oscillator the latter can be driven far from equilibrium. Blue detuned driving leads to a population inversion in the qubit and a bi-stability with lasing behavior of the oscillator; for red detuning the qubit cools the oscillator. This behavior persists at the symmetry point where the qubit-oscillator coupling is quadratic and decoherence effects are m…
We consider ultracold atoms in a far detuned optical lattice orientated across a high-Q optical resonator. Applying an external driving laser to the atoms, which is red detuned from the cavity mode by one vibrational quantum, induces cavity-enhanced sideband cooling. For a dense and cold enough atomic ensemble we predict an oscillation threshold for optical Raman sideband lasing concurrent with coherent matter-wave amplification. Above this oscillation threshold photons and atoms in the lowest band are dominantly created pairwise via stimulated emission with a strong suppression of competing s…
We show that it is possible to realize simultaneous Raman lasing at two different frequencies using a double-$Λ$ system pumped by a bi-frequency field. The Raman lasers are phase-locked to one another, and the beat-frequency matches the energy difference between the two meta-stable ground states. Akin to a conventional Raman laser, the phase-locked Raman laser pair is expected to be subluminal. As such, it is expected to be highly stable against perturbations in cavity length, and have a quantum noise limited linewidth that is far below that of a conventional laser. Because of these properties…
Nonlinear Heisenberg-Langevin equations are solved analytically by operator Fourier-expansion for the laser in the LED regime. Fluctuations of populations of lasing levels are taken into account as perturbations. Spectra of operator products are calculated as convolutions, preserving Bose commutations for the lasing field operators. It is found that fluctuations of population significantly affect spontaneous and stimulated emissions into the lasing mode, increase the radiation rate, the number of lasing photons and broad the spectrum of a bad cavity thresholdless and the superradiant lasers. T…
In a sequence of single spins interacting longitudinally with a mechanical oscillator, and using the micromaser model with random injection, we show that after an appropriate post-selection of each spin, a phonon laser analog with Poisson statistics is created with nearly perfect coherence, evidenced by the second order coherence function that goes asymptotically to one. The non-linear gain of the system depends crucially on the properly post-selected spin state as well as the pump. Our model and results suggest that the mechanism of interaction followed by a post-selected state or partial tra…
Stimulated emission is the process fundamental to laser operation, thereby producing coherent photon output. Despite negatively-charged nitrogen-vacancy (NV$^-$) centres being discussed as a potential laser medium since the 1980's, there have been no definitive observations of stimulated emission from ensembles of NV$^-$ to date. Reasons for this lack of demonstration include the short excited state lifetime and the occurrence of photo-ionisation to the neutral charge state by light around the zero-phonon line. Here we show both theoretical and experimental evidence for stimulated emission fro…
Simultaneous strong coherent pumping of the two transitions of a V-level atom with very differentdecay rates has been predicted to create almost perfect inversion on the narrower transition. Usingthe example of the blue and red transitions in Strontium we show that for suitable operatingconditions the corresponding resonant gain can be used to continuously operate a laser on thenarrow transition. In particular, for a strong detuning of the pump field with respect to the narrowtransition, coherent laser emission occurs close to the bare atomic transition frequency exhibitingonly a negligible co…
We introduce the concept of a squeezed laser, in which a squeezed cavity mode develops a macroscopic photonic occupation due to stimulated emission. Above the lasing threshold, the emitted light retains both the spectral purity inherent of a laser and the photon correlations characteristic of a photonic mode with squeezed quadratures. Our proposal, which can be implemented in optical setups, relies on the parametric driving of the cavity and dissipative stabilization by a broadband squeezed vacuum. The squeezed laser can find applications that go beyond those of standard lasers thanks to the s…
We theoretically investigate the emission properties of a single-mode cavity coupled to a mesoscopic number of incoherently pumped quantum emitters. We propose an operational measure for the medium cooperativity, valid both in the bad and in the good cavity regimes. We show that the opposite regimes of subradiance and superradiance correspond to negative and positive cooperativity, respectively. The lasing regime is shown to be characterized by nonnegative cooperativity. In the bad cavity regime we show that the cooperativity defines the transitions from subradiance to superradiance. In the go…
We propose a magnetomechanical device that exhibits many properties of a laser. The device is formed by a nanocantilever and dynamically polarized paramagnetic nuclei of a solid sample in a strong external magnetic field. The corresponding quantum oscillator and effective two-level systems are coupled by the magnetostatic dipole-dipole interaction between a permanent magnet on the cantilever tip and the magnetic moments of the spins, so that the entire system is effectively described by the Jaynes-Cummings model. We consider the possibility of observing transient and cw lasing in this system, …
The spatial formation of coherent random laser modes in strongly scattering disordered random media is a central feature in the understanding of the physics of random lasers. We derive a quantum field theoretical method for random lasing in disordered samples of complex amplifying Mie resonators which is able to provide self-consistently and free of any fit parameter the full set of transport characteristics at and above the laser phase transition. The coherence length and the correlation volume respectively is derived as an experimentally measurable scale of the phase transition at the laser …
Amplification by stimulated emission of nitrogen vacancy centres in a diamond-loaded fibre cavity
Macquarie University（麦考瑞大学）；Fraunhofer Institut für Angewandte Festkörperphysik (IAF)（弗劳恩霍夫应用固体物理研究所）；National Institutes for Quantum and Radiological Science and Technology（量子科学技术研究机构）；University of Tokyo（东京大学）；RMIT University（皇家墨尔本理工大学）
Stimulated emission of photons from a large number of atoms into the mode of a strong light field is the principle mechanism for lasing in "classical" lasers. The onset of lasing is marked by a threshold which can be characterised by a sharp increase in photon flux as a function of external pumping strength. The same is not necessarily true for the fundamental building block of a laser: a single trapped atom interacting with a single optical radiation mode. It has been shown that such a "quantum" laser can exhibit thresholdless lasing in the regime of strong coupling between atom and radiation…
Cavity optomechanical phenomena, such as cooling, amplification or optomechanically induced transparency, emerge due to a strong imbalance in the dissipation rates of the parametrically coupled electromagnetic and mechanical resonators. Here we analyze the reversed dissipation regime where the mechanical energy relaxation rate exceeds the energy decay rate of the electromagnetic cavity. We demonstrate that this regime allows for mechanically-induced amplification (or cooling) of the electromagnetic mode. Gain, bandwidth, and added noise of this electromagnetic amplifier are derived and compare…
We study the quantum dynamics of an ultracold atomic gas in a deep optical lattice within an optical high-$Q$ resonator. The atoms are coherently illuminated with the cavity resonance tuned to a blue vibrational sideband, so that photon scattering to the resonator mode is accompanied by vibrational cooling of the atoms. This system exhibits a threshold above which pairwise stimulated generation of a cavity photon and an atom in the lowest vibrational band dominates spontaneous scattering and we find a combination of optical lasing with a buildup of a macroscopic population in the lowest lattic…
The surprising recent observation of highly emissive triplet-states in lead halide perovskites accounts for their orders-of-magnitude brighter optical signals and high quantum efficiencies compared to other semiconductors. This makes them attractive for future optoelectronic applications, especially in bright low-threshold nano-lasers. Whilst non-resonantly pumped lasing from all-inorganic lead-halide perovskites is now well-established as an attractive pathway to scalable low-power laser sources for nano-optoelectronics, here we showcase a resonant optical pumping scheme on a fast triplet-sta…
We study a single incoherently pumped atom moving within an optical high-Q resonator in the strong coupling regime. Using a semiclassical description for the atom and field dynamics, we derive a closed system of differential equations to describe this coupled atom-field dynamics. For sufficiently strong pumping the system starts lasing when the atom gets close to a field antinode, and the associated light forces provide for self-trapping of the atom. For a cavity mode blue detuned with respect to the atomic transition frequency this is combined with cavity induced motional cooling allowing for…
We present a single solid-state laser system to cool, coherently manipulate and detect $^{25}$Mg$^+$ ions. Coherent manipulation is accomplished by coupling two hyperfine ground state levels using a pair of far-detuned Raman laser beams. Resonant light for Doppler cooling and detection is derived from the same laser source by means of an electro-optic modulator, generating a sideband which is resonant with the atomic transition. We demonstrate ground-state cooling of one of the vibrational modes of the ion in the trap using resolved-sideband cooling. The cooling performance is studied and disc…
We demonstrate phase locking of two ultraviolet laser sources by modulating a fundamental infrared laser with 4th-order sidebands using an electro-optic modulator and phase locking of one sideband to a second fundamental infrared laser. Subsequent sum frequency generation and second harmonic generation successfully translates the frequency offset to the ultraviolet domain. The phase lock at 139 GHz is confirmed through stimulated Raman transitions for thermometry of $^9$Be$^+$ ions confined in a cryogenic Penning trap. This technique might be used for sideband cooling of single $^9$Be$^+$ ions…
We present a solid-state laser system that generates 750 mW of continuous-wave single-frequency output at 313 nm. Sum-frequency generation with fiber lasers at 1550 nm and 1051 nm produces up to 2 W at 626 nm. This visible light is then converted to UV by cavity-enhanced second-harmonic generation. The laser output can be tuned over a 495 GHz range, which includes the 9Be+ laser cooling and repumping transitions. This is the first report of a narrow-linewidth laser system with sufficient power to perform fault-tolerant quantum-gate operations with trapped 9Be+ ions by use of stimulated Raman t…
