We study high-field phase diagram and low-energy excitations of three-dimensional quantum helimagnets. Slightly below the saturation field, the emergence of magnetic order may be viewed as Bose-Einstein condensation (BEC) of magnons. The method of dilute Bose gas enables a quantitative analysis of quantum effects in these helimagnets and thereby three phases are found: cone, coplanar fan and a phase-separated one. As an application, we map out the phase diagram of a 3D helimagnet which consists of frustrated J1-J2 chains as a function of frustration and an interchain coupling. Moreover, we also calculate the stability of the 2-magnon bound state to investigate the possibility of the bound-magnon BEC.
We report studies of thermal conductivity as functions of magnetic field and temperature in the helimagnetic insulator Cu$_2$OSeO$_3$ that reveal novel features of the spin-phase transitions as probed by magnon heat conduction. The tilted conical spiral and low-temperature skyrmion phases, recently identified in small-angle neutron scattering studies, are clearly identified by sharp signatures in the magnon thermal conductivity. Magnon scattering associated with the presence of domain boundaries in the tilted conical phase and regions of skyrmion and conical-phase coexistence are identified.
The magnon spectral problem is solved in terms of the spectrum of a diagonalizable operator for a generic class of magnetic states that includes several types of domain walls and the chiral solitons of monoaxial helimagnets. Focusing on the isolated solitons of monoaxial helimagnets, it is shown that the spin waves scattered (reflected and transmitted) by the soliton suffer a lateral displacement analogous to the Goos-Hanchen effect of optics. The displacement is a fraction of the wavelength, but can be greatly enhanced by using an array of well separated solitons. Contrarily to the Goos-Hanch…
Anisotropic low-temperature properties of the cubic spinel helimagnet ZnCr2Se4 in the single-domain spin-spiral state are investigated by a combination of neutron scattering, thermal conductivity, ultrasound velocity, and dilatometry measurements. In an applied magnetic field, neutron spectroscopy shows a complex and nonmonotonic evolution of the spin-wave spectrum across the quantum-critical point that separates the spin-spiral phase from the field-polarized ferromagnetic phase at high fields. A tiny spin gap of the pseudo-Goldstone magnon mode, observed at wave vectors that are structurally …
The metallic compound FeP belongs to the class of materials that feature a complex noncollinear spin order driven by magnetic frustration. While its double-helix magnetic structure with a period $λ_{\text{s}} \approx 5c$, where $c$ is the lattice constant, was previously well determined, the relevant spin-spin interactions that lead to that ground state remain unknown. By performing extensive inelastic neutron scattering measurements, we obtained the spin-excitation spectra in a large part of the momentum-energy space. The spectra show that the magnons are gapped with a gap energy of $\sim$5 m…
Disorder instability of the magnon condensate in a frustrated spin ladder
利用体磁测量和热力学测量研究了无序对受抑自旋梯化合物H8 C4 SO2 Cu 2（Cl[1-x]Brx）4的场诱导量子相变的影响.母体材料（x=0）是一种量子自旋液体，在应用领域中，已知它会形成具有长程螺旋磁序的磁振子凝聚体。我们表明，债券的随机性引入的非磁性halogene网站上的化学取代破坏这个相变在非常低的浓度，已经为x=0.01。磁振子凝聚体的极端脆弱性归因于无公度态中的随机挫折。
Spin waves in chiral magnetic materials are strongly influenced by the Dzyaloshinskii-Moriya interaction resulting in intriguing phenomena like non-reciprocal magnon propagation and magnetochiral dichroism. Here, we study the non-reciprocal magnon spectrum of the archetypical chiral magnet MnSi and its evolution as a function of magnetic field covering the field-polarized and conical helix phase. Using inelastic neutron scattering, the magnon energies and their spectral weights are determined quantitatively after deconvolution with the instrumental resolution. In the field-polarized phase the …
The phase diagram of cubic helimagnets near the critical temperature is obtained from a Landau-Ginzburg model, including fluctuations to gaussian level. The free energy is evaluated via a saddle point expansion around the local minima of the Landau-Ginzburg functional. The local minima are computed by solving the Euler-Lagrange equations with appropriate boundary conditions, preserving manifestly the full nonlinearity that is characteristic of skyrmion states. It is shown that the fluctuations stabilize the skyrmion lattice in a region of the phase diagram close to the critical temperature, wh…
We theoretically study the electrical conductivity in a one-dimensional helimagnet whose spin texture changes from helimagnetic to conical magnetic, and to forced ferromagnetic state while increasing the magnetic field along the helical axis. We find that the conductivity in the helimagnetic state at zero field depends on the electron filling and the coefficient of the spin-charge coupling. We also find that the conductivity in the conical magnetic state changes nonlinearly to the applied field, and the magnetoresistance becomes negative and positive depending on the model parameters.
Giant dielectric nonlinearities at a magnetic Bose-Einstein condensation
实验研究了低维带隙量子磁体Cu $_2$ Cl $_{4}\cdot$ H $_8$ C $_4$ SO $_2$在磁场诱导的量子临界点附近的介电响应，该临界点分离了量子无序态和螺旋基态.观察到的磁电容效应源于转变的不适当的铁电性质，这本身也许是磁振子的玻色-爱因斯坦凝聚的最著名的实现之一。尽管如此，我们发现，与过渡相关的磁电容效应表现出巨大的和非常不寻常的非谐性。
We report a comprehensive neutron scattering study of low energy magnetic excitations in the breathing pyrochlore helimagnetic $\text{Cu}_2\text{OSeO}_3$. Fully documenting the four lowest energy magnetic modes that leave the ferrimagnetic configuration of the "strong tetrahedra" intact ($|\hbarω|<13$ meV), we find gapless quadratic dispersion at the $Γ$ point for energies above 0.2 meV, two doublets separated by 1.6(2) meV at the $R$ point, and a bounded continuum at the $X$ point. Our constrained rigid spin cluster model relates these features to Dzyaloshinskii-Moriya (DM) interactions and t…
We employed small-angle neutron scattering to demonstrate that the magnetic skyrmion lattice can be realized in bulk chiral magnets as a thermodynamically stable state at temperatures much lower than the ordering temperature of the material. This is in the regime where temperature fluctuations become completely irrelevant to the formation of the topologically non-trivial magnetic texture. In this attempt we focused on the model helimagnet MnSi, in which the skyrmion lattice was previously well characterized and shown to exist only in a very narrow phase pocket close to the Curie temperature of…
Chirality is breaking of mirror symmetry in matter. In the fields of biology and chemistry, this is particularly important because some of the essential molecules in life such as amino acids and DNA have chirality. It is a long-standing mystery how one of the enantiomers was chosen at the beginning stage of life. The understanding of the emergence of homochirality under some conditions is indispensable for the study of the origin of life as well as pharmaceutical science. The chirality is also emergent in magnetic structures. The longitudinal helical magnetic structure is the chiral object com…
Quintuplet condensation in the skyrmionic insulator Cu2OSeO3 at ultrahigh magnetic fields
Shizuoka University（静冈大学）；Loughborough University（拉夫堡大学）；Leibniz Institute for Solid State and Materials Research Dresden（德累斯顿莱布尼茨固体与材料研究所）；University of Tokyo（东京大学）
Frustration of harmonic and solitonic helimagnetism on the body-centered tetragonal lattice of GdAlSi
The University of Tokyo（东京大学）；Korea Advanced Institute of Science and Technology（韩国科学技术院）；RIKEN Center for Emergent Matter Science (CEMS)（理化学研究所 新兴物质科学中心）；Institute for Solid State Physics, The University of Tokyo（东京大学固体物理研究所）；High Energy Accelerator Research Organization（高能加速器研究机构）；Nagoya University Synchrotron Radiation Research Center (NUSR), Nagoya University（名古屋大学同步辐射研究中心）
Magnetic skyrmions are nano-sized topological spin textures stabilized by a delicate balance of magnetic energy terms. The chemical substitution of the underlying crystal structure of skyrmion-hosting materials offers a route to manipulate these energy contributions, but also introduces additional effects such as disorder and pinning. While the effects of doping and disorder have been well studied in B20 metallic materials such as Fe$_{1-x}$Co$_x$Si and Mn$_{1-x}$Fe$_x$Si, the consequences of chemical substitution in the magnetoelectric insulator Cu$_2$OSeO$_3$ have not been fully explored. In…
SANS and magnetometry study of the magnetic phase diagram of the B20 helimagnet FeRhSi
Saint Petersburg State University（圣彼得堡国立大学）；Vereshchagin Institute for High Pressure Physics, Russian Academy of Sciences（俄罗斯科学院韦列夏金高压物理研究所）；Mozhaisky Military Space Academy（莫扎伊斯基军事航天学院）
Breaking of spatial inversion symmetry (SIS) induces unique phenomena in condensed matter. Besides the classic examples such as natural optical activity and piezoelectricity, the spin-orbit interaction further enriches the effect of SIS breaking, as exemplified by the Rashba effect. In particular, by combining this symmetry with magnetic fields or another type of time-reversal symmetry (TRS) breaking, noncentrosymmetric materials can be made to exhibit nonreciprocal responses, which are responses that differ for rightward and leftward stimuli. For example, resistivity becomes directionally dep…
Bose-Einstein condensation (BEC) of triplet excitations triggered by a magnetic field, sometimes called magnon BEC, in dimerized antiferromagnets gives rise to a long-range antiferromagnetic order in the plane perpendicular to the applied magnetic field. To explore the effects of spin-orbit coupling on magnon condensation, we study a spin model on a distorted honeycomb lattice with dimerized Heisenberg exchange ($J$ terms) and uniform off-diagonal exchange ($Γ'$ terms) interactions. Via variational Monte Carlo calculations and spin-wave theory, we find that an out-of-plane magnetic field can i…
We performed a comprehensive electron spin resonance, magnetization and heat capacity study on the field-induced magnetic phase transitions in the kagome antiferromagnet $α-Cu_3Mg(OH)_6Br_2$. With the successful preparation of single crystals, we mapped out the magnetic phase diagrams under the $c$-axis and $ab$-plane directional magnetic fields $B$. For $B\|c$, the three-dimensional (3D) magnon Bose-Einstein condensation (BEC) is evidenced by the power law scaling of the transition temperature, $T_c\propto (B_c-B)^{2/3}$. For $B\|ab$, the transition from the canted antiferromagetic (CAFM) sta…
In three-dimensional (3D) quantum magnets, magnonic Weyl points (WPs) featuring linear band crossing of two non-degenerate magnon branches can emerge in certain lattice geometry when time-reversal symmetry is broken macroscopically. Unfortunately, there are very limited 3D quantum magnets that host magnonic WPs, and they are yet to be observed experimentally because the intrinsic perturbative interactions that break time-reversal symmetry macroscopically can be very negligible. Here, we present an alternative means via photo-irradiation, in which magnonic WPs can emerge in 3D quantum magnets w…
Ground-state phase diagram and magnetic properties of a tetramerized spin-1/2 J_1-J_2 model: BEC of bound magnons and absence of the transverse magnetization
The microscopic conditions for the emergence of nonreciprocal magnon excitations in noncentrosymmetric magnets are theoretically investigated. We show that asymmetric magnon excitations appear when a bond magnetic toroidal dipole becomes active, which is defined as a parallel component between the Dzyaloshinskii-Moriya vector and the averaged spin moments at the ends of the bonds. Depending on magnetic structures accompanying the bond magnetic toroidal dipoles, the higher-rank magnetic toroidal multipoles can also be activated in a magnetic cluster, which describes various angle dependences of…
We use recently proposed four-spin bond-operator technique (BOT) to discuss spectral properties of frustrated spin-$\frac12$ $J_1$--$J_2$ Heisenberg antiferromagnet on square lattice at $J_2<0.4J_1$ (i.e., in the Néel ordered phase). This formalism is convenient for the consideration of low-lying excitations which appear in conventional approaches as multi-magnon bound states (e.g., the Higgs excitation) because separate bosons describe them in BOT. At $J_2=0$, the obtained magnon spectrum describes accurately available experimental data. However, calculated one-magnon spectral weights and the…
Topologically protected magnon surface states are highly desirable as an ideal platform to engineer low-dissipation spintronics devices. However, theoretical prediction of topological magnons in strongly correlated materials proves to be challenging because the ab initio density functional theory calculations fail to reliably predict magnetic interactions in correlated materials. Here, we present a symmetry-based approach, which predicts topological magnons in magnetically ordered crystals, upon applying external perturbations such as magnetic/electric fields and/or mechanical strains. We appl…
Combining the technologies of quantum optics and magnonics, we find that the circularly polarized laser can dynamically realize the quasiequilibrium magnon Bose-Einstein condensates (BEC). The Zeeman coupling between the laser and spins generates the optical Barnett field, and its direction is controllable by switching the laser chirality. We show that the optical Barnett field develops the total magnetization in insulating ferrimagnets with reversing the local magnetization, which leads to the quasiequilibrium magnon BEC. This laser-induced magnon BEC transition through optical Barnett effect…
