We propose a multiterminal nanostructure for electrical probing of the quantum spin Hall effect (QSHE) in two-dimensional (2D) topological insulators. The device consists of a ferromagnetic (FM) island with precessing magnetization that pumps (in the absence of any bias voltage) pure spin current symmetrically into the left and right adjacent 2D TIs modeled as graphene nanoribbons with the intrinsic spin-orbit (SO) coupling. The QSH regime of the six-terminal TI|FM|TI nanodevice, attached to two longitudinal and four transverse normal metal electrodes, is characterized by the SO-coupling-induced energy gap, chiral spin-filtered edge states within finite length TI regions, and quantized spin Hall conductance when longitudinal bias voltage is applied, despite the presence of the FM island. The same unbiased device, but with precessing magnetization of the central FM island, blocks completely pumping of total spin and charge currents into the longitudinal electrodes while generating DC transverse charge Hall currents. Although these transverse charge currents are not quantized, their induction together with zero longitudinal charge current is a unique electrical response of TIs to pumped pure spin current that cannot be mimicked by SO-coupled but topologically trivial systems. In the corresponding two-terminal inhomogeneous TI|FM|TI nanostructures, we image spatial profiles of local spin and charge currents within TIs which illustrate transport confined to chiral spin-filtered edges states while revealing concomitantly the existence of interfacial spin and charge currents flowing around TI|FM interfaces and penetrating into the bulk of TIs over some short distance.
We report direct electrical detection of spin pumping, using a lateral normal metal/ferromagnet/normal metal device, where a single ferromagnet in ferromagnetic resonance pumps spin polarized electrons into the normal metal, resulting in spin accumulation. The resulting backflow of spin current into the ferromagnet generates a d.c. voltage due to the spin dependent conductivities of the ferromagnet. By comparing different contact materials (Al and /or Pt), we find, in agreement with theory, that the spin related properties of the normal metal dictate the magnitude of the d.c. voltage.
We study spin and charge currents pumped by precessing magnetization of a single ferromagnetic layer within F|I|N or F|I|F (F-ferromagnet; I-insulator; N-normal-metal) multilayers of nanoscale thickness attached to two normal metal electrodes with no applied bias voltage between them. Both simple one-dimensional model, consisting of a single precessing spin and a potential barrier as the "sample," and realistic three-dimensional devices are investigated. In the rotating reference frame, where the magnetization appears to be static, these junctions are mapped onto a four-terminal dc circuit who…
The Josephson current in a diffusive superconductor/ferromagnet/superconductor junction with precessing magnetization is calculated within the quasiclassical theory of superconductivity. When the junction is phase-biased, a stationary current (without a.c. component) can flow through it despite the non-equilibrium condition. A large critical current is predicted due to a dynamically induced long range triplet proximity effect. Such effect could be observed in a conventional hybrid device close to the ferromagnetic resonance.
We report the manipulation of nitrogen vacancy (NV) spins in diamond when nearby ferrimagnetic insulator, yttrium iron garnet, is driven into precession. The change in NV spin polarization, as measured by changes in photoluminescence, is comparable in magnitude to that from conventional optically detected magnetic resonance, but relies on a distinct mechanism as it occurs at a microwave frequency far removed from the magnetic resonance frequency of the NV spin. This observation presents a new approach to transferring ferromagnetic spin information into a paramagnet and then transducing the res…
A linear-response formulation of the dc spin pumping, i.e., a spin injection from a precessing ferromagnet into an adjacent spin sink, is developed in view of describing many-body effects caused by spin fluctuations in the spin sink. It is shown that, when an itinerant ferromagnet near Tc is used as the spin sink, the spin pumping is largely increased owing to the fluctuation enhancement of the spin conductance across the precessing ferromagnet/spin sink interface. As an example, the enhanced spin pumping from permalloy into nickel palladium alloy (Tc ~ 20K) is analyzed by means of a self-cons…
Using the charge-conserving Floquet-Green function approach to open quantum systems driven by external time periodic potential, we analyze how spin current pumped (in the absence of any dc bias voltage) by the precessing magnetization of a ferromagnetic (F) layer is injected {\em laterally} into the interface with strong spin-orbit coupling (SOC) and converted into charge current flowing in the same direction. In the case of metallic interface with the Rashba SOC used in experiments [Nature Comm. {\bf 4}, 2944 (2013)], both spin $I^{S_α}$ and charge $I$ current flow within it where $I/I^{S_α} …
We propose a method to control surface phonon transport by weak magnetic fields based on the pumping of surface acoustic waves (SAWs) by magnetostriction. We predict that the magnetization dynamics of a nanowire on top of a dielectric films injects SAWs with opposite angular momenta into opposite directions. Two parallel nanowires form a phononic cavity that at magnetic resonances pump a unidirectional SAW current into half of the substrate.
We theoretically investigate pumping of phonons by the dynamics of a magnetic film into a non-magnetic contact. The enhanced damping due to the loss of energy and angular momentum shows interference patterns as a function of resonance frequency and magnetic film thickness that cannot be described by viscous ("Gilbert") damping. The phonon pumping depends on magnetization direction as well as geometrical and material parameters and is observable, e.g., in thin films of yttrium iron garnet on a thick dielectric substrate.
Precessing magnetization in a thin film magnetic insulator pumps spins into adjacent metals; however, this phenomenon is not quantitatively understood. We present a theory for the dependence of spin-pumping on the transverse mode number and in-plane wave vector. For long-wavelength spin waves, the enhanced Gilbert damping for the transverse mode volume waves is twice that of the macrospin mode, and for surface modes, the enhancement can be ten or more times stronger. Spin-pumping is negligible for short-wavelength exchange spin waves. We corroborate our analytical theory with numerical calcula…
We study the magnetization dynamics in thin ferromagnetic films and small ferromagnetic particles in contact with paramagnetic conductors. A moving magnetization vector causes \textquotedblleft pumping\textquotedblright of spins into adjacent nonmagnetic layers. This spin transfer affects the magnetization dynamics similar to the Landau-Lifshitz-Gilbert phenomenology. The additional Gilbert damping is significant for small ferromagnets, when the nonmagnetic layers efficiently relax the injected spins, but the effect is reduced when a spin accumulation build-up in the normal metal opposes the s…
We investigate two schemes for pumping spin adiabatically from a ferromagnet through an interacting quantum dot into a normal lead, which exploit the possibility to vary in time the ferromagnet's magnetization, either its amplitude or its direction. For this purpose, we extend a diagrammatic real-time technique for pumping to situations in which the leads' properties are time dependent. In the first scheme, the time-dependent magnetization amplitude is combined with a time-dependent level position of the quantum dot to establish both a charge and a spin current. The second scheme uses a unifor…
We demonstrate electrical magnetization switching and spin pumping in magnetically doped Weyl semimetals. The Weyl semimetal is a new class of topological semimetals, known to have nontrivial coupling between the charge and the magnetization due to the chiral anomaly. By solving the Landau-Lifshitz-Gilbert equation for a multilayer structure of a Weyl semimetal, an insulator and a metal whilst taking the charge-magnetization coupling into account, magnetization dynamics is analyzed. It is shown that the magnetization dynamics can be driven by the electric voltage. Consequently, switching of th…
We demonstrate spin pumping, i.e. the generation of a pure spin current by precessing magnetization, without application of microwave radiation commonly used in spin pumping experiments. We use femtosecond laser pulses to simultaneously launch the magnetization precession in each of two ferromagnetic layers of a Galfenol-based spin valve and monitor the temporal evolution of the magnetizations. The spin currents generated by the precession cause a dynamic coupling of the two layers. This coupling has dissipative character and is especially efficient when the precession frequencies in the two l…
Recent experiments demonstrated generation of spin currents by ultrasound. We can understand this acoustically induced spin pumping in terms of the coupling between magnetization and lattice waves. Here we study the parametric excitation of magnetization by longitudinal acoustic waves and calculate the acoustic threshold power. The induced magnetization dynamics can be detected by the spin pumping into an adjacent normal metal that displays the inverse spin Hall effect.
The polarization of the spin current pumped by a precessing ferromagnet into an adjacent normal metal has a constant component parallel to the precession axis and a rotating one normal to the magnetization. The former component is now routinely detected in the form of a DC voltage induced by the inverse spin Hall effect (ISHE). Here we compute AC-ISHE voltages much larger than the DC signals for various material combinations and discuss optimal conditions to observe the effect. Including the backflow of spins is essential for distilling parameters such as the spin Hall angle from ISHE-detected…
The interplay between spin, charge, and orbital degrees of freedom has led to the development of spintronic devices like spin-torque oscillators, spin-logic devices, and spin-transfer torque magnetic random-access memories. In this development spin pumping, the process where pure spin-currents are generated from magnetisation precession, has proved to be a powerful method for probing spin physics and magnetisation dynamics. The effect originates from direct conversion of low energy quantised spin-waves in the magnet, known as magnons, into a flow of spins from the precessing magnet to adjacent…
"Pumping" of phonons by a dynamic magnetization promises to extend the range and functionality of magnonic devices. We explore the impact of phonon pumping on room-temperature ferromagnetic resonance (FMR) spectra of bilayers of thin yttrium iron garnet (YIG) films on thick gadolinium gallium garnet substrates over a wide frequency range. At low frequencies the Kittel mode hybridizes coherently with standing ultrasound waves of a bulk acoustic resonator to form magnon polarons that induce rapid oscillations of the magnetic susceptibility, as reported before. At higher frequencies, the phonon r…
A mechanism of current-induced magnetization reversal based on the parametric resonance is described. The source of the magnetization reversal is a current-induced magnetic field, which is applied perpendicularly to the easy axis of magnetic anisotropy of a ferromagnetic nanomagnet. The current-induced magnetic field was measured in a FeCoB nanomagnet to be 60 Gauss at a current density of 65 mA/um2. Two mechanisms of the magnetization reversal are described and calculated. The first mechanism is the reversal by a RF electrical current, which modulated at a frequency close to the precession fr…
We derive a non-perturbative solution to the Floquet-nonequilibrium Green function (Floquet-NEGF) describing open quantum systems periodically driven by an external field of arbitrary strength of frequency. By adopting the reduced-zone scheme, we obtain expressions rendering conserved charge currents for any given maximum number of photons, distinguishable from other existed Floquet-NEGF-based expressions where, less feasible, infinite number of photons needed to be taken into account to ensure the conservation. To justify our derived formalism and to investigate spin-charge conversions by spi…
We formulate a phenomenological description of thin ferromagnetic layers with inversion asymmetry where the single-domain magnetic dynamics experiences magnon current-induced torques and leads to magnon-motive forces. We first construct a phenomenological theory based on irreversible thermodynamics, taking into account the symmetries of the system. Furthermore, we confirm that these effects originate from Dzyaloshinskii-Moriya interactions from the analysis based on the stochastic Landau-Lifshitz-Gilbert equation. Our phenomenological results generalize to a general form of Dzyaloshinskii-Mori…
Voltage induced magnetization dynamics of magnetic thin films is a valuable tool to study anisotropic fields, exchange couplings, magnetization damping and spin pumping mechanism. A particularly well established technique is the ferromagnetic resonance (FMR) generated by the coupling of microwave photons and magnetization eigenmodes in the GHz range. Here we review the basic concepts of the so-called acoustic ferromagnetic resonance technique (a-FMR) induced by the coupling of surface acoustic waves (SAW) and magnetization of thin films. Interestingly, additional to the benefits of the microwa…
We derive boundary conditions at the interfaces of magnetoelastic heterostructures under ferromagnetic resonance for arbitrary magnetization directions and interface shapes. We apply our formalism to magnet$\vert$nonmagnet bilayers and magnetic grains embedded in a nonmagnetic thin film, revealing a nontrivial magnetization angle dependence of acoustic phonon pumping.
We develop a time-dependent nonequilibrium Green function (NEGF) approach to the problem of spin pumping by precessing magnetization in one of the ferromagnetic layers within F/I/F magnetic tunnel junctions (MTJs) or F/I/N semi-MTJs in the presence of intrinsic Rashba spin-orbit coupling (SOC) at the F/I interface or the extrinsic SOC in the bulk of F layers of finite thickness (F-ferromagnet; N-normal metal; I-insulating barrier). To express the time-averaged pumped charge current, or the corresponding dc voltage signal in open circuits that was measured in recent experiments on semi-MTJs [T.…
We investigate magnetization dynamics in asymmetric interlayer exchange coupled Py/Ru/Py trilayers using both vector network analyzer-based and electrically detected ferromagnetic resonance techniques. Two different ferromagnetic resonance modes, in-phase and out-of-phase, are observed across all three regimes of the static magnetization configurations, through antiparallel alignment at low fields, the spin-flop transition at intermediate fields, and parallel alignment at high fields. The nonmonotonic behavior of the modes as a function of the external field is explained in detail by analyzing…
A magnet with precessing magnetization pumps a spin current into adjacent leads. As a special case of this spin pumping, a precessing macrospin (magnetization) can assist electrons in tunneling. In small systems, however, the Coulomb blockade effect can block the transport of electrons. Here, we investigate the competition between macrospin-assisted tunneling and Coulomb blockade for the simplest system where both effects meet; namely, for a single tunnel junction between a normal metal and a metallic ferromagnet with precessing magnetization. By combining Fermi's golden rule with magnetizatio…
To study the effect of spin-orbit coupling (SOC) on spin-transfer torque in magnetic materials, we have implemented two theoretical formalisms that can accommodate SOC. Using the "charge-pumping" formalism, we find two contributions to the out-of-plane spin-transfer torque parameter $β$ in ballistic Ni domain walls (DWs). For short DWs, the nonadiabatic reflection of conduction electrons caused by the rapid spatial variation of the exchange potential results in an out-of-plane torque that increases rapidly with decreasing DW length. For long DWs, the Fermi level conduction channel anisotropy t…
We study the effects of the coupling between magnetization dynamics and the electronic degrees of freedom in a heterostructure of a metallic nanomagnet with dynamic magnetization coupled with a superconductor containing a steady spin-splitting field. We predict how this system exhibits a non-linear spin torque, which can be driven either with a temperature difference or a voltage across the interface. We generalize this notion to arbitrary magnetization precession by deriving a Keldysh action for the interface, describing the coupled charge, heat and spin transport in the presence of a precess…
We study the quantum spin pumping of an antiferromagnetic spin-1/2 chain with competing exchange interactions. We show that spatially periodic potential modulated in space and time acts as a quantum spin pump. In our model system, an applied electric field causes a spin gap to its critical ground state by introducing bond-alternation exchange interactions. We study quantum spin pumping at different quantized magnetization states and also explain physically the presence and absence of quantum spin pumping at different fractionally quantized magnetization states.
We investigate pure spin pumping in graphene by imposing a ferromagnet (F) with rotating magnetization on top of it. Using the generalized scattering approach for adiabatic spin pumping, we obtain the spin current pumped through magnetic graphene to a neighboring normal (N) region. The spin current can be easily controlled by gate voltages and under certain conditions, becomes sufficiently large to be measurable in current experimental setups. In fact it reaches a maximum value when one of the spins are completely filtered due to the vanishing density of states of the corresponding spin specie…
A theoretical formalism is developed to simultaneously solve equation of motion of the magnetizations in two ferromagnets and the spin-pumping induced spin transport equation. Based on the formalism, a coupled motion of the magnetizations in a self-oscillation state is studied. The spin pumping is found to induce an in-phase synchronization of the magnetizations for the oscillation around the easy axis. For an out-of-plane self-oscillation around the hard axis, on the other hand, the spin pumping leads to an in-phase synchronization in a small current region, whereas an antiphase synchronizati…
Generally the adiabatic quantum pumping phenomenon can be interpreted by the surface integral of the Berry curvature inside the cyclic loop. Spin angular momentum flow without charge current can be pumped out by magnetization precession in ferromagnet-based structures. When an electron is scattered by a helimagnet, spin-dependent diffraction occurs due to the spatial modulation of the spiral. In this work, we consider the charge and spin flow driven by magnetization precession in normal-metal/multiferroic-helimagnet/ferromagnet heterostructures. The pumping behavior is governed by the diffract…
We describe electrical detection of spin pumping in metallic nanostructures. In the spin pumping effect, a precessing ferromagnet attached to a normal-metal acts as a pump of spin-polarized current, giving rise to a spin accumulation. The resulting spin accumulation induces a backflow of spin current into the ferromagnet and generates a dc voltage due to the spin dependent conductivities of the ferromagnet. The magnitude of such voltage is proportional to the spin-relaxation properties of the normal-metal. By using platinum as a contact material we observe, in agreement with theory, that the v…
The magnetization dynamics induced by standing elastic waves excited in a thin ferromagnetic film is described with the aid of micromagnetic simulations taking into account the magnetoelastic coupling between spins and lattice strains. The simulations have been performed for the 2 nm thick Fe81Ga19 film dynamically strained by longitudinal and transverse standing waves with various frequencies, which span a wide range around the resonance frequency nu_res of coherent magnetization precession in unstrained Fe81Ga19 film. It is found that standing elastic waves give rise to complex local magneti…
The critical current of the spin transfer torque-driven magnetization dynamics was studied by taking into account both spin pumping and the finite penetration depth of the transverse spin current. We successfully reproduced the recent experimental results obtained by Chen et al. [Phys. Rev. B {\bf 74}, 144408 (2006)] and found that the critical current remains finite even in the zero-thickness limit of the free layer. We showed that the remaining value of the critical current is determined mainly by spin pumping.
We analyze the statistics of charge and energy currents and spin torque in a metallic nanomagnet coupled to a large magnetic metal via a tunnel contact. We derive a Keldysh action for the tunnel barrier, describing the stochastic currents in the presence of a magnetization precessing with the rate $Ω$. In contrast to some earlier approaches, we include the geometric phases that affect the counting statistics. We illustrate the use of the action by deriving spintronic fluctuation relations, the quantum limit of pumped current noise, and consider the fluctuations in two specific cases: the situa…
Spin transfer torque and spin pumping are central reciprocal phenomena in spintronics. These phenomena occur in hybrid systems of normal metals and magnets. Spin transfer is the conversion of spin currents in metals to a torque on the magnetization of magnets. Spin pumping is the emission of spin currents from precessing magnets. Here, we demonstrate a general way to understand these effects within a quantum out-of-equilibrium path-integral model. Our results agree with known expressions for spin transfer and spin pumping in terms of transverse (mixing) conductances when there are no fluctuati…
We consider an antiferromagnetic insulator that is in contact with a metal. Spin accumulation in the metal can induce spin-transfer torques on the staggered field and on the magnetization in the antiferromagnet. These torques relate to spin pumping: the emission of spin currents into the metal by a precessing antiferromagnet. We investigate how the various components of the spin-transfer torque are affected by spin-independent disorder and spin-flip scattering in the metal. Spin-conserving disorder reduces the coupling between the spins in the antiferromagnet and the itinerant spins in the met…
Spin pumping by a moving magnetization gives rise to an electric voltage over a spin valve. Thermal fluctuations of the magnetization manifest themselves as increased thermal voltage noise with absorption lines at the ferromagnetic resonance frequency and/or zero frequency. The effect depends on the magnetization configuration and can be of the same order of magnitude as the Johnson-Nyquist thermal noise. Measuring colored voltage noise is an alternative to ferromagnetic resonance experiments for nano-scale ferromagnetic circuits.
We study the ac charge and -spin transport through an orbital of a magnetic molecule with spin precessing in a constant magnetic field. We assume that the source and drain contacts have time-dependent chemical potentials. We employ the Keldysh nonequilibrium Green's functions method to calculate the spin and charge currents to linear order in the time-dependent potentials. The molecular and electronic spins are coupled via exchange interaction. The time-dependent molecular spin drives inelastic transitions between the molecular quasienergy levels, resulting in a rich structure in the transport…
We present a theoretical analysis of current driven ferromagnetic resonance in a ferromagnet/normal-metal/ferromagnet tri-layer. This method of driving ferromagnetic resonance was recently realized experimentally by Tulapurkar et al. [Nature 438, 339 (2005)] and Sankey et al. [Phys. Rev. Lett. 96, 227601 (2006)]. The precessing magnetization rectifies the alternating current applied to drive the ferromagnetic resonance and leads to the generation of a dc voltage. Our analysis shows that a second mechanism to generate a dc voltage, rectification of spin currents emitted by the precessing magnet…
Spin pumping is the emission of a spin current by a magnetization dynamics while spin transfer stands for the excitation of magnetization by spin currents. Using Onsager's reciprocity relations we prove that spin pumping and spin-transfer torques are two fundamentally equivalent dynamic processes in magnetic structures with itinerant electrons. We review the theory of the coupled motion of the magnetization order parameter and electron for textured bulk ferromagnets (e.g. containing domain walls) and heterostructures (such as spin valves). We present first-principles calculations for the mater…
We report a theoretical study of the quantized spin pump in a traditional two-parameter quantum pump device that is based on the helical edge states of a quantum spin Hall insulator. By introducing two time-dependent magnetizations out of phase as the pumping parameters, we found that when the Fermi energy resides in the energy gap opened by magnetization, an integer number of charges or spins can be pumped out in a pumping cycle and ascribed to the possible topological interface state born in between the two pumping potentials. The quantized pump current can be fully spin-polarized, spin-unpo…
Here, we investigate spin Hall angle of Pt in Ni80Fe20/Pt bilayer system by using a broadband spin pumping and inverse spin Hall effect measurement. An out-of-plane excitation geometry with application of external magnetic field perpendicular to the charge current direction is utilized in order to suppress unwanted galvanomagnetic effects. Magnetization precession angle on ferromagnetic resonance for wide excitation frequency range (4-14 GHz) is estimated from the rectification voltage of anisotropic magnetoresistance (AMR) and a conventional method of using microwave power in a coplanar waveg…
Rectification of microwave oscillations of magnetization in a permalloy film is realized using planar Hall effect. Two different rectified signals are obtained: a signal from the linearly excited uniform magnetization precession at the frequency of the external pumping and a signal from the pairs of contra-propagating short-wavelength spin waves parametrically generated at a half of the pumping frequency. The second, most unusual, rectified signal is caused by the uniform component of the dynamic magnetization created due to the interference of the phase correlated pairs of parametric spin wav…
We study proximity effect in diffusive ferromagnet/normal-metal/superconductor junction with precessing magnetization of the ferromagnet. We find that the odd-frequency pairing induced in the normal metal is modified by spin pumping from the ferromagnet and hence can be tuned by changing the precessional frequency. At the frequency corresponding to twice the superconducting gap, the odd-frequency pairing is strongly enhanced. We find a crossover from the even- to the odd-frequency superconductivity in the normal metal by tuning the precessional frequency. This gives a clearcut signature of the…
We present a study of dynamical spin injection from a three-dimensional ferromagnet into two-dimensional single-layer graphene. Comparative ferromagnetic resonance (FMR) studies of ferromagnet/graphene strips buried underneath the central line of a coplanar waveguide show that the FMR linewidth broadening is the largest when the graphene layer protrudes laterally away from the ferromagnetic strip, indicating that the spin current is injected into the graphene areas away from the area directly underneath the ferromagnet being excited. Our results confirm that the observed damping is indeed a si…
We report a theory for the coherent and incoherent chiral pumping of spin waves into thin magnetic films through the dipolar coupling with a local magnetic transducer, such as a nanowire. The ferromagnetic resonance of the nanowire is broadened by the injection of unidirectional spin waves that generate a non-equilibrium magnetization in only half of the film. A temperature gradient between the local magnet and film leads to a unidirectional flow of incoherent magnons, i.e., a chiral spin Seebeck effect.
In metallic ferromagnets, the spin-transfer torque and spin-motive force are known to exhibit a reciprocal relationship. Recent experiments on ferromagnets with strong spin-orbit coupling have revealed a rich complexity in the interaction between itinerant charge carriers and magnetization, but a full understanding of this coupled dynamics is lacking. Here, we develop a general phenomenology of the two reciprocal processes of charge pumping by spin-motive forces and current-driven magnetization dynamics. The formalism is valid for spin-orbit coupling of any strength and presents a systematic s…
We would like to point out the blind spots of the approach combining the spin pumping theory proposed by Tserkovnyak et al. with the Landau-Lifshitz-Gilbert equation; this method has been widely used for interpreting vast experimental results. The essence of the spin pumping effect is the quantum fluctuation. Thus, localized spin degrees of freedom should be quantized, i.e. be treated as magnons not as classical variables. Consequently, the precessing ferromagnet can be regarded as a magnon battery. This point of view will be useful for further progress of spintronics.
In this study, current pumping by an external potential is studied on the basis of the Keldysh Green's function method, and a pumping formula written in terms of retarded and advanced Green's functions is obtained. It is shown that pumping is essentially driven by a change of particle distribution before and after an external perturbation. The formula is used to study the spin pumping effect in the case of strong sd exchange interaction, and the driving field is identified to be the spin gauge field. At the lowest order in the precession frequency of magnetization, the spin gauge field works a…
