Voltage induced magnetization dynamics of magnetic thin films is a valuable tool to study anisotropic fields, exchange couplings, magnetization damping and spin pumping mechanism. A particularly well established technique is the ferromagnetic resonance (FMR) generated by the coupling of microwave photons and magnetization eigenmodes in the GHz range. Here we review the basic concepts of the so-called acoustic ferromagnetic resonance technique (a-FMR) induced by the coupling of surface acoustic waves (SAW) and magnetization of thin films. Interestingly, additional to the benefits of the microwave excited FMR technique, the coupling between SAW and magnetization also offers fertile ground to study magnon-phonon and spin rotation couplings. We describe the in-plane magnetic field angle dependence of the a-FMR by measuring the absorption / transmission of SAW and the attenuation of SAW in the presence of rotational motion of the lattice, and show the consequent generation of spin current by acoustic spin pumping.
Recent experiments demonstrated generation of spin currents by ultrasound. We can understand this acoustically induced spin pumping in terms of the coupling between magnetization and lattice waves. Here we study the parametric excitation of magnetization by longitudinal acoustic waves and calculate the acoustic threshold power. The induced magnetization dynamics can be detected by the spin pumping into an adjacent normal metal that displays the inverse spin Hall effect.
We study transport in ferromagnetic-superconductor/normal-metal systems. It is shown that charge and spin currents are pumped from ferromagnetic superconductors into adjacent normal metals by adiabatic changes in the order parameters induced by external electromagnetic fields. Spin and charge pumping identify the symmetry of the superconducting order parameter, e.g., singlet pairing or triplet pairing with opposite or equal spin pairing. Consequences for ferromagnetic-resonance experiments are discussed.
The linear and nonlinear interactions between spin waves (magnons) and acoustic waves (phonons) in magnetostrictive materials provide an exciting opportunity for realizing novel microwave signal processing devices and spintronic circuits. Here we demonstrate the parametric pumping of spin waves by acoustic waves, the possibility of which has long been theoretically anticipated but never experimentally realized. Spin waves propagating in a thin film of yttrium iron garnet (YIG), a magnetostrictive ferrimagnet with low spin and acoustic wave damping, are pumped using an acoustic resonator driven…
Surface acoustic waves (SAWs) in the GHz frequency range can inject spin currents dynamically into adjacent nonmagnetic layers via spin pumping effect associated with ferromagnetic resonance. Here, we demonstrate an enhancement of acoustic ferromagnetic resonance and spin current generation by a pair of SAW reflector gratings, which form an acoustic analogue of the distributed Bragg reflector cavity. In the experiment, we confirmed 2.04 $\pm$ 0.02 times larger SAW power absorption in a device with cavity than in case of no acoustic cavity. We confirmed up to 2.96 $\pm$ 0.02 times larger spin c…
The spin waves and ferromagnetic resonance (FMR) contribution to the spin pumping signal is studied in the Ta/CoFeB interface under different excitation bias fields. Ferromagnetic resonance is excited utilizing a coplanar waveguide and a microwave generator. Using a narrow waveguide of about 3 μm, magnetostatic surface spin waves with large wavevector (k) of about 0.81 μm^-1 are excited. A large k value results in dissociation of spin waves and FMR frequencies according to the surface spin wave dispersion relation. Spin waves and FMR contribution to the spin pumping are calculated based on the…
Adiabatic pumping of electrons induced by surface acoustic waves (SAWs) in a ballistic quasi-1D quantum channel is considered using an exactly solvable tight-binding model for non-interacting electrons. The single-electron degrees of freedom, responsible for acoustoelectric current quantization, are related to the transmission resonances. We study the influence of experimentally controllable parameters (SAW power, gate voltage, source-drain bias, amplitude and phase of a secondary SAW beam) on the plateau-like structure of the acoustoelectric current. The results are consistent with existing e…
We present a realization of quantized charge pumping. A lateral quantum dot is defined by metallic split gates in a GaAs/AlGaAs heterostructure. A surface acoustic wave whose wavelength is twice the dot length is used to pump single electrons through the dot at a frequency f=3GHz. The pumped current shows a regular pattern of quantization at values I=nef over a range of gate voltage and wave amplitude settings. The observed values of n, the number of electrons transported per wave cycle, are determined by the number of electronic states in the quantum dot brought into resonance with the fermi …
Using a multilayer structure containing (cobalt detector layer)/(copper spacer)/(Permalloy source layer), we show experimentally how the non-reorientable spin-orbit torque generated by the Permalloy source layer (the component of spin-orbit torque that does not change when the Permalloy magnetization is rotated) can be measured using spin-torque ferromagnetic resonance (ST-FMR) with lineshape analysis. We find that dynamic spin pumping between the magnetic layers exerts torques on the magnetic layers as large or larger than the spin-orbit torques, so that if dynamic spin pumping is neglected t…
We investigate the spin-pumping-induced electric current on the surface of a three-dimensional topological insulator hybridized with a ferromagnet, namely, ferromagnetic topological insulator. In order to do this, we establish the microscopic formalism and construct the perturbation theory using a Keldysh Green's function approach. We analyze how this electric current is generated by an exchange interaction and an external ac magnetic field, which is the driving force of ferromagnetic resonance as well as the spin pumping. The mechanism is as follows. First, the ferromagnetic resonance is driv…
A general definition of the Spintronics concept of spin-pumping is proposed as generalized forces conjugated to the spin degrees of freedom in the framework of the theory of mesoscopic non-equilibrium thermodynamics. It is shown that at least three different kinds of spin-pumping forces and associated spin-currents can be defined in the most simple spintronics system (the Ferromagnetic/Non-Ferromagnetic metal interface). Furthermore, the generalized force associated to the ferromagnetic collective variable is also introduced in an equal footing, in order to describe the coexistence of the spin…
We study adiabatic pumping of electrons through quantum dots attached to ferromagnetic leads. Hereby we make use of a real-time diagrammatic technique in the adiabatic limit that takes into account strong Coulomb interaction in the dot. We analyze the degree of spin polarization of electrons pumped from a ferromagnet through the dot to a nonmagnetic lead (N-dot-F) as well as the dependence of the pumped charge on the relative leads' magnetization orientations for a spin-valve (F-dot-F) structure. For the former case, we find that, depending on the relative coupling strength to the leads, spin …
The features of phonon-magnon interconversion in acoustic resonator determine the efficiency of spin pumping from YIG into Pt that may be detected electrically through the inverse spin Hall effect (ISHE). Based on the methods developed in previous works for calculating resonator structures with a piezoelectric (ZnO) and a magnetoelastic layer in contact with the heavy metal (YIG/Pt), we present the results of numerical calculations of YIG film thickness influence on acoustically driven spin waves. We obtain some YIG film thickness regions with various behavior of dc ISHE voltage $U_{ISHE}$. At…
We investigate adiabatic quantum pumping of Dirac fermions on the surface of a strong 3D topological insulator. Two different geometries are studied in detail, a normal metal -- ferromagnetic -- normal metal (NFN) junction and a ferromagnetic -- normal metal -- ferromagnetic (FNF) junction. Using a scattering matrix approach, we first calculate the tunneling conductance and then the adiabatically pumped current using different pumping mechanisms for both types of junctions. We explain the oscillatory behavior of the conductance by studying the condition for resonant transmission in the junctio…
We determined the spin-transport properties of Pd and Pt thin films by measuring the increase in ferromagnetic resonance damping due to spin-pumping in ferromagnetic (FM)-nonferromagnetic metal (NM) multilayers with varying NM thicknesses. The increase in damping with NM thickness depends strongly on both the spin- and charge-transport properties of the NM, as modeled by diffusion equations that include both momentum- and spin-scattering parameters. We use the analytical solution to the spin-diffusion equations to obtain spin-diffusion lengths for Pt and Pd. By measuring the dependence of cond…
We describe electrical detection of spin pumping in metallic nanostructures. In the spin pumping effect, a precessing ferromagnet attached to a normal-metal acts as a pump of spin-polarized current, giving rise to a spin accumulation. The resulting spin accumulation induces a backflow of spin current into the ferromagnet and generates a dc voltage due to the spin dependent conductivities of the ferromagnet. The magnitude of such voltage is proportional to the spin-relaxation properties of the normal-metal. By using platinum as a contact material we observe, in agreement with theory, that the v…
Based on spin-dependent transport theory and thermodynamics, we develop a generalized theory of the Joule heating in the presence of a spin current. Along with the conventional Joule heating consisting of an electric current and electrochemical potential, it is found that the spin current and spin accumulation give an additional dissipation because the spin-dependent scatterings inside bulk and ferromagnetic/nonmagnetic interface lead to a change of entropy. The theory is applied to investigate the dissipation due to pure spin-current generated by spin pumping across a ferromagnetic/nonmagneti…
We investigated the dependence of the seed [Ta/Pt, Ta/Au] and capping [Pt/Ta, Au/Ta] layers on spin pumping effect in the ferromagnetic 3 nm thick Co thin film using ferromagnetic resonance spectroscopy. The data is fitted with Kittel equation to evaluate damping constant and g-factor. A strong dependence of seed and capping layers on spin pumping has been discussed. The value of damping constant {alpha} is found to be relatively large i.e. 0.0326 for the Ta{3}/Pt{3}/Co{3}/Pt{3}/Ta{3} {nm} multi-layer structure, while it is 0.0104 for Ta{3}/Co{3}/Ta{3} {nm}. Increase in {alpha} is observed due…
Spin pumping in nonmagnetic/ferromagnetic metal multilayers is studied both theoretically and experimentally. We show that the line widths of the ferromagnetic resonance (FMR) spectrum depend on the thickness of the ferromagnetic metal layers, which must not be in resonance with the oscillating magnetic field. We also show that the penetration depths of the transverse spin current in ferromagnetic metals can be determined by analyzing the line widths of their FMR spectra. The obtained penetration depths in NiFe, CoFe and CoFeB were 3.7 [nm], 2.5 [nm] and 12.0 [nm], respectively.
Spin pumping by ferromagnetic resonance is one of the most common technique to determine spin hall angles, Edelstein lengths or spin diffusion lengths of a large variety of materials. In recent years, rising concerns have appeared regarding the interpretation of these experiments, underlining that the signal could arise purely from thermoelectric effects, rather than from coherent spin pumping. Here, we propose a method to evaluate the presence or absence of thermal effects in spin pumping signals, by combining bolometry and spin pumping by ferromagnetic resonance measurements, and comparing t…
The magnetic behaviour of ultrathin ferromagnetic films deposited on substrates is strongly affected by the properties of the substrate. We investigate the spin pumping rate, interlayer exchange coupling and dynamic exchange coupling between ultrathin ferromagnetic films through palladium, a non-magnetic substrate that displays strong Stoner enhancement. We find that the interlayer exchange coupling, both in the static and dynamic versions, is qualitatively affected by the substrate's Stoner enhancement. For instance, the oscillatory behavior that is a hallmark property of the RKKY exchange co…
The magnon pumping effect in ferromagnetic insulators under an external time-dependent transverse magnetic field is theoretically studied. Generation of a magnon current is discussed by calculating the magnon source term in the spin continuity equation. This term represents the non-conservation of magnons arising from an applied transverse magnetic field. The magnon source term has a resonance structure as a function of the angular frequency of the transverse field, and this fact is useful to enhance the pumping effect.
We have demonstrated spin pumping from a paramagnetic state of an insulator La2NiMnO6 into a Pt film. Single-crystalline films of La2NiMnO6 which exhibit a ferromagnetic order at TC ~ 270 K were grown by pulsed laser deposition. The inverse spin Hall voltage induced by spin-current injection has been observed in the Pt layer not only in the ferromagnetic phase of La2NiMnO6 but also in a wide temperature range above TC. The efficient spin pumping in the paramagnetic phase is ascribable to ferromagnetic correlation, not to ferromagnetic order.
The relative contribution of spin pumping and spin rectification from the ferromagnetic resonance of CoFeB/non-magnetic bilayers was investigated as a function of non-magnetic electrode resistance. Samples with highly resistive electrodes of Ta or Ti exhibit a stronger spin rectification signal, which may result in over-(or under-)estimation of the spin Hall angle of the materials, while those with low resistive electrodes of Pt or Pd show the domination of the inverse spin Hall effect from spin pumping. By comparison with samples of single FM layer and an inverted structure, we provide a prop…
Quantized charge pumping is a robust adiabatic phenomenon uniquely existing in topologically nontrivial systems. Such topological pumping not only brings fundamental insights to the evolution of states under the protection of topology but also provides a vital approach for the study of higher-dimensional topological phases. In this work, we demonstrate topological pumping in an acoustic waveguide system by showing the successful pumping of topological boundary states (TBSs) across the bulk to the opposite edge. By exploring the finite-size induced mini-gap between two TBS bands, we unveil the …
We study spin pumping into an anisotropic Dirac electron system induced by microwave irradiation to an adjacent ferromagnetic insulator theoretically. We formulate the Gilbert damping enhancement due to the spin current flowing into the Dirac electron system using second-order perturbation with respect to the interfacial exchange coupling. As an illustration, we consider the anisotropic Dirac system realized in bismuth to show that the Gilbert damping varies according to the magnetization direction in the ferromagnetic insulator. Our results indicate that this setup can provide helpful informa…
We theoretically consider spin pumping in a junction between a ferromagnetic insulator (FI) and a two-dimensional electron gas (2DEG) in which the Rashba and Dresselhaus spin-orbit interactions coexist. Using second-order perturbation theory, we derive an increase in linewidth in the case of an interfacial exchange coupling in a ferromagnetic resonance (FMR) experiment. We clarify how the enhancement of Gilbert damping depends on the resonant frequency and spin orientation of the FI. We show that this setup of an FMR experiment can provide information on the spin texture of 2DEG at the Fermi s…
We measure electrically detected ferromagnetic resonance in microdevices patterned from ultra-thin Co/Pt bilayers. Spin pumping and rectification voltages are observed and distinguished via their angular dependence. The spin-pumping voltage shows an unexpected increase as the cobalt thickness is reduced below 2 nm. This enhancement allows more efficient conversion of spin to charge current and motivates a theory modelling the dependence of impurity scattering on surface roughness.
Laughlin pumping assisted by surface acoustic waves
International Center for Quantum Materials, Peking University（北京大学量子材料科学中心）；Department of Electrical Engineering, Princeton University（普林斯顿大学电气工程系）；Hefei National Laboratory（合肥国家实验室）；School of Physics and Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology（华中科技大学物理学院与武汉国家强磁场中心）
We study the magnetization dynamics in thin ferromagnetic films and small ferromagnetic particles in contact with paramagnetic conductors. A moving magnetization vector causes \textquotedblleft pumping\textquotedblright of spins into adjacent nonmagnetic layers. This spin transfer affects the magnetization dynamics similar to the Landau-Lifshitz-Gilbert phenomenology. The additional Gilbert damping is significant for small ferromagnets, when the nonmagnetic layers efficiently relax the injected spins, but the effect is reduced when a spin accumulation build-up in the normal metal opposes the s…
We investigate pure spin pumping in graphene by imposing a ferromagnet (F) with rotating magnetization on top of it. Using the generalized scattering approach for adiabatic spin pumping, we obtain the spin current pumped through magnetic graphene to a neighboring normal (N) region. The spin current can be easily controlled by gate voltages and under certain conditions, becomes sufficiently large to be measurable in current experimental setups. In fact it reaches a maximum value when one of the spins are completely filtered due to the vanishing density of states of the corresponding spin specie…
We study the spin current injected by spin pumping into single layer graphene and the two-dimensional electron gas (2DEG) with ferromagnetic contacts using scattering theory. The spin currents pumped into graphene are very distinct from that into the 2DEG since importantly affected by Klein tunneling.
Spin pumping by a moving magnetization gives rise to an electric voltage over a spin valve. Thermal fluctuations of the magnetization manifest themselves as increased thermal voltage noise with absorption lines at the ferromagnetic resonance frequency and/or zero frequency. The effect depends on the magnetization configuration and can be of the same order of magnitude as the Johnson-Nyquist thermal noise. Measuring colored voltage noise is an alternative to ferromagnetic resonance experiments for nano-scale ferromagnetic circuits.
We develop a method for universally resolving the important issue of separating spin pumping (SP) from spin rectification (SR) signals in bilayer spintronics devices. This method is based on the characteristic distinction of SP and SR, as revealed in their different angular and field symmetries. It applies generally for analyzing charge voltages in bilayers induced by the ferromagnetic resonance (FMR), independent of FMR line shape. Hence, it solves the outstanding problem that device specific microwave properties restrict the universal quantification of the spin Hall angle in bilayer devices …
We report on the experimental observation of excitation and detection of parametric spin waves and spin currents in the bulk acoustic wave resonator. The hybrid resonator consists of ZnO piezoelectric film, yttrium iron garnet (YIG) films on gallium gadolinium garnet substrate, and a heavy metal Pt layer. Shear bulk acoustic waves are electrically excited in the ZnO layer due to piezoeffect at the resonant frequencies of the resonator. The magnetoelastic interaction in the YIG film emerges magnons (spin waves) excitation by acoustic waves either on resonator's eigenfrequencies or the half-valu…
We calculate adiabatic charge and spin pumping through a serial double quantum dot with strong Coulomb interaction, coupled to normal metal or ferromagnetic contacts. We use a real-time diagrammatic approach in the regime of weak coupling to the reservoirs. In the case of weak interdot tunnel coupling we investigate the influence of tunnel-induced renormalization effects due to charge fluctuations on the pumped charge and spin. We show that tunneling through thermally excited states can play an important role in the strong interdot coupling regime. In particular, for ferromagnetic contacts, bo…
We derive boundary conditions at the interfaces of magnetoelastic heterostructures under ferromagnetic resonance for arbitrary magnetization directions and interface shapes. We apply our formalism to magnet$\vert$nonmagnet bilayers and magnetic grains embedded in a nonmagnetic thin film, revealing a nontrivial magnetization angle dependence of acoustic phonon pumping.
We theoretically investigate spin transport at the interface between the ferromagnetic insulator(FI) and a superconductor(SC). Considering a simple FI-SC interface model, we derive formulas for the spin current and spin-current noise induced by microwave irradiation (spin pumping) or the temperature gradient (the spin Seebeck effect). We show how the superconducting coherence factor affects the temperature dependence of the spin current. We also calculate the spin-current noise in thermal equilibrium and in non-equilibrium states induced by the spin pumping, and compare them quantitatively for…
In the normal metal/ferromagnetic insulator bilayer (such as Pt/Y$_{3}$Fe$_{5}$O$_{12}$) and the normal metal/ferromagnetic metal/oxide trilayer (such as Pt/Co/AlO$_{x}$) where spin injection and ejection are achieved by the spin Hall effect in the normal metal, we propose a minimal model based on quantum tunneling of spins to explain the spin-transfer torque and spin pumping caused by the spin Hall effect. The ratio of their damping-like to field-like component depends on the tunneling wave function that is strongly influenced by generic material properties such as interface $s-d$ coupling, i…
Ultrafast optical pumping of spatially nonuniform magnetic textures is known to induce far-from-equilibrium spin transport effects. Here, we use ultrafast x-ray diffraction with unprecedented dynamic range to study the laser-induced dynamics of labyrinth domain networks in ferromagnetic CoFe/Ni multilayers. We detected azimuthally isotropic, odd order, magnetic diffraction rings up to 5th order. The amplitudes of all three diffraction rings quench to different degrees within 1.6 ps. In addition, all three of the detected diffraction rings both broaden by 15% and radially contract by 6% during …
A Thouless pump can be regarded as a dynamical version of the integer quantum Hall effect. In a finite-size configuration, such topological pump displays edge modes that emerge dynamically from one bulk-band and dive into the opposite bulk-band, an effect that can be reproduced with both quantum and classical systems. Here, we report the first un-assisted dynamic energy transfer across a metamaterial, via pumping of such topological edge modes. The system is a topological aperiodic acoustic crystal, with a phason that can be fast and periodically driven in adiabatic cycles. When one edge of th…
"Pumping" of phonons by a dynamic magnetization promises to extend the range and functionality of magnonic devices. We explore the impact of phonon pumping on room-temperature ferromagnetic resonance (FMR) spectra of bilayers of thin yttrium iron garnet (YIG) films on thick gadolinium gallium garnet substrates over a wide frequency range. At low frequencies the Kittel mode hybridizes coherently with standing ultrasound waves of a bulk acoustic resonator to form magnon polarons that induce rapid oscillations of the magnetic susceptibility, as reported before. At higher frequencies, the phonon r…
We investigate quantum charge and spin pumping in armchair graphene nanoribbons under a single ac gate voltage connected with nonmagnetic/ferromagnetic leads via the nonequilibrium Green's function method. In the case of nonmagnetic leads, where only part of the nanoribbon is subject to an ac gate voltage to break the left-right spatial symmetry, we discover that peaks of the charge pumping current appear at the Fermi energies around the subband edges in the ac-field-free region of the nanoribbon. In the case of ferromagnetic leads with the lead magnetizations being antiparallel to break the l…
Controlled spin transport in magnetic stacks is required to realize pure spin current-driven logic and memory devices. The control over the generation and detection of the pure spin current is achieved by tuning the spin to charge conversion efficiency of the heavy metal interfacing with ferromagnets. Here, we demonstrate the direct tunability of spin angular momentum transfer and thereby spin pumping, in CoFeB/Pt stack, with interfacial magnetic anisotropy. The ultra-low thickness of CoFeB thin film tilts the magnetic easy axis from in-plane to out-of-plane due to surface anisotropy. The Ferr…
The richness in both the dispersion and energy of antiferromagnetic magnons has spurred the magnetism community to consider antiferromagnets for future spintronic/magnonic applications. However, the excitation and control of antiferromagnetic magnons remains challenging, especially when compared to ferromagnetic counterparts. A middle ground is found with synthetic antiferromagnet metamaterials, where acoustic and optical magnons exist at GHz frequencies. In these materials, the magnon energy spectrum can be tuned by static symmetry-breaking external fields or dipolar interactions hybridizing …
We measured spin transport in nonferromagnetic (NM) metallic multilayers from the contribution to damping due to spin pumping from a ferromagnetic Co90Fe10 thin film. The multilayer stack consisted of NM1/NM2/Co90Fe10(2 nm)/NM2/NM3 with varying NM materials and thicknesses. Using conventional theory for one dimensional diffusive spin transport in metals, we show that the effective damping due to spin pumping can be strongly affected by the spin transport properties of each NM in the multilayer, which permits the use of damping measurements to accurately determine the spin transport properties …
Spin pumping is a recently established means for generating a pure spin current, whereby spins are pumped from a magnet into the adjacent target material under the ferromagnetic resonance condition. We theoretically investigate the spin pumping from an insulating ferromagnet into spin glass materials. Combining a dynamic theory of spin glasses with the linear-response formulation of the spin pumping, we calculate temperature dependence of the spin pumping near the spin glass transition. The analysis predicts that a characteristic peak appears in the spin pumping signal, reflecting that the spi…
By combining Floquet theory with Green's function formalism, we present non-adiabatic quantum spin and charge pumping through a zigzag ferromagnetic graphene nanoribbon including a double-barriers structure driven weakly by two local $ac$ gate voltages operating with a phase-lag. Over a wide range of Fermi energies, interesting quantum pumping such as i) pure spin pumping with zero net charge pumping, ii) pure charge pumping and iii) fully spin polarized pumping can be achieved by tuning and manipulating driving frequency in the non-adiabatic regime. Spin polarized pumping which is measurable …
We study spin and charge currents pumped by precessing magnetization of a single ferromagnetic layer within F|I|N or F|I|F (F-ferromagnet; I-insulator; N-normal-metal) multilayers of nanoscale thickness attached to two normal metal electrodes with no applied bias voltage between them. Both simple one-dimensional model, consisting of a single precessing spin and a potential barrier as the "sample," and realistic three-dimensional devices are investigated. In the rotating reference frame, where the magnetization appears to be static, these junctions are mapped onto a four-terminal dc circuit who…
We show that the magnetization of a thin ferromagnetic (Ga,Mn)As layer can be modulated by picosecond acoustic pulses. In this approach a picosecond strain pulse injected into the structure induces a tilt of the magnetization vector M, followed by the precession of M around its equilibrium orientation. This effect can be understood in terms of changes in magneto-crystalline anisotropy induced by the pulse. A model where only one anisotropy constant is affected by the strain pulse provides a good description of the observed time-dependent response.
Probing Interfacial Spin Dynamics and Temperature Dependent Asymmetry in Spin Pumping Across Ni80Fe20/Cu/Cr1.12Te2 Interfaces
Department of Physics, Indian Institute of Technology Kanpur（印度坎普尔理工学院物理系）；Natural Sciences and Science Education, National Institute of Education, Nanyang Technological University（南洋理工大学国立教育学院自然科学与科学教育）
