We report a theory for the coherent and incoherent chiral pumping of spin waves into thin magnetic films through the dipolar coupling with a local magnetic transducer, such as a nanowire. The ferromagnetic resonance of the nanowire is broadened by the injection of unidirectional spin waves that generate a non-equilibrium magnetization in only half of the film. A temperature gradient between the local magnet and film leads to a unidirectional flow of incoherent magnons, i.e., a chiral spin Seebeck effect.
We investigate adiabatic quantum pumping of chiral Majorana states in a system composed of two Mach--Zehnder type interferometers coupled via a quantum point contact. The pumped current is generated by periodic modulation of the phases accumulated by traveling around each interferometer. Using scattering matrix formalism we show that the pumped current reveals a definite signature of the chiral nature of the Majorana states involved in transport in this geometry. Furthermore, by tuning the coupling between the two interferometers the pump can operate in a regime where finite pumped current and…
Chiral spin pumping is the generation of a unidirectional spin current in half of ferromagnetic films or conductors by dynamic dipolar stray fields from close-by nanomagnets. We formulate a general theory of long-range chiral interactions between magnets mediated by unidirectional traveling waves, e.g., spin waves in a magnetic film or microwaves in a waveguide. The traveling waves emitted by an excited magnet can be perfectly trapped by a second, initially passive, magnet by a dynamical interference effect. When both magnets are excited by a uniform microwave, the chiral interaction between t…
Studying many-body versions of Landau-Zener-like problems of non-interacting electrons in the Slater formalism for several $k \cdot p$ models representing Weyl and Dirac semimetals, we systematically include non-adiabatic corrections to a quantum limit of chiral charge pumping in these models. In this paper, we show that relative homotopy invariant [Sun et al., Phys. Rev. Lett. 121, 106402 (2018)] and Euler class invariant [Bouhon et al., Nat. Phys. 16, 1137 (2020)] non-trivially manifest in the non-adiabatic corrections to the quantum limit of chiral charge pumping. These corrections could af…
We demonstrate that a sizable chiral charge pumping can be achieved at room temperature in graphene/Yttrium Iron Garnet (YIG) bilayer systems. The effect, which cannot be attributed to the ordinary spin pumping, reveals itself in the creation of a dc electric field/voltage in graphene as a response to the dynamic magnetic excitations (spin waves) in an adjacent out-of-plane magnetized YIG film. We show that the induced voltage changes its sign when the orientation of the static magnetization is reversed, clearly indicating the broken spatial inversion symmetry in the studied system. The streng…
We extend the theory of dipole moments in crystalline insulators to higher multipole moments. In this paper, we expand in great detail the theory presented in Ref. 1, and extend it to cover associated topological pumping phenomena, and a novel class of 3D insulator with chiral hinge states. In quantum-mechanical crystalline insulators, higher multipole bulk moments manifest themselves by the presence of boundary-localized moments of lower dimension, in exact correspondence with the electromagnetic theory of classical continuous dielectrics. In the presence of certain symmetries, these moments …
We investigate charge pumping in ferromagnet/triplet superconductor junctions where the magnetization of the ferromagnet is inhomogeneous and dynamical. It is shown that charge current is pumped due to the coupling of the localized spin with triplet vector spin chirality, vector spin chirality formed by the triplet vector of Cooper pairing. Physical mechanism of the charge pumping is also discussed.
Solids with topologically robust electronic states exhibit unusual electronic and optical transport properties that do not exist in other materials. A particularly interesting example is chiral charge pumping, the so-called chiral anomaly, in recently discovered topological Weyl semimetals, where simultaneous application of parallel DC electric and magnetic fields creates an imbalance in the number of carriers of opposite topological charge (chirality). Here, using time-resolved terahertz measurements on the Weyl semimetal TaAs in a magnetic field, we optically interrogate the chiral anomaly b…
The angular momentum of evanescent light fields has been studied in nano-optics and plasmonics, but not in the microwave regime. Here we predict non-contact pumping of electron spin currents in conductors by the evanescent stray fields of excited magnetic nanostructures. The coherent transfer of the photon to the electron spin is proportional to the $g$-factor, which is large in narrow-gap semiconductors and surface states of topological insulators. The spin pumping current is chiral when the spin susceptibility displays singularities that indicate collective states. However, 1D systems with l…
Spin pumping is a recently established means for generating a pure spin current, whereby spins are pumped from a magnet into the adjacent target material under the ferromagnetic resonance condition. We theoretically investigate the spin pumping from an insulating ferromagnet into spin glass materials. Combining a dynamic theory of spin glasses with the linear-response formulation of the spin pumping, we calculate temperature dependence of the spin pumping near the spin glass transition. The analysis predicts that a characteristic peak appears in the spin pumping signal, reflecting that the spi…
By combining Floquet theory with Green's function formalism, we present non-adiabatic quantum spin and charge pumping through a zigzag ferromagnetic graphene nanoribbon including a double-barriers structure driven weakly by two local $ac$ gate voltages operating with a phase-lag. Over a wide range of Fermi energies, interesting quantum pumping such as i) pure spin pumping with zero net charge pumping, ii) pure charge pumping and iii) fully spin polarized pumping can be achieved by tuning and manipulating driving frequency in the non-adiabatic regime. Spin polarized pumping which is measurable …
We study resonant all-electric adiabatic spin pumping through a quantum dot with two nearby levels by using a Fermi liquid approach in the strongly interacting regime, combined with a projective numerical renormalization group (NRG) theory. Due to spin-orbit coupling, a strong spin pumping resonance emerges at every charging transition, which allows for the transfer of a spin $~ \hbar/2$ through the device in a single pumping cycle. Depending on the precise geometry of the device, controlled pure spin pumping is also possible.
We propose schemes for generating spin currents into a semiconductor by adiabatic or non-adiabatic pumping of electrons through interacting quantum dots. The appeal of such schemes lies in the possibility to tune the pumping characteristics via gate voltages that control the properties of the quantum dot. The calculations are based on a systematic perturbation expansion in the tunnel-coupling strength and the pumping frequency, expressed within a diagrammatic real-time technique. Special focus is put on the possibility of pure spin pumping, i.e., of pumping spin currents without charge current…
Based on the Floquet scattering theory, we analytically investigate the topological spin pumping for an exactly solvable model. Floquet spin Chern numbers are introduced to characterize the periodically time-dependent system. The topological spin pumping remains robust both in the presence and in the absence of the time-reversal symmetry, as long as the pumping frequency is smaller than the band gap, where the electron transport involves only the Floquet evanescent modes in the pump. For the pumping frequency greater than the band gap, where the propagating modes in the pump participate in the…
The spin-pumping mechanism is probed through a tunnelling MgO interlayer in Fe/Pt bilayers. We show by ferromagnetic resonance technique and spin-pumping experiments that spin currents can tunnel through the MgO interlayer for thickness up to 2~{nm} and can produce significant voltages in the Pt layer. The electrical detection of spin-pumping furthermore reveals the critical role of rectification and shunting effects on the generated voltages. The non zero spin current transport through a few monolayers of an insulating interlayer might initiate further studies on the role of very thin oxides …
We present a prescription for generating pure spin current or spin selective current, based on adiabatic quantum pumping in a tight-binding model of a one dimensional conductor. A formula for the instantaneous pumped current is derived without introducing the scattering matrix. Our calculations indicate that some pumping cycles produce the maximum value 2 of pumped spin while others reverse the direction of current as a result of small alterations of the pumping cycle. We find pumping cycles which produce essentially any ratio of spin current to charge current.
We have proposed a method to synchronize multiple spin-transfer torque oscillators based on spin pumping, inverse spin Hall, and spin Hall effects. The proposed oscillator system consists of a series of nano-magnets in junction with a normal metal with high spin-orbit coupling, and an accumulative feedback loop. We conduct simulations to demonstrate the effect of modulated charge currents in the normal metal due to spin pumping from each nano-magnet. We show that the interplay between the spin Hall effect and inverse spin Hall effect results in synchronization of the nano-magnets.
Recent experiments demonstrated generation of spin currents by ultrasound. We can understand this acoustically induced spin pumping in terms of the coupling between magnetization and lattice waves. Here we study the parametric excitation of magnetization by longitudinal acoustic waves and calculate the acoustic threshold power. The induced magnetization dynamics can be detected by the spin pumping into an adjacent normal metal that displays the inverse spin Hall effect.
We propose an experimental scheme to realize adiabatic topological spin and valley pumping by using silicene subject to an in-plane $ac$ electric field with amplitude $E_{y}$ and a vertical electric field consisting of an electrostatic component and an $ac$ component with amplitudes $E_{z}^{0}$ and $E_{z}^{1}$. By tuning $E_{z}^{0}$ and $E_{z}^{1}$, topological valley pumping or spin-valley pumping can be achieved. The noisefree valley and spin currents generated could be useful in valleytronic and spintronic applications. This work demonstrates that bulk topological spin or valley pumping is …
High spin to charge conversion efficiency is the requirement for the spintronics devices which is governed by spin pumping and inverse spin Hall effect (ISHE). In last one decade, ISHE and spin pumping are heavily investigated in ferromagnet/ heavy metal (HM) heterostructures. Recently antiferromagnetic (AFM) materials are found to be good replacement of HMs because AFMs exhibit terahertz spin dynamics, high spin-orbit coupling, and absence of stray field. In this context we have performed the ISHE in CoFeB/ IrMn heterostructures. Spin pumping study is carried out for $Co_{40}Fe_{40}B_{20} (12…
We experimentally investigate spin-orbit torques and spin pumping in NiFe/Pt bilayers with direct and interrupted interfaces. The damping-like and field-like torques are simultaneously measured with spin-torque ferromagnetic resonance tuned by a dc bias current, whereas spin pumping is measured electrically through the inverse spin Hall effect using a microwave cavity. Insertion of an atomically thin Cu dusting layer at the interface reduces the damping-like torque, field-like torque, and spin pumping by nearly the same factor of ~1.4. This finding confirms that the observed spin-orbit torques…
We investigate parametric pumping of a spin-polarized current through a nearly-closed quantum dot in a perpendicular magnetic field. Pumping is achieved by tuning the tunnel couplings to the left and right lead - thereby operating the quantum dot as a turnstile - and changing either the magnetic field or a gate-voltage. We analyze the quantum dynamics of a pumping cycle and the limiting time scales for operating the quantum dot turnstile as a pure spin pump. The proposed device can be used as a fully controllable double-sided and bipolar spin filter and to inject spins "on demand".
We study the spin current injected by spin pumping into single layer graphene and the two-dimensional electron gas (2DEG) with ferromagnetic contacts using scattering theory. The spin currents pumped into graphene are very distinct from that into the 2DEG since importantly affected by Klein tunneling.
Chiral anomaly, a non-conservation of chiral charge pumped by the topological nontrivial gauge fields, has been predicted to exist in Weyl semimetals. However, until now, the experimental signature of this effect exclusively relies on the observation of negative longitudinal magnetoresistance at low temperatures. Here, we report the field-modulated chiral charge pumping process and valley diffusion in Cd3As2. Apart from the conventional negative magnetoresistance, we observe an unusual nonlocal response with negative field dependence up to room temperature, originating from the diffusion of va…
In this study, current pumping by an external potential is studied on the basis of the Keldysh Green's function method, and a pumping formula written in terms of retarded and advanced Green's functions is obtained. It is shown that pumping is essentially driven by a change of particle distribution before and after an external perturbation. The formula is used to study the spin pumping effect in the case of strong sd exchange interaction, and the driving field is identified to be the spin gauge field. At the lowest order in the precession frequency of magnetization, the spin gauge field works a…
We investigate an adiabatic spin pumping through a quantum dot with a single orbital energy level under the Zeeman effect. Electron pumping is produced by two periodic time dependent parameters, a magnetic field and a difference of the dot-lead coupling between the left and right barriers of the dot. The maximum charge transfer per cycle is found to be $e$, the unit charge in the absence of a localized moment in the dot. Pumped charge and spin are different, and spin pumping is possible without charge pumping in a certain situation. They are tunable by changing the minimum and maximum value of…
The combination of parametric pumping and spin-transfer torque is a powerful approach that enables high-level control over magnetic excitations in thin-film ferromagnets. The excitation parameters, such as pumping power and external field strength, affect the instabilities of individual magnon modes. We theoretically explore how the simultaneous effects of parametric pumping and spin transfer torque influence these magnetic instabilities in a thin-film ferromagnet. Within the Landau-Lifshitz-Gilbert framework, we perform micromagnetic simulations of magnon excitations in yttrium iron garnet by…
Based on spin-dependent transport theory and thermodynamics, we develop a generalized theory of the Joule heating in the presence of a spin current. Along with the conventional Joule heating consisting of an electric current and electrochemical potential, it is found that the spin current and spin accumulation give an additional dissipation because the spin-dependent scatterings inside bulk and ferromagnetic/nonmagnetic interface lead to a change of entropy. The theory is applied to investigate the dissipation due to pure spin-current generated by spin pumping across a ferromagnetic/nonmagneti…
Precessing magnetization in a thin film magnetic insulator pumps spins into adjacent metals; however, this phenomenon is not quantitatively understood. We present a theory for the dependence of spin-pumping on the transverse mode number and in-plane wave vector. For long-wavelength spin waves, the enhanced Gilbert damping for the transverse mode volume waves is twice that of the macrospin mode, and for surface modes, the enhancement can be ten or more times stronger. Spin-pumping is negligible for short-wavelength exchange spin waves. We corroborate our analytical theory with numerical calcula…
A general definition of the Spintronics concept of spin-pumping is proposed as generalized forces conjugated to the spin degrees of freedom in the framework of the theory of mesoscopic non-equilibrium thermodynamics. It is shown that at least three different kinds of spin-pumping forces and associated spin-currents can be defined in the most simple spintronics system (the Ferromagnetic/Non-Ferromagnetic metal interface). Furthermore, the generalized force associated to the ferromagnetic collective variable is also introduced in an equal footing, in order to describe the coexistence of the spin…
Generally the adiabatic quantum pumping phenomenon can be interpreted by the surface integral of the Berry curvature inside the cyclic loop. Spin angular momentum flow without charge current can be pumped out by magnetization precession in ferromagnet-based structures. When an electron is scattered by a helimagnet, spin-dependent diffraction occurs due to the spatial modulation of the spiral. In this work, we consider the charge and spin flow driven by magnetization precession in normal-metal/multiferroic-helimagnet/ferromagnet heterostructures. The pumping behavior is governed by the diffract…
Spin currents can be obtained through adiabatic pumping by means of electrical gating only. This is possible by making use of the tunability of the Rashba spin-orbit coupling in semiconductor heterostructures. We demonstrate the principles of this effect by considering a single-channel wire with a constriction. We also consider realistic structures, consisting of several open channels where subband spin-mixing and disorder are present, and we confirm our predictions. Two different ways to detect the spin-pumping effect, either using ferromagnetic leads or applying a magnetic field, are discuss…
The review chapter starts by a pedagogical introduction to the general concept of the scattering theory: from the fundamental wave-function picture to the second-quantization language, with the aim to clear possible ambiguity in conventional textbooks. Recent progress in applying the method to current fluctuations and oscillating-parameter driven quantum pumping processes is presented with inclusion of contributions by Büttiker, Brouwer, Moskalets, Zhu, etc. In particular, the spin-orbit-coupling affected shot noise can be dealt with by taking into account the spin-dependent scattering process…
The adiabatic topological pumping is proposed by periodically modulating a semiconductor nanowire double-quantum-dot chain. We demonstrate that the quantized charge transport can be achieved by a nontrivial modulation of the quantum-dot well and barrier potentials. When the quantum-dot well potential is replaced by a time-dependent staggered magnetic field, the topological spin pumping can be realized by periodically modulating the barrier potentials and magnetic field. We also demonstrate that in the presence of Rashba spin-orbit interaction, the double-quantum-dot chain can be used to implem…
We study the adiabatic quantum pumping and quantum size effects of spin-torque in a magnetic tunnel junction within a scattering matrix approach. Quantum size effects are predicted in the presence of a dc bias as a function of the thickness of the normal metal layer inserted between two magnetic layers and of the fixed magnetic layer. In the presence of ac voltages, the results for the spin-torque show a peculiar magnification effect and advantages of spin-torque pumping in actual devices are also discussed.
We contend that Microwave Spin Pumping was first predicted and observed - albeit using a different and more sensitive detection mechanism than Inverse Spin Hall Effect - in the 1950's. This discovery was the founding step in the widely used analytical tool that is now known as Dynamic Nuclear Polarisation. Recognising this hitherto unsung connection between 20th Century Magnetic Resonance and 21st Century Spintronics not only helps to explain and unify contemporary metallic spin pumping observations: it is also the key to unlocking the immense and very sophisticated toolbox of Magnetic Resonan…
We study transport in ferromagnetic-superconductor/normal-metal systems. It is shown that charge and spin currents are pumped from ferromagnetic superconductors into adjacent normal metals by adiabatic changes in the order parameters induced by external electromagnetic fields. Spin and charge pumping identify the symmetry of the superconducting order parameter, e.g., singlet pairing or triplet pairing with opposite or equal spin pairing. Consequences for ferromagnetic-resonance experiments are discussed.
We theoretically investigate the fluctuation of a pure spin current induced by the spin Seebeck effect and spin pumping in a normal metal (NM)/ferromagnet (FM) bilayer system. Starting with a simple FI--NM interface model with both spin-conserving and spin-non-conserving processes, we derive general expressions of the spin current and the spin-current noise at the interface within second-order perturbation of the FI--NM coupling strength, and estimate them for an yttrium iron garnet (YIG) --platinum interface. We show that the spin-current noise can be used to determine the effective spin carr…
The spin waves and ferromagnetic resonance (FMR) contribution to the spin pumping signal is studied in the Ta/CoFeB interface under different excitation bias fields. Ferromagnetic resonance is excited utilizing a coplanar waveguide and a microwave generator. Using a narrow waveguide of about 3 μm, magnetostatic surface spin waves with large wavevector (k) of about 0.81 μm^-1 are excited. A large k value results in dissociation of spin waves and FMR frequencies according to the surface spin wave dispersion relation. Spin waves and FMR contribution to the spin pumping are calculated based on the…
The linear and nonlinear interactions between spin waves (magnons) and acoustic waves (phonons) in magnetostrictive materials provide an exciting opportunity for realizing novel microwave signal processing devices and spintronic circuits. Here we demonstrate the parametric pumping of spin waves by acoustic waves, the possibility of which has long been theoretically anticipated but never experimentally realized. Spin waves propagating in a thin film of yttrium iron garnet (YIG), a magnetostrictive ferrimagnet with low spin and acoustic wave damping, are pumped using an acoustic resonator driven…
Over the last two decades organic spintronics has developed into a striving field with exciting reports of long spin diffusion lengths and spin relaxation times in organic semiconductors (OSCs). Easily processed and inexpensive, OSCs are considered a potential alternative to inorganic materials for use in spintronic applications. Spin currents have been detected in a wide range of materials, however, there is still uncertainty over the origin of the signals. Recently, we explored spin transport through an organic semiconductor with lateral spin injection and detection architectures, where the …
The linear band crossings of 3D Dirac and Weyl semimetals are characterized by a charge chirality, the parallel or anti-parallel locking of electron spin to its momentum. Such materials are believed to exhibit a ${\bf E} \cdot {\bf B}$ chiral magnetic effect that is associated with the near conservation of chiral charge. Here, we use magneto-terahertz spectroscopy to study epitaxial Cd$_3$As$_2$ films and extract their conductivities $σ(ω)$ as a function of ${\bf E} \cdot {\bf B}$. As field is applied, we observe a remarkably sharp Drude response that rises out of the broader background. Its a…
A highly asymmetric dynamic nuclear spin pumping is observed in a single self assembled InGaAs quantum dot subject to resonant optical pumping of the neutral exciton transition leading to a large maximum polarization of 54%. This dynamic nuclear polarization is found to be much stronger following pumping of the higher energy Zeeman state. Time-resolved measurements allow us to directly monitor the buildup of the nuclear spin polarization in real time and to quantitatively study the dynamics of the process. A strong dependence of the observed dynamic nuclear polarization on the applied magnetic…
Magnetic thin films at ferromagnetic resonance (FMR) leak angular momentum, which may be absorbed by adjacent layers. This phenomenon, known as spin pumping, is manifested by an increase in the resonance linewidth ($ΔH$), and the closely related Gilbert damping. Another effect of this transfer of spin currents is a dynamical and long-range coupling that can drive two magnetic layers into a collective precession when their FMR frequencies coincide. A collective behavior is also found in magnetic trilayers with interlayer exchange coupling (IEC). In this study we investigate the interplay betwee…
Circuit theory has been tremendously successful in translating physical equations into circuit elements in organized form for further analysis and proposing creative designs for applications. With the advent of new materials and phenomena in the field of spintronics and nanomagnetics, it is imperative to construct the spin circuit representations for different materials and phenomena. Spin pumping is a phenomenon by which a pure spin current can be injected into the adjacent layers. If the adjacent layer is a material with a high spin orbit coupling, a considerable amount of charge voltage can…
The dc voltage obtained from the inverse spin Hall effect (iSHE) due to spin pumping in ferromagnet/normal-metal (NM) bilayers can be unintentionally superimposed with magnetoresistive rectification of ac charge currents in the ferromagnetic layer. We introduce a geometry in which these spurious rectification voltages vanish while the iSHE voltage is maximized. In this geometry, a quantitative study of the dc iSHE is performed in a broad frequency range for Permalloy/NM multilayers with NM={Pt, Ta, Cu/Au, Cu/Pt}. The experimentally recorded voltages can be fully ascribed to the iSHE due to spi…
We propose a four-terminal device designed to manipulate by all electrical means the spin of a magnetic adatom positioned at the edge of a quantum spin Hall insulator. We show that an electrical gate, able to tune the interface resistance between a quantum spin Hall insulator and the source and drain electrodes, can switch the device between two regimes: one where the system exhibits spin pumping and the other where the adatom remains in its ground state. This demonstrates an all-electrical route to control single spins by exploiting helical edge states of topological materials.
The polarization of the spin current pumped by a precessing ferromagnet into an adjacent normal metal has a constant component parallel to the precession axis and a rotating one normal to the magnetization. The former component is now routinely detected in the form of a DC voltage induced by the inverse spin Hall effect (ISHE). Here we compute AC-ISHE voltages much larger than the DC signals for various material combinations and discuss optimal conditions to observe the effect. Including the backflow of spins is essential for distilling parameters such as the spin Hall angle from ISHE-detected…
Using a multilayer structure containing (cobalt detector layer)/(copper spacer)/(Permalloy source layer), we show experimentally how the non-reorientable spin-orbit torque generated by the Permalloy source layer (the component of spin-orbit torque that does not change when the Permalloy magnetization is rotated) can be measured using spin-torque ferromagnetic resonance (ST-FMR) with lineshape analysis. We find that dynamic spin pumping between the magnetic layers exerts torques on the magnetic layers as large or larger than the spin-orbit torques, so that if dynamic spin pumping is neglected t…
Spin transfer torque and spin pumping are central reciprocal phenomena in spintronics. These phenomena occur in hybrid systems of normal metals and magnets. Spin transfer is the conversion of spin currents in metals to a torque on the magnetization of magnets. Spin pumping is the emission of spin currents from precessing magnets. Here, we demonstrate a general way to understand these effects within a quantum out-of-equilibrium path-integral model. Our results agree with known expressions for spin transfer and spin pumping in terms of transverse (mixing) conductances when there are no fluctuati…
