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arXiv 0901.3810cond-mat.supr-con
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Ba_2Ca_3Cu_4O_8(F_ yO_{1-y})_2(T_c=55-102 K)的反铁磁相变:Cu-和F-NMR研究

Antiferromagnetic phase transition in four-layered high-T_c superconductors Ba_2Ca_3Cu_4O_8(F_yO_{1-y})_2 with T_c=55-102 K: Cu- and F-NMR studies

S. Shimizu, H. Mukuda, Y. Kitaoka, H. Kito, Y. Kodama, P. M. Shirage, A. Iyo

摘要:

本文报道了用Cu-和F-NMR方法研究顶端含氟的四层结构Ba_2Ca_3Cu_4O_8(F_ yO_{1-y})_2超导体的磁特性。氧取代氟使载流子密度(Nh)和T_c从55 K提高到102 K。NMR测量结果表明,在Nh = 0.15之前,存在与超导性均匀共存的反铁磁有序,这比五层化合物的量子临界点Nh = 0.17要小一些。四层化合物的QCP向载流子密度较低的区域移动的事实保证了CuO_2层数的减少使层间磁耦合减弱。

英文摘要:

We report on magnetic characteristics in four-layered high-T_c superconductors Ba_2Ca_3Cu_4O_8(F_yO_{1-y})_2 with apical fluorine through Cu- and F-NMR measurements. The substitution of oxygen for fluorine at the apical site increases the carrier density (N_h) and T_c from 55 K up to 102 K. The NMR measurements reveal that antiferromagnetic order, which can uniformly coexist with superconductivity, exists up to N_h = 0.15, which is somewhat smaller than N_h = 0.17 being the quantum critical point (QCP) for five-layered compounds. The fact that the QCP for the four-layered compounds moves to a region of lower carrier density than for five-layered ones ensures that the decrease in the number of CuO_2 layers makes an interlayer magnetic coupling weaker.

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