NMR揭示的CaK(Fe1-xNix)4As 4中Hedgehog自旋涡旋晶体反铁磁量子临界性
Hedgehog Spin-vortex Crystal Antiferromagnetic Quantum Criticality in CaK(Fe1-xNix)4As4 Revealed by NMR
摘要:
在大多数铁基超导体(SC)中观察到两种有序态,即反铁磁性和向列性。与这些SC相反,新发现的SC CaK(Fe $_{1-x}$ Ni $_x$)$_4$ As $_4$显示出反铁磁(AFM)状态,称为刺猬自旋涡旋晶体结构,没有无序,为研究自旋涨落与SC之间的关系提供了机会,而没有任何自旋涨落的影响。我们对CaK(Fe $^{75}$ Ni $_x$)$_4$ As $_4$(0 $\le x\le$ 0.049)的核磁共振研究表明,CaK Fe $_4$ As $_4$位于接近隐藏的刺猬SVC AFM量子临界点(QCP)。在CaK(Fe $_{1-x}$ Ni $_x$)$_4$ As $_4$中没有向列性的磁性QCP突出了铁基SC中自旋涨落与超导电性的紧密联系。化学计量组成的优点也使得CaKFe $_4$ As $_4$成为进一步详细研究无无序效应的铁基SC中磁性QCP与超导性之间关系的理想平台。
英文摘要:
Two ordering states, antiferromagnetism and nematicity, have been observed in most iron-based superconductors (SCs). In contrast to those SCs, the newly discovered SC CaK(Fe$_{1-x}$Ni$_x$)$_4$As$_4$ exhibits an antiferromagnetic (AFM) state, called hedgehog spin-vortex crystal structure, without nematic order, providing the opportunity for the investigation into the relationship between spin fluctuations and SC without any effects of nematic fluctuations. Our $^{75}$As nuclear magnetic resonance studies on CaK(Fe$_{1-x}$Ni$_x$)$_4$As$_4$ (0$\le x\le$ 0.049) revealed that CaKFe$_4$As$_4$ is located close to a hidden hedgehog SVC AFM quantum-critical point (QCP). The magnetic QCP without nematicity in CaK(Fe$_{1-x}$Ni$_x$)$_4$As$_4$ highlights the close connection of spin fluctuations and superconductivity in iron-based SCs. The advantage of stoichiometric composition also makes CaKFe$_4$As$_4$ an ideal platform for further detailed investigation of the relationship between magnetic QCP and superconductivity in iron-based SCs without disorder effects.
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