arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2301.06336cond-mat.str-elcond-mat.supr-con
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CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$中的反铁磁序及其与超导的相互影响

Antiferromagnetic order and its interplay with superconductivity in CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$

J. M. Wilde, A. Sapkota, Q. -P. Ding, M. Xu, W. Tian, S. L. Bud'ko, Y. Furukawa, A. Kreyssig, P. C. Canfield

AI总结:

本文利用NMR、穆斯堡尔谱学和中子衍射研究Mn掺杂CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$,发现其具有与超导共存的刺猬状自旋涡旋晶体序,并推断出隐藏于超导穹顶下的量子相变。

摘要:

本文通过核磁共振(NMR)、穆斯堡尔谱学和中子衍射研究了几种CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$成分的磁序。我们对Mn掺杂1144化合物的观察结果与之前在Ni掺杂CaKFe4As4中发现的刺猬状自旋涡旋晶体(hSVC)序一致。hSVC态的特征是具有条纹型传播矢量(π 0)和(0 π),这与掺杂的122化合物相同。hSVC态在Fe位点上保持四方对称性,并且只有这种沿c轴简单AFM堆叠的SVC图案与我们使用NMR、穆斯堡尔谱学和中子衍射的所有观察结果一致。我们发现Mn掺杂1144化合物中的hSVC态与超导(SC)共存,通过结合中子散射和穆斯堡尔谱学数据,我们可以推断出一个量子相变,它隐藏在超导穹顶之下,与在x≈0.01时反铁磁转变温度(T_N)被抑制至零相关。此外,与几种122化合物和Ni掺杂1144不同,未观察到有序磁矩在低于超导转变温度(T_c)时减小。

英文摘要:

The magnetic order for several compositions of CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$ has been studied by nuclear magnetic resonance (NMR), Mössbauer spectroscopy, and neutron diffraction. Our observations for the Mn-doped 1144 compound are consistent with the hedgehog spin vortex crystal (hSVC) order which has previously been found for Ni-doped $\text{Ca}\text{K}\text{Fe}_4\text{As}_4$. The hSVC state is characterized by the stripe-type propagation vectors $(π\,0)$ and $(0\,π)$ just as in the doped 122 compounds. The hSVC state preserves tetragonal symmetry at the Fe site, and only this SVC motif with simple AFM stacking along $\textbf{c}$ is consistent with all our observations using NMR, Mössbauer spectroscopy, and neutron diffraction. We find that the hSVC state in the Mn-doped 1144 compound coexists with superconductivity (SC), and by combining the neutron scattering and Mössbauer spectroscopy data we can infer a quantum phase transition, hidden under the superconducting dome, associated with the suppression of the AFM transition temperature ($T_\text{N}$) to zero for $x\approx0.01$. In addition, unlike several 122 compounds and Ni-doped 1144, the ordered magnetic moment is not observed to decrease at temperatures below the superconducting transition temperature ($T_\text{c}$).

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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