Following the recent observation of the quantum spin Hall (QSH) effect in HgTe quantum wells, an important issue is to understand the effect of impurities on transport in the QSH regime. Using linear response and renormalization group methods, we calculate the edge conductance of a QSH insulator as a function of temperature in the presence of a magnetic impurity. At high temperatures, Kondo and/or two-particle scattering give rise to a logarithmic temperature dependence. At low temperatures, for weak Coulomb interactions in the edge liquid the conductance is restored to unitarity with unusual power-laws characteristic of a `local helical liquid', while for strong interactions transport proceeds by weak tunneling through the impurity where only half an electron charge is transferred in each tunneling event.
We show that the paradigmatic Ruderman-Kittel-Kasuya-Yosida (RKKY) description of two local magnetic moments coupled to propagating electrons breaks down in helical Luttinger Liquids when the electron interaction is stronger than some critical value. In this novel regime, the Kondo effect overwhelms the RKKY interaction over all macroscopic inter-impurity distances. This phenomenon is a direct consequence of the helicity (realized, for instance, at edges of a time-reversal invariant topological insulator) and does not take place in usual (non-helical) Luttinger Liquids.
The combined effect of Rashba and Dresselhaus spin-orbit interactions on the physics of a helical Luttinger liquid coupled to a Kondo impurity is studied. A Rashba coupling can potentially destroy the Kondo singlet formation in certain parameter regimes [Phys. Rev. B 86, 161103(R) (2012)]. This effect is here shown to vanish for sufficiently strong Dresselhaus interaction. The transport properties of the system are investigated by calculating electrical conductance, current and current fluctuations, and thermal conductance.
The Kondo cloud, represented by the correlations between the magnetic moment and the spin density in the leads of a Kondo setup, is until now eluding its observation. We exploit the unique coupling of spin and direction of motion of the recently discovered helical liquids in a setup with two leads to establish a proportionality between the Kondo cloud and the time resolved current cross correlations. This relation holds around a specific choice of model parameters. Thereby, we provide a new and direct way to detect the Kondo cloud.
We investigate theoretically the quantum phase transition (QPT) between the one-channel Kondo (1CK) and two-channel Kondo (2CK) fixed points in a quantum dot coupled to helical edge states of interacting 2D topological insulators (2DTI) with Luttinger parameter $0<K<1$. The model has been studied in Ref. 21, and was mapped onto an anisotropic two-channel Kondo model via bosonization. For K<1, the strong coupling 2CK fixed point was argued to be stable for infinitesimally weak tunnelings between dot and the 2DTI based on a simple scaling dimensional analysis[21]. We re-examine this model beyond…
We analyze the screening of a magnetic quantum dot with spin 1/2 coupled to two helical liquids. Interestingly, we find two qualitatively different sets of Toulouse points, i.e., nontrivial parameters for which we can solve the two channel Kondo model exactly. This enables us to calculate the temperature and voltage dependent Kondo screening cloud, which develops oscillations for an applied spin voltage $μ_s$. Such a spin voltage can be conveniently applied by a charge bias in a four-terminal helical liquid setup.
We study a quantum dot coupled to two edge states of a quantum spin Hall insulator through electron tunnelings in the presence of a Rashba spin-orbital interaction induced by an external electric field. We show that if the electron interactions on the edge states are repulsive, there are two possible phases, depending on the Luttinger liquid parameter $K$. For $1/2<K<1$, the low-temperature physics is controlled by a previously identified two-channel Kondo fixed point. For the edge states with even stronger repulsive interactions, i.e. $1/4<K<1/2$, the system reaches another phase at low tempe…
Ballistic transport of helical edge modes in two-dimensional topological insulators is protected by time-reversal symmetry. Recently it was pointed out [1] that coupling of non-interacting helical electrons to an array of randomly anisotropic Kondo impurities can lead to a spontaneous breaking of the symmetry and, thus, can remove this protection. We have analyzed effects of the interaction between the electrons using a combination of the functional and the Abelian bosonization approaches. The suppression of the ballistic transport turns out to be robust in a broad range of the interaction str…
We study one-dimensional Kondo Lattices (KL) which consist of itinerant electrons interacting with Kondo impurities (KI) - localized quantum magnetic moments. We focus on KL with isotropic exchange interaction between electrons and KI and with a high KI density. The latter determines the principal róle of the indirect interaction between KI for the low energy physics. Namely, the Kondo physics becomes suppressed and all properties are governed by spin ordering. We present a first-ever comprehensive analytical theory of such KL at an arbitrary doping and predict a variety of regimes with differ…
One-dimensional (1D) quantum wires, which are functionalized by magnetic ad-atoms, can host ballistic helical transport. Helicity protects transport from an undesirable influence of material imperfections, and it makes the magnetically doped wire a very promising element for nanoelectronics and spintronics. However, fabricating purely 1D conductors is experimentally very challenging and not always feasible. In this paper, we show that the protected helical transport can exist even in quasi-1D wires. We model the quasi-1D magnetically doped wire as two coupled dense 1D Kondo chains. Each chain …
The long-thought charge Kondo effects have recently been experimentally realized in the quantum Hall regime. This experiment, supported by numerics, exemplifies the realization of two-channel Kondo state, a non-Fermi Liquid, and its crossover to the one-channel counterpart, a Fermi liquid. Scaling up such a platform, we find a hierarchy of non-Fermi Liquids and their tunable crossovers based on a renormalization group analysis. Utilizing results from a conformal field theory, we further examine the universal conductances of this strongly correlated system and their finite temperature scaling, …
The enhanced spin Hall effect in Au metal due to the resonant skew scattering is studied with first-principles band structure calculations. Especially the gigantic spin Hall angle $γ_S \cong 0.1$ observed recently (T.Seki et al., Nature Materials {\bf 7}, 125 (2008)) is attributed to the orbital-dependent Kondo effect of Fe in the Au host metal, where the $t_{2g}$-orbitals are in the mixed-valence region while $e_g$-orbitals are in the Kondo limit. The enhanced spin-orbit interaction by the electron correlation in the $t_{2g}$-orbitals leads to the gigantic spin Hall effect. Impurities with 5d…
We study the coupling between a quantum dot and the edge of a non-Abelian fractional quantum Hall state which is spatially separated from it by an integer quantum Hall state. Near a resonance, the physics at energy scales below the level spacing of the edge states of the dot is governed by a $k$-channel Kondo model when the quantum Hall state is a Read-Rezayi state at filling fraction $ν=2+k/(k+2)$ or its particle-hole conjugate at $ν=2+2/(k+2)$. The $k$-channel Kondo model is channel isotropic even without fine tuning in the former state; in the latter, it is generically channel anisotropic. …
The anomalous Hall effect (AHE) in strongly disordered magnetic systems has been buried in persistent confusion despite its long history. We report the AHE in perpendicularly magnetized L10-MnAl epitaxial films with variable orbital two-channel Kondo (2CK) effect arising from the strong coupling of conduction electrons and the structural disorders of two-level systems. The AHE is observed to excellently scale with pAH/f=a0pxx0+bpxx2 at high temperatures where phonon scattering prevails. In contrast, significant deviation occurs at low temperatures where the orbital 2CK effect becomes important…
We theoretically investigate the non-equilibrium current through a quantum dot coupled to one- dimensional electron leads, utilizing a controlled frequency-dependent renormalization group (RG) approach. We compute the non-equilibrium conductance for large bias voltages and address the interplay between decoherence, Kondo entanglement and Luttinger physics. The combined effect of large bias voltage and strong interactions in the leads, known to stabilize two-channel Kondo physics, leads to non-trivial modifications of the conductance. For weak interactions, we build an analogy to a dot coupled …
Quantum dots in the quantum Hall regime can have pairs of single Slater determinant states that are degenerate in energy. We argue that these pairs of many body states may give rise to a Kondo effect which can be mapped into an ordinary Kondo effect in a fictitious magnetic field. We report on several properties of this Kondo effect using scaling and numerical renormalization group analysis. We suggest an experiment to investigate this Kondo effect.
A mapping between fractional quantum Hall (FQH) junctions and the two-channel Kondo model is presented. We discuss in detail this relation for the particular case of a junction of a FQH state at $ν= 1/3$ and a normal metal. We show that in the strong coupling regime this junction has a non-Fermi liquid fixed point. At this fixed point the electron Green's function has a branch cut, and the entropy has a non-zero value equal to $S={1/2} \ln{2}$. We construct the space of perturbations at the strong coupling fixed point and find that the dimensions of the tunneling operator is 1/2. These behavio…
In this work, a quantum dot couples to two helical edge states of a 2D topological insulator through weak tunnelings is studied. We show that if the electron interactions on the edge states are repulsive, with Luttinger liquid parameter $ K < 1 $, the system flows to a stable two-channel fixed point at low temperatures. This is in contrast to the case of a quantum dot couples to two Luttinger liquid leads. In the latter case, a strong electron-electron repulsion is needed, with $ K<1/2 $, to reach the two-channel fixed point. This two-channel fixed point is described by a boundary Sine-Gordon …
We show that edges of Quantum Spin Hall topological insulators represent a natural platform for realization of exotic supersolid phase. On one hand, fermionic edge modes are helical due to the nontrivial topology of the bulk. On the other hand, a disorder at the edge or magnetic adatoms may produce a dense array of localized spins interacting with the helical electrons. The spin subsystem is magnetically frustrated since the indirect exchange favors formation of helical spin order and the direct one favors (anti)ferromagnetic ordering of the spins. At a moderately strong direct exchange, the c…
Domain walls in fractional quantum Hall ferromagnets are gapless helical one-dimensional channels formed at the boundaries of topologically distinct quantum Hall (QH) liquids. Naïvely, these helical domain walls (hDWs) constitute two counter-propagating chiral states with opposite spins. Coupled to an s-wave superconductor, helical channels are expected to lead to topological superconductivity with high order non-Abelian excitations. Here we investigate transport properties of hDWs in the $ν=2/3$ fractional QH regime. Experimentally we found that current carried by hDWs is substantially smalle…
We report on a Kondo correlated quantum dot connected to two-dimensional leads where we demonstrate the renormalization of the g-factor in the pure Zeeman case i.e, for magnetic fields parallel to the plane of the quantum dot. For the same system we study the influence of orbital effects by investigating the quantum Hall regime i.e. a perpendicular magnetic field is applied. In this case an unusual behaviour of the suppression of the Kondo effect and of the split zero-bias anomaly is observed. The splitting decreases with magnetic field and shows discontinuous changes which are attributed to t…
We study the Ruderman-Kittel-Kasuya-Yoshida (RKKY) interaction mediated by helical edge states in quantum spin hall system. The helical edge states induce an in-plane noncollinear exchange coupling between two local spins, in contrast to the isotropic coupling induced in normal metal. The angle between the two local spins in the ground state depends on the Fermi level. This property may be used to control the angle of spins by tuning the electric gate.
Transport in an ideal two-dimensional quantum spin Hall device is dominated by the counterpropagating edge states of electrons with opposite spins, giving the universal value of the conductance, $2e^2/h$. We study the effect on the conductance of a magnetic impurity, which can backscatter an electron from one edge state to the other. In the case of isotropic Kondo exchange we find that the correction to the electrical conductance caused by such an impurity vanishes in the dc limit, while the thermal conductance does acquire a finite correction due to the spin-flip backscattering.
We propose a general capacitive model for an antidot, which has two localized edge states with different spins in the quantum Hall regime. The capacitive coupling of localized excess charges, which are generated around the antidot due to magnetic flux quantization, and their effective spin fluctuation can result in Coulomb blockade, h/(2e) Aharonov-Bohm oscillations, and the Kondo effect. The resultant conductance is in qualitative agreement with recent experimental data.
Among the most interesting predictions in two-dimensional materials with a Dirac cone is the existence of the zeroth Landau level (LL), equally filled by electrons and holes with opposite chirality. The gapless edge states with helical spin structure emerge from Zeeman splitting at the LL filling factor $ν=0$ gapped quantum Hall state. We present observations of a giant nonlocal four-terminal transport in zero-gap HgTe quantum wells at the $ν=0$ quantum Hall state. Our experiment clearly demonstrates the existence of the robust helical edge state in a system with single valley Dirac cone mater…
We study theoretically the two interacting one-dimensional helical modes at the edges of the quantum spin Hall systems. A new type of inter-edge correlated liquid (IECL) without the spin gap is found. This liquid shows the diverging density wave (DW) and superconductivity (SC) correlations much stronger than those of the spinfull electrons. Possible experimental observations are also discussed.
A quantum Hall edge state provides a rich foundation to study electrons in 1-dimension (1d) but is limited to chiral propagation along a single direction. Here, we demonstrate a versatile platform to realize new 1d systems made by combining quantum Hall edge states of opposite chiralities in a graphene electron-hole bilayer. Using this approach, we engineer helical 1d edge conductors where the counterpropagating modes are localized in separate electron and hole layers by a tunable electric field. These helical conductors exhibit strong nonlocal transport signals and suppressed backscattering d…
The recent experimental observations of the quantum Hall effect in 3D topological semimetals have attracted great attention, but there are still debates on its origin. We systematically study the dependence of the quantum Hall effect in topological semimetals on the thickness, Fermi energy, and growth direction, taking into account the contributions from the Fermi-arc surface states, confinement-induced bulk subbands, and helical side-surface edge states. In particular, we focus on the intensively studied Dirac semimetal Cd$_{3}$As$_{2}$ and its slabs grown along experimentally accessible dire…
We consider chiral electrons moving along the 1D helical edge of a 2D topological insulator and interacting with a disordered chain of Kondo impurities. Assuming the electron-spin couplings of random anisotropies, we map this system to the problem of the pinning of the charge density wave by the disordered potential. This mapping proves that arbitrary weak anisotropic disorder in coupling of chiral electrons with spin impurities leads to the Anderson localization of the edge states.
We have experimentally confirmed the quantum Hall ferromagnetic state with Chern number ν=0, characterized by the helical edge state, in a layered organic Dirac fermion system α-(BEDT-TTF)_2I_3. The interlayer resistance saturates at low temperatures and high magnetic fields. It does not scale with the sample cross-sectional area in the saturating region, and resonantly depends on the magnetic field direction. These results strongly suggest that the helical edge state dominates transport. This is the first observation of the topological phase in organic molecular crystals.
Electronic systems harboring one dimensional helical modes, where the spin and momentum of the electron are locked, have lately become an important field of its own. When coupled to a conventional superconductor, such systems are expected to manifest topological superconductivity, a unique phase that gives rise to exotic Majorana zero modes. Even more interesting are fractional helical states which have not been observed before and which open the route for the realization of the generalized para fermions quasiparticles. Possessing non abelian exchange statistics, these quasiparticles may serve…
We show that burying of the Dirac point in semiconductor-based quantum-spin-Hall systems can generate unexpected robustness of edge states to magnetic fields. A detailed ${\bf k\cdot p}$ band-structure analysis reveals that InAs/GaSb and HgTe/CdTe quantum wells exhibit such buried Dirac points. By simulating transport in a disordered system described within an effective model, we further demonstrate that buried Dirac points yield nearly quantized edge conduction out to large magnetic fields, consistent with recent experiments.
The rich phase diagram of quantum spin-ladder systems has attracted much attention in the theoretical literature. The progress in experimental realisations of this fascinating physics however has been much slower. While materials with a ladder-like structure exist, one always has coupling between the ladders to muddy the waters. In addition, such materials exhibit limited (if any) tunability in terms of the magnetic exchange parameters, and experimental probing of the different phases is a great challenge. In this work, we show that a realisation of spin-ladder physics can occur in an engineer…
The conductance of graphene subject to a strong, tilted magnetic field exhibits a dramatic change from insulating to conducting behavior with tilt-angle, regarded as evidence for the transition from a canted antiferromagnetic (CAF) to a ferromagnetic (FM) ν=0 quantum Hall state. We develop a theory for the electric transport in this system based on the spin-charge connection, whereby the evolution in the nature of collective spin excitations is reflected in the charge-carrying modes. To this end, we derive an effective field theoretical description of the low-energy excitations, associated wit…
We consider a four-terminal setup of a two-dimensional topological insulator (quantum spin Hall insulator) with local tunneling between the upper and lower edges. The edge modes are modeled as helical Luttinger liquids and the electron-electron interactions are taken into account exactly. Using perturbation theory in the tunneling, we derive the cumulant generating function for the inter-edge current. We show that different possible transport channels give rise to different signatures in the current noise and current cross-correlations, which could be exploited in experiments to elucidate the …
The ground state of charge neutral graphene under perpendicular magnetic field was predicted to be a quantum Hall topological insulator with a ferromagnetic order and spin-filtered, helical edge channels. In most experiments, however, an otherwise insulating state is observed and is accounted for by lattice-scale interactions that promote a broken-symmetry state with gapped bulk and edge excitations. We tuned the ground state of the graphene zeroth Landau level to the topological phase via a suitable screening of the Coulomb interaction with a SrTiO$_3$ high-$k$ dielectric substrate. We observ…
We report on the observation of a helical Luttinger-liquid in the edge of InAs/GaSb quantum spin Hall insulator, which shows characteristic suppression of conductance at low temperature and low bias voltage. Moreover, the conductance shows power-law behavior as a function of temperature and bias voltage. The results underscore the strong electron-electron interaction effect in transport of InAs/GaSb edge states. Because of the fact that the Fermi velocity of the edge modes is controlled by gates, the Luttinger parameter can be fine tuned. Realization of a tunable Luttinger-liquid offers a one-…
We report low-temperature transport measurements in strained InAs/Ga0.68In0.32Sb quantum wells, which supports time-reversal symmetry-protected helical edge states. The temperature and bias voltage dependence of the helical edge conductance for devices of various sizes are consistent with the theoretical expectation of a weakly interacting helical edge state. Moreover, we found that the magnetoresistance of the helical edge states is related to the edge interaction effect and the disorder strength.
We study Berry curvature driven and Zeeman magnetic field dependent electric current responses of two-dimensional electron system with spin-orbit coupling. New non-dissipative component of the electric current occurring in the applied in-plane magnetic field is described. This component is transverse to the electric field, odd in the magnetic field, and depends only on one particular direction of the magnetic field defined by the spin-orbit coupling. We show that the effect can be observed in a number of systems with $C_{3v}$ symmetry.
We demonstrate that electrostatic interactions between helical electrons at the edge of a quantum spin Hall insulator and a dynamical impurity can induce quasi-elastic backscattering. Modelling the impurity as a two-level system, we show that transitions between counterpropagating Kramers-degenerate electronic states can occur without breaking time-reversal symmetry, provided that the impurity also undergoes a transition. The associated electrical resistance has a weak temperature dependence down to a non-universal temperature scale. Our results extend the range of known backscattering mechani…
We investigate nuclear spin effects in a two-dimensional electron gas in the quantum Hall regime modeled by a weakly coupled array of interacting quantum wires. We show that the presence of hyperfine interaction between electron and nuclear spins in such wires can induce a phase transition, ordering electrons and nuclear spins into a helix in each wire. Electron-electron interaction effects, pronounced within the one-dimensional stripes, boost the transition temperature up to tens to hundreds of millikelvins in GaAs. We predict specific experimental signatures of the existence of nuclear spin …
We calculate the anomalous Hall conductivity $σ_{xy}$ of the surface states {in cubic topological Kondo insulators}. We consider a generic model for the surface states with three Dirac cones on the (001) surface. The Fermi velocity, the Fermi momentum and the Zeeman energy in different Dirac pockets may be unequal. The microscopic impurity potential mediates mixed intra and interband extrinsic scattering processes. Our calculation of $σ_{xy}$ is based on the Kubo-Streda diagrammatic approach. It includes diffractive skew scattering contributions originating from the rare two-impurity complexes…
We theoretically study tunneling of Cooper pairs from a superconductor spanning a two-dimensional topological insulator strip into its helical edge states. The coherent low-energy electron-pair tunneling sets off positive current cross correlations along the edges, which reflect an interplay of two quantumentanglement processes. Most importantly, superconducting spin pairing dictates a Cooper pair partitioning into the helical edge liquids, which transport electrons in opposite directions for opposite spin orientations. At the same time, Luttinger-liquid correlations fractionalize electrons in…
We propose and analyze inter-edge tunneling in a quantum spin Hall corner junction as a means to probe the helical nature of the edge states. We show that electron-electron interactions in the one-dimensional helical edge states result in Luttinger parameters for spin and charge that are intertwined, and thus rather different than those for a quantum wire with spin rotation invariance. Consequently, we find that the four-terminal conductance in a corner junction has a distinctive form that could be used as evidence for the helical nature of the edge states.
A two-dimensional time-reversal symmetric topological superconductor is a fully gapped system possessing a helical Majorana mode on the edges. This helical Majorana edge mode (HMEM), which is a Kramer's pair of two chiral Majorana edge modes in the opposite propagating directions, is robust under time-reversal symmetry protection. We propose a feasible setup and accessible measurement to provide the preliminary step of the HMEM realization by studying superconducting antiferromagnetic quantum spin Hall insulators. Since this antiferromagnetic topological insulator hosts a helical electron edge…
We study an electrically controlled quantum spin Hall antidot embedded in a two-dimensional topological insulating bar. Helical edge states around the antidot and along the edges of the bar are tunnel coupled. The close connection between spin and chirality, typical of helical systems, allows to generate a spin-polarized current flowing across the bar. This current is studied as a function of the external voltages, by varying the asymmetry between the barriers. For asymmetric setups, a switching behavior of the spin current is observed as the bias is increased, both in the absence and in the p…
It is well known that quantum spin Hall (QSH) edge modes being helical are immune to backscattering due to non-magnetic disorder within the sample. Thus, quantum spin Hall edge modes are non-localized and show a vanishing Hall resistance along with quantized 2-terminal, longitudinal and non-local resistances even in presence of sample disorder. However, this is not the case for contact disorder. This paper shows that when all contacts are disordered in an N-terminal quantum spin Hall sample, then transport via these helical QSH edge modes can have a significant localization correction. All the…
We study the electronic transport across an electrostatically-gated lateral junction in a HgTe quantum well, a canonical 2D topological insulator, with and without applied magnetic field. We control carrier density inside and outside a junction region independently and hence tune the number and nature of 1D edge modes propagating in each of those regions. Outside the 2D gap, magnetic field drives the system to the quantum Hall regime, and chiral states propagate at the edge. In this regime, we observe fractional plateaus which reflect the equilibration between 1D chiral modes across the juncti…
We study the plasmon excitations and the electromagnetic response of the magnetically doped single layer and multilayer of ``helical metals'', which emerge at the surfaces of topological insulators. For the single layer case, we find a ``spin-plasmon'' mode with the rotating spin texture due to the combination of the spin-momentum locking of ``helical metals'' and the Hall response from magnetization. For the multilayers case, we investigate the electromagnetic response due to the plasmon excitations, including the Faraday rotation for the light propagating normal to the helical metal layers a…
We give a theory of the inverse spin Hall effect (ISHE) in ferromagnetic metals based on skew scattering via collective spin fluctuations. This extends Kondo's theory of the anomalous Hall effect (AHE) to include short-range spin-spin correlations. We find a relation between the ISHE and the four-spin correlations near the Curie temperature TC. Such four-spin correlations do not contribute to the AHE, which relates to the three-spin correlations. Thus our theory shows an essential difference between the AHE and ISHE, providing an essential complement to Kondo's classic theory of the AHE in met…
Helical metals realized at the surfaces of topological insulators have recently attracted wide attention due to their potential applications in spintronics. In this paper we propose to realize helical metals through the application of THz light on common two-dimensional semiconductors and discuss their observable properties. We show that the application of circularly polarized light enables coherent manipulation of magnetization. Moreover, for a range of chemical potentials the system behaves as a helical metal, exhibiting a large anomalous Hall conductivity and associated magnetoelectric effe…
The gapless edge modes of the Quantum Spin Hall insulator form a helical liquid in which the direction of motion along the edge is determined by the spin orientation of the electrons. In order to probe the Luttinger liquid physics of these edge states and their interaction with a magnetic (Kondo) impurity, we consider a setup where the helical liquid is tunnel-coupled to a semiconductor quantum dot which is excited by optical absorption, thereby inducing an effective quantum quench of the tunneling. At low energy, the absorption spectrum is dominated by a power-law singularity. The correspondi…
Quantum spin Hall insulator is characterized by the helical edge states, with the spin polarization of electron being locked to its direction of motion. Although the edge-state conduction has been observed, unambiguous evidence of the helical spin texture is still lacking. Here, we investigate the coherent edge-state transport in an interference loop pinched by two point contacts. Due to the helical character, the forward inter-edge scattering enforces a $π$ spin rotation. Two successive processes can only produce a nontrivial $2π$ or trivial $0$ spin rotation, which can be controlled by the R…
The two-dimensional electron gas in a bilayer graphene in the Bernal stacking supports a variety of uniform broken-symmetry ground states in Landau level N=0 at integer filling factors $ν\in [-3,4].$ When an electric potential difference (or bias) is applied between the layers at filling factors $ν=-1,3$, the ground state evolves from an interlayer coherent state at small bias to a state with orbital coherence at higher bias where \textit{electric} dipoles associated with the orbital pseudospins order spontaneously in the plane of the layers. In this paper, we show that by further increasing t…