We report complete characterization of an optical memory based on electromagnetically induced transparency. We recover the superoperator associated with the memory, under two different working conditions, by means of a quantum process tomography technique that involves storage of coherent states and their characterization upon retrieval. In this way, we can predict the quantum state retrieved from the memory for any input, for example, the squeezed vacuum or the Fock state. We employ the acquired superoperator to verify the nonclassicality benchmark for the storage of a Gaussian distributed set of coherent states.
We investigate frequency correlations in multiple scattered light that are present in the quantum fluctuations. The memory effect for quantum and classical noise is compared, and found to have markedly different frequency scaling, which was confirmed in a recent experiment. Furthermore, novel mesoscopic correlations are predicted that depend on the photon statistics of the incoming light.
Recent experiments demonstrating atomic quantum memory for light [B. Julsgaard et al., Nature 432, 482 (2004)] involve two macroscopic samples of atoms, each with opposite spin polarization. It is shown here that a single atomic cell is enough for the memory function if the atoms are optically pumped with suitable linearly polarized light, and quadratic Zeeman shift and/or ac Stark shift are used to manipulate rotations of the quadratures. This should enhance the performance of our quantum memory devices since less resources are needed and losses of light in crossing different media boundaries…
We develop the theory of an optical quantum memory protocol based on the three pulse photon echo (PE) in an optically dense medium with controlled reversible inhomogeneous broadening (CRIB). The wave-function of the retrieved photon echo field is derived explicitly as a function of an arbitrary input Data light field. The storage and retrieval of time-bin qubit states based on the described quantum memory is discussed, and it is shown that the memory allows to measure the path length difference in an imbalanced interferometer using short light pulses.
It has been shown recently (Phys. Rev. Lett. 106, 090504 (2011)) that entangled light with Einstein-Podolsky-Rosen (EPR) correlations retrieves information from digital memory better than any classical light. In identifying this, a model of digital memory with each cell consisting of reflecting medium with two reflectivities (each memory cell encoding the binary numbers 0 or 1) is employed. The readout of binary memory essentially corresponds to discrimination of two Bosonic attenuator channels characterized by different reflectivities. The model requires an entire mathematical paraphernalia o…
We report on coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr3+:Y2SiO5 to spin-waves in the hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of 5 temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory i…
We propose a new method for efficient storage and recall of non-stationary light fields, e.g. single photon time-bin qubits, in optically dense atomic ensembles. Our approach to quantum memory is based on controlled, reversible, inhomogeneous broadening. We briefly discuss experimental realizations of our proposal.
We report an experiment on mapping a quantum state of light onto the ground state spin of an ensemble of Cs atoms with the life time of 2 milliseconds. Quantum memory for one of the two quadrature phase operators of light is demonstrated with vacuum and squeezed states of light. The sensitivity of the mapping procedure at the level of approximately one photon/sec per Hz is shown. The results pave the road towards complete (storing both quadrature phase observables) quantum memory for Gaussian states of light. The experiment also sheds new light on fundamental limits of sensitivity of the magne…
We propose and investigate a protocol for Gaussification of quantum states of traveling light beams in an atomic quantum memory that couples to light via quantum non-demolition interaction. The protocol relies on a periodic switching between two different QND couplings and the total coupling strength scales only logarithmically with number of Gaussified light modes. The present scheme can be used to prepare entangled states of two distant atomic ensembles and to purify and Gaussify noisy non-Gaussian entangled states of light while simultaneously storing the purified state in atomic memories.
We implement the ROSE protocol in an erbium doped solid, compatible with the telecom range. The ROSE scheme is an adaptation of the standard 2-pulse photon echo to make it suitable for a quantum memory. We observe an efficiency of 40% in a forward direction by using specific orientations of the light polarizations, magnetic field and crystal axes.
The information carrier of today's communications, a weak pulse of light, is an intrinsically quantum object. As a consequence, complete information about the pulse cannot, even in principle, be perfectly recorded in a classical memory. In the field of quantum information this has led to a long standing challenge: how to achieve a high-fidelity transfer of an independently prepared quantum state of light onto the atomic quantum state? Here we propose and experimentally demonstrate a protocol for such quantum memory based on atomic ensembles. We demonstrate for the first time a recording of an …
We propose an efficient method for mapping and storage of a quantum state of propagating light in atoms. The quantum state of the light pulse is stored in two sublevels of the ground state of a macroscopic atomic ensemble by activating a synchronized Raman coupling between the light and atoms. We discuss applications of the proposal in quantum information processing and in atomic clocks operating beyond quantum limits of accuracy. The possibility of transferring the atomic state back on light via teleportation is also discussed.
A scheme for control and read-out of diffracted spins waves to propagating light fields is presented. Diffraction is obtained via sinusoidally varying lights shifts and ideal one-to-one mapping to light is realized using a gradient echo quantum memory. We also show that dynamical control of the diffracted spin waves spatial orders can be implemented to realize a quantum pulse sequencer for temporal modes that have high time-bandwidth products. Full numerical solutions suggest that both co-propagating and couterpropagating light shift geometries can be used, making the proposal applicable to ho…
We propose a quantum memory for light that is analogous to the NMR gradient echo. Our proposal is ideally perfectly efficient and provides simplifications to current 3-level quantum memory schemes based on controlled inhomogeneous broadening. Our scheme does not require auxiliary light fields. Instead the input optical pulse interacts only with two-level atoms that have linearly increasing Stark shifts. By simply reversing the sign of the atomic Stark shifts, the pulse is retrieved in the forward direction. We present analytical, numerical and experimental results of this scheme. We report exp…
In a recent continuous-variable quantum memory experiment, one quadrature of light pulse is directly uploaded by the light-atom coupling whereas complementary quadrature is obtained by homodyne measurement of the out-coupled light. Subsequently, information from homodyne mea- surement is written into the memory by feed-back electro-optical control of the atomic state. Using the same experimental set-up, a deterministic noise excess free record of unknown quantum states to continuous-variable quantum atomic memory is proposed. Further, the memory experiment is extended by the pre-squeezing of t…
The possibilities of recording, storage and reconstruction of short single photon wave packets in the photon echo technique are analyzed. The influence of the photon field and medium parameters on the quality and precision of the photon quantum state reconstruction is theoretically studied.
We describe a technique for generating pulses of light with controllable photon numbers, propagation direction, timing, and pulse shapes. The technique is based on preparation of an atomic ensemble in a state with a desired number of atomic spin excitations, which is later converted into a photon pulse. Spatio-temporal control over the pulses is obtained by exploiting long-lived coherent memory for photon states and electromagnetically induced transparency (EIT) in an optically dense atomic medium. Using photon counting experiments we observe generation and shaping of few-photon sub-Poissonian…
We discuss theoretically quantum interface between light and a spin polarized ensemble of atoms with the spin >= 1 based on an off-resonant Raman scattering. We present the spectral theory of the light-atoms interaction and show how particular spectral modes of quantum light couple to spatial modes of the extended atomic ensemble. We show how this interaction can be used for quantum memory storage and retrieval and for deterministic entanglement protocols. The proposed protocols are attractive due to their simplicity since they involve just a single pass of light through atoms without the need…
We extend the theory to describe the quantum light memory in type atoms with considering (lower levels coherency decay rate) and detuning for the probe and the control fields. We obtain that with considering these parameters, group velocity of the probe pulse does not tend to zero by turning off the control field. We show that there are considerable decay for the probe pulse and the stored information. Also, it is inferred that the light field does not tend to zero when the control field is turned off. In addition, we obtain that in the off-resonance case there is considerable distortion of th…
Cavity-assisted storage and retrieval of single-photon wave packets in optically thin spatially extended resonant materials are analyzed. It is shown that the use of cavity tuning allows one to store and recall time-symmetric double-sided exponential pulses with near unit efficiency. The optimal regime of the cavity tuning is determined and the effect of time jitter on the storage efficiency is analyzed.
We present two protocols, one for the storage of light in an atomic ensemble and the subsequent retrieval, and another one for the generation of entanglement between light and atoms. They rely on two passes of a single pulse through the ensemble, Larmor precessing in an external field. Both protocols work deterministically and the relevant figures of merit - such as the fidelity or the EPR variance - scale exponentially in the coupling strength. We solve the corresponding Maxwell-Bloch equations describing the scattering process and determine the resulting input-output relations which only inv…
We present a light-storage experiment in a praseodymium-doped crystal where the light is mapped onto an inhomogeneously broadened optical transition shaped into an atomic frequency comb. After absorption of the light the optical excitation is converted into a spin-wave excitation by a control pulse. A second control pulse reads the memory (on-demand) by reconverting the spin-wave excitation to an optical one, where the comb structure causes a photon-echo type rephasing of the dipole moments and directional retrieval of the light. This combination of photon echo and spin-wave storage allows us …
We consider a quantum memory scheme based on the conversion of a signal pulse into a long-lived spin coherence via stimulated off-resonant Raman process. For a storing medium consisting of alkali atoms, we have calculated the Autler-Townes resonance structure created by a strong control field. By taking into account the upper hyperfine states of the D1 optical transition, we show important deviations from the predictions of the usual three-level Lambda-scheme approximation and we demonstrate an enhancement of the process for particular detunings of the control. We estimate the memory efficienc…
We investigate the transient phenomenon or property of the propagation of an optical probe field in a medium consisting of many $Λ$-type three-level atoms coupled to this probe field and an classical driven field. We observe a hidden symmetry and obtain an exact solution for this light propagation problem by means of the spectral generating method. This solution enlightens us to propose a practical protocol implementing the quantum memory robust for quantum decoherence in a crystal. As an transient dynamic process this solution also manifests an exotic result that a wave-packet of light will s…
We review a series of quantum memory protocols designed to store the quantum information carried by light into atomic ensembles. In particular, we show how a simple semiclassical formalism allows to gain insight into various memory protocols and to highlight strong analogies between them. These analogies naturally lead to a classification of light storage protocols into two categories, namely photon echo and slow-light memories. We focus on the storage and retrieval dynamics as a key step to map the optical information into the atomic excitation. We finally review various criteria adapted for …
Nowadays the most intriguing features of wave particle complementarity of single photon is exemplified by the famous Wheeler's delayed choice experiment in linear optics, nuclear magnetic resonance and integrated photonic device systems. Studying the wave particle behavior in light and matter interaction at single photon level is challenging and interesting, which gives how single photons complement in light and matter interaction. Here, we demonstrate a Wheeler's delayed choice experiment in an interface of light and atomic memory, in which the cold atomic memory makes the heralded single pho…
Here we demonstrate generating and storing entanglement in a solid state spin-wave quantum memory with on-demand read out using the process of rephased amplified spontaneous emission (RASE). Amplified spontaneous emission (ASE), resulting from an inverted ensemble of Pr$^{3+}$ ions doped into a Y$_2$SiO$_5$ crystal, generates entanglement between collective states of the praseodymium ensemble and the output light. The ensemble is then rephased using a four-level photon echo technique. Entanglement between the ASE and its echo is confirmed and the inseparability violation preserved when the RAS…
We propose an original quantum memory protocol. It belongs to the class of rephasing processes and is closely related to two-pulse photon echo. It is known that the strong population inversion produced by the rephasing pulse prevents the plain two-pulse photon echo from serving as a quantum memory scheme. Indeed gain and spontaneous emission generate prohibitive noise. A second $π$-pulse can be used to simultaneously reverse the atomic phase and bring the atoms back into the ground state. Then a secondary echo is radiated from a non-inverted medium, avoiding contamination by gain and spontaneo…
We extend the theory of quantum light memory in atomic ensemble of Lambda type atoms with considering lower levels coherence decay rate and one and two-photon detunings from resonances in low intensity and adiabatic passage limit. We obtain that with considering these parameters, that there will be a considerable decay of probe pulse and stored information; also, we obtain that the group velocity of probe (light) pulse and its amplitude does not tend to zero by turning off the control field. We propose a method to keep the probe pulse in small values in turn off time of control field and to re…
Quantum memories for light are essential components in quantum technologies like long-distance quantum communication and distributed quantum computing. Recent studies have shown that long optical and spin coherence lifetimes can be observed in rare earth doped nanoparticles, opening exciting possibilities over bulk materials e.g. for enhancing coupling to light and other quantum systems, and material design. Here, we report on coherent light storage in Eu$^{3+}$:Y$_2$O$_3$ nanoparticles using the Stark Echo Modulation Memory (SEMM) quantum protocol. We first measure a nearly constant Stark coe…
We demonstrate a solid state spin-wave optical memory based on stopped light in a spectral hole. A long lived narrow spectral hole is created by optical pumping in the inhomogeneous absorption profile of a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. Optical pulses sent through the spectral hole experience a strong reduction of their group velocity and are spatially compressed in the crystal. A short Raman pulse transfers the optical excitation to the spin state before the light pulse exits the crystal, effectively stopping the light. After a controllable delay, a second Raman pulse is sent, which leads to…
We propose a method to implement a quantum memory for light based on ensembles of two-level atoms. Our protocol is based on controlled reversible inhomogeneous broadening (CRIB), where an external field first dephases the atomic polarization and thereby stores an incoming light pulse into collective states of the atomic ensemble, and later a reversal of the applied field leads to a rephasing of the atomic polarization and a reemission of the light. As opposed to previous proposals for CRIB based quantum memories we propose to only apply the broadening for a short period after most of the pulse…
An ideal and reversible transfer technique for the quantum state between light and metastable collective states of matter is presented and analyzed in detail. The method is based on the control of photon propagation in coherently driven 3-level atomic media, in which the group velocity is adiabatically reduced to zero. Form-stable coupled excitations of light and matter (``dark-state polaritons'') associated with the propagation of quantum fields in Electromagnetically Induced Transparency are identified, their basic properties discussed and their application for quantum memories for light ana…
We have considered theoretically the feasibility of the broadband quantum memory based on the resonant tripod-type atomic configuration. In this case, the writing of a signal field is carried out simultaneously into two channels, and characterized by an excitation of two spin waves of the atomic ensemble. With simultaneous read out from both channels quantum properties of the original signal are mapped on the retrieval pulse no worse than in the case of memory based on Lambda-type atomic configuration. At the same time new possibilities are opened up for manipulation of quantum states associat…
We have found a new hidden symmetry of time reversal light-atom interaction in the photon echo quantum memory with Raman atomic transition. The time-reversed quantum memory creates generalized conditions for ideal compression/decompression of time duration of the input light pulses and its wavelength. Based on a general analytical approach to this scheme, we have studied the optimal conditions for the light field compression/decompression in resonant atomic systems characterized by realistic spectral properties. The demonstrated necessary conditions for the effective quantum conversion of the …
A new protocol of the optical quantum memory based on the resonant interactions of the multi atomic system with a cavity light mode is proposed. The quantum memory is realized using a controllable inversion of the inhomogeneous broadening of the resonant atomic transition and impact interaction (on request) of additional short 2 - laser pulse resonant to an adjacent atomic transition. We demonstrate that the quantum memory protocol is effective for arbitrary storage time and can be used for new quantum manipulations with transient entangled states in the field-atoms evolution. The effect of th…
We produce a 600-ns pulse of 1.86-dB squeezed vacuum at 795 nm in an optical parametric amplifier and store it in a rubidium vapor cell for 1 us using electromagnetically induced transparency. The recovered pulse, analyzed using time-domain homodyne tomography, exhibits up to 0.21+-0.04 dB of squeezing. We identify the factors leading to the degradation of squeezing and investigate the phase evolution of the atomic coherence during the storage interval.
We propose a feasible scheme of quantum state storage and manipulation via electromagnetically induced transparency (EIT) in flexibly $united$ multi-ensembles of three-level atoms. For different atomic array configurations, one can properly steer the signal and the control lights to generate different forms of atomic entanglement within the framework of linear optics. These results shed new light on designing the versatile quantum memory devices by using, e.g., an atomic grid.
Matter-light quantum interface and quantum memory for light are important ingredients of quantum information protocols, such as quantum networks, distributed quantum computation, etc. In this Letter we present a spatially multimode scheme for quantum memory for light, which we call a quantum hologram. Our approach uses a multi-atom ensemble which has been shown to be efficient for a single spatial mode quantum memory. Due to the multi-atom nature of the ensemble it is capable of storing many spatial modes, a feature critical for the present proposal. A quantum hologram has a higher storage cap…
In this paper, we examined a possibility of preservation of a substantially multimode radiation in a single cell of quantum memory. As a light source we considered a synchronously pumped optical parametric oscillator (SPOPO). As it was shown in [1-4], SPOPO radiation has a large number of the correlated modes making it attractive for the purposes of the quantum communication and computing. We showed that these correlations can be mapped on the longitudinal spin waves of the memory cell and be restored later in the readout light. The efficiencies of the writing and readout depend on the mode st…
Duan-Lukin-Cirac-Zoller (DLCZ) quantum repeater protocol, which was proposed to realize long distance quantum communication, requires usage of quantum memories. Atomic ensembles interacting with optical beams based on off-resonant Raman scattering serve as convenient on-demand quantum memories. Here, a complete free space, three-dimensional theory of the associated read and write process for this quantum memory is worked out with the aim of understanding intrinsic retrieval efficiency. We develop a formalism to calculate the transverse mode structure for the signal and the idler photons and us…
We develop a three-dimensional theory for quantum memories based on light storage in ensembles of Lambda-type atoms, where two long-lived atomic ground states are employed. We consider light storage in an ensemble of finite spatial extent and we show that within the paraxial approximation the Fresnel number of the atomic ensemble and the optical depth are the only important physical parameters determining the quality of the quantum memory. We analyze the influence of these parameters on the storage of light followed by either forward or backward read-out from the quantum memory. We show that f…
Slow-light-enhanced Atomic Frequency Comb Quantum Memory in Stoichiometric EuCl$_3 \cdot$ 6D$_2$O
International Quantum Academy, and Shenzhen Branch, Hefei National Laboratory（国际量子学院，合肥国家实验室深圳分院）；Southern University of Science and Technology（南方科技大学）
Distribution of light-matter quantum correlations with a temporally multiplexed solid-state quantum memory array
ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科技研究所）；ICREA, Institucio Catalana de Recerca i Estudis Avançats（ICREA，加泰罗尼亚研究与高级研究学院）
We consider the coherent stimulated Raman process developing in an optically dense and disordered atomic medium in application to the quantum memory scheme. Our theoretical model predicts that the hyperfine interaction in the excited state of alkali atoms can positively affect on the quantum memory efficiency. Based on the concept of the coherent information transfer we analyze and compare the memory requirements for storage of single photon and macroscopic multi-photon light pulses.
The paper studies the Raman quantum memory protocol as applied to quantum light with orbital angular momentum. The memory protocol is implemented on an ensemble of three-level cold atoms with the $Λ$- configuration of energy levels. The possibility of storing quantum statistics of light with an orbital momentum is analysed in the case when the driving field could be treated as a plane wave. The efficiency analysis shows that examined storage/retrieval processes do not cause the efficiency decreasing compared with the spatial multimode memory protocol considered in [Golubeva et al. 2012]]. We a…
Photon echo schemes are excellent candidates for high efficiency coherent optical memory. They are capable of high-bandwidth multi-pulse storage, pulse resequencing and have been shown theoretically to be compatible with quantum information applications. One particular photon echo scheme is the gradient echo memory (GEM). In this system, an atomic frequency gradient is induced in the direction of light propagation leading to a Fourier decomposition of the optical spectrum along the length of the storage medium. This Fourier encoding allows precision spectral manipulation of the stored light. I…
Light-cones in many-body open quantum systems with memory
Max Planck Institute of Quantum Optics（马克斯·普朗克量子光学研究所）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）；Department Physics, University of Washington（华盛顿大学物理系）
The unusual features of quantum mechanics are enabling the development of technologies not possible with classical physics. These devices utilize nonclassical phenomena in the states of atoms, ions, and solid-state media as the basis for many prototypes. Here we investigate molecular states as a distinct alternative. We demonstrate a memory for light based on storing photons in the vibrations of hydrogen molecules. The THz-bandwidth molecular memory is used to store 100-fs pulses for durations up to 1ns, enabling 10,000 operational time bins. The results demonstrate the promise of molecules fo…
The ability to efficiently realize storage and readout of optical squeezed states plays a key roll in continuous-variables quantum information processing. Here we study the quantum memory (QM) for squeezed state of propagating light in atoms based on the hybrid photon echo re-phasing (HYPER). The optical quantum state is recorded in two sublevels of the ground state of an atomic ensemble to realize long-lived QM. Taking into account the noise effect due to atomic decay, our estimation indicates that, with currently available technique, high fidelities larger than the classical fidelity thresho…
The efficiency of an ensemble-based optical quantum memory depends critically on the strength of the atom-light coupling. An optical cavity is an effective method to enhance atom-light coupling strength, with the drawback that cavities can be difficult to integrate into a memory setup. In this work we show coherent enhancement of atom-light coupling via an interference effect. The light to be absorbed into the atomic ensemble is split and used to drive the atoms from opposite ends of the ensemble. We compare this method theoretically to a cavity enhanced scheme and present experimental results…
We propose a quantum memory protocol based on dynamically changing the resonance frequency of an ensemble of two-level atoms. By sweeping the atomic frequency in an adiabatic fashion, photons are reversibly transferred into atomic coherences. We present a polaritonic description for this type of storage, which shares some similarities with Electromagnetically Induced Transparency (EIT) based quantum memories. On the other hand the proposed memory is also linked to the Gradient Echo Memory (GEM) due to the effective spatial gradient that pulses experience in the medium. We discuss a possible im…
Quantum networks promise to revolutionise computing, simulation, and communication. Light is the ideal information carrier for quantum networks, as its properties are not degraded by noise in ambient conditions, and it can support large bandwidths enabling fast operations and a large information capacity. Quantum memories, devices that store, manipulate, and release on demand quantum light, have been identified as critical components of photonic quantum networks, because they facilitate scalability. However, any noise introduced by the memory can render the device classical by destroying the q…
A long-lived quantum memory was developed based on light-compensated cold $^{87}$Rb atoms in a dipole trap. The lifetime of the quantum memory was improved by 40 folds, from 0.67 ms to 28 ms with the help of a compensation laser beam. Oscillations of the memory efficiency due to the transverse mode breathing of the singly-excited spin wave have been clearly observed and clarified with a Monte-Carlo simulation procedure. With detailed analysis of the decoherence processes of the spin wave in cold atomic ensembles, this experiment provides a benchmark for the further development of high-quality …
