B. Kraus, W. Tittel, N. Gisin, M. Nilsson, S. Kroll, J. I. Cirac
We propose a new method for efficient storage and recall of non-stationary light fields, e.g. single photon time-bin qubits, in optically dense atomic ensembles. Our approach to quantum memory is based on controlled, reversible, inhomogeneous broadening. We briefly discuss experimental realizations of our proposal.
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We present a detailed analysis of a quantum memory for photons based on controlled and reversible inhomogeneous broadening (CRIB). The explicit solution of the equations of motion is obtained in the weak excitation regime, making it possible to gain insight into the dependence of the memory efficiency on the optical depth, and on the width and shape of the atomic spectral distributions. We also study a simplified memory protocol which does not require any optical control fields.
A novel method of multi-bit quantum optical data storage is presented, where the storage time can be lengthened far beyond the spin phase-decay time in a reversible spin inhomogeneous system excited by consecutive resonant Raman optical data pulses. The ultralong storage time is obtained by an optical population locking mechanism of modified rephasing process. This gives potentials to quantum repeaters utilizing quantum memories for long distance quantum communications, in which ultralong storage time plays a major role.
We study the evolution of an inverted spin ensemble coupled to a cavity. The inversion itself presents an inherent instability of the system; however, the inhomogeneous broadening of spin-resonance frequencies presents a stabilizing mechanism, and a stability criterion is derived. The detailed behavior of mean values and variances of the spin components and of the cavity field is accounted for under both stable and unstable conditions.
Spontaneous Raman emission in atomic gases provides an attractive source of photon pairs with a controllable delay. We show how this technique can be implemented in solid state systems by appropriately shaping the inhomogeneous broadening. Our proposal is eminently feasible with current technology and provides a realistic solution to entangle remote rare-earth doped solids in a heralded way.
A new scheme of photon echo based quantum memory in the optimal optical QED cavity with off-resonant Raman atomic transition is proposed. The scheme employs the atomic ensembles characterized by an optically thin resonant transition and natural inhomogeneous broadening of the resonant line composed of the arbitrary narrow homogeneous spectral components. The scheme provides robust and quite simple coherent control of the light-atoms dynamics that can be implemented by using an existing optical technique and opens a practical way for realization of the efficient long-lived multi-mode optical qu…
A long-lived qubit is usually well-isolated from all other systems and the environments, and so is not easy to couple with measurement apparatus. It is sometimes difficult to implement reliable projective measurements on such a qubit. One potential solution is spin amplification with many ancillary qubits. Here, we propose a spin amplification technique, where the ancillary qubits state change depending on the state of the target qubit. The technique works even in the presence of inhomogeneous broadening. We show that fast and accurate amplification is possible even if the coupling and frequen…
In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)] and in the two preceding papers [Gorshkov et al., Phys. Rev. A 76, 033804 (2007); 76, 033805 (2007)], we used a universal physical picture to optimize and demonstrate equivalence between a wide range of techniques for storage and retrieval of photon wave packets in homogeneously broadened Lambda-type atomic media, including the adiabatic reduction of the photon group velocity, pulse-propagation control via off-resonant Raman techniques, and photon-echo-based techniques. In the present paper, we generalize this treatment to…
Photon echo quantum memory with complete use of natural inhomogeneous broadening
本文提出一种新型原子重定相主动机制，可在任意初始非均匀展宽下完美恢复存储光场，并利用所有共振原子最大化光学深度，为高效光子回波量子存储器的实际实现开辟了广阔道路。
Removing inhomogeneous broadening in cross-relaxation spectra via hole burning
研究基于金刚石NV中心的量子弛豫测量技术中，非均匀展宽限制交叉弛豫谱分辨率的问题，提出用烧孔技术，利用弱泵浦场耗尽特定NV中心，保留便利性与灵敏度，开辟高分辨率磁共振光谱新途径。
Electromagnetically induced transparency (EIT) has been often proposed for generating nonlinear optical effects at the single photon level; in particular, as a means to effect a quantum non-demolition measurement of a single photon field. Previous treatments have usually considered homogeneously broadened samples, but realisations in any medium will have to contend with inhomogeneous broadening. Here we reappraise an earlier scheme [Munro \textit{et al.} Phys. Rev. A \textbf{71}, 033819 (2005)] with respect to inhomogeneities and show an alternative mode of operation that is preferred in an in…
Transition from inhomogeneous to homogeneous broadening at a lasing prethreshold
本文研究非均匀展宽激光器在临界泵浦速率附近的谱形转变，揭示特殊锁定模式先于激光形成并使光谱由高斯型转为洛伦兹型，同时给出阈值与产生频率表达式。
In order to better understand the underlying fundamental physical processes in nitrogen-vacancy centers in diamond, and to realize improvements in the use of this system for technological applications, it is imperative to gain new insight into the origins of the apparent inhomogeneous broadening. In this work we make use of a novel type of spectroscopy developed specifically for this task. The pump-probe spectroscopy closely follows Doppler-free spectroscopy used in atomic vapor. We show that the origin of inhomogeneous broadening comes from local magnetic field variations in the diamond latti…
It is shown that inhomogeneous broadening of the spectral line of active impurities may sustain simultaneously parity (P) and time (T) symmetries of a medium, in a finite range of field frequencies, what is forbidden by the causality principle in media without broadening. If a spectral width of a propagating pulse is less than the inhomogeneous broadening, the medium for such a pulse becomes quasi-PT symmetric. The effect of the broadband quasi-PT symmetry in a finite frequency domain, is illustrated on examples of unidirectional diffraction of pulses in Bragg and Laue geometries, propagating …
Inhomogeneous broadening of energy levels is one of the principal limiting factors for achieving "slow" or "stationary" light in solid state media by means of electromagnetically induced transparency (EIT), a quantum version of stimulated Raman adiabatic passage (STIRAP). Stark-shift-chirped rapid-adiabatic-passage (SCRAP) has been shown to be far less sensitive to inhomogeneous broadening than STIRAP, a population transfer technique to which it is closely related. We further optimise the pulses used in SCRAP to be even less sensitive to inhomogeneous broadening in a lambda-type three-level sy…
We examine the effect of inhomogeneous broadening on the collective response of a planar metamaterial consisting of asymmetric split ring resonators. We show that such a response leads to a transmission resonance that can persist when the broadening of individual meta-atom resonance frequencies is roughly one half the frequency characterizing the split ring asymmetry. We also find that larger degrees of inhomogeneous broadening can drastically alter the cooperative response, destroying this resonance. The reduced effect of cooperative response due to inhomogeneous broadening may find applicati…
Optical quantum memory with generalized time-reversible atom-light interactions
本文提出一种基于可控退相干的量子存储方案，将光与原子系综的时间可逆相互作用从弱场线性情形推广到强场非线性情形，并建立统一框架以涵盖受控可逆非均匀展宽和原子频率梳等不同实现方式。
A transducer of single photons between microwave and optical frequencies can be used to realize quantum communication over optical fiber links between distant superconducting quantum computers. A promising scalable approach to constructing such a transducer is to use ensembles of quantum emitters interacting simultaneously with electromagnetic fields at optical and microwave frequencies. However, inhomogeneous broadening in the transition frequencies of the emitters can be detrimental to this collective action. In this article, we utilise a gradient-based optimization strategy to design the te…
We present a method for performing quantum state reconstruction on qubits and qubit registers in the presence of decoherence and inhomogeneous broadening. The method assumes only rudimentary single qubit rotations as well as knowledge of decoherence and loss mechanisms. We show that full state reconstruction is possible even in the case where single qubit rotations may only be performed imperfectly. Furthermore we show that for ensemble quantum computing proposals, quantum state reconstruction is possible even if the ensemble experiences inhomogeneous broadening and if only imperfect qubit man…
We show that atoms from wide velocity interval can be concurrently involved in Doppler-free two-photon resonant far from frequency degenerate four-wave mixing with the aid of auxiliary electromagnetic field. This gives rise to substantial enhancement of the output radiation generated in optically thick medium. Numerical illustrations addressed to typical experimental conditions are given.
We study photon emission by an ensemble of two-level systems, with strong inhomogeneous broadening and coupled to a cavity mode whose frequency has linear time-dependence. The analysis shows that, regardless the distribution of energy level splittings, a sharp phase transition occurs between the weak and strong cooperative emission phases near a critical photonic frequency sweeping rate. The associated scaling exponent is determined. We suggest that this phase transition can be observed in an ensemble of negatively charged NV centers in diamond interacting with a microwave half-wavelength cavi…
In large ensembles of identical atoms or spins, the interaction with a mode of the electromagnetic radiation field concentrates in a single superradiant degree of freedom with a collectively enhanced coupling. Given a controllable inhomogeneous broadening, such ensembles may be used for multi-mode storage of quantum states of the radiation field with applications in quantum communication networks and quantum computers. In this paper we analyze how the width and shape of the inhomogeneous broadening influence the collective enhancement and the dynamics of the cavity-ensemble system with focus o…
We demonstrate precision measurement and control of inhomogeneous broadening in a multi-ion clock consisting of three $^{176}$Lu$^+$ ions. Microwave spectroscopy between hyperfine states in the $^3D_1$ level is used to characterise differential systematic shifts between ions, most notably those associated with the electric quadrupole moment. By appropriate alignment of the magnetic field, we demonstrate suppression of these effects to the $\sim 10^{-17}$ level relative to the $^1S_0\leftrightarrow{}^3D_1$ optical transition frequency. Correlation spectroscopy on the optical transition demonstr…
Collective effects in the interaction of light with ensembles of identical scatterers play an important role in many fields of physics. However, often the term ``identical'' is not accurate due to the presence of hyperfine fields which induce inhomogeneous transition shifts and splittings. Here we develop a formalism based on the Green function method to model the linear response of such inhomogeneous ensembles in one-dimensional waveguides. We obtain a compact formula for the collective spectrum, which exhibits deviations from the uniform frequency shift and broadening expected of two level s…
Spin self-organization in an optical cavity facilitated by inhomogeneous broadening
本研究揭示非均匀多普勒展宽可促进光学腔中热原子系综的自旋自组织，降低临界驱动阈值，并引发密度调制与非热态等协同动力学。
A method of reversible quantum optical data storage is presented using resonant Raman field excited spin coherence, where the spin coherence is stored in an inhomogeneously broadened spin ensemble. Unlike the photon echo method, present technique uses a 2 pi Raman optical rephasing pulse, and multimode (parallel) optical channels can be utilized, where the multimode access gives a great benefit to both all-optical and quantum information processing.
We study, theoretically and experimentally, electromagnetically induced transparency (EIT) in two different solid-state systems. Unlike many implementations in homogeneously broadened media, these systems exhibit inhomogeneous broadening of their optical and spin transitions typical of solid-state materials. We observe EIT lineshapes typical of atomic gases, including a crossover into the regime of Autler-Townes splitting, but with the substitution of the inhomogeneous widths for the homogeneous values. We obtain quantitative agreement between experiment and theory for the width of the transpa…
Controlling the Inhomogeneous Broadening and Impedance Matching of a Spin Ensemble
研究通过反亥姆霍兹线圈施加磁场梯度控制自旋系综光谱分布，实现其与传输线阻抗匹配及-50dB吸收，为量子存储器迈出第一步，还建模预测响应并调节耦合转变。
Collective emission of subwavelengths atom-like emitter arrays in the presence of inhomogeneous broadening
实验证明，即使非均匀展宽超过自然线宽两个数量级，金刚石中硅空位中心的亚波长阵列仍能观察到集体发射效应，理论分析解释了非均匀性下集体效应得以保持的机制。
We experimentally demonstrate optical trapping of 87Rb atoms using a two-color evanescent field around an optical nanofiber. In our trapping geometry, a blue-detuned traveling wave whose polarization is nearly parallel to the polarization of a red-detuned standing wave produces significant vector light shifts that lead to broadening of the absorption profile of a near-resonant beam at the trapping site. A model that includes scalar, vector, and tensor light shifts of the probe transition $5S_{1/2}$-$5P_{3/2}$ from the trapping beams, weighted by the temperature-dependent position of the atoms …
We demonstrate photon echoes in Eu$^{3+}$:Y$_{2}$SiO$_{5}$ by controlling the inhomogeneous broadening of the Eu$^{3+}$ $^{7}$F$_{0}\leftrightarrow^{5}$D$_{0}$ optical transition. This transition has a linear Stark shift and we induce inhomogeneous broadening by applying an external electric field gradient. After optical excitation, reversing the polarity of the field rephases the ensemble, resulting in a photon echo. This is the first demonstration of such a photon echo and its application as a quantum memory is discussed.
We investigate theoretically the coupling of a cavity mode to a continuous distribution of emitters. We discuss the influence of the emitters inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Under certain conditions the coupling to the cavity protects the polaritonic states from inhomogeneous broadening, resulting in a longer storage time for a quantum memory based on emitters ensembles. When two different ensembles of emitters are couple…
We address the propagation of a single photon pulse with two polarization components, i.e., a polarization qubit, in an inhomogeneously broadened "phaseonium" Λ-type three-level medium. We combine some of the non-trivial propagation effects characteristic for this kind of coherently prepared systems and the controlled reversible inhomogeneous broadening technique to propose several quantum information processing applications, such as a protocol for polarization qubit filtering and sieving as well as a tunable polarization beam splitter. Moreover, we show that, by imposing a spatial variation o…
Here we propose a solid-state quantum memory that does not require spectral holeburning, instead using strong rephasing pulses like traditional photon echo techniques. The memory uses external broadening fields to reduce the optical depth and so switch off the collective atom-light interaction when desired. The proposed memory should allow operation with reasonable efficiency in a much broader range of material systems, for instance Er3+ doped crystals which have a transition at 1.5 um. We present analytic theory supported by numerical calculations and initial experiments.
We propose a multi-mode quantum memory protocol able to store the quantum state of the field in a microwave resonator into an ensemble of electronic spins. The stored information is protected against inhomogeneous broadening of the spin ensemble by spin-echo techniques resulting in memory times orders of magnitude longer than previously achieved. By calculating the evolution of the first and second moments of the spin-cavity system variables for realistic experimental parameters, we show that a memory based on NV center spins in diamond can store a qubit encoded on the |0> and |1> Fock states …
On Maxwell-Bloch systems with inhomogeneous broadening and one-sided nonzero background
本文针对非均匀展宽两能级系统的Maxwell-Bloch方程，发展了逆散射变换方法，处理未来非零背景的光学脉冲，发现无反射解不存在且孤子伴随辐射，介质最终衰减至基态。
Based on the recent experiments on the hybrid quantum system of a superconducting microwave cavity coupling strongly to an inhomogeneous broadening spin ensemble under an external driving field, we use the exact master equation approach to investigate its non-Markovian decoherence dynamics. Here the spin ensemble is made by negatively charged nitrogen-vacancy (NV) defects in diamond. Our exact master equation theory for open systems depicts the experimental decoherence results and reveals the mechanism how the decoherence induced by the inhomogeneous broadening is suppressed in the strong-coup…
Ensembles of solid state defects in diamond make promising quantum sensors with high sensitivity and spatiotemporal resolution. The inhomogeneous broadening and drive amplitude variations across such ensembles have differing impacts on the sensitivity depending on the sensing scheme used, adding to the challenge of choosing the optimal sensing scheme for a particular sensing regime. In this work, we numerically investigate and compare the predicted sensitivity of schemes based on continuous-wave (CW) optically detected magnetic resonance (ODMR) spectroscopy, pi-pulse ODMR and Ramsey interferom…
We demonstrate that reversible dephasing via inhomogeneous broadening can greatly reduce collective quantum state rotation errors, and observe the suppression of rotation errors by more than 21 dB in the context of collective population measurements of the spin states of an ensemble of $2.1 \times 10^5$ laser cooled and trapped $^{87}$Rb atoms. The large reduction in rotation noise enables direct resolution of spin state populations 13(1) dB below the fundamental quantum projection noise limit. Further, the spin state measurement projects the system into an entangled state with 9.5(5) dB of di…
Origin of the inhomogeneous linewidth in a solid state $^{229}$Th:CaF$_2$ nuclear clock
本研究通过实验与理论结合，揭示固态$^{229}$Th核钟中非均匀线宽源于局部电场梯度变化，随钍浓度线性增加，为设计低展宽核钟材料提供指导。
We propose a scheme for sensing of an oscillating field in systems with large inhomogeneous broadening and driving field variation by applying sequences of phased, adiabatic, chirped pulses. The latter act as a double filter for dynamical decoupling, where the adiabatic changes of the mixing angle during the pulses rectify the signal and partially remove frequency noise. The sudden changes between the pulses act as instantaneous $π$ pulses in the adiabatic basis for additional noise suppression. We also use the pulses' phases to correct for other errors, e.g., due to non-adiabatic couplings. O…
Stability of macroscopic spin ensembles against inhomogeneous dephasing
本文研究自旋猫态在非均匀展宽下的退相干行为，发现小振幅下奇猫态比偶猫态更脆弱，并通过平均场分析揭示驱动-耗散系统中的同步相变及耗散稳定机制，为大振幅自旋猫态的稳定性提供估计。
We study the dynamics of a spin ensemble strongly coupled to a single-mode resonator driven by external pulses. When the mean frequency of the spin ensemble is in resonance with the cavity mode, damped Rabi oscillations are found between the spin ensemble and the cavity mode which we describe very accurately, including the dephasing effect of the inhomogeneous spin broadening. We demonstrate that a precise knowledge of this broadening is crucial both for a qualitative and a quantitative understanding of the temporal spin-cavity dynamics. On this basis we show that coherent oscillations between…
We demonstrate active control of inhomogeneous dephasing and rephasing for single collective atomic spin excitations (spin-waves) created by spontaneous Raman scattering in a quantum memory based on cold $^{87}$Rb atoms. The control is provided by a reversible external magnetic field gradient inducing an inhomogeneous broadening of the atomic hyperfine levels. We demonstrate experimentally that active rephasing preserves the single photon nature of the retrieved photons. Finally, we show that the control of the inhomogeneous dephasing enables the creation of time-separated spin-waves in a sing…
Enhancement of femtosecond photon echo signals from an inhomogeneously broadened InAs quantum dot ensemble using chirped pulses
本文实验演示了利用啁啾脉冲实现绝热快速通过增强的飞秒光子回波，在InAs量子点系综中实现3.2倍回波效率提升，为太赫兹超快光通信提供稳健方案。
We theoretically investigate the transport properties of a weak coherent input field scattered by an ensemble of $Λ$-type atoms coupled to a one-dimensional photonic crystal waveguide. In our model, the atoms are randomly located in the lattice along the crystal axis. We analyze the transmission spectrum mediated by the tunable long-range atomic interactions, and observe the highest-energy dip. The results show that the highest-energy dip location is associated with the number of the atoms, which provides an accurate measuring tool for the emitter-waveguide system. We also quantify the influen…
The possibility of using a solid medium to store few-photon laser pulses as coupled excitations between light and matter is investigated. The role of inhomogeneous broadening and nonadiabaticity are considered, and conditions governing the feasibility of the scheme are derived. The merits of a number of classes of solid are examined.
We have analyzed an efficient integration of the multi-qubit echo quantum memory into the quantum computer scheme on the atomic resonant ensembles in quantum electrodynamics cavity. Here, one atomic ensemble with controllable inhomogeneous broadening is used for the quantum memory node and other atomic ensembles characterized by the homogeneous broadening of the resonant line are used as processing nodes. We have found optimal conditions for efficient integration of multi-qubit quantum memory modified for this analyzed physical scheme and we have determined a specified shape of the self tempor…
Continuous change of the propagation direction of a classical control field in the process of its off-resonant Raman interaction with a weak signal field in a three-level atomic medium is suggested for quantum storage of a single-photon wave packet. It is shown that due to phase matching condition such an angular control allows one to reversibly map the single-photon wave packet to the Raman spatial coherence grating. Thus, quantum storage and retrieval can be realized without using inhomogeneous broadening of the atomic transitions or manipulating the amplitude of the control field. Under som…
We introduce a figure of merit for a quantum memory which measures the preservation of entanglement between a qubit stored in and retrieved from the memory and an auxiliary qubit. We consider a general quantum memory system consisting of a medium of two level absorbers, with the qubit to be stored encoded in a single photon. We derive an analytic expression for our figure of merit taking into account Gaussian fluctuations in the Hamiltonian parameters, which for example model inhomogeneous broadening and storage time dephasing. Finally we specialize to the case of an atomic quantum memory wher…
We investigate the performance of inhomogeneously broadened spin ensembles as quantum memories under continuous dynamical decoupling. The role of the continuous driving field is two-fold: first, it decouples individual spins from magnetic noise; second and more important, it suppresses and reshapes the spectral inhomogeneity of spin ensembles. We show that a continuous driving field, which itself may also be inhomogeneous over the ensemble, can enhance the decay of the tails of the inhomogeneous broadening distribution considerably. This fact enables a spin ensemble based quantum memory to exp…
Optimally Controlled Storage of a Qubit in an Inhomogeneous Spin Ensemble
研究通过优化腔体调制，提升自旋集体中量子比特寿命，克服不均匀展宽和腔体衰减的影响。
Lineshape Optimization in Inhomogeneous $Λ$-type Quantum Memory
本研究针对非均匀展宽$\Lambda$型量子存储器，优化激发态线形以提升存储效率，并与AFC协议对比，通过数值方法实现协议无关的最优线形设计。
We perform spectroscopy on the hyperfine splitting of $^{85}$Rb atoms trapped in far-off-resonance optical traps. The existence of a spatially dependent shift in the energy levels is shown to induce an inherent dephasing effect, which causes a broadening of the spectroscopic line and hence an inhomogeneous loss of atomic coherence at a much faster rate than the homogeneous one caused by spontaneous photon scattering. We present here a number of approaches for reducing this inhomogeneous broadening, based on trap geometry, additional laser fields, and novel microwave pulse sequences. We then sh…
We study the processes in a quantum dot and its surrounds under resonant excitation with the addition of weak non-resonant light. We observe a decrease in inhomogeneous emission linewidth, as well as previously observed enhancement of resonant fluorescence (RF). Scanning excitation and detection frequencies, we distinguish between homogeneous and inhomogeneous broadening. Monte Carlo simulations model the enhanced RF only if we include charge-carrier loss from the quantum dot induced by the resonant laser. The cause of the linewidth narrowing is predominantly independent of the enhanced RF.
Parrondo's paradox in quantum walks with inhomogeneous coins
本文研究离散时间量子行走中的 Parrondo 悖论，证明仅采用时空依赖的非均匀硬币即可实现两种失败策略组合获胜，无需高维硬币或退相干，从而提升实验可行性并拓展量子输运应用。
A very promising recent trend in applied quantum physics is to combine the advantageous features of different quantum systems into what is called "hybrid quantum technology". One of the key elements in this new field will have to be a quantum memory enabling to store quanta over extended periods of time. Systems that may fulfill the demands of such applications are comb-shaped spin ensembles coupled to a cavity. Due to the decoherence induced by the inhomogeneous ensemble broadening, the storage time of these quantum memories is, however, still rather limited. Here we demonstrate how to overco…
We characterize the positively charged exciton (X1+) in single InGaAs quantum dots using resonant laser spectroscopy. Three samples with different dopant species (Be or C as acceptors, Si as a donor) are compared. The p-doped samples exhibit larger inhomogeneous broadening (x3) and smaller absorption contrast (x10) than the n-doped sample. For X1+ in the Be-doped sample, a dot dependent non-linear Fano effect is observed, demonstrating coupling to degenerate continuum states. However, for the C-doped sample the X1+ lineshape and saturation broadening follows isolated atomic transition behaviou…
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