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arXiv 0812.3713cond-mat.mes-hall
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单分子磁体自旋偏置驱动的磁化反转及无损检测

Spin-bias driven magnetization reversal and nondestructive detection in a single molecular magnet

Hai-Zhou Lu, Bin Zhou, Shun-Qing Shen

摘要:

利用速率方程,对具有自旋相关化学势分裂(自旋偏置)的弱耦合单分子磁体(SMM)的磁化反转进行了理论研究.反转点的雪崩动力学证明了反转的微观机制。作为自旋偏置的函数的磁化强度示出了可由栅极电压调谐并且随温度变化的磁滞回线。通过测量小自旋偏压下的全极化电流,实现了SMM中巨自旋取向的无损测量。对于Mn $_{12}$ ac分子,其小的横向各向异性仅略微违反上述结果。当SMM的易磁化轴和电极的自旋量子化方向之间存在夹角时,也进行了研究。

英文摘要:

The magnetization reversal in a single molecular magnet (SMM) weakly coupled to an electrode with spin-dependent splitting of chemical potentials (spin bias) is theoretically investigated by means of the rate equation. A microscopic mechanism for the reversal is demonstrated by the avalanche dynamics at the reversal point. The magnetization as a function of the spin bias shows hysteresis loops tunable by the gate voltage and varying with temperature. The nondestructive measurement to the orientation of giant spin in SMM is presented by measuring the fully polarized electric current in the response to a small spin bias. For Mn$_{12}$ac molecule, its small transverse anisotropy only slightly violates the results above. The situation when there is an angle between the easy axis of the SMM and the spin quantization direction of the electrode is also studied.

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