We have considered the effect of different spin-orbit interaction mechanisms on the process of demagnetization under the influence of short-pulse lasers. All-optical magnetization reversal of perpendicularly magnetized thin films can occur if there are sufficient strong spin-Hall, skew scattering, and Rashba interactions. In the presence of spin-orbit interactions, the transient charge currents provide the generation of transverse-spin currents and accumulations, which eventually exert spin-transfer torque on the magnetization. By combining the optically excited spin-dependent diffusive transport with the spin and charge currents due to skew scattering, spin-Hall, inverse spin-Hall and Rashba interactions, into a numerical model, we demonstrate a possibility of ultra-fast all-optical magnetization reversal. This understanding provokes intriguing, more in-depth experimental studies on the role of spin-orbit interaction mechanisms in optimizing structures for all-optical magnetization reversal.
We show theoretically that strong electron coupling to circularly polarized photons in non-singly-connected nanostructures results in the appearance of an artificial gauge field that changes the electron phase. The effect arises from the breaking of time-reversal symmetry and is analogous to the well-known Aharonov-Bohm phase effect. It can manifest itself in the oscillations of conductance as a function of the intensity and frequency of the illumination. The theory of the effect is elaborated for mesoscopic rings in both ballistic and diffusive regimes.
The diversity of various manganese types and its complexes in the Mn-doped ${\rm A^{III}B^V}$ semiconductor structures leads to a number of intriguing phenomena. Here we show that the interplay between the ordinary substitutional Mn acceptors and interstitial Mn donors as well as donor-acceptor dimers could result in a reversal of electron magnetization. In our all-optical scheme the impurity-to-band excitation via the Mn dimers results in direct orientation of the ionized Mn-donor $d$ shell. A photoexcited electron is then captured by the interstitial Mn and the electron spin becomes parallel…
We report measurements of thermopower oscillations $vs$ magnetic field in a diffusive Andreev interferometer. Upon the increase of the dc current applied to the heater electrodes, the amplitude of these oscillations first increases then goes to zero as one would expect. Surprisingly, the oscillations reappear at yet higher heater currents with their phase being $π$-shifted compared to low current values. From direct measurements of the temperature gradient we estimate the amplitude of the oscillations to be orders of magnitude smaller than predicted by theory.
The asymptotic behavior of switching time as a function of current for a uniaxial macrospin under the effects of both spin-torque and thermal noise is explored analytically by focusing on its diffusive energy space dynamics. The scaling dependence ($I\rightarrow 0$, $<τ\propto\exp(-ξ(1-I)^2)$) is shown to confirm recent literature results. The analysis shows the mean switching time to be functionally independent of the angle between the spin current and magnet's uniaxial axes. These results have important implications for modeling the energetics of thermally assisted magnetization reversal of …
Near-infrared magneto-optical spectroscopy of single-walled carbon nanotubes reveals two absorption peaks with an equal strength at high magnetic fields ($>$ 55 T). We show that the peak separation is determined by the Aharonov-Bohm phase due to the tube-threading magnetic flux, which breaks the time-reversal symmetry and lifts the valley degeneracy. This field-induced symmetry breaking thus overcomes the Coulomb-induced intervalley mixing which is predicted to make the lowest exciton state optically inactive (or ``dark'').
We present an extensive Monte Carlo study on light transport in optically thin slabs, addressing both axial and transverse propagation. We completely characterize the so-called ballistic-to-diffusive transition, notably in terms of the spatial variance of the transmitted/reflected profile. We test the validity of the prediction cast by diffusion theory, that the spatial variance should grow independently of absorption and, to a first approximation, of the sample thickness and refractive index contrast. Based on a large set of simulated data, we build a freely available look-up table routine al…
Monolayer valley semiconductors, such as tungsten diselenide (WSe$_2$), possess valley pseudospin degrees of freedom that are optically addressable but degenerate in energy. Lifting the energy degeneracy by breaking time-reversal symmetry is vital for valley manipulation. This has been realized by directly applying magnetic fields or via pseudo-magnetic fields generated by intense circularly polarized optical pulses. However, sweeping large magnetic fields is impractical for devices, and the pseudo-magnetic fields are only effective in the presence of ultrafast laser pulses. The recent rise of…
We theoretically study spin and charge currents through finite-size two-dimensional $s$-wave superconductor/uniform ferromagnet/s-wave superconductor (SFS) junctions with intrinsic spin-orbit interactions (ISOIs) using a quasiclassical approach. Considering experimentally realistic parameters, we demonstrate that the combination of spontaneously broken time-reversal symmetry and lack of inversion symmetry can result in spontaneously accumulated spin currents at the edges of finite-size two-dimensional magnetic SF hybrids. Due to the spontaneous edge spin accumulation, the corners of the F wire…
We present Fokker-Planck equations that describe transport of heat and spin in dirty unconventional superconducting quantum wires. Four symmetry classes are distinguished, depending on the presence or absence of time-reversal and spin rotation invariance. In the absence of spin-rotation symmetry, heat transport is anomalous in that the mean conductance decays like $1/\sqrt{L}$ instead of exponentially fast for large enough length $L$ of the wire. The Fokker-Planck equations in the presence of time-reversal symmetry are solved exactly and the mean conductance for quasiparticle transport is calc…
The conductance of a quantum wire with off-diagonal disorder that preserves a sublattice symmetry (the random hopping problem with chiral symmetry) is considered. Transport at the band center is anomalous relative to the standard problem of Anderson localization both in the diffusive and localized regimes. In the diffusive regime, there is no weak-localization correction to the conductance and universal conductance fluctuations are twice as large as in the standard cases. Exponential localization occurs only for an even number of transmission channels in which case the localization length does…
Many proposed experiments involving topological insulators (TIs) require spatial control over time-reversal symmetry and chemical potential. We demonstrate reconfigurable micron-scale optical control of both magnetization (which breaks time-reversal symmetry) and chemical potential in ferromagnetic thin films of Cr-(Bi,Sb)$_2$Te$_3$ grown on SrTiO$_3$. By optically modulating the coercivity of the films, we write and erase arbitrary patterns in their remanent magnetization, which we then image with Kerr microscopy. Additionally, by optically manipulating a space charge layer in the underlying …
We study the quantum diffusive transport of multivalley massive Dirac cones, where time-reversal symmetry requires opposite spin orientations in inequivalent valleys. We show that the intervalley scattering and intravalley scattering can be distinguished from the quantum conductivity that corrects the semiclassical Drude conductivity, due to their distinct symmetries and localization trends. In immediate practice, it allows transport measurements to estimate the intervalley scattering rate in hole-doped monolayers of group-VI transition metal dichalcogenides (e.g., molybdenum dichalcogenides a…
The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely valuable stimuli for the all-optical magnetisation reversal in ferrimagnetic and ferromagnetic alloys and multilayers, while this remains elusive in elementary ferromagnets. Here we demonstrate that a single laser pulse with sub-picosecond duration can lead to the reversal of the magnetisation of bulk nickel, in tandem with the expected demagnetisation. As …
The low sensitivity of photons to external magnetic fields is one of the major challenges for the engineering of photonic lattices with broken time-reversal symmetry. Here we show that time-reversal symmetry can be broken for microcavity polaritons in the absence of any external magnetic field thanks to polarization dependent polariton interactions. Circularly polarized excitation of carriers in a micropillar induces a Zeeman-like energy splitting between polaritons of opposite polarizations. In combination with optical spin-orbit coupling inherent to semiconductor microstructures, the interac…
We describe a theoretical approach for spin-polarized hot-electron transport, as it occurs after excitation by ultrafast optical pulses in heterostructures formed by ferromagnetic and normal metals. We formulate a spin-dependent particle-in-cell model that solves the Boltzmann equation for excited electrons. It includes lifetimes and transmission coefficients as parameters, which can be taken from ab-initio calculations or experiment, and can be easily extended to multilayer systems. This approach is capable of describing electron transport in the ballistic, super-diffusive and diffusive regim…
We present a description of spin-polarized transport in mesoscopic ferromagnet-superconductor (F/S) systems, where the transport is diffusive, and the interfaces are transparent. It is shown that the spin reversal associated with Andreev reflection generates an excess spin density close to the F/S interface, which leads to a spin contact resistance. Expressions for the contact resistance are given for two terminal and four terminal geometries. In the latter the sign depends on the relative magnetization of the ferromagnetic electrodes.
Polariton polarization can be described in terms of a pseudospin which can be oriented along the $x,\,y,$ or $z$ axis, similarly to electron and hole spin. Unlike electrons and holes where time-reversal symmetry requires that the spin-orbit interaction be odd in the momentum, the analogue of the spin-orbit interaction for polaritons, the so-called TE-TM splitting, is even in the momentum. We calculate and compare spin transport of polariton, electron, and hole systems, in the diffusive regime of many scatterings. After dimensional rescaling diffusive systems with spatially uniform particle den…
We report about the anomalous Hall effect in 4f 3d metallic alloys measured using terahertz time-domain spectroscopy. The strength of the observed terahertz spin-dependent transport phenomenon is in good agreement with expectations based on electronic transport measurements. Employing this effect, we succeeded to reveal ultrafast dynamics of the anomalous Hall effect which accompanies the sub-100 picosecond optically induced magnetization reversal in a GdFeCo alloy. The experiments demonstrate the ability to control currents at terahertz frequencies in spintronic devices magnetically and ultra…
