We demonstrate that left-handed resonance transmission from metallic metamaterial, composed of periodically arranged double rings, can be extended to visible spectrum by introducing an active medium layer as the substrate. The severe ohmic loss inside metals at optical frequencies is compensated by stimulated emission of radiation in this active system. Due to the resonance amplification mechanism of recently proposed lasing spaser, the left-handed transmission band can be restored up to 610 nm wavelength, in dependence on the gain coefficient of the active layer. Additionally, threshold gains for different scaling levels of the double-ring unit are investigated to evaluate the gain requirement of left-handed transmission restoration at different frequency ranges.
We derive the formula of the complex Doppler shift in a two-dimensional, dispersive metamaterial and we show that a moving, monochromatic radiation source generates multiple frequency modes. The role of the group velocity is stressed and the Doppler shifted radiation field exhibits features of the Cherenkov effect. The presented theory is also applicable to the case of a moving, nonoscillating charge and explains many peculiar characteristics of the Cherenkov radiation in lefthanded metamaterials such as the backward direction of power emission, the constant radiation angle and the lack of vel…
The Doppler shift is investigated in one-dimensional system with moving source. Theoretical findings are confirmed in numerical simulations of optical and acoustical waves propagation in simple metamaterial model, showing the reversed shift and the existence of multiple frequency modes. The properties of these waves are discussed. The effect of absorption on the phenomenon is outlined.
In recent years, there has been increasing interest in studying the quantum characteristics in plasmonic metamaterials. By using the Hamiltonian combined with second quantization, we have investigated the basic excitation of the coupled metamaterials and presented a quantum description of them. The interaction between the excitation of the coupled metamaterial and the exciton in the quantum dot material has been further considered with the aid of the interaction Hamiltonian. In such a damping system, a set of Langevin equations has been used to deal with the quantum motion of the system. And t…
We compute the SBS gain for a metamaterial comprising a cubic lattice of dielectric spheres suspended in a background dielectric material. Theoretical methods are presented to calculate the optical, acoustic, and opto-acoustic parameters that describe the SBS properties of the material at long wavelengths. Using the electromagnetic and strain energy densities we accurately characterise the optical and acoustic properties of the metamaterial. From a combination of energy density methods and perturbation theory, we recover the appropriate terms of the photoelastic tensor for the metamaterial. We…
A bulk left-handed metamaterial with fishnet structure is investigated to show the optical loss compensation via surface plasmon amplification, with the assistance of a Gaussian gain in PbS quantum dots. The optical resonance enhancement around 200 THz is confirmed by the retrieval method. By exploring the dependence of propagation loss on the gain coefficient and metamaterial thickness, we verify numerically that the left-handed response can endure a large propagation thickness with ultralow and stable loss under a certain gain coefficient.
Using full opto-acoustic numerical simulations, we demonstrate enhancement and suppression of the SBS gain in a metamaterial comprising a subwavelength cubic array of dielectric spheres suspended in a dielectric background material. We develop a general theoretical framework and present several numerical examples using technologically important materials. For As$_2$S$_3$ spheres in silicon, we achieve a gain enhancement of more than an order of magnitude compared to pure silicon, and for GaAs spheres in silicon, full suppression is obtained. The gain for As$_2$S$_3$ glass can also be strongly …
In this paper we explored the scattering behavior of thin cylinders made of LHM and coated by a monoatomic graphene layer. A spectral tunability of the resonance peaks is evidenced by altering the chemical potential of the graphene coating, a fact that occurs at any state of polarization of the incident plane wave in opposition to the case of scatterers of dielectric core. On the contrary, no invisibility condition can be satisfied for dielectric environments. A singular performance is also found for cylinders with permittivity and permeability near zero. Practical implementations of our resul…
We perform a theoretical investigation on the Goos-Hächen (GH) shift in one-dimensional photonic crystals (1DPCs) containing left-handed metamaterials (LHMs). We find an unusal effect of the GH shift near the photonic band-crossing structure, which is located at the condition, $% -k_{z}^{(A)}d_{A}=k_{z}^{(B)}d_{B}=mπ$ $(m=1,2,3...)$, under the inclined incident angle, here A denotes the LHM layer and B denotes the dielectric layer. Above the frequency of the band-crossing point (BCP), the GH shift changes from negative to positive as the incident angle increases, while the GH shift changes rev…
Electromagnetic metamaterials are man-made structures that have novel properties such as a negative refraction index, not attainable in naturally occurring materials. Although negative index materials (NIMs) in microwave frequencies were demonstrated in 2001, it has remained challenging to design NIMs for optical frequencies especially those with both negative permittivity and negative permeability [known as left-handed metamaterials (LHMs)]. Here, by going beyond the traditional concept of the combination of artificial electronic and magnetic meta-atoms to design NIMs, we propose a novel LHM …
We suggest a principle for isolation of circularly polarized waves in magnetically active extreme-parameter metamaterials. Using theoretical analysis and numerical simulations, we show that metamaterials with extreme parameters, such as epsilon-near-zero materials (ENZ), when merged with magneto-optical materials, become transparent for forward circularly polarized waves of a given handedness and opaque for backward propagating waves of the same handedness. We theoretically study two possible implementations of such hybrid materials: (1) the case of metal-dielectric stacks; and (2) rectangular…
Using detailed simulations we investigate the magnetic response of metamaterials consisting of pairs of parallel slabs or combinations of slabs with wires (including the fishnet design) as the length-scale of the structures is reduced from mm to nm. We observe the expected saturation of the magnetic resonance frequency when the structure length-scale goes to the sub-micron regime, as well as weakening of the effective permeability resonance and reduction of the spectral width of the negative permeability region. All these results are explained by using an equivalent resistor-inductor-capacitor…
It is shown that artificial magnetism with relatively large frequency bandwidth can be obtained from periodic arrangements of dielectric rings. Combined with dielectric rods, dielectric rings can provide 3D isotropic left-handed metamaterials being an advantageous alternative to metallic split ring resonators and/or metallic wires when un-detectability by low frequency external magnetic fields is desired. Furthermore it is shown that dielectric rings can be also combined with natural plasma-like media to obtain a left-handed metamaterial.
The electronic Lorentz theory is employed to determine the electromagnetic response of planar split-ring metamaterials. Starting from the dynamics of individual free carriers, the effective permittivity tensor of the metamaterial is calculated. Whenever the split ring lacks in-plane mirror symmetry, the corresponding permittivity tensor has a crystallographic structure of an elliptically dichroic medium, and the metamaterial exhibits optical properties of planar chiral structures. Its transmission spectra are different for right-handed vs. left-handed circular polarization of the incident wave…
We show for the first time that a planar metamaterial, an array of coupled metal split-ring resonators with a unit cell lacking mirror symmetry, exhibits asymmetric transmission of terahertz radiation (0.25-2.5 THz) propagating through it in opposite directions. This intriguing effect, that is compatible with Lorentz reciprocity and time-reversal, depends on a directional difference in conversion efficiency of the incident circularly polarized wave into one of opposite handedness, that is only possible in lossy low-symmetry planar chiral metamaterials. We show that asymmetric transmission is l…
We investigate numerically Fano resonances excited in periodic arrays of dielectric, metallic and left-handed cylinders. Of particular interest are Fano resonances excited in the linear array of cylin- ders. We analyze spatial distribution and symmetry of electromagnetic field and discuss the relation between observed Fano resonances and frequency spectra of two-dimensional arrays of cylinders.
Anisotropic homogeneous metamaterials that are neither wholly dissipative nor wholly active at a specific frequency are permitted by classical electromagnetic theory. Well-established homogenization formalisms indicate that such a metamaterial may be realized quite simply as a random mixture of electrically small (possibly nanoscale) spheroidal particles of at least two different isotropic dielectric materials, one of which must be dissipative but the other active. The dielectric properties of this metamaterial are influenced by the volume fraction, spatial distribution, particle shape and siz…
In nature, the beetle Chrysina gloriosa derives its iridescence by selectively reflecting left-handed circularly polarized light only. Here, for the first time, we introduce and demonstrate the optical analogue based on an ultrathin metamaterial, which we term circular dichroic metamirror. A general method to design the circular dichroic metasmirror is presented under the framework of Jones calculus. It is analytically shown that the metamirror can be realized by two layers of anisotropic metamaterial structures, in order to satisfy the required simultaneous breakings of n-fold rotational (n>2…
We review some recent (mostly ours) results on the Anderson localization of light and electron waves in complex disordered systems, including: (i) left-handed metamaterials, (ii) magneto-active optical structures, (iii) graphene superlattices, and (iv) nonlinear dielectric media. First, we demonstrate that left-handed metamaterials can significantly suppress localization of light and lead to an anomalously enhanced transmission. This suppression is essential at the long-wavelength limit in the case of normal incidence, at specific angles of oblique incidence (Brewster anomaly), and in the vici…
We have developed an approach allowing us to resolve the problem of non-conventional Anderson localization emerging in bilayered periodic-on-average structures with alternating layers of right-handed and left-handed materials. Recently, it was numerically discovered that in such structures with weak fluctuations of refraction indices, the localization length $L_{loc}$ can be enormously large for small wave frequencies $ω$. Within the fourth order of perturbation theory in disorder, $σ^2 \ll 1$, we derive the expression for $L_{loc}$ valid for any $ω$. In the limit $ω\rightarrow 0$ one gets a q…
We provide rigorous numerical calculations (using the rigorous coupled-wave analysis) of transmission spectra of various metallic and metamaterial one-dimensional gratings and identify plasmonic resonances responsible for enhanced transmission. We argue that the most important mechanism which influences the resonant transmission is the coupling of incident electromagnetic wave with two plasmonic waves: lengthwise plasmons, which propagates along the grating, and crosswise plasmons excited in air gaps.
Isotropic negative index metamaterials (NIMs) are highly desired, particularly for the realization of ultra-high resolution lenses. However, existing isotropic NIMs function only two-dimensionally and cannot be miniaturized beyond microwaves. Direct laser writing processes can be a paradigm shift toward the fabrication of three-dimensionally (3D) isotropic bulk optical metamaterials, but only at the expense of an additional design constraint, namely connectivity. Here, we demonstrate with a proof of-principle design that the requirement connectivity does not preclude fully isotropic left-hande…
Recently it was discovered that periodic lattices of metamaterial scatterers show optical activity, even if the scatterers or lattice show no 2D or 3D chirality, if the illumination breaks symmetry. In this Letter we demonstrate that such `pseudo-chirality' is intrinsic to any single planar metamaterial scatterer and in fact has a well-defined value at a universal bound. We argue that in any circuit model, a nonzero electric and magnetic polarizability derived from a single resonance automatically imply strong bianisotropy, i.e., magneto-electric cross polarizability at the universal bound set…
Chirality Inversion and Giant Optical Activity in Scalable Self-Assembled Metamaterials
Max Planck Institute of Colloids and Interfaces (MPIKG)（马克斯·普朗克胶体与界面研究所）；Department of Chemistry, University of Cambridge（剑桥大学化学系）；Institute of Light and Matter, Claude Bernard University Lyon 1, CNRS（里昂第一大学克劳德·贝尔纳大学光与物质研究所，法国国家科学研究中心）
We explore the optical properties of periodic layered media containing left-handed metamaterials. This study is based on several analogies between the propagation of light in metamaterials and charge transport in graphene. We derive the conditions for these two problems become equivalent, i.e., the equations and the boundary conditions when the corresponding wave functions coincide. We show that the photonic band-gap structure of a periodic system built of alternating left- and right-handed dielectric slabs contains conical singularities similar to the Dirac points in the energy spectrum of ch…
Optical systems with gain and loss that respect Parity-Time (PT) symmetry can have real eigenvalues despite their non-Hermitian character. Chiral systems impose circularly polarized waves which do not preserve their handedness under the combined space- and time- reversal operations and, as a result, seem to be incompatible with systems possessing PT symmetry. Nevertheless, in this work we show that in certain configurations, PT symmetric permittivity, permeability and chirality is possible; in addition, real eigenvalues are maintained even if the chirality goes well beyond PT symmetry. By obta…
Chiroptical effects, characterized by different optical responses for left- (LCP) and right- handed circularly polarized light (RCP), are powerful and valuable tools in optics with wide applications in polarization resolved imaging and sensing. Previously observed strong chiroptical effects are limited to metamaterials with complex three-dimensional chiral structures at the sub-wavelength scale. Although asymmetrical transmission of LCP and RCP have been investigated in planar chiral metasurfaces, the observed weak chiroptical effects result from anisotropic Ohmic dissipation of the metal cons…
We report on the theoretical investigation of the plasmonic wave propagation in the coaxial cylindrical cables fabricated of both right-handed medium (RHM) [with $ε>0$, $μ>0$] and left-handed medium (LHM) [with $ε(ω) <0$, $μ(ω) <0$], using a Green-function (or response function) theory in the absence of an applied magnetic field. The Green-function theory generalized to be applicable to such quasi-one dimensional systems enables us to derive explicit expressions for the corresponding response functions (associated with the EM fields), which can in turn be used to derive various physical proper…
The polarization controlled optical signal routing has many important applications in photonics such as polarization beam splitter. By using two-dimensional transmission lines with lumped elements, we experimentally demonstrate the selective excitation of guided modes in waveguides composed of two kinds of single-negative metamaterials. A localized, circularly polarized emitter placed near the interface of the two kinds of single-negative metamaterials only couples with one guided mode with a specific propagating direction determined by the polarization handedness of the source. Moreover, this…
It is evidenced by numerical calculations that optically pumped graphene is suitable for compensating inherent loss in terahertz (THz) metamaterials. In a first step, the complex conductivity of graphene under optical pumping is calculated and the proper conditions for terahertz amplification in single layer graphene are determined. It is shown that amplification in graphene occurs for temperatures up to room temperature and for moderate pump intensities when pumped at a telecommunication wavelength $λ=1.5~\mathrm{μm}$. Furthermore, the amplification properties of graphene are evaluated and di…
Although the invention of the metamaterials has stimulated the interest of many researchers and possesses many important applications, the basic design idea is very simple: composing effective media from many small structured elements and controlling its artificial EM properties. According to the effective-media model, the coupling interactions between the elements in metamaterials are somewhat ignored; therefore, the effective properties of metamaterials can be viewed as the "averaged effect" of the resonance property of the individual elements. However, the coupling interaction between eleme…
Over the past two decades, metamaterials have led to an increasing number of biosensing and nanophotonic applications due to the possibility of a careful control of light propagating through subwavelength features. Chiral nanostructures (characterized by the absence of any mirror symmetry), in particular, give rise to unique chiro-optical properties such as circular dichroism and optical activity. Here, we present a gyroid optical metamaterial with a periodicity of 65 nm exhibiting a strong circular dichroism at visible wavelengths. Our bottom-up approach, based on metallic replication of the …
