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arXiv 0810.3502cond-mat.str-el
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LaMn $_{1-x}$ Fe $_{x}$ O $_3$中的极化子弛豫和跳跃电导

Polaron relaxation and hopping conductivity in LaMn$_{1-x}$Fe$_{x}$O$_3$

A. Karmakar, S. Majumdar, S. Giri

摘要:

研究了LaMn $_{1-x}$ Fe $_{x}$ O $_3$(0 $\leq x \leq$ 1.0)样品的直流和交流输运性质以及电模量谱。体直流电阻率示出了与在低温下的可变范围跳跃机制和在高温下的Arrhenius机制一致的温度变化。已经发现,在有限的温度和频率范围内,交流电导率遵循幂律行为,其中安德森局域化在所有组合物的传输机制中起着重要作用。在低温下,所有组合物的大直流电阻率和介电弛豫行为与载流子的极化性质一致。缩放的模量谱表明,电荷传输动力学是独立的温度为一个特定的组合物,但强烈依赖于不同的组合物可能是由于不同的载流子浓度和结构特性。

英文摘要:

Dc and ac transport properties as well as electric modulus spectra have been investigated for the samples LaMn$_{1-x}$Fe$_{x}$O$_3$ with compositions 0 $\leq x \leq$ 1.0. The bulk dc resistivity shows a temperature variation consistent with the variable range hopping mechanism at low temperature and Arrhenius mechanism at high temperatures. The ac conductivity has been found to follow a power law behavior at a limited temperature and frequency region where Anderson-localization plays a significant role in the transport mechanism for all the compositions. At low temperatures large dc resistivities and dielectric relaxation behavior for all the compositions are consistent with the polaronic nature of the charge carriers. Scaling of the modulus spectra shows that the charge transport dynamics is independent of temperature for a particular composition but depends strongly on different compositions possibly due to different charge carrier concentrations and structural properties.

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