We describe an ion-based cavity-QED system in which the internal dynamics of an atom is coupled to the modes of an optical cavity by vacuum-stimulated Raman transitions. We observe Raman spectra for different excitation polarizations and find quantitative agreement with theoretical simulations. Residual motion of the ion introduces motional sidebands in the Raman spectrum and leads to ion delocalization. The system offers prospects for cavity-assisted resolved-sideband ground-state cooling and coherent manipulation of ions and photons.
We have constructed an apparatus containing a linear ion trap and a high-finesse optical cavity in the ultraviolet spectral range. In our construction, we have avoided all organic materials inside the ultrahigh vacuum chamber. We show that, unlike previously reported, the optical cavity does not degrade in performance over a time scale of 9 months.
We report on the first observation of stimulated Raman scattering from a Lambda-type three-level atom, where the stimulation is realized by the vacuum field of a high-finesse optical cavity. The scheme produces one intracavity photon by means of an adiabatic passage technique based on a counter-intuitive interaction sequence between pump laser and cavity field. This photon leaves the cavity through the less-reflecting mirror. The emission rate shows a characteristic dependence on the cavity and pump detuning, and the observed spectra have a sub-natural linewidth. The results are in excellent a…
An extensive characterization of high finesse optical cavities used in cavity QED experiments is described. Different techniques in the measurement of the loss and phase shifts associated with the mirror coatings are discussed and their agreement shown. Issues of cavity field mode structure supported by the dielectric coatings are related to our effort to achieve the strongest possible coupling between an atom and the cavity.
Transits of single atoms through higher-order Hermite-Gaussian transverse modes of a high-finesse optical cavity are observed. Compared to the fundamental Gaussian mode, the use of higher-order modes increases the information on the atomic position. The experiment is a first experimental step towards the realisation of an atomic kaleidoscope.
Individual laser cooled atoms are delivered on demand from a single atom magneto-optic trap to a high-finesse optical cavity using an atom conveyor. Strong coupling of the atom with the cavity field allows simultaneous cooling and detection of individual atoms for time scales exceeding 15 s. The single atom scatter rate is studied as a function of probe-cavity detuning and probe Rabi frequency, and the experimental results are in good agreement with theoretical predictions. We demonstrate the ability to manipulate the position of a single atom relative to the cavity mode with excellent control…
We report on collective non-linear dynamics in an optical lattice formed inside a high finesse ring cavity in a so far unexplored regime, where the light shift per photon times the number of trapped atoms exceeds the cavity resonance linewidth. We observe bistability and self-induced squeezing oscillations resulting from the retro-action of the atoms upon the optical potential wells. We can well understand most of our observations within a simplified model assuming adiabaticity of the atomic motion. Non-adiabatic aspects of the atomic motion are reproduced by solving the complete system of cou…
We present a novel microfabricated optical cavity, which combines a very small mode volume with high finesse. In contrast to other micro-resonators, such as microspheres, the structure we have built gives atoms and molecules direct access to the high-intensity part of the field mode, enabling them to interact strongly with photons in the cavity for the purposes of detection and quantum-coherent manipulation. Light couples directly in and out of the resonator through an optical fibre, avoiding the need for sensitive coupling optics. This renders the cavity particularly attractive as a component…
The quadrupole S$_{1/2}$ -- D$_{5/2}$ optical transition of a single trapped Ca$^+$ ion, well suited for encoding a quantum bit of information, is coherently coupled to the standing wave field of a high finesse cavity. The coupling is verified by observing the ion's response to both spatial and temporal variations of the intracavity field. We also achieve deterministic coupling of the cavity mode to the ion's vibrational state by selectively exciting vibrational state-changing transitions and by controlling the position of the ion in the standing wave field with nanometer-precision.
Cross-phase modulation at the single-photon level has a wide variety of fundamental applications in quantum optics including the generation of macroscopic entangled states. Here we describe a practical method for producing a weak cross-phase modulation at the single-photon level using metastable xenon in a high finesse cavity. We estimate the achievable phase shift and give a brief update on the experimental progress towards its realization. A single-photon cross-phase modulation of approximately 20 milliradians is predicted by both a straightforward perturbation theory calculation and a numer…
When an off-resonant light field is coupled with atomic spins, its polarization can rotate depending on the direction of the spins via a Faraday rotation which has been used for monitoring and controlling the atomic spins. We observed Faraday rotation by an angle of more than 10 degrees for a single 1/2 nuclear spin of 171Yb atom in a high-finesse optical cavity. By employing the coupling between the single nuclear spin and a photon, we have also demonstrated that the spin can be projected or weakly measured through the projection of the transmitted single ancillary photon.
We propose two novel schemes to engineer four-partite entangled Greenberger-Horne-Zeilinger (GHZ) and W states in a deterministic way by using chains of (two-level) Rydberg atoms within the framework of cavity QED. These schemes are based on the resonant interaction of the atoms with a bimodal cavity that simultaneously supports, in contrast to a single-mode cavity, two independent modes of the photon field. In addition, we suggest the schemes to reveal the non-classical correlations for the engineered GHZ and W states. It is shown how these schemes can be extended in order to produce general …
We predict that the collective excitations of an atomic array become entangled with the light of a high-finesse cavity mode when they are suitably coupled. This entanglement is of Einstein-Podolsky-Rosen type, it is robust against cavity losses and is a stationary property of the coupled system. It is generated when the atomic array is aligned along the cavity axis and driven transversally by a laser, when coherent scattering of photons into the cavity mode is suppressed because of phase-mismatching. We identify the parameter regimes under which entanglement is found and show that these are co…
We experimentally investigate the interaction between one and two atoms and the field of a high-finesse optical resonator. Laser-cooled caesium atoms are transported into the cavity using an optical dipole trap. We monitor the interaction dynamics of a single atom strongly coupled to the resonator mode for several hundred milliseconds by observing the cavity transmission. Moreover, we investigate the position-dependent coupling of one and two atoms by shuttling them through the cavity mode. We demonstrate an alternative method, which suppresses heating effects, to analyze the atom-field intera…
We investigate theoretically the mechanical effects of light on atoms trapped by an external potential, whose dipole transition couples to the mode of an optical resonator and is driven by a laser. We derive an analytical expression for the quantum center-of-mass dynamics, which is valid in presence of a tight external potential. This equation has broad validity and allows for a transparent interpretation of the individual scattering processes leading to cooling. We show that the dynamics are a competition of the mechanical effects of the cavity and of the laser photons, which may mutually int…
We study spontaneous emission of an atom near a nanofiber with two fiber-Bragg-grating (FBG) mirrors. We show that the coupling between the atom and the guided modes of the nanofiber can be significantly enhanced by the FBG cavity even when the cavity finesse is moderate. We find that, when the fiber radius is 200 nm and the cavity finesse is about 30, up to 94% of spontaneous emission from the atom can be channeled into the guided modes in the overdamped-cavity regime. We show numerically and analytically that vacuum Rabi oscillations and strong coupling can occur in the FBG cavity even when …
An optical lattice with rubidium atoms ($^{85}Rb$) is formed inside a ring resonator with a finesse of $1.8 \times 10^5$ and a large mode volume of 1.3 $mm^3$. We typically trap several times $10^6$ atoms at densities up to $10^{12} cm^{-3}$ and temperatures between 25 and 125 $μK$. Despite of the narrow bandwidth (17.3 kHz) of the cavity, heating due to intra--cavity intensity fluctuations is kept at a low level, such that the time evolution of the temperature is determined by evaporative cooling.
We have realized a fiber-based Fabry-Perot cavity with CO2 laser-machined mirrors. It combines very small size, high finesse F>=130000, small waist and mode volume, and good mode matching between the fiber and cavity modes. This combination of features is a major advance for cavity quantum electrodynamics (CQED), as shown in recent CQED experiments with Bose-Einstein condensates enabled by this cavity [Y. Colombe et al., Nature 450, 272 (2007)]. It should also be suitable for a wide range of other applications, including coupling to solid-state emitters, gas detection at the single-particle le…
Strong saturated absorption at nanowatt power levels has been demonstrated using metastable xenon in a high-finesse optical cavity. The use of metastable xenon allows a high quality factor of Q=2*10^8 to be achieved at relatively high atomic densities without any contamination or damage to the optical surfaces, which is often a problem when using high-density rubidium or other alkali atoms. This technique provides a relatively straightforward way to produce nonlinearities at the single-photon level with possible applications in quantum communications and computing.
We propose two novel schemes to generate the two-dimensional 2xN and 3xN cluster states by using a chain of (two-level) Rydberg atoms in the framework of cavity QED. These schemes work in a completely deterministic way and are based on the resonant interaction of the atoms in a chain with a bimodal cavity that supports two independent modes of the photon field. We demonstrate that a 2xN cluster state can be generated efficiently with only a single bimodal cavity, while two such cavities are needed in order to construct a 3xN cluster state. It is shown, moreover, how these schemes can be extend…
We study the dynamics of a supersonic molecular beam in a low-finesse optical cavity and demonstrate that most molecules in the beam can be decelerated to zero central velocity by the intracavity optical field in a process analogous to electrostatic Stark deceleration. We show that the rapid switching of the optical field for slowing the molecules is automatically generated by the cavity-induced dynamics. We further show that $\sim1\%$ of the molecules can be optically trapped at a few millikelvin in the same cavity.
Strong light interaction with a subwavelength object has been a long pursuing goal with difficulties mainly arising from the diffraction limit. We propose a high finesse cavity with one mirror made of a subwavelength resonant particle as a platform to enhance this interaction. High-quality eigenmode solutions are obtained for such a highly non-paraxial cavity with a very high field concentration at the particle. The eigenmode solutions interact with the small particle in a more general way than by the electric dipole approximation. With the help of the anapole excitation in the dipole term, th…
We present an experimental study of cavity assisted Rydberg atom electromagnetically induced transparency (EIT) using a high-finesse optical cavity ($F \sim 28000$). Rydberg atoms are excited via a two-photon transition in a ladder-type EIT configuration. A three-peak structure of the cavity transmission spectrum is observed when Rydberg EIT is generated inside the cavity. The two symmetrically spaced side peaks are caused by bright-state polaritons, while the central peak corresponds to a dark-state polariton. Anti-crossing phenomenon and the effects of mirror adsorbate electric fields are st…
The topic of this thesis is the theoretical analysis of the optomechanical coupling effects in a high-finesse optical cavity, and the experimental realization of such a device. Radiation pressure exerted by light limits the sensitivity of high precision optical measurements. In particular, the sensitivity of interferometric measurements of gravitational wave is limited by the so called standard quantum limit. cavity with a movable mirror. The internal field stored in such cavity can be orders of magnitude greater than the input field, and it's radiation pressure force can change the physical l…
We report a high-finesse bow-tie cavity designed for atomic physics experiments with Rydberg atom arrays. The cavity has a finesse of $51,000$ and a waist of $7.1$ $μ$m at the cesium D2 line ($852$ nm). With these parameters, the cavity is expected to induce strong coupling between a single atom and a single photon, corresponding to a cooperativity per traveling mode of $35$ at the cavity waist. To trap and image atoms, the cavity setup utilizes two in-vacuum aspheric lenses with numerical aperture ($NA$) of $0.35$ and is capable of housing $NA=0.5$ microscope objectives. In addition, the larg…
Concentric cavities can lead to strong photon-atom coupling without a need for high finesse or small physical-cavity volume. In a proof-of-principle experiment of this concept we demonstrate coupling of single Rb atoms to a 11mm long near-concentric cavity with a finesse F=138(2). Operating the cavity 1.65(1)$μ$m shorter than the critical length, we observe an atom-cavity coupling constant $g_0=2π\times 5.0(2)\,$MHz which exceeds the natural dipole decay rate $γ$ by a factor $g_0/γ=1.7(1)$.
We demonstrate continuous loading of strontium atoms into a high finesse ring cavity and observe continuous strong collective coupling in the form of a vacuum Rabi splitting between the atoms and the cavity on the 7.5 kHz transition $^1{\rm S}_0$ to $^3{\rm P}_1$. The atoms are loaded into the cavity from a 3D narrow linewidth molasses, thus avoiding large magnetic field gradients and associated broadening of transition frequencies. The ring cavity allows us to realize a deterministic conveyor belt to transport atoms away from the loading region where the laser cooling beams lead to broadening…
We present the results of theoretical and experimental studies of dispersively coupled (or "membrane in the middle") optomechanical systems. We calculate the linear optical properties of a high finesse cavity containing a thin dielectric membrane. We focus on the cavity's transmission, reflection, and finesse as a function of the membrane's position along the cavity axis and as a function of its optical loss. We compare these calculations with measurements and find excellent agreement in cavities with empty-cavity finesses in the range 10^4 to 10^5. The imaginary part of the membrane's index o…
We show that a low finesse cavity can be efficient for detecting neutral atoms. The low finesse can be compensated for by decreasing the mode waist of the cavity. We have used a near concentric resonator with a beam waist of 12$μ$m and a finesse of only 1100 to detect magnetically guided Rb atoms with a detection sensitivity of 0.1 atom in the mode volume. For future experiments on single atom detection and cavity QED applications, it should be very beneficial to use miniaturized optical resonator integrated on atom chips.
We have fabricated an atom chip device which combines the circuitry for magnetic trapping of cold atoms with high-finesse optical resonators suitable for cavity QED in the single-atom strong coupling regime. Fabry-Perot optical resonators with finesse F > 2 X 10^5 were formed between a micropatterned on-chip planar mirror with lateral dimension of < 100 um and a curved mirror suspended above the chip. The strong and rapid thermal coupling between on-chip electrical and optical elements was utilized to stabilize the cavity mirror separation with servo bandwidth exceeding 100 kHz during simulate…
Orthogonal temporal modes (TMs) form a field-orthogonal, continuous-variable degree of freedom that is in principle infinite dimensional, and create a promising resource for quantum information science and technology. The ideal quantum pulse gate (QPG) is a device that multiplexes and demultiplexes temporally orthogonal optical pulses that have the same carrier frequency, spatial mode, and polarization. The QPG is the chief enabling technology for usage of orthogonal temporal modes as a basis for high-dimensional quantum information storage and processing. The greatest hurdle for QPG implement…
We study the quantum dynamics of the cavity optomechanical system formed by a Fabry-Perot cavity with a thin vibrating membrane at its center. We first derive the general multimode Hamiltonian describing the radiation pressure interaction between the cavity modes and the vibrational modes of the membrane. We then restrict the analysis to the standard case of a single cavity mode interacting with a single mechanical resonator and we determine to what extent optical absorption by the membrane hinder reaching a quantum regime for the cavity-membrane system. We show that membrane absorption does n…
We analyze the dynamics of a chain of singly-charged ions confined in a linear Paul trap and which couple with the mode of a high-finesse optical resonator. In these settings the ions interact via the Coulomb repulsion and are subject to the mechanical forces due to scattering of cavity photons. We show that the interplay of these interactions can give rise to bistable equilibrium configurations, into which the chain can be cooled by cavity-enhanced photon scattering. We characterize the resulting equilibrium structures by determining the stationary state in the semiclassical limit for both ca…
We present a numerical study of a MEMS-based design of a fiber cavity integrated with an ion trap system. Each fiber mirror is supported by a microactuator that controls the mirror's position in three dimensions. The mechanical stability is investigated by a feasibility analysis showing that the actuator offers a stable support of the fiber. The actuators move the fibers' positions continuously with a stroke of more than 10 $μ$m, with mechanical resonance frequencies on the order of kHz. A calculation of the trapping potential shows that a separation between ion and fiber consistent with stron…
We demonstrate the fabrication of ultra-low-loss, all-fiber Fabry-Pérot cavities containing a nanofiber section, optimized for cavity quantum electrodynamics. By continuously monitoring the finesse and fiber radius during fabrication of a nanofiber between two fiber Bragg gratings, we are able to precisely evaluate taper transmission as a function of radius. The resulting cavities have an internal round-trip loss of only 0.31% at a nanofiber waist radius of 207 nm, with a total finesse of 1380, and a maximum expected internal cooperativity of $\sim$ 1050 for a cesium atom on the nanofiber surf…
We study the spectra of emission of a system composed by an atom, tightly confined inside a high-finesse resonator, when the atom is driven by a laser and is at steady state of the cooling dynamics induced by laser and cavity field. In general, the spectrum of resonance fluorescence and the spectrum at the cavity output contain complementary information about the dynamics undergone by the system. In certain parameter regimes, quantum interference effects between the scattering processes induced by cavity and laser field lead to the selective suppression of features of the resonance fluorescenc…
We present two schemes for driving Raman transitions between the ground state hyperfine manifolds of a single atom trapped within a high-finesse optical cavity. In both schemes, the Raman coupling is generated by standing-wave fields inside the cavity, thus circumventing the optical access limitations that free-space Raman schemes must face in a cavity system. These cavity-based Raman schemes can be used to coherently manipulate both the internal and the motional degrees of freedom of the atom, and thus provide powerful tools for studying cavity quantum electrodynamics. We give a detailed theo…
Optical high-finesse cavities are a well-known mean to enhance light-matter interactions. Despite large progress in the realization of strongly coupled light-matter systems, the controlled positioning of single solid emitters in cavity modes remains a challenge. We pursue the idea to use nanofibers with sub-wavelength diameter as a substrate for such emitters. This paper addresses the question how strongly optical nanofibers influence the cavity modes. We analyze the influence of the fiber position for various fiber diameters on the finesse of the cavity and on the shape of the modes.
We study the collective motion of atoms confined in an optical lattice operating inside a high finesse ring cavity. A simplified theoretical model for the dynamics of the system is developed upon the assumption of adiabaticity of the atomic motion. We show that in a regime where the light shift per photon times the number of atoms exceeds the line width of the cavity resonance, the otherwise tiny retro-action of the atoms upon the light field becomes a significant feature of the system, giving rise to dispersive optical bistability of the intra-cavity field. A solution of the complete set of c…
Entanglement is a fundamental resource that allows quantum sensors to surpass the standard quantum limit set by the quantum collapse of independent atoms. Collective cavity-QED systems have succeeded in generating large amounts of directly observed entanglement involving the internal degrees of freedom of laser-cooled atomic ensembles. Here we demonstrate cavity-QED entanglement of external degrees of freedom to realize a matter-wave interferometer of 700 atoms in which each individual atom falls freely under gravity and simultaneously traverses two paths through space while also entangled wit…
We study the scattering problem of photon and polariton in a one-dimensional coupled-cavity system. Analytical approximate analysis and numerical simulation show that a photon can stimulate the photon emission from a polariton through polariton-photon collisions. This observation opens the possibility of photon-stimulated transition from insulating to radiative phase in a coupled-cavity QED system. Inversely, we also find that a polariton can be generated by a two-photon Raman scattering process. This paves the way towards single photon storage by the aid of atom-cavity interaction.
We describe a fiber ring resonator comprised of a relatively long loop of standard single-mode fiber with a short nanofiber segment. The evanescent mode of the nanofiber segment allows the cavity-enhanced field to interact with atoms in close proximity to the nanofiber surface. We report on an experiment using a warm atomic vapor and low-finesse cavity, and briefly discuss the potential for reaching the strong coupling regime of cavity QED by using trapped atoms and a high-finesse cavity of this kind.
By integrating the techniques of laser cooling and trapping with those of cavity quantum electrodynamics (QED), single Cesium atoms have been trapped within the mode of a small, high finesse optical cavity in a regime of strong coupling. The observed lifetime for individual atoms trapped within the cavity mode is $τ\approx 28$ms, and is limited by fluctuations of light forces arising from the far-detuned intracavity field. This initial realization of trapped atoms in cavity QED should enable diverse protocols in quantum information science.
The dynamics of a vibronic system in a lossy two-mode cavity is studied, with the first mode being resonant to the electronic transition and the second one being nearly resonant due to Raman transitions. We derive analytical solutions for the dynamics of this system. For a properly chosen detuning of the second mode from the exact Raman resonance, we obtain conditions that are closely related to the phenomenon of Rabi resonance as it is well known in laser physics. Such resonances can be observed in the spontaneous emission spectra, where the spectrum of the second mode in the case of weak Ram…
The transmission spectrum of a high-finesse optical cavity containing an arbitrary number of trapped atoms is presented. We take spatial and motional effects into account and show that in the limit of strong coupling, the important spectral features can be determined for an arbitrary number of atoms, N. We also show that these results have important ramifications in limiting our ability to determine the number of atoms in the cavity.
We investigate the coherent manipulation of interacting Rydberg atoms placed inside a high-finesse optical cavity for the deterministic preparation of strongly coupled light-matter systems. We consider a four-level diamond scheme with one common Rydberg level for N interacting atoms. One side of the diamond is used to excite the atoms into a collective `superatom' Rydberg state using either π-pulses or stimulated Raman adiabatic passage (STIRAP) pulses. The upper transition on the other side of the diamond is used to transfer the collective state to one that is coupled to a field mode of an op…
Raman heterodyne spectroscopy is a powerful tool for characterizing the energy and dynamics of spins. The technique uses an optical pump to transfer coherence from a spin transition to an optical transition where the coherent emission is more easily detected. Here Raman heterodyne spectroscopy is used to probe an isotopically purified ensemble of erbium dopants, in a yttrium orthosilicate (Y$_2$SiO$_5$) crystal coupled to a microwave cavity. Because the erbium electron spin transition is strongly coupled to the microwave cavity, we observed Raman heterodyne signals at the resonant frequencies …
We present a scheme to realise the basic two-quibit logic gates such as quantum phase gate and controlle-NOT gate using a detuned optical cavity interacting with a three-level Raman system. We discuss the role of Stark shifts which are as important as the terms leading to two-photon transition. The operation of the proposed logic gates involves metastable states of the atom and hence is not affected by spontaneous emission. These ideas can be extended to produce multiparticle entanglement.
We study the quantum limits in an optomechanical sensor based on a detuned high-finesse cavity with a movable mirror. We show that the radiation pressure exerted on the mirror by the light in the detuned cavity induces a modification of the mirror dynamics and makes the mirror motion sensitive to the signal. This leads to an amplification of the signal by the mirror dynamics, and to an improvement of the sensor sensitivity beyond the standard quantum limit, up to an ultimate quantum limit only related to the mechanical dissipation of the mirror. This improvement is somewhat similar to the one …
We investigate the dynamics of a cold trapped ion coupled to the quantized field inside a high-finesse cavity. We have used an approach for preparing the SC states of motion of ion. This approach, based on unitary transformating the Hamiltonian, allows its exact diagonalization without performing the Lamb-Dicke aproximation. We show that is possible to generate a SC states having rather simple initial state preparation, e.g., the vacuum sate for both cavity field and the ion motion.
Light scattering by a two-dimensional photonic crystal slab (PCS) can result in dramatic interference effects associated with Fano resonances. Such devices offer appealing alternatives to distributed Bragg reflectors or filters for various applications such as optical wavelength and polarization filters, reflectors, semiconductor lasers, photodetectors, bio-sensors, or non-linear optical components. Suspended PCSs also find natural applications in the field of optomechanics, where the mechanical modes of a suspended slab interact via radiation pressure with the optical field of a high finesse …
Squeezing ensemble of spins provides a way to surpass the standard quantum limit (SQL) in quantum metrology and test the fundamental physics as well, and therefore attracts broad interest. Here we propose an experimentally accessible protocol to squeeze a giant ensemble of spins via the geometric phase control. Using the cavity-assisted Raman transitions in a double $Λ$-type system, we realize an effective Dicke model. Under the condition of vanishing effective spin transition frequency, we find a particular evolution time where the cavity decouples from the spins and the spin ensemble is sque…
A new scheme of photon echo based quantum memory in the optimal optical QED cavity with off-resonant Raman atomic transition is proposed. The scheme employs the atomic ensembles characterized by an optically thin resonant transition and natural inhomogeneous broadening of the resonant line composed of the arbitrary narrow homogeneous spectral components. The scheme provides robust and quite simple coherent control of the light-atoms dynamics that can be implemented by using an existing optical technique and opens a practical way for realization of the efficient long-lived multi-mode optical qu…
Plasmonic dimer cavities can induce extreme electric-field hot spots that allow one to access ultrastrong coupling regimes using Raman-type spectroscopy on single vibrating molecules. Using a generalized master equation, we study resonant Raman scattering in the strong coupling regime of cavity-QED, when also in the vibrational ultrastrong coupling regime, leading to "phonon-dressed polaritons". The master equation rigorously includes spectral baths for the cavity and vibrational degrees of freedom, as well as a pure dephasing bath for the resonant two-level system, which play a significant ro…
The energy-level structure of a single atom strongly coupled to the mode of a high-finesse optical cavity is investigated. The atom is stored in an intracavity dipole trap and cavity cooling is used to compensate for inevitable heating. Two well-resolved normal modes are observed both in the cavity transmission and the trap lifetime. The experiment is in good agreement with a Monte Carlo simulation, demonstrating our ability to localize the atom to within $λ/10$ at a cavity antinode.
