The energy-level structure of a single atom strongly coupled to the mode of a high-finesse optical cavity is investigated. The atom is stored in an intracavity dipole trap and cavity cooling is used to compensate for inevitable heating. Two well-resolved normal modes are observed both in the cavity transmission and the trap lifetime. The experiment is in good agreement with a Monte Carlo simulation, demonstrating our ability to localize the atom to within $λ/10$ at a cavity antinode.
We show that photon coincidence spectroscopy can provide an unambiguous signature of two atoms simultaneously interacting with a quantised cavity field mode. We also show that the single-atom Jaynes-Cummings model can be probed effectively via photon coincidence spectroscopy, even with deleterious contributions to the signal from two-atom events. In addition, we have explicitly solved the eigenvectors and eigenvalues of two two-level atoms coupled to a quantised cavity mode for differing coupling strengths.
An array of $N$ closely spaced dipole coupled quantum emitters exhibits super- and subradiance with characteristic tailorable spatial radiation patterns. Optimizing their geometry and distance with respect to the spatial profile of a near resonant optical cavity mode allows to increase the ratio between light scattering into the cavity mode and free space by several orders of magnitude. This leads to a distinct nonlinear particle number scaling of the relative strength of coherent light-matter interactions versus decay. In particular, for subradiant states the collective cooperativity increase…
We describe an ion-based cavity-QED system in which the internal dynamics of an atom is coupled to the modes of an optical cavity by vacuum-stimulated Raman transitions. We observe Raman spectra for different excitation polarizations and find quantitative agreement with theoretical simulations. Residual motion of the ion introduces motional sidebands in the Raman spectrum and leads to ion delocalization. The system offers prospects for cavity-assisted resolved-sideband ground-state cooling and coherent manipulation of ions and photons.
We present evidence of cavity quantum electrodynamics from a sparse density of strongly quantum-confined Pb-chalcogenide nanocrystals (between 1 and 10) approaching single-dot levels on moderately high-Q mesoscopic silicon optical cavities. Operating at important near-infrared (1500-nm) wavelengths, large enhancements are observed from devices and strong modifications of the QD emission are achieved. Saturation spectroscopy of coupled QDs is observed at 77K, highlighting the modified nanocrystal dynamics for quantum information processing.
Photon coincidence spectroscopy relies on detecting multiphoton emissions from the combined atom-cavity system in atomic beam cavity quantum electrodynamics experiments. These multiphoton emissions from the cavity are nearly simultaneous approximately on the cavity lifetime scale. We determine the optimal time for the detection window of photon pairs in two-photon coincidence spectroscopy. If the window time is too short, some photon pairs will not be detected; if the window time is too long, too many nearly coincident independent single photons will be falsely interpreted as being a photon pa…
In recent experiments on coupled quantum dot (QD) optical cavity systems a pronounced interaction between the dot and the cavity has been observed even for detunings of many cavity linewidths. This interaction has been attributed to an incoherent phonon-mediated scattering process and is absent in atomic systems. Here, we demonstrate that despite its incoherent nature, this process preserves the signatures of coherent interaction between a QD and a strong driving laser, which may be observed via the optical emission from the off-resonant cavity. Under bichromatic driving of the QD, the cavity …
Raman heterodyne spectroscopy is a powerful tool for characterizing the energy and dynamics of spins. The technique uses an optical pump to transfer coherence from a spin transition to an optical transition where the coherent emission is more easily detected. Here Raman heterodyne spectroscopy is used to probe an isotopically purified ensemble of erbium dopants, in a yttrium orthosilicate (Y$_2$SiO$_5$) crystal coupled to a microwave cavity. Because the erbium electron spin transition is strongly coupled to the microwave cavity, we observed Raman heterodyne signals at the resonant frequencies …
We investigate the limits of intracavity absorption spectroscopy with nonlinear media. Using a common theoretical framework, we compare the detection of a trace gas within an undriven cavity with gain near and above threshold, a driven cavity with gain kept just below threshold, and a cavity driven close to the saturation point of a saturable absorber. These phase-transition-based metrology methods are typically quantum-limited by spontaneous emission, and we compare them to the empty cavity shotnoise-limited case. Although the fundamental limits achievable with nonlinear media do not surpass …
We investigate the transmission spectrum of an optical cavity coupled with four-level atoms. Multiple normal-mode splitting peaks of the strongly coupled atom-cavity system are obtained as single cavity mode couples three separated atomic transitions simultaneously. We employ a confocal optical cavity and an ensemble of cold Rb-85 atoms for cavity quantum electrodynamics. We observe four normal-mode splitting peaks of the cavity transmission in the strong coupling regime due to collective enhancement of the atom-cavity coupling strength by ensemble of cold atoms. The experimental observations …
Multi-normal-mode splitting peaks are experimentally observed in a system with Doppler-broadened two-level atoms inside a relatively long optical cavity. In this system, the atoms-cavity interaction can reach the ``superstrong coupling" condition with atoms-cavity coupling strength $g\sqrt{N}$ to be near or larger than the cavity free-spectral range $Δ_{FSR}$. In such case, normal-mode splitting can occur in many cavity longitudinal modes to generate the multi-normal-mode splitting peaks, which can be well explained by the linear dispersion enhancement due to the largely increased atomic densi…
We present experimental investigations on the non-resonant dot-cavity coupling of a single quantum dot inside a micro-pillar where the dot has been resonantly excited in the s-shell, thereby avoiding the generation of additional charges in the QD and its surrounding. As a direct proof of the pure single dot-cavity system, strong photon anti-bunching is consistently observed in the autocorrelation functions of the QD and the mode emission, as well as in the cross-correlation function between the dot and mode signals. Strong Stokes and anti-Stokes-like emission is observed for energetic QD-mode …
We theoretically analyze measurements of the transient field leaving a cavity as a tool for studying non-Markovian dynamics in cavity quantum electrodynamics (QED). Combined with a dynamical decoupling pulse sequence, transient spectroscopy can be used to recover spectral features that may be obscured in the stationary cavity transmission spectrum due to inhomogeneous broadening. The formalism introduced here can be leveraged to perform in situ noise spectroscopy, revealing a robust signature of quantum noise arising from non-commuting observables, a purely quantum effect.
We study Stokes and anti-Stokes processes in cavity optomechanics in the regime of strong coupling. The Stokes and anti-Stokes signals exhibit prominently the normal-mode splitting. We report gain for the Stokes signal. We also report lifetime splitting when the pump power is less than the critical power for normal-mode splitting. The nonlinear Stokes processes provide a useful method for studying strong coupling regime of cavity optomechanics. We also investigate the correlations between the Stokes and anti-Stokes photons produced spontaneously by the optomechanical system. At zero temperatur…
We study a system of periodic Bose condensed atoms coupled to cavity photons using the input-output formalism. We show that the cavity will either act as a through pass Lorentzian filter when the superfluid fraction of the condensate is minimum or completely reflect the input field when the superfluid fraction is maximum. We show that by monitoring the ratio between the transmitted field and the reflected field, one can estimate the superfluid fraction.
We study how an optical parametric amplifier inside the cavity can affect the normal mode splitting behavior of the coupled movable mirror and the cavity field. We work in the resolved sideband regime. The spectra exhibit a double-peak structure as the parametric gain is increased. Moreover, for a fixed parametric gain, the double-peak structure of the spectrum is more pronounced with increasing the input laser power. We give results for mode splitting. The widths of the split lines are sensitive to parametric gain.
Photon coincidence spectroscopy is a promising technique for probing the nonlinear regime of cavity quantum electrodynamics in the optical domain, however its accuracy is mitigated by two factors: higher-order photon correlations, which contribute to an enhanced pair count rate, and non-simultaneity of emitted photon pairs from the optical cavity. We show that the technique of photon coincidence spectroscopy is effective in the presence of these effects if the quantitative predictions are adjusted to include non-simultaneity and higher-order correlations.
A novel regime of atom-cavity physics is explored, arising when large atom samples dispersively interact with high-finesse optical cavities. A stable far detuned optical lattice of several million rubidium atoms is formed inside an optical ring resonator by coupling equal amounts of laser light to each propagation direction of a longitudinal cavity mode. An adjacent longitudinal mode, detunedby about 3 GHz, is used to perform probe transmission spectroscopy of the system. The atom-cavity coupling for the lattice beams and the probe is dispersive and dissipation results only from the finite pho…
The efficiency of the frequency conversion process at the heart of Raman heterodyne spectroscopy was improved by nearly four orders of magnitude by resonant enhancement of both the pump and signal optical fields. Our results using an erbium doped Y$_2$SiO$_5$ crystal at temperatures near 4K suggest that such an approach is promising for the quantum conversion of microwave to optical photons.
We report on a combined experimental and theoretical investigation into the normal modes of an all-fiber coupled cavity-quantum-electrodynamics system. The interaction between atomic ensembles and photons in the same cavities, and that between the photons in these cavities and the photons in the fiber connecting these cavities, generates five non-degenerate normal modes. We demonstrate our ability to excite each normal mode individually. We study particularly the `cavity dark mode', in which the two cavities coupled directly to the atoms do not exhibit photonic excitation. Through the observat…
Strong coupling of molecular vibrations to an infrared cavity mode affects their nature by creating dressed polariton states. We show how the single and double vibrational polariton manifolds may be controlled by varying the cavity coupling strength, and probed by a time domain 2DIR technique, Double Quantum Coherence (DQC). Applications are made to the amide-I ($CO$) and amide-II ($CN$) bond vibrations of $N-methylacetamide$ (NMA).
In the viewpoint of quasi normal modes, we describe a novel decoherence mechanism of charge qubit of Josephson Junctions (JJ) in a lossy micro-cavity, which can appear in the realistic experiment for quantum computation based on JJ qubit. We show that the nonlinear coupling of a charge qubit to quantum cavity field can result in an additional dissipation of resonant mode due to its effective interaction between those non-resonant modes and a resonant mode, which is induced by the charge qubit itself. We calculate the characterized time of the novel decoherence by making use of the system plus …
We investigate theoretically how the spectroscopy of an ancillary qubit can probe cavity (circuit) QED ground states containing photons. We consider three classes of systems (Dicke, Tavis-Cummings and Hopfield-like models), where non-trivial vacua are the result of ultrastrong coupling between N two-level systems and a single-mode bosonic field. An ancillary qubit detuned with respect to the boson frequency is shown to reveal distinct spectral signatures depending on the type of vacua. In particular, the Lamb shift of the ancilla is sensitive to both ground state photon population and correlat…
In this work we realize a narrow spectroscopic feature using a technique that we refer to as magnetically-induced optical transparency. A cold ensemble of $^{88}$Sr atoms interacts with a single mode of a high-finesse optical cavity via the 7.5kHz linewidth, spin forbidden $^1$S$_0$ to $^3$P$_1$ transition. By applying a magnetic field that shifts two excited state Zeeman levels, we open a transmission window through the cavity where the collective vacuum Rabi splitting due to a single level would create destructive interference for probe transmission. The spectroscopic feature approaches the …
We present a microscopic theory for nonlinear optical spectroscopy of N molecules in an optical cavity. A quantum Langevin analytical expression is derived for the time- and frequency-resolved signals accounting for arbitrary numbers of vibrational excitations. We identify clear signatures of the polariton-polaron interaction from multidimensional projections of the signal, e.g., pathways and timescales. Cooperative dynamics of cavity polaritons against intramolecular vibrations is revealed, along with a cross talk between long-range coherence and vibronic coupling that may lead to localizatio…
We report on a novel non-invasive method to determine the normal mode frequencies of ion Coulomb crystals in traps based on the resonance enhanced collective coupling between the electronic states of the ions and an optical cavity field at the single photon level. Excitations of the normal modes are observed through a Doppler broadening of the resonance. An excellent agreement with the predictions of a zero-temperature uniformly charged liquid plasma model is found. The technique opens up for investigations of the heating and damping of cold plasma modes, as well as the coupling between them.
We report on the coupling of the emission from a single europium-doped nanocrystal to a fiber-based microcavity under cryogenic conditions. As a first step, we study the sample properties and observe a strong correlation between emission lifetime and brightness, as well as a lifetime reduction for nanocrystals embedded in a polymer film. This is explained by differences in the local density of states. We furthermore quantify the scattering loss of a nanocrystal inside the cavity and use this to deduce the crystal size. Finally, by resonantly coupling the cavity to a selected transition, we per…
We have studied the coherent excitation of a strongly coupled QD/photonic crystal cavity system. Time-resolved reflectivity measurements show the vacuum Rabi oscillation of the dot in the cavity. Next, we considered the resonant driving of a cavity-detuned dot, which efficiently populates the cavity mode. This cavity-controlled read-out channel allows high-resolution single quantum dot spectroscopy. Autocorrelation measurements on the cavity mode show antibunching and suggest the use of the resonantly driven QD/cavity system as an on-demand source of single photons with potentially near-unity …
Efficient quantum memory is of paramount importance for long-distance quantum communications, as well as for complex large-scale computing architectures. We investigate the capability of Er$^{3+}$:Y$_2$SiO$_5$ crystal to serve as a quantum memory for the travelling microwave photons by employing techniques developed for dense optical ensembles. In our efforts to do so, we have performed high-resolution microwave spectroscopy of Er$^{3+}$:Y$_2$SiO$_5$, where we identified electronic spin as well as hyperfine transitions. Furthermore, we have explored spectral hole burning technique and studied …
We explore the potential of direct spectroscopy of ultra-narrow optical transitions of atoms localized in an optical cavity. In contrast to stabilization against a reference cavity, which is the approach currently used for the most highly stabilized lasers, stabilization against an atomic transition does not suffer from Brownian thermal noise. Spectroscopy of ultra-narrow optical transitions in a cavity operates in a very highly saturated regime in which non-linear effects such as bistability play an important role. From the universal behavior of the Jaynes-Cummings model with dissipation, we …
We present robust radio frequency (rf) pulses that tolerate a factor of six inhomogeneity in the B1 field, significantly enhancing the potential of toroid cavity resonators for NMR spectroscopic applications. Both point-to-point (PP) and unitary rotation (UR) pulses were optimized for excitation, inversion, and refocusing using the gradient ascent pulse engineering (GRAPE) algorithm based on optimal control theory. In addition, the optimized parameterization (OP) algorithm applied to the adiabatic BIR-4 UR pulse scheme enabled ultra-short (50 microsec) pulses with acceptable performance compar…
We study the normal mode splitting in a system consisting of a Bose Einstein condensates (BECs) trapped inside a Fabry Perot cavity driven by a single mode laser field. We analyze the variations in frequency and damping rate of the collective density excitation of a BEC imparted by the optical field. We study the occurrence of normal mode splitting which appears as consequences of the hybridization of the fluctuations of the intracavity field and the condensate mode. It is shown that normal mode splitting vanishes for weak coupling between the condensate mode and the intracavity field. Moreove…
We study an accumulation mode Si/SiGe double quantum dot (DQD) containing a single electron that is dipole coupled to microwave photons in a superconducting cavity. Measurements of the cavity transmission reveal dispersive features due to the DQD valley states in Si. The occupation of the valley states can be increased by raising temperature or applying a finite source-drain bias across the DQD, resulting in an increased signal. Using cavity input-output theory and a four-level model of the DQD, it is possible to efficiently extract valley splittings and the inter- and intra-valley tunnel coup…
Ultraviolet (UV) diode lasers are widely used in many photonics applications. But their frequency stabilization schemes are not as mature as frequency-doubling lasers, mainly due to some limitations in the UV spectral region. Here we developed a high-performance UV frequency stabilization technique implemented directly on UV diode lasers by combining the dichroic atomic vapor laser lock and the resonant transfer cavity lock. As an example, we demonstrate a stable locking with frequency standard deviations of approximately 200 KHz and 300 KHz for 399nm and 370nm diode lasers in 20 minutes. We a…
We propose a special cavity design that is constructed by terminating a one-dimensional waveguide with a perfect mirror at one end and doping a two-level atom at the other. We show that this atom plays the intrinsic role of a semi-transparent mirror for single photon transports such that quasi-normal modes (QNM's) emerge spontaneously in the cavity system. This atomic mirror has its reflection coefficient tunable through its level spacing and its coupling to the cavity field, for which the cavity system can be regarded as a two-end resonator with a continuously tunable leakage. The overall inv…
The coherent interaction of Rydberg helium atoms with microwave fields in a $λ/4$ superconducting coplanar waveguide resonator has been exploited to probe the spectral characteristics of an individual resonator mode. This was achieved by preparing the atoms in the 1s55s$^3$S$_1$ Rydberg level by resonance enhanced two-color two-photon excitation from the metastable 1s2s$^3$S$_1$ level. The atoms then travelled over the resonator in which the third harmonic microwave field, at a frequency of $ω_{\mathrm{res}}=2π\times19.556$ GHz, drove the two-photon 1s55s$^3$S$_1\rightarrow$1s56s$^3$S$_1$ tran…
A fiber taper waveguide is used to perform direct optical spectroscopy of a microdisk-quantum-dot system, exciting the system through the photonic (light) channel rather than the excitonic (matter) channel. Strong coupling, the regime of coherent quantum interactions, is demonstrated through observation of vacuum Rabi splitting in the transmitted and reflected signals from the cavity. The fiber coupling method also allows the examination of the system's steady-state nonlinear properties, where saturation of the cavity-QD response is observed for less than one intracavity photon.
Delayed Formation of Landau Polaritons in Phase-Resolved THz Spectroscopy
Centera Labs, Institute of High Pressure Physics, Polish Academy of Sciences（波兰科学院高压物理研究所）；Centera, Cezamat, Warsaw University of Technology（华沙理工大学）；Weitzman Institute of Science（魏茨曼科学研究所）；Faculty of Physics, University of Warsaw（华沙大学物理学院）
Sideband transitions are spectroscopically probed in a system consisting of a Cooper pair box strongly but non-resonantly coupled to a superconducting transmission line resonator. When the Cooper pair box is operated at the optimal charge bias point the symmetry of the hamiltonian requires a two photon process to access sidebands. The observed large dispersive ac-Stark shifts in the sideband transitions induced by the strong non-resonant drives agree well with our theoretical predictions. Sideband transitions are important in realizing qubit-photon and qubit-qubit entanglement in the circuit q…
In this paper we explore the rich structure of macroscopic many-particle quantum states for Bose- Einstein condensate in an optical cavity with the tunable nonlinear atom-photon interaction [Nature (London) 464, 1301 (2010)]. Population inversion, bistable normal phases and the coexistence of normal{superradiant phases are revealed by adjusting of the experimentally realizable interaction strength and pump-laser frequency. For the negative (effective) cavity-frequency we observe remark- ably an inverted quantum phase transition (QPT) from the superradiant to normal phases with the increase of …
Optical nonlinearities typically require macroscopic media, thereby making their implementation at the quantum level an outstanding challenge. Here we demonstrate a nonlinearity for one atom enclosed by two highly reflecting mirrors. We send laser light through the input mirror and record the light from the output mirror of the cavity. For weak laser intensity, we find the vacuum-Rabi resonances. But for higher intensities, we find an additional resonance. It originates from the fact that the cavity can accommodate only an integer number of photons and that this photon number determines the ch…
We report on a low-noise diode laser oscillator at 972 nm actively stabilized to an ultra-stable vibrationally- and thermally compensated reference cavity. To increase the fraction of laser power in the carrier we designed a 20 cm long external cavity diode laser with an intra-cavity electro-optical modulator. The fractional power in the carrier reaches 99.9% which corresponds to a rms phase noise of $ϕ^2_\textrm{rms}=1\,\textrm{mrad}^2$ in 10\,MHz bandwidth. Using this oscillator we recorded 1S-2S spectra in atomic hydrogen and have not observed any significant loss of the excitation efficien…
We perform an investigation into the properties of Pr3+:Y2SiO5 whispering gallery mode resonators as a first step towards achieving the strong coupling regime of cavity QED with rare-earth-ion doped crystals. Direct measurement of cavity QED parameters are made using photon echoes, giving good agreement with theoretical predictions. By comparing the ions at the surface of the resonator to those in the center it is determined that the physical process of making the resonator does not negatively affect the properties of the ions. Coupling between the ions and resonator is analyzed through the ob…
