We present experimental investigations on the non-resonant dot-cavity coupling of a single quantum dot inside a micro-pillar where the dot has been resonantly excited in the s-shell, thereby avoiding the generation of additional charges in the QD and its surrounding. As a direct proof of the pure single dot-cavity system, strong photon anti-bunching is consistently observed in the autocorrelation functions of the QD and the mode emission, as well as in the cross-correlation function between the dot and mode signals. Strong Stokes and anti-Stokes-like emission is observed for energetic QD-mode detunings of up to ~100 times the QD linewidth. Furthermore, we demonstrate that non-resonant dot-cavity coupling can be utilized to directly monitor and study relevant QD s-shell properties like fine-structure splittings, emission saturation and power broadening, as well as photon statistics with negligible background contributions. Our results open a new perspective on the understanding and implementation of dot-cavity systems for single-photon sources, single and multiple quantum dot lasers, semiconductor cavity quantum electrodynamics, and their implementation, e.g. in quantum information technology.
We describe a scheme of deterministic single-photon subtraction in a solid-state system consisting of a charged quantum dot coupled to a bimodal photonic-crystal cavity with a moderate magnetic field applied in a Voigt configuration. We numerically simulate injection of optical pulses into one of the modes of the bimodal cavity and show that the system deterministically transfers one photon into the second cavity mode for input pulses in the form of both Fock states and coherent states.
Cryogenic spectroscopy of ultra-low density colloidal lead chalcogenide quantum dots on chip-scale optical cavities towards single quantum dot near-infrared cavity QED
Coherence has been remaining a key resource for numerous applications of quantum physics ranging from quantum metrology to quantum information. Here, we report a theoretical work on how maximally created coherence results in the squeezing of cavity field coupled to a coherently driven single quantum dot. We employ a recently developed polaron master equation theory for accurately incorporating the impact of exciton-phonon coupling on squeezing.
The quantum Rabi oscillations in a coherently driven quantum dot embedded in a high-Q doubly resonant semiconductor micro-cavity in the presence of a strong second-order nonlinear medium is investigated theoretically. It is shown that the second order nonlinearity effect the Rabi oscillations in a significant manner.
A new analytic approach to investigate the zero-temperature time evolution of the Jaynes-Cummings system with cavity losses is developed. With the realistic coupling between the cavity and the environment assumed, a simple master equation is derived, leading to the explicit analytic solution for the resonant case. This solution is suitable for the analyses not only on the single excitation states but also on many excitation states, which enables us to investigate the photon coherent state and to observe sharp collapses and revivals under dissipation. For the off-resonant case, on the other han…
We investigate the photon induced tunneling phenomena in a photonic crystal cavity containing a strongly coupled quantum dot and describe how this tunneling can be used to generate photon states consisting mainly of a particular Fock state. Additionally, we study experimentally the photon-induced tunneling as a function of excitation laser power and frequency and show the signature of second rung of the Jaynes-Cummings Hamiltonian in the observed photon-statistics.
The ability to generate mode-engineered single photons to interface with disparate quantum systems is of importance for building a quantum network. Here we report on the generation of a pulsed, heralded single photon source with a sub-GHz spectral bandwidth that couples to indium arsenide quantum dots centered at 942 nm. The source is built with a type-II PPKTP down-conversion crystal embedded in a semi-confocal optical cavity and pumped with a 76 MHz repetition rate pulsed laser to emit collinear, polarization-correlated photon pairs resonant with a single quantum dot. In order to demonstrate…
We theoretically investigate the unexpected occurrence of an extra emission peak that has been experimentally observed in off-resonant studies of cavity QED systems. Our results within the Markovian master equation approach successfully explain why the central peak arises, and how it reveals that the system is suffering a dynamical phase transition induced by the phonon-mediated coupling. Our findings are in perfect agreement with previous reported experimental results and for the first time the fundamental physics behind this quantum phenomenon is understood.
We describe how quantum dot semiconductor cavity systems can be engineered to realize anisotropy-induced dipole-dipole coupling between orthogonal dipole states in a single quantum dot. Quantum dots in single-mode cavity structures as well as photonic crystal waveguides coupled to spin states or linearly polarized excitons are considered. We demonstrate pronounced dipole-dipole coupling to control the radiative decay rate of excitons and form pure entangled states in the long time limit. We investigate both field-free entanglement evolution and coherently pumped exciton regimes, and show how a…
We predict dominating cooperative two-photon emission from two quantum dots coupled with a single mode photonic crystal cavity. The cooperative two photon emission occurs when excitons in two off-resonantly coupled quantum dots decay simultaneously. The interaction with common cavity field leads to cavity induced two-photon emission which is strongly inhibited by electron phonon coupling. The interaction with common phonon bath produces phonon induced two-photon emission which increases on increasing temperature. For identical quantum dots cavity induced two-photon emission is negligible but p…
We observe the unconventional photon blockade effect in quantum dot cavity QED, which, in contrast to conventional photon blockade, operates in the weak coupling regime. A single quantum dot transition is simultaneously coupled to two orthogonally polarized optical cavity modes, and by careful tuning of the input and output state of polarization, the unconventional photon blockade effect is observed. We find a minimum second-order correlation $g^{(2)}(0)\approx0.37$ which corresponds to $g^{(2)}(0)\approx0.005$ when corrected for detector jitter, and observe the expected polarization dependenc…
We use a versatile model to evaluate the multipartite entanglement and the nonclassical light generation in optical parametric oscillators, exploring the differences between doubly and triply resonant cavity configurations. We demonstrate the entanglement of the pump mode with converted fields in both situations, and the fundamental differences of oscillators using parametric down conversion and four wave mixing processes as the intracavity amplification technique. The strong correlations involving the sidebands of the pump and converted fields gives the signatures of a rich dynamic of multipa…
We investigate the generation of single photons and photon pairs in a cavity quantum electrodynamics system of a four-level quantum dot coupled to bimodal cavity. By tuning frequencies and intensity ratio of the driving lasers, sub-Poissonian and super-Poissonian photon statistics are obtained in each nondegenerate cavity mode respectively. Single photon emission is characterized as zero-delay second-order correlation function g^2(0)~0.15. Photon pair emission under the two-photon resonance excitation is quantified by Mandel parameter as Q~0.04. The mean cavity photon number in both scenarios …
We theoretically demonstrate the enhanced and dephasing immune squeezing in the resonance fluorescence of a single quantum dot (QD) confined to a pillar-microcavity and driven by a continuous wave laser. We employ a formalism based on Polaron master equation theory for incorporating the influence of exciton-phonon coupling quite accurately in the dot-cavity system. We show a significant enhancement of squeezing due to cavity coupling of the QD as compared to that of an ideal single two-level system in free space. Particularly, we show a four-fold enhancement in squeezing as compared to that of…
In this paper we investigate an implementation of a quantum gate for quantum information processing in a system of quantum dots in an optical cavity manipulated by collinear laser fields. For simplicity we give theoretical and numerical results only for simulations of two quantum dots in a cavity interacting with two collinear fields. Extension to the system of many quantum dots in a cavity can be done in similar manner as the two dots system. It is shown that due to the collinear fields are used, a two qubit gate operation can be acheived by choosing properly detunings and amplitudes of the c…
Two main mechanisms dictate the tunneling process in a double quantum dot: overlap of excited wave functions, effectively described as a tunneling rate, and phonon-assisted tunneling. In this paper, we study different regimes of tunneling that arise from the competition between these two mechanisms in a double quantum dot molecule immersed in a unimodal optical cavity. We show how such regimes affect the mean number of excitations in each quantum dot and in the cavity, the spectroscopic resolution and emission peaks of the photoluminescence spectrum, and the second-order coherence function whi…
Charged quantum dots containing an electron or hole spin are bright solid-state qubits suitable for quantum networks and distributed quantum computing. Incorporating such quantum dot spin into a photonic crystal cavity creates a strong spin-photon interface, in which the spin can control a photon by modulating the cavity reflection coefficient. However, previous demonstrations of such spin-photon interfaces have relied on quantum dots that are charged randomly by nearby impurities, leading to instability in the charge state, which causes poor contrast in the cavity reflectivity. Here we demons…
We propose methods for realization of continuous two photon source using coherently pumped quantum dot embedded inside a photonic crystal cavity. We analyze steady state population in quantum dot energy levels and field inside the cavity mode. We find conditions for population inversion in coherently pumped and incoherently pumped quantum dot. We show that squeezing in the output for two two photon laser is not visible using coherent as well as incoherent pump. We discuss effect of phonon coupling using recently developed polaron transformed master equation at low temperatures. We also propose…
Scalable architectures for quantum information technologies require to selectively couple long-distance qubits while suppressing environmental noise and cross-talk. In semiconductor materials, the coherent coupling of a single spin on a quantum dot to a cavity hosting fermionic modes offers a new solution to this technological challenge. Here, we demonstrate coherent coupling between two spatially separated quantum dots using an electronic cavity design that takes advantage of whispering-gallery modes in a two-dimensional electron gas. The cavity-mediated long-distance coupling effectively min…
The on-demand preparation of higher-order Fock states is of fundamental importance in quantum information sciences. We propose and compare different protocols to generate higher-order Fock states in solid state quantum-dot--cavity systems. The protocols make use of a series of laser pulses to excite the quantum dot exciton and off-resonant pulses to control the detuning between dot and cavity. Our theoretical studies include dot and cavity loss processes as well as the pure-dephasing type coupling to longitudinal acoustic phonons in a numerically complete fashion. By going beyond the two-level…
Quantum confinement leads to the formation of discrete electronic states in quantum dots. Here we probe electron-phonon interactions in a suspended InAs nanowire double quantum dot (DQD) that is electric-dipole coupled to a microwave cavity. We apply a finite bias across the wire to drive a steady state population in the DQD excited state, enabling a direct measurement of the electron-phonon coupling strength at the DQD transition energy. The amplitude and phase response of the cavity field exhibit features that are periodic in the DQD energy level detuning due to the phonon modes of the nanow…
