We observe the unconventional photon blockade effect in quantum dot cavity QED, which, in contrast to conventional photon blockade, operates in the weak coupling regime. A single quantum dot transition is simultaneously coupled to two orthogonally polarized optical cavity modes, and by careful tuning of the input and output state of polarization, the unconventional photon blockade effect is observed. We find a minimum second-order correlation $g^{(2)}(0)\approx0.37$ which corresponds to $g^{(2)}(0)\approx0.005$ when corrected for detector jitter, and observe the expected polarization dependency and photon bunching and anti-bunching very close-by in parameter space, which indicates the abrupt change from phase to amplitude squeezing.
We have observed the unconventional photon blockade effect for microwave photons using two coupled superconducting resonators. As opposed to the conventional blockade, only weakly nonlinear resonators are required. The blockade is revealed through measurements of the second order correlation function $g^{(2)}(t)$ of the microwave field inside one of the two resonators. The lowest measured value of $g^{(2)}(0)$ is 0.4 for a resonator population of approximately $10^{-2}$ photons. The time evolution of $g^{(2)}(t)$ exhibits an oscillatory behavior, which is characteristic of the unconventional p…
A strong photon-photon nonlinear interaction is a necessary condition for photon blockade. Moreover, this nonlinearity can also result a bistable behavior in the cavity field. We analyze the relation between detecting field and photon blockade in a superconducting circuit QED system, and show that photon blockade cannot occur when the detecting field is in the bistable regime. This photon blockade is the microwave-photonics analog of the Coulomb blockade. We further demonstrate that the photon transmission through such system can be controlled (from photon blockade to transparency) by the dete…
We theoretically investigate the three-photon blockade phenomenon in a two atoms cavity QED system, where two atoms are driven by a coherent field. In the case of in-phase radiations, we show that the three-photon blockade with bunched two photons can be realized in a small regime of the driving field Rabi frequency. However, in the case of out-of-phase radiations, the one-photon excitations are prohibited due to the destructive interference, and three-photon blockade can be realized in a wide regime of driving field Rabi frequency. In addition, the three-photon blockade phenomenon can be sign…
We theoretically study a quantum destructive interference (QDI) induced photon blockade in a two-qubit driven cavity QED system with dipole-dipole interaction (DDI). In the absence of dipole-dipole interaction, we show that a QDI-induced photon blockade can be achieved only when the qubit resonance frequency is different from the cavity mode frequency. When DDI is introduced the condition for this photon blockade is strongly dependent upon the pump field frequency, and yet is insensitive to the qubit-cavity coupling strength. Using this tunability feature we show that the conventional energy-l…
We theoretically study the quantum interference induced photon blockade phenomenon in atom cavity QED system, where the destructive interference between two different transition pathways prohibits the two-photon excitation. Here, we first explore the single atom cavity QED system via an atom or cavity drive. We show that the cavity-driven case will lead to the quantum interference induced photon blockade under a specific condition, but the atom driven case can't result in such interference induced photon blockade. Then, we investigate the two atoms case, and find that an additional transition …
We present a study of manipulating the multiphoton blockade phenomenon in a single mode cavity with two ladder-type three-level atoms. Combining the cavity QED with electromagnetically induced transparency technique, we show that it is possible to actively manipulate the photon blockade when two atoms are in phase radiations. As a result, the two-photon blockade can be changed to three-photon blockade by changing the control field Rabi frequency. In the case of out-phase radiations, we show that the three-photon blockade can be improved with enhanced mean photon number. In addition, we show th…
Photon blockade is a dynamical quantum-nonlinear effect that occurs in driven systems with an anharmonic excitation ladder. For a single atom strongly coupled to an optical cavity, we show that driving the atom gives a decisively larger optical nonlinearity than driving the cavity. This enhances single-photon blockade and allows for the implementation of two-photon blockade where the absorption of two photons suppresses the absorption of further photons. As a signature, we report on three-photon antibunching with simultaneous two-photon bunching observed in the light emitted from the cavity. O…
We propose how to achieve quantum nonreciprocity via unconventional photon blockade (UPB) in a compound device consisting of an optical harmonic resonator and a spinning optomechanical resonator. We show that, even with an extremely weak single-photon nonlinearity, nonreciprocal UPB can emerge in this system, i.e., strong photon antibunching can emerge only by driving the device from one side, but not from the other side. This nonreciprocity results from the Fizeau drag, leading to different splitting of the resonance frequencies for the counter-circulating modes. Such nonreciprocal quantum UP…
The most simple and seemingly straightforward application of the photon blockade effect, in which the transport of one photon prevents the transport of others, would be to separate two incoming indistinguishable photons to different output ports. We show that time-energy uncertainty relations inherently prevent this ideal situation when the blockade is implemented by a two-level system. The fundamental nature of this limit is revealed in the fact that photon blockade in the strong coupling regime of cavity QED, resulting from the nonlinearity of the Jaynes-Cummings energy level structure, exhi…
We use the scattering matrix formalism to analyze photon blockade in coherently-driven CQED systems with a weak drive. By approximating the weak coherent drive by an input single- and two-photon Fock state, we reduce the computational complexity of the transmission and the two-photon correlation function from exponential to polynomial in the number of emitters. This enables us to easily analyze cavity-based systems containing $\sim$50 quantum emitters with modest computational resources. Using this approach we study the coherence statistics of polaritonic photon blockade while increasing the n…
We propose how to achieve strong photon antibunching effect in a cavity-QED system coupled with two Rydberg-Rydberg interaction atoms. Via calculating the equal time second order correlation function g(2)(0), we find that the unconventional photon blockade and the conventional photon blockade appear in the atom-driven scheme, and they are both significantly affected by the Rydberg-Rydberg interaction. We also find that under appropriate parameters, the photon antibunching and the mean photon number can be significantly enhanced by combining the conventional photon blockade and the unconvention…
We review the unconventional photon blockade mechanism. This quantum effect remarkably enables a strongly sub-Poissonian light statistics, even from a system characterized by a weak single photon nonlinearity. We revisit the past results, which can be interpreted in terms of quantum interferences or optimal squeezing, and show how recent developments on input-output field mixing can overcome the limitations of the original schemes towards passive and integrable single photon sources. We finally present some valuable alternative schemes for which the unconventional blockade can be directly adap…
Unconventional photon blockade refers to the suppression of multi-photon states in weakly nonlinear optical resonators via the destructive interference of different excitation pathways. It has been studied in a pair of coupled nonlinear resonators and other few-mode systems. Here, we show that unconventional photon blockade can be greatly enhanced in a chain of coupled resonators. Specifically, the strength of the nonlinearity in each resonator needed to achieve unconventional photon blockade is suppressed exponentially with lattice size. The analytic derivation, based on a weak drive approxim…
Cavity quantum electrodynamics (QED), wherein a quantum emitter is coupled to electromagnetic cavity modes, is a powerful platform for implementing quantum sensors, memories, and networks. However, due to the fundamental tradeoff between gate fidelity and execution time, as well as limited scalability, the use of cavity-QED for quantum computation was overtaken by other architectures. Here, we introduce a new element into cavity-QED - a free charged particle, acting as a flying qubit. Using free electrons as a specific example, we demonstrate that our approach enables ultrafast, deterministic …
We study the unconventional photon blockade, recently proposed for a coupled-cavity system, in presence of input and output quantum fields. Mixing of the input or output channels still allows strong photon antibunching of the output field, but for optimal values of the system parameters that differ substantially from those that maximize antibunching of the intracavity field. This result shows that the specific input-output geometry in a photonic system determines the optimal design in view of single-photon device operation. We provide a compact analytical formula that allows finding the optima…
It is shown that non-centrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably engineered coupled microcavities. The proposed scheme exploits the unconventional photon blockade of a coherent driving field at the input of a coupled cavity system, where one of the two cavities is engineered to resonate at both fundamental and second harmonic frequencies, respectively. Remarkably, the unconventional blockade mechanism occurs with reasonably low …
Phonon nonlinearities play an important role in hybrid quantum networks and on-chip quantum devices. We investigate the phonon statistics of a mechanical oscillator in hybrid systems composed of an atom and one or two standard optomechanical cavities. An efficiently enhanced atom-phonon interaction can be derived via a tripartite atom-photon-phonon interaction, where the atom-photon coupling depends on the mechanical displacement without practically changing a cavity frequency. This novel mechanism of optomechanical interactions, as predicted recently by Cotrufo et al. [Phys. Rev. Lett. 118, 1…
In the recent publications [Phys. Rev. A 92,023838 (2015)], the unconventional photon blockade are studied in a two-mode-second-order-nonlinear system with nonlinear coupling between the low frequency and high frequency modes. In this paper, we study the unconventional photon blockade in a three-mode system with weakly coupled nonlinear cavities via $χ^{(2)}$ nonlinearity. By solving the master equation in the steady-state limit and calculating the zero-delay time second-order correlation function, we obtain the conditions of strong photon antibunching in the low frequency mode. The numerical …
We study the photon blockade effect in a coupled cavity system, which is formed by a linear cavity coupled to a Kerr-type nonlinear cavity via a photon-hopping interaction. We explain the physical phenomenon from the viewpoint of the conventional and unconventional photon blockade effects. The corresponding physical mechanisms of the two kinds of photon blockade effects are based on the anharmonicity in the eigenenergy spectrum and the destructive quantum interference between two different transition paths, respectively. In particular, we find that the photon blockade via destructive quantum i…
We show that in laser-driven coupled optomechanical systems, photon antibunching can occur under weak optomechanical coupling, contrarily to common expectation. This unconventional photon blockade originates from destructive quantum interference between different excitation pathways bringing from the ground to two-photon states. Using a quantum open-system approach, we study the antibunching as a function of driving field amplitude, temperature, and pure dephasing rate, and derive optimal values of the system parameters for its occurrence. These values are remarkably close to those characteriz…
We analyze the photon correlations in an optomechanical system containing two nonlinear optical modes and one mechanical mode which are coupled via a three-mode mixing. Under a weak driving condition, we determine the optimal conditions for photon antibunching in the weak Kerr-nonlinear regime and we find that the analytical calculations are consistent with the numerical results. The photon blockade effect is attributed to destructive quantum interference in the two-photon excitation pathways created as a result of the three-mode interaction.
We propose a scheme to realize strong photon antibunching with lower photon nonlinearity in a photonic molecule consisting of two photonic cavities, one of which contains a quantum dot (QD). This strong photon antibunching is attributed to destructive quantum interference effect which suppresses the two-photon excitation of the cavity field. That g^2 (0)~10^(-4) can be achieved with modest QD-cavity coupling strength g=1.1k and cavity tunneling strength J=3k when the system is driven by single laser field. To further reduce the requisite tunneling and make the system tunable, two laser fields …
Photon antibunching is a quantum phenomenon typically observed in strongly nonlinear systems where photon blockade suppresses the probability for detecting two photons at the same time. Antibunching has also been reported with Gaussian states, where optimized amplitude squeezing yields classically forbidden values of the intensity correlation, $g^{(2)}(0)<1$. As a consequence, observing antibunching is not necessarily a signature of photon-photon interactions. To clarify the significance of the intensity correlations, we derive a sufficient condition for deducing if a field is non-Gaussian bas…
The driven-damped Jaynes-Cummings model in the regime of strong coupling is found to exhibit a coexistence between the quantum photon blockaded state and a quasi-coherent bright state. We characterize the slow time scales and the basin of attraction of these metastable states using full quantum simulations. This form of bistability can be useful for implementing a qubit readout scheme that does not require additional circuit elements. We propose a coherent control sequence that makes use of a simple linear chirp of drive amplitude and frequency as well as qubit frequency. By optimizing the par…
We present a scheme for implementing the unconventional geometric two-qubit phase gate with nonzero dynamical phase by using the two-channel Raman interaction of two atoms in a cavity. We show that the dynamical phase acquired in a cyclic evolution is proportional to the geometric phase acquired in the same cyclic evolution, hence the the total phase possesses the same geometric features as the geometric phase. In our scheme the atomic excited state is adiabatically eliminated and the operation of the proposed logic gate involves only in the metastable states of the atom and hence is not affec…
We investigate theoretically the model of a cavity-quantum-electrodynamics (QED) system that consists of two two-level atoms coupled to a single-mode cavity in the weak coupling regime, where the system is driven by quantum light. The dynamics behavior of the entire system is tackled in the framework of a cascaded quantum system. We find that the two-photon blockade with two-photon bunching and three-photon antibunching can be obtained even when the strong system dissipation is included. This result shows that our work has potential for realizing entangled photon pairs in a weakly coupled cavi…
The lack of suitable quantum emitters in silicon and silicon-based materials has prevented the realization of room temperature, compact, stable, and integrated sources of single photons in a scalable on-chip architecture, so far. Current approaches rely on exploiting the enhanced optical nonlinearity of silicon through light confinement or slow-light propagation, and are based on parametric processes that typically require substantial input energy and spatial footprint to reach a reasonable output yield. Here we propose an alternative all-silicon device that employs a different paradigm, namel…
Based on the four wave mixing, a three mode nonlinear system is proposed. The single photon blockade is discussed through analytical analysis and numerical calculation. The analytical analysis shows that the conventional photon blockade and unconventional photon blockade can be realized at the same time, and the analytical conditions of the two kinds of blockade are the same. The numerical results show that the system not only has the maximum average photon number in the blockade region, but also can have strong photon anti-bunching in the region with small nonlinear coupling coefficient, whic…
We study a 2D system of trion-polaritons at the quantum level and demonstrate that for monolayer semiconductors they can exhibit a strongly nonlinear optical response. The effect is due to the composite nature of trion-based excitations resulting in their nontrivial quantum statistical properties, and enhanced phase space filling effects. We present the full quantum theory to describe the statistics of trion-polaritons, and demonstrate that the associated nonlinearity persists at the level of few quanta, where two qualitatively different regimes of photon antibunching are present for weak and …
There is generally no obvious evidence in any direct relation between photon blockade and atomic coherence. Here instead of only illustrating the photon statistics, we show an interesting relation between the steady-state photon blockade and the atomic coherence by designing a weakly driven cavity QED system with a two-level atom trapped. It is shown for the first time that the maximal atomic coherence has a perfect correspondence with the optimal photon blockade. The negative effects of the strong dissipations on photon statistics, atomic coherence and their correspondence are also addressed.…
A two-level system interacting with a cavity field is an important model for investigating the photon blockade (PB) effect. Most work on this topic has been based on the assumption that the atomic transition frequency is resonant with the fundamental mode frequency of the cavity. We relax this constraint and reexamine PB in a more general atom--cavity system with arbitrary atomic and cavity detunings from a driving field. The results show that when the signs of the atomic and cavity detunings are the same, PB occurs only in the strong-coupling regime, but for opposite signs of the atomic and c…
Manipulating photons is an essential technique in quantum communication and computation. Combining the Raman electromagnetically induced transparency technology, we show that the photon blockade behavior can be actively controlled by using an external control field in a two atoms cavity-QED system. As a result, a versatile photon gateway can be achieved in this system, which changes the cavity photons from classical to quantum property and allows one photon, two photon and classical field leaking from the cavity. The proposal presented here has many potential applications for quantum informati…
The hybrid microwave optomechanical-magnetic system has recently emerged as a promising candidate for coherent information processing because of the ultrastrong microwave photon-magnon coupling and the longlife of the magnon and phonon. As a quantum information processing device, the realization of a single excitation holds special meaning for the hybrid system. In this paper, we introduce a single two-level atom into the optomechanical-magnetic system and show that an unconventional blockade due to destructive interference cannot offer a blockade of both the photon and magnon. Meanwhile, unde…
We propose a scheme for realizing two-qubit quantum phase gates via an unconventional geometric phase shift with atoms in a cavity. In the scheme the atoms interact simultaneously with a highly detuned cavity mode and a classical field. The atoms undergo no transitions during the gate operation, while the cavity mode is displaced along a circle in the phase space, aquiring a geometric phase conditional upon the atomic state. Under certain conditions, the atoms are disentangled with the cavity mode and thus the gate is insensitive to both the atomic spontaneous emission and the cavity decay.
The discovery of topological materials has challenged our understanding of condensed matter physics and led to novel and unusual phenomena. This has motivated recent developments to export topological concepts into photonics to make light behave in exotic ways. Here, we predict several unconventional quantum optical phenomena that occur when quantum emitters interact with a topological waveguide QED bath, namely, the photonic analogue of the Su-Schrieffer-Hegger model. When the emitters frequency lies within the topological band-gap, a chiral bound state emerges, which is located at just one s…
Chiral cavity-magnonic system for the unidirectional photon blockade
School of Physics and Information Technology, Shaanxi Normal University（陕西师范大学物理与信息技术学院）；Xi’an Key Laboratory of Optical Information Manipulation and Augmentation（西安光学信息操纵与增强重点实验室）
Photon correlations, as measured by Glauber's $n$-th order coherence functions $g^{(n)}$, are highly sought to be minimized and/or maximized. In systems that are coherently driven, so-called blockades can give rise to strong correlations according to two scenarios based on level-repulsion (conventional blockade) or interferences (unconventional blockade). Here we show how these two approaches relate to the admixing of a coherent state with a quantum state such as a squeezed state for the simplest and most recurrent case. The emission from a variety of systems, such as resonance fluorescence, t…
The photon blockade (PB) effect in emitter-cavity systems depends on the anharmonicity of the ladder of dressed energy eigenstates. The recent developments in color center photonics are leading toward experimental demonstrations of multi-emitter-cavity solid-state systems with an expanded set of energy levels compared to the traditionally studied single-emitter systems. We focus on the case of N = 2 nonidentical quasi-atoms strongly coupled to a nanocavity in the bad cavity regime (with parameters within reach of the color center systems), and discover three PB mechanisms: polaritonic, subradi…
We propose a mechanism of unconventional Rydberg pumping (URP) via simultaneously driving each Rydberg atom by two classical fields with different strengths of Rabi frequencies. This mechanism differs from the general Rydberg blockade or Rydberg antiblockade since it is closely related to the ground states of atoms, i.e. two atoms in the same ground state are stable while two atoms in different ground states are resonantly excited. Furthermore, we find the URP can be employed to simplify some special quantum information processing tasks, such as implementation of a three-qubit controlled phase…
We study the interaction between a quantum-dot and a bi-mode micro/nano-optical cavity composed of second-order nonlinear materials. Compared with the Jaynes-Cummings (J-C) model, except for a coherent weak driving field, a strong pump light illuminates the two-mode optical cavity. Analytical results indicate that the model exhibits abundant non-classical optical phenomena, such as conventional photon blockade induced by the nonlinear interaction between polaritons. It constitutes unconventional photon blockade induced by quantum interference due to parametric driving. We compare the photon st…
Kinetically constrained cavity QED: from blockaded ferromagnetism to long-range quantum scars
Institute of Physics, Johannes Gutenberg University Mainz（约翰内斯·古腾堡大学美因茨物理研究所）；Department of Physics, University of Konstanz（康斯坦茨大学物理系）；ICFO—Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology（巴塞罗那科技学院光子科学研究所）；ICREA—Institució Catalana de Recerca i Estudis Avançats（加泰罗尼亚高级研究学院）；Max-Planck-Institut für Quantenoptik（马克斯·普朗克量子光学研究所）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）；Fakultät für Physik, Ludwig-Maximilians-Universität（路德维希-马克西米利安大学物理学院）；Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）；Department of Physics, The State University of New York at Buffalo（纽约州立大学布法罗分校物理系）
