We propose a mechanism of unconventional Rydberg pumping (URP) via simultaneously driving each Rydberg atom by two classical fields with different strengths of Rabi frequencies. This mechanism differs from the general Rydberg blockade or Rydberg antiblockade since it is closely related to the ground states of atoms, i.e. two atoms in the same ground state are stable while two atoms in different ground states are resonantly excited. Furthermore, we find the URP can be employed to simplify some special quantum information processing tasks, such as implementation of a three-qubit controlled phase gate with only a single Rabi oscillation, preparation of two- and three-dimensional steady-state entanglement with two identical atoms, and realization of the autonomous quantum error correction in a Rydberg-atom-cavity system. The feasibility of the above applications is certified explicitly by the state-of-the-art technology.
Compared with the idea of universal quantum computation, a direct synthesis of a multiqubit logic gate can greatly improve the efficiency of quantum information processing tasks. Here we propose an efficient scheme to implement a three-qubit controlled-not (Toffoli) gate of neutral atoms based on unconventional Rydberg pumping. By adjusting the strengths of Rabi frequencies of driving fields, the Toffoli gate can be achieved within one step, which is also insensitive to the fluctuation of the Rydberg-Rydberg interaction. Considering different atom alignments, we can obtain a high-fidelity Toff…
We extend the recent result of bipartite Bell singlet [Carr and Saffman, Phys. Rev. Lett. {\bf111}, (2013)] to a stationary three-dimensional entanglement between two-individual neutral Rydberg atoms. This proposal makes full use of the coherent dynamics provided by Rydberg mediated interaction and the dissipative factor originating from the spontaneous emission of Rydberg state. The numerical simulation of the master equation reveals that both the target state negativity ${\cal N}(\hatρ_{\infty})$ and fidelity ${\cal F}(\hatρ_{\infty})$ can exceed 99.90%. Furthermore, a steady three-atom sing…
The resonant dipole-dipole interaction between highly excited Rydberg levels dominates the interaction of neutral atoms at short distances scaling as $1/r^3$. Here we take advantage of the combined effects of strong dipole-dipole interaction and multifrequency driving fields to propose one type of selective Rydberg pumping mechanism. In the computational basis of two atoms $\{|00\rangle, |01\rangle,|10\rangle,|11\rangle\}$, this mechanism allows $|11\rangle$ to be resonantly pumped upwards to the single-excited Rydberg states while the transitions of the other three states are suppressed. From…
Inspired by recent work [A. W. Carr and M. Saffman, Phys. Rev. Lett. 111, 033607 (2013)], we propose a simplified scheme to prepare the two-atom maximally entangled states via dissipative Rydberg pumping. Compared with the former scheme, the simplified one involves less classical laser fields and Rydberg interactions, and the asymmetric Rydberg interactions are avoided. Master equation simulations demonstrate that the fidelity and the Clauser-Horne-Shimony-Holt correlation of the maximally entangled state could reach up to 0.999 and 2.821, respectively, under certain conditions. Furthermore, w…
We propose how to achieve strong photon antibunching effect in a cavity-QED system coupled with two Rydberg-Rydberg interaction atoms. Via calculating the equal time second order correlation function g(2)(0), we find that the unconventional photon blockade and the conventional photon blockade appear in the atom-driven scheme, and they are both significantly affected by the Rydberg-Rydberg interaction. We also find that under appropriate parameters, the photon antibunching and the mean photon number can be significantly enhanced by combining the conventional photon blockade and the unconvention…
We propose and analyze an approach for preparation of high fidelity entanglement and antiferromagnetic states using Rydberg mediated interactions with dissipation. Using asymmetric Rydberg interactions the two-atom Bell singlet is a dark state of the Rydberg pumping process. Master equation simulations demonstrate Bell singlet preparation fidelity $\mcF=0.998$. Antiferromagnetic states are generated on a four spin plaquette in agreement with results found from diagonalization of the transverse field Ising Hamiltonian.
Inspired by a recent work [Reiter, Reeb, and Sørensen, Phys. Rev. Lett. {\bf117}, 040501 (2016)], we present a simplified proposal for dissipatively preparing a Greenberger-Horne-Zeilinger (GHZ) state of three Rydberg atoms in a cavity. The $Z$ pumping is implemented under the action of the spontaneous emission of $Λ$-type atoms and the quantum Zeno dynamics induced by strong continuous coupling. In the meantime, a dissipative Rydberg pumping breaks up the stability of the state $|{\rm GHZ}_+\rangle$ in the process of $Z$ pumping, making $|{\rm GHZ}_-\rangle$ be the unique steady state of syst…
Interaction-enabled topological pumping of Rydberg electrons
University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校）；The Pennsylvania State University（宾夕法尼亚州立大学）；Xi’an Jiaotong University（西安交通大学）；Rice University（莱斯大学）
We consider strongly interacting systems of effective spins, subject to dissipative spin-flip processes associated with optical pumping. We predict the existence of novel magnetic phases in the steady-state of this system, which emerge due to the competition between coherent and dissipative processes. Specifically, for strongly anisotropic spin-spin interactions, we find ferromagnetic, antiferromagnetic, spin-density-wave, and staggered-XY steady states, which are separated by nonequilibrium phase transitions meeting at a Lifshitz point. These transitions are accompanied by quantum correlation…
Nonadiabatic geometric quantum computation (NGQC) has been developed to realize fast and robust geometric gate. However, the conventional NGQC is that all of the gates are performed with exactly the sameamount of time, whether the geometric rotation angle is large or small, due to the limitation of cyclic condition. Here, we propose an unconventional scheme, called nonadiabatic noncyclic geometric quantum computation(NNGQC), that arbitrary single- and two-qubit geometric gate can be constructed via noncyclic non-Abeliangeometric phase. Consequently, this scheme makes it possible to accelerate …
We propose a cooling scheme to prepare stationary entanglement of neutral atoms in the Rydberg blockade regime by combination of periodically collective laser pumping and dissipation. In each cycle, the controlled unitary dynamics process can selectively pump atoms away from the non-target state while maintaining the target state unchanged. The subsequent dissipative process redistributes the populations of ground states through the engineered spontaneous emission. After a number of cycles, the system will be eventually stabilized into the desired steady state independent of the initial state.…
We show that in parametrically driven systems and, more generally, in systems in coherent states, off-resonant pumping can cause a transition from a continuum energy spectrum of the system to a discrete one, and result in quantum revivals of the initial state. The mechanism responsible for quantum revivals in the present case is different from that in the non-linear wavepacket dynamics of systems such as Rydberg atoms. We interpret the reported phenomena as an optical analog of Bloch oscillations realized in Fock space and propose a feasible scheme for inducing Bloch oscillations in trapped io…
Non-equilibrium quantum dynamics represents an emerging paradigm for condensed matter physics, quantum information science, and statistical mechanics. Strongly interacting Rydberg atoms offer an attractive platform to study driven-dissipative dynamics of quantum spin models with long-range order. Here, we explore the conditions under which stationary many-body entanglement persists with near-unit fidelity and high scalability. In our approach, coherent many-body dynamics is driven by Rydberg-mediated laser transitions, while atoms at the lattice boundary reduce the entropy of the many-body sta…
Preparation of entangled steady states via dissipation and pumping in Rydberg atoms has been recently found to be useful for quantum information processing. The driven-dissipative dynamics is closely related to the natural linewidth of the Rydberg states and can be usually modulated by engineering the thermal reservior. Instead of modifying the effectively radiative decay, we propose an alternatively optimized scheme, which combines the resonant Rydberg antiblockade excitation and the Lyapunov control of the ground states to speed up the prepration of the singlet state for two interacting Rydb…
Strong dipole-exchange interactions due to spontaneously produced contaminant states can trigger rapid dephasing in many-body Rydberg ensembles [E. Goldschmidt et al., PRL 116, 113001 (2016)]. Such broadening has serious implications for many proposals to coherently use Rydberg interactions, particularly Rydberg dressing proposals. The dephasing arises as a runaway process where the production of the first contaminant atoms facilitates the creation of more contaminant atoms. Here we study the time dependence of this process with stroboscopic approaches. Using a pump-probe technique, we create …
The multipartite Greenberger-Horne-Zeilinger (GHZ) states are indispensable elements for various quantum information processing tasks. Here we put forward two deterministic proposals to dissipatively prepare tripartite GHZ states in a neutral atom system. The first scheme can be considered as an extension of a recent work [T. M. Wintermantel, Y. Wang, G. Lochead, \textit{et al}, {Phys. Rev. Lett. \textbf{124}, 070503 (2020)}]. By virtue of the polychromatic driving fields and the engineered spontaneous emission, a multipartite GHZ state with odd numbers of atoms are generated with a high effic…
We study nonlinear optical effects in the laser excitation of Rydberg states. $5S_{1/2}$ and $5P_{3/2}$ levels of $^{85}$Rb are strongly coupled by a strong laser field and probed by a weak laser tuned to the $5P_{3/2} - 44D$ Rydberg resonance. We observe high contrast Autler-Townes spectra which are dependent on the pump polarization, intensity and detuning. The observed behavior agrees with calculations, which include the effect of optical pumping.
We present a scheme for engineering quantum transport dynamics of spin excitations in a chain of laser-dressed Rydberg atoms, mediated by synthetic spin-exchange arising from diagonal van der Waals interaction. The dynamic tunability and long-range interaction feature of our scheme allows for the exploration of transport physics unattainable in conventional spin systems. As two concrete examples, we first demonstrate a topological exciton pumping protocol that facilitates quantized entanglement transfer, and secondly we discuss a highly nonlocal correlated transport phenomenon which persists e…
Versatile controllability of interactions in ultracold atomic and molecular gases has now reached an unprecedented era where quantum correlations and unconventional many-body phases can be studied with no corresponding analogs in solid state systems. Recent experiments in Rydberg atomic gases have achieved exquisite control over non-local interactions, allowing novel quantum phases unreachable with the usual local interactions in atomic systems. Here, we study Rydberg dressed atomic fermions in a three dimensional optical lattice predicting the existence of hitherto unheard-of exotic mixed top…
Following Feynman and as elaborated on by Lloyd, a universal quantum simulator (QS) is a controlled quantum device which reproduces the dynamics of any other many particle quantum system with short range interactions. This dynamics can refer to both coherent Hamiltonian and dissipative open system evolution. We investigate how laser excited Rydberg atoms in large spacing optical or magnetic lattices can provide an efficient implementation of a universal QS for spin models involving (high order) n-body interactions. This includes the simulation of Hamiltonians of exotic spin models involving n-…
We describe a quantum simulator for the Hubbard--Holstein model (HHM), comprising two dressed Rydberg atom species held in a monolayer by independent painted potentials, predicting that boson-mediated preformed pairing, and Berezinskii--Kosterlitz--Thouless (BKT) transition temperatures are experimentally accessible. The HHM is important for modeling the essential physics of unconventional superconductors. Experimentally realizable quantum simulators for HHMs are needed: (1) since HHMs are difficult to solve numerically and analytically, (2) to explore how competition between electron-phonon i…
We discuss in detail the implementation of an open-system quantum simulator with Rydberg states of neutral atoms held in an optical lattice. Our scheme allows one to realize both coherent as well as dissipative dynamics of complex spin models involving many-body interactions and constraints. The central building block of the simulation scheme is constituted by a mesoscopic Rydberg gate that permits the entanglement of several atoms in an efficient, robust and quick protocol. In addition, optical pumping on ancillary atoms provides the dissipative ingredient for engineering the coupling between…
Samples with few hundred atoms within a few micrometer sized region of space are large enough to provide efficient cooperative absorption and emission of light, and small enough to ensure strong dipole-dipole interactions when atoms are excited into high-lying Rydberg states. Based on a recently proposed collective encoding scheme, we propose to build few-qubit quantum registers in such samples. The registers can store and transmit quantum information in the form of single photons, and they can employ entanglement pumping protocols to perform ideally in networks for scalable quantum computing …
Dynamical quantum phase transitions (DQPTs) feature singular temporal behavior in transient quantum states during nonequilibrium real-time evolution. In this work we show that DQPTs in random Ising chains exhibit critical behavior with nontrivial exponents that are not integer valued and not of mean-field type. By means of an exact renormalization group transformation we estimate the exponents with high accuracy eliminating largely any finite-size effects. We further discuss how the considered dynamical phenomena can be made accessible in current Rydberg atom platforms. In this context we expl…
Quantum state transport is an important way to study the energy or information flow. By combining the unconventional Rydberg pumping mechanism and the diagonal form of van der Waals interactions, we construct a theoretical model via second-order perturbation theory to realize a long-range coherent transport inside the ground-state manifold of neutral atoms system. With the adjustment of the Rabi frequencies and the interatomic distance, this model can be used to simulate various single-body physics phenomena such as Heisenberg $XX$ spin chain restricted in the single-excitation manifold, coher…
We develop a general theory to study the electromagnetically induced transparency (EIT) in ultracold quantum gases, applicable for both Bose and Fermi gases with arbitrary inter-particle interaction strength. We show that, in the weak probe field limit, the EIT spectrum is solely determined by the single particle Green's function of the ground state atoms, and reflects interesting quantum many-body effects when atoms are virtually coupled to the low-lying Rydberg states. As an example, we apply our theory to 1D Luttinger liquid, Bose-Mott insulator state, and the superfluid state of two-compon…
