Coherent spin states in semiconductor quantum dots offer promise as electrically controllable quantum bits (qubits) with scalable fabrication. For few-electron quantum dots made from gallium arsenide (GaAs), fluctuating nuclear spins in the host lattice are the dominant source of spin decoherence. We report a method of preparing the nuclear spin environment that suppresses the relevant component of nuclear spin fluctuations below its equilibrium value by a factor of ~ 70, extending the inhomogeneous dephasing time for the two-electron spin state beyond 1 microsecond. The nuclear state can be readily prepared by electrical gate manipulation and persists for > 10 seconds.
The optimal $N$-pulse dynamical decoupling discovered by Uhrig for a spin-boson mmodel [Phys. Rev. Lett, {\bf 98}, 100504 (2007)] is proved to be universal in suppressing to $O(T^{N+1})$ the pure dephasing or the longitudinal relaxation of a qubit (or spin-1/2) coupled to a generic bath in a short-time evolution of duration $T$. It is also found that for the purpose of suppressing the longitudinal relaxation, an ideal Uhrig $π$-pulse sequence can be generalized to a sequence consisting of the ideal one superimposed with finite-duration pulses satisfying certain symmetry requirements.
We show that dephasing of individual atoms destroys the superradiance transition of the Dicke model, but that adding individual decay toward the spin down state can restore this transition. To demonstrate this, we present a method to give an exact solution for the $N$ atom problem with individual dephasing which scales polynomially with $N$. By comparing finite size scaling of our exact solution to a cumulant expansion, we confirm the destruction and restoration of the superradiance transition holds in the thermodynamic limit.
We investigate theoretically under which conditions a stable and high-fidelity preparation of the biexciton state in a quantum dot can be realized by means of adiabatic rapid passage in the presence of acoustic phonon coupling. Our analysis is based on a numerically complete real-time path integral approach and comprises different schemes of optical driving using frequency-swept (chirped) pulses. We show that depending on the size of the biexciton binding energy, resonant two-photon excitations or two-color schemes can be favorable. It is demonstrated that the carrier-phonon interaction strong…
The coupling between single-photon emitters and phonons opens many possibilities to store and transmit quantum properties. In this paper we apply the independent boson model to describe the coupling between an optically driven two-level system and a discrete phonon mode. Tailored optical driving allows not only to generate coherent phonon states, but also to generate coherent superpositions in the form of Schrödinger cat states in the phonon system. We analyze the influence of decay and dephasing of the two-level system on these phonon preparation protocols. We find that the decay transforms t…
We study dephasing in electron transport through a large quantum dot (a Fabry-Perot interferometer) in the fractional quantum Hall regime with filling factor $2/3$. In the regime of sequential tunneling, dephasing occurs due to electron fractionalization into counterpropagating charge and neutral edge modes on the dot. In particular, when the charge mode moves much faster than the neutral mode, and at temperatures higher than the level spacing of the dot, electron fractionalization combined with tje fractional statistics of the charge mode leads to the dephasing selectively suppressing $h/e$ A…
Unwanted interaction between a quantum system and its fluctuating environment leads to decoherence and is the primary obstacle to establishing a scalable quantum information processing architecture. Strategies such as environmental and materials engineering, quantum error correction and dynamical decoupling can mitigate decoherence, but generally increase experimental complexity. Here we improve coherence in a qubit using real-time Hamiltonian parameter estimation. Using a rapidly converging Bayesian approach, we precisely measure the splitting in a singlet-triplet spin qubit faster than the s…
Motivated by fundamental questions about the loss of phase coherence at low temperature we consider relaxation, dephasing and renormalization effects in quantum two-level systems which are coupled to a dissipative environment. We observe that experimental conditions, e.g., details of the initial state preparation, determine to which extent the environment leads to dephasing or to renormalization effects. We analyze an exactly solvable limit where the relation between both can be demonstrated explicitly. We also study the effects of dephasing and renormalization on response functions.
We report a study of suppressed spin dephasing for quasi-one-dimensional electron ensembles in wires etched into a GaAs/AlGaAs heterojunction system. Time-resolved Kerr-rotation measurements show a suppression that is most pronounced for wires along the [110] crystal direction. This is the fingerprint of a suppression that is enhanced due to a strong anisotropy in spin-orbit fields that can occur when the Rashba and Dresselhaus contributions are engineered to cancel each other. A surprising observation is that this mechanisms for suppressing spin dephasing is not only effective for electrons i…
We present an experimental realization of the transmon qubit, an improved superconducting charge qubit derived from the Cooper pair box. We experimentally verify the predicted exponential suppression of sensitivity to 1/f charge noise [J. Koch et al., Phys. Rev. A 76, 042319 (2007)]. This removes the leading source of dephasing in charge qubits, resulting in homogenously broadened transitions with relaxation and dephasing times in the microsecond range. Our systematic characterization of the qubit spectrum, anharmonicity, and charge dispersion shows excellent agreement with theory, rendering t…
A robust scheme for state preparation and state trapping for the spins of two electrons in a semiconductor double quantum dot is presented. The system is modeled by two spins coupled to two independent bosonic reservoirs. Decoherence effects due to this environment are minimized by application of optimized control fields which make the target state to the ground state of the isolated driven spin system. We show that stable spin entanglement with respect to pure dephasing is possible. Specifically, we demonstrate state trapping in a maximally entangled state (Bell state) in the presence of deco…
The resistivity of disordered metallic layer sandwiched by two ferromagnetic layers at low-temperature is investigated theoretically. It is shown that the magnetic field acting at the interface does not affect the classical Boltzmann resistivity but causes a dephasing among electrons in the presence of the spin-orbit interaction, suppressing the anti-localization due to the spin-orbit interaction. The dephasing turns out to be stronger in the case where the magnetization of the two layers is parallel, contributing to a positive magnetoresistance close to a switching field at low temperature.
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps and …
We investigate the effect of electron-electron interactions on Aharonov-Bohm (AB) current oscillations in nanorings formed by a chain of metallic quantum dots. We demonstrate that electron-electron interactions cause electron dephasing thereby suppressing the amplitude of AB oscillations at all temperatures down to T=0. The crossover between thermal and quantum dephasing is found to be controlled by the ring perimeter. Our predictions can be directly tested in future experiments.
A spin qubit in semiconductor quantum dots holds promise for quantum information processing for scalability and long coherence time. An important semiconductor qubit system is a double quantum dot trapping two electrons or holes, whose spin states encode either a singlet-triplet qubit or two single-spin qubits coupled by exchange interaction. In this article, we report progress on spin dephasing of two exchange-coupled spins in a double quantum dot. We first discuss the schemes of two-qubit gates and qubit encodings in gate-defined quantum dots or donor atoms based on the exchange interaction.…
Carrier spins in semiconductor nanocrystals are promising candidates for quantum information processing. Using a combination of time-resolved Faraday rotation and photoluminescence spectroscopies, we demonstrate optical spin polarization and coherent spin precession in colloidal CsPbBr3 nanocrystals that persists up to room temperature. By suppressing the influence of inhomogeneous hyperfine fields with a small applied magnetic field, we demonstrate inhomogeneous hole transverse spin-dephasing times (T2*) that approach the nanocrystal photoluminescence lifetime, such that nearly all emitted ph…
A key insight from recent studies is that noise, such as dephasing, can improve the efficiency of quantum transport by suppressing coherent single-particle interference effects. However, it is not yet clear whether dephasing can enhance transport in an interacting many-body system. Here, we address this question by analyzing the transport properties of a boundary driven spinless fermion chain with nearest-neighbor interactions subject to bulk dephasing. The many-body nonequilibrium stationary state is determined using large-scale matrix product simulations of the corresponding quantum master e…
We present a systematic, perturbative method for correcting quantum gates to suppress errors that take the target system out of a chosen subspace. It addresses the generic problem of non-adiabatic errors in adiabatic evolution and state preparation, as well as general leakage errors due to spurious couplings to undesirable states. The method is based on the Magnus expansion: by correcting control pulses, we modify the Magnus expansion of an initially-given, imperfect unitary in such a way that the desired evolution is obtained. Applications to adiabatic quantum state transfer, superconducting …
We consider the problem of pulsed biexciton preparation in a quantum dot and show that a pulse-sequence with a simple on-off-on modulation can achieve complete preparation of the target state faster than the commonly used constant and hyperbolic secant pulses. The durations of the pulses composing the sequence are obtained from the solution of a transcendental equation. Furthermore, using numerical optimal control, we demonstrate that for a wide range of values of the maximum pulse amplitude, the proposed pulse-sequence prepares the biexciton state in the numerically obtained minimum time, for…
We demonstrate high-fidelity, quantum nondemolition, single-shot readout of a superconducting flux qubit in which the pointer state distributions can be resolved to below one part in 1000. In the weak excitation regime, continuous measurement permits the use of heralding to ensure initialization to a fiducial state, such as the ground state. This procedure boosts readout fidelity to 93.9% by suppressing errors due to spurious thermal population. Furthermore, heralding potentially enables a simple, fast qubit reset protocol without changing the system parameters to induce Purcell relaxation.
Dynamical error suppression techniques are commonly used to improve coherence in quantum systems. They reduce dephasing errors by applying control pulses designed to reverse erroneous coherent evolution driven by environmental noise. However, such methods cannot correct for irreversible processes such as energy relaxation. In this work, we investigate a complementary, stochastic approach to reducing errors: instead of deterministically reversing the unwanted qubit evolution, we use control pulses to shape the noise environment dynamically. In the context of superconducting qubits, we implement…
Superconducting transmon qubits comprise one of the most promising platforms for quantum information processing due to their long coherence times and to their scalability into larger qubit networks. However, their weakly anharmonic spectrum leads to spectral crowding in multiqubit systems, making it challenging to implement fast, high-fidelity gates while avoiding leakage errors. To address this challenge, we use a protocol known as SWIPHT [Phys. Rev. B 91, 161405(R) (2015)], which yields smooth, simple microwave pulses designed to suppress leakage without sacrificing gate speed through spectr…
We solve the long-standing central spin problem for a general set of inhomogeneous bath couplings and a large class of initial bath states. We compute the time evolution of the coherence of a central spin coupled to a spin bath by resumming all orders of the time-convolutionless master equation, thus avoiding the need to assume weak coupling to the bath. The fully quantum, non-Markovian solution is obtained in the large-bath limit and is valid up to a timescale set by the largest coupling constant. Our result captures the full decoherence of an electron spin qubit coupled to a nuclear spin bat…
We experimentally demonstrate an ultrafast method for preparing spin states of donor-bound electrons in GaAs with single laser pulses. Each polarization state of a preparation pulse has a direct mapping onto a spin state, with bijective correspondence between the Poincaré-sphere (for photon polarization) and Bloch-sphere (for spin) state representations. The preparation is governed by a stimulated Raman process and occurs orders of magnitude faster than the spontaneous emission and spin dephasing. Similar dynamics governs our ultrafast optical Kerr detection of the spin coherence, thus getting…
We report theoretical studies of adiabatic population transfer using dressed spin states. Quantum optimal control using the algorithm of Chopped Random Basis (CRAB) has been implemented in a negatively charged diamond nitrogen vacancy center that is coupled to a strong and resonant microwave field. We show that the dressed spin states are highly effective in suppressing effects of spin dephasing on adiabatic population transfer. The numerical simulation also demonstrates that CRAB-based quantum optimal control can enable an efficient and robust adiabatic population transfer.
Dissipative preparation and stabilization of d-mode multinomial cat states
Institute for Quantum Materials and Technology, Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院量子材料与技术研究所）；Institute for Theory of Condensed Matter, Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院凝聚态理论研究所）；Institut de Science et d’Ingénierie Supramoléculaires (ISIS, UMR7006), University of Strasbourg and CNRS（斯特拉斯堡大学及法国国家科学研究中心超分子科学与工程研究所）
This work presents epitaxial growth and optical spectroscopy of CdTe quantum dots (QDs) in (Cd,Zn,Mg)Te barriers placed on the top of (Cd,Zn,Mg)Te distributed Bragg reflector. The formed photonic mode in our half-cavity structure permits to enhance the local excitation intensity and extraction efficiency of the QD photoluminescence, while suppressing the reflectance within the spectral range covering the QD transitions. This allows to perform coherent, nonlinear, resonant spectroscopy of individual QDs. The coherence dynamics of a charged exciton is measured via four-wave mixing, with the esti…
Over the past decade we have seen an explosion of demonstrations of quantum coherence in atomic, optical, and condensed matter systems. These developments have placed a new emphasis on the production of robust and optimal quantum control techniques in the presence of environmental noise. We discuss the use of dynamical decoupling as a form of open-loop quantum control capable of suppressing the effects of dephasing in quantum coherent systems. We introduce the concept of dynamical decoupling pulse-sequence construction as a filter-design problem, making connections with filter design from cont…
We propose a dissipative method for the preparation of many-body steady entangled states in spin and fermionic chains. The scheme is accomplished by means of an engineered set of Lindbladians acting over the eigenmodes of the system, whose spectrum is assumed to be resolvable. We apply this idea to prepare a particular entangled state of a spin chain described by the XY model, emphasizing its generality and experimental feasibility. Our results show that our proposal is capable of achieving high fidelities and purities for a given target state even when dephasing and thermal dissipative proces…
Methods that preserve coherence broadly impact all quantum information processing and metrology applications. Dynamical decoupling methods accomplish this by protecting qubits in noisy environments but are typically constrained to the limit where the qubits themselves are non-interacting. Here we consider the alternate regime wherein the inter-qubit couplings are of the same order as dephasing interactions with the environment. We propose and demonstrate a multi-pulse protocol that protects transverse spin states by suitably Hamiltonian engineering the inter-spin coupling while simultaneously …
The nuclear spins in nanostructured semiconductors play a central role in quantum applications. The nuclear spins represent a useful resource for generating local magnetic fields but nuclear spin noise represents a major source of dephasing for spin qubits. Controlling the nuclear spins enhances the resource while suppressing the noise. NMR techniques are challenging: the group III and V isotopes have large spins with widely different gyromagnetic ratios; in strained material there are large atom-dependent quadrupole shifts; and nanoscale NMR is hard to detect. We report NMR on 100,000 nuclear…
Hyperfine interactions with a nuclear spin environment fundamentally limit the coherence properties of confined electron spins in the solid-state. Here, we show that a quantum interference effect in optical absorption from two electronic spin states of a solid-state emitter can be used to prepare the surrounding environment of nuclear spins in well-defined states, thereby suppressing electronic spin dephasing. The evolution of the coupled electron-nuclei system into a coherent population trapping state by optical excitation induced nuclear spin diffusion can be described in terms of Levy fligh…
A controlled quantum system can alter its environment by feedback, leading to reduced-entropy states of the environment and to improved system coherence. Here, using a quantum dot electron spin as control and probe, we prepare the quantum dot nuclei under the feedback of coherent population trapping and measure the evolution from a thermal to a reduced-entropy state, with the immediate consequence of extended qubit coherence. Via Ramsey interferometry on the electron spin, we directly access the nuclear distribution following its preparation, and measure the emergence and decay of correlations…
We report here on results of experimental-theoretical investigation of high-order harmonic generation (HHG) in layers of CdSe semiconductor quantum dots of different sizes and a reference bulk CdSe thin film. We observe a strong decrease in the efficiency, up to complete suppression of HHG with energies of quanta above the bandgap for the smallest dots, whereas the intensity of below bandgap harmonics remains weakly affected by the dot size. In addition, it is observed that the ratio between suppression of above gap harmonics versus below gap harmonics increases with driving wavelength. We sug…
We provide a general method to calculate and maximize the purity of a qubit interacting with an anisotropic non-Markovian environment. Counter to intuition, we find that the purity is often maximized by preparing and storing the qubit in a superposition of non-interacting eigenstates. For a model relevant to decoherence of a heavy-hole spin qubit in a quantum dot or for a singlet-triplet qubit for two electrons in a double quantum dot, we show that preparation of the qubit in its non-interacting ground state can actually be the worst choice to maximize purity. We further give analytical result…
Rapid and efficient preparation, manipulation and transfer of quantum states through an array of quantum dots (QDs) is a demanding requisite task for quantum information processing and quantum computation in solid-state physics. Conventional adiabatic protocols, as coherent transfer by adiabatic passage (CTAP) and its variations, provide slow transfer prone to decoherence, which could lower the fidelity to some extent. To achieve the robustness against decoherence, we propose a protocol of speeding up the adiabatic charge transfer in multi-QD systems, sharing the concept of "Shortcuts to Adiab…
