We describe an effective resonant interaction between two localized wave modes of different nature: a plasmon-polariton at a metal surface and a self-focusing beam (spatial soliton) in a non-linear dielectric medium. Propagating in the same direction, they represent an exotic coupled-waveguide system, where the resonant interaction is controlled by the soliton amplitude. This non-linear system manifests hybridized plasmon-soliton eigenmodes, mutual conversion, and non-adiabatic switching, which offer exciting opportunities for manipulation of plasmons via spatial solitons.
This paper deals with the temporal nonlinear dynamics of plasmon-solitons in a plasmonic waveguide. Duffing equation is recognized as the temporal part of the nonlinear amplitude equation governing the plasmonic waveguide. It is shown that Duffing oscillator waveforms stand for the temporal nonlinear dynamics of plasmon-soliton waves. The exchange of Lorentz-type bright and dark solitons energies gives rise to a Fano resonance. It is thus shown that the interaction of solitons and the formation of plasmon-solitons is inherently nonlinear. It is accordingly indicated that the nonlinear modulati…
We demonstrate that soliton-plasmon bound states appear naturally as propagating eigenmodes of nonlinear Maxwell's equations for a metal/dielectric/Kerr interface. By means of a variational method, we give an explicit and simplified expression for the full-vector nonlinear operator of the system. Soliplasmon states (propagating surface soliton-plasmon modes) can be then analytically calculated as eigenmodes of this non-selfadjoint operator. The theoretical treatment of the system predicts the key features of the stationary solutions and gives physical insight to understand the inherent stabili…
We theoretically show the existence of cascaded second-order surface plasmon solitons propagating at the interface between metal and linear dielectric. Nonlocal multipole nonlinearities originating from free conduction electron plasma of a metal lead to strong interaction between co-propagating surface plasmon polariton beams at fundamental and second harmonic frequencies. Finite element numerical modelling for effective two-dimensional medium explicitly demonstrates the solitons formation, confirming the theoretical results. The non-diffractive regime of propagation has been demonstrated at s…
Nonlinear properties of a multi-layer stack of graphene sheets are studied. It is predicted that such a structure may support dissipative plasmon-solitons generated and supported by an external laser radiation. Novel nonlinear equations describing spatial dynamics of the nonlinear plasmons driven by a plane wave in the Otto configuration are derived and the existence of single and multi-hump dissipative solitons in the graphene structure is predicted.
Formation of a novel hybrid-vector spatial plasmon-soliton in a Kerr slab embedded in-between metal plates is predicted and analyzed with a modified NLSE, encompassing hybrid vector field characteristics. Assisted by the transverse plasmonic effect, the self trapping dimension of the plasmon-soliton was substantially compressed (compared to the dielectrically cladded slab case) when reducing the slab width. The practical limitation of the Plasmon-soliton size reduction is determined by available nonlinear materials and metal loss. For the extreme reported values of nonlinear index change, we p…
We consider the process of light scattering by optical solitons in a planar waveguide with homogeneous and inhomogeneous refractive index core. We observe resonant reflection (Fano resonances) as well as resonant transmission of light by optical solitons. All resonant effects can be controlled in experiment by changing the soliton intensity.
We study the interband self-induced transmission of surface plasmon polaritons in a gold film surrounded by an external Kerr medium. We model the optical propagation by using a version of the generalized nonlinear Schrodinger equation for the field envelope coupled to Bloch equations for valence electrons of gold, predicting self-induced transparency of ultrashort plasmon solitons with a pulse duration below 10 fs. We demonstrate that the Kerr nonlinearity from the surrounding dielectric can be used to compensate for the group velocity dispersion, and that the impact of dephasing and decay pro…
We examine the dynamics of a dissipative photonic Josephson junction formed by the weak coupling of an optical soliton in a nonlinear dielectric waveguide and a co-propagating surface plasmon along a parallel metal surface with a linear dielectric spacer. We employ a heuristic model with a coupling function that depends on the soliton amplitude, and consider two phenomenological dissipation mechanisms separately: angular velocity dissipation and population imbalance dissipation. In the former dissipation mechanism, the system exhibits phase-slip phenomenon where the odd-πphase modes decay into…
We study nonlinear modes in one-dimensional arrays of doped graphene nanodisks with Kerr-type nonlinear response in the presence of an external electric field. We present the theoretical model describing the evolution of the disks' polarizations, taking into account intrinsic graphene losses and dipole-dipole coupling between the graphene nanodisks. We reveal that this nonlinear system can support discrete dissipative scalar solitons of both longitudinal and transverse polarizations, as well as vector solitons composed of two mutually coupled polarization components. We demonstrate the formati…
We consider the linear and nonlinear models of generation of the surface plasmon-polaritons on the boundary of nonmagnetic dielectric medium and nonmagnetic metal. We have shown how the three-dimensional incident wave is transformed to the fluxes of surface plasmon-polaritons at the first and second harmonics of the TM-mode. These "slow" and "fast" fluxes of the surface plasmon-polaritons are formed at the both harmonics at the weak interaction. We obtain that the pulses of surface plasmon-polaritons propagate as the bright and dark solitons at the strong interaction of the first and second ha…
Controlling low power light beam self-confinement with ultrafast response time opens up opportunities for the development of signal processing in microdevices. The combination of highly nonlinear medium with the tight confinement of plasmonic waves offers a viable but challenging configuration to reach this goal. Here, we report the experimental observation of plasmon-soliton waves propagating in a chalcogenide-based four-layer planar geometry engineered to limit plasmon propagation losses while exhibiting efficient Kerr self-focusing at moderate power. The observations reveal a strongly enhan…
Assuming that the resonant surface plasmons on a spherical nanoparticle is formed by standing waves of two counter-propagating surface plasmon waves along the surface, by using Mie theory simulation, we find that the dispersions of surface plasmon resonant modes supported by silver nanospheres match that of the surface plasmons on a semi-infinite medium-silver interface very well. This suggests that the resonant surface plasmons of a metal nanosphere can be treated as a propagating surface plasmon wave.
The properties of optical solitons in periodic nonlinear media are reviewed. The emphasis is on solitons in periodically refractive media (Bragg gratings) incorporating a periodic set of thin layers of two-level systems resonantly interacting with the field. Such media support a variety of bright and dark `gap solitons' propagating in the band gaps of the Bragg gratings, as well as their multi - dimensional analogs (light bullets). These novel gap solitons differ substantially from their counterparts in periodic media with either cubic or quadratic off-resonant nonlinearities.
We study the formation of gap solitons in the presence of parametric pump. It is shown that parametric pump can stabilize stationary solitons continuously emitting dispersive waves. The resonant interactions of the radiation and the solitons are studied and it is shown that the solitons can be effectively controlled by the radiation. In particular it is shown that the solitons can collide or to get pinned to inhomogeneities due to the interactions mediated by the resonant radiation.
We present three complementary methods to study stationary nonlinear solutions in one-dimensional nonlinear metal-dielectric structures. Two of them use an approximate treatment of the Kerr type nonlinear term taking into account only the leading electric field component, while the third one allows for an exact treatment of the nonlinearity. A direct comparison of the results obtained with all three models is presented and the excellent agreement between them justifies the assumptions that have been used to construct the models. A systematic study of the configurations made of two, three, or f…
We demonstrate a multi-spectral polarization sensitive mid-infrared dots-in-a-well (DWELL) photodetector utilizing surface-plasmonic resonant elements, with tailorable frequency response and polarization selectivity. The resonant responsivity of the surface-plasmon detector shows an enhancement of up to 5 times that of an unpatterned control detector. As the plasmonic resonator involves only surface patterning of the top metal contact, this method is independent of light-absorbing material and can easily be integrated with current focal plane array processing for imaging applications.
A rigorous theory of photon emission accompanied inelastic tunnelling inside the gap of plasmonic nanoantennas has been developed. The disappointingly low efficiency of the electrical excitation of surface plasmon polaritons in these structures can be increased by orders of magnitude when a resonant tunnelling structure is incorporated inside the gap. Resonant tunnelling assisted surface plasmon emitter may become a key element in future electrically-driven nanoplasmonic circuits.
We study the propagation of surface plasmon polaritons (SPPs) on a metal surface which hosts a thin film of a liquid dielectric. The ohmic losses, that are inherently present due to the coupling of SPPs to conductors' electron plasma, induce temperature gradients and fluid deformation driven by the thermocapillary effect, which lead to a nonlinear and nonlocal change of the effective dielectric constant. The latter extends beyond the regions of highest optical intensity, and constitutes a novel thermally self-induced mechanism that affects the propagation of the SPPs. We derive the nonlinear a…
We theoretically investigate the spontaneous emission process of an optical, dipolar emitter in metal-dielectric-metal slab and slot waveguide structures. We find that both structures exhibit strong off-resonant emission enhancements due to the tight confinement of modes between two metallic plates. The large enhancement of surface plasmon-polariton excitation enables dipole emission to be preferentially coupled into plasmon waveguide modes. These structures find applications in creating nanoscale local light sources or in generating guided single plasmons in integrated optical circuits.
A matrix balanced version of the Recursive Centered T Matrix Algorithm (RCTMA) applicable to systems possessing resonant inter-particle couplings is presented. Possible domains of application include systems containing interacting localized plasmon resonances, surface resonances, and photonic jet phenomena. This method is of particular interest when considering modifications to complex systems. The numerical accuracy of this technique is demonstrated in a study of particles with strongly interacting localized plasmon resonances.
We report on the existence of a novel kind of squeezing in photonic crystal fibers which is conceptually intermediate between the four-wave mixing induced squeezing, in which all the participant waves are monochromatic waves, and the self-phase modulation induced squeezing for a single pulse in a coherent state. This hybrid squeezing occurs when an arbitrary short soliton emits quasi-monochromatic resonant radiation near a zero group velocity dispersion point of the fiber. Photons around the resonant frequency become strongly correlated due to the presence of the classical soliton, and a reduc…
We study the effect of off-resonant plasmon modes on spaser threshold in nanoparticle-based spasers. We develop an analytical semiclassical model and derive spaser threshold condition accounting for gain coupling to higher-order plasmons. We show that such a coupling originates from inhomogeneity of gain distribution near the metal surface and leads to an upward shift of spaser frequency and population inversion threshold. This effect is similar, albeit significantly weaker, to quenching of plasmon-enhanced fluorescence near metal nanostructures due to excitation of off-resonant modes with wid…
We analytically and numerically study the direct soliton generation in a cw-pumped doubly resonant degenerate optical parametric oscillator via pump frequency scanning. By means of bifurcation and linear stability analysis of the homogeneous solutions, we discriminate distinctive soliton forming mechanisms and corresponding dynamics, depending on pump and signal group velocity dispersions (GVDs). To the best of our knowledge, this is the first study regarding the dynamics of pure quadratic solitons. In addition, we discuss how to extend soliton existing regime and easily access quadratic solit…
We consider the process of low-power light scattering by optical solitons in a slab waveguide with homogeneous and inhomogeneous refractive index core. We observe resonant reflection (Fano resonance) as well as resonant transmission of light by optical solitons at certain incident angles. The resonance position can be controlled experimentally by changing the soliton intensity and the relative frequency detuning between the soliton and the probe light beams.
We study analytically and numerically a kind of diffractive resonant radiation emitted by spatial solitons, which is generated in waveguide arrays with Kerr nonlinearity. The phase matching condition between soliton and radiation is derived and agrees well with direct pulse propagation simulations. The folded dispersion due to the Brillouin zone leads to a peculiar anomalous soliton recoil that we describe in detail. A linear potential applied across the array generates the analogue of the Raman self-frequency shift in optical fibers, only now applied to the wavenumber. We demonstrate that it …
We present an electrically tunable terahertz two dimensional plasmonic interferometer with an integrated detection element that down converts the terahertz fields to a DC signal. The integrated detector utilizes a resonant plasmonic homodyne mixing mechanism that measures the component of the plasma waves in-phase with an excitation field functioning as the local oscillator. Plasmonic interferometers with two independently tuned paths are studied. These devices demonstrate a means for developing a spectrometer-on-a-chip where the tuning of electrical length plays a role analogous to that of ph…
Vertical gold-nanogaps are created on microtubular cavities to explore the coupling between resonant light supported by the microcavities and surface plasmons localized at the nanogaps. Selective coupling of optical axial modes and localized surface plasmons critically depends on the exact location of the gold-nanogap on the microcavities which is conveniently achieved by rolling-up specially designed thin dielectric films into three dimensional microtube ring resonators. The coupling phenomenon is explained by a modified quasi-potential model based on perturbation theory. Our work reveals the…
Here, we study the possibility of selective high-harmonic generation (HHG) based on the concept of charge transfer plasmons (CTP) in bridged nanoparticle assemblies. By choosing plasmonic dimer nanoantenna, as a fundamental member of nanoclusters family, and bridging the gap space between the proximal nanoparticles with an optothermally controllable substance, we selectively produced two different harmonics at different states of the functional bridge. To this end, the conductive connection between the nanoparticles is mediated with Ge2Sb2Te5 (GST), which inherently has opposite optical and el…
A plasmonic coupled-cavity system, which consists of a quarter-wave coupler cavity, a resonant Fabry-Perot detector nanocavity, and an off-resonant reflector cavity, is used to enhance the localization of surface plasmons in a plasmonic detector. The coupler cavity is designed based on transmission line theory and wavelength scaling rules in the optical regime, while the reflector cavity is derived from off-resonant resonator structures to attenuate transmission of plasmonic waves. We observed strong coupling of the cavities in simulation results, with an 86% improvement of surface plasmon loc…
We demonstrate that the relatively small power induced changes in the soliton wavenumber comparable with splitting of the effective indexes of the orthogonally polarized waveguide modes result in significant changes of the efficiency of the interaction between solitons and dispersive waves and can be used to control energy transfer between the soliton and newly generated waves and to delay or accelerate solitons.
Evanescent waves in a metal thin film with nonlocality are found to propagate in normal direction to film surface with quenched (to zero) energy dissipation associated with intra-band electron transitions when wave numbers satisfy a resonant condition. It is shown that resonant quenching of energy dissipation (RQED) effect occurs in metal films with thicknesses of less or larger than, but still on the order of, the nonlocality scale length. RQED ceases to exist in metal films whose thickness exceeds a cutoff length or in metal films with local dielectric permittivity. Resonant quenching of ene…
Surface plasmon polaritons (SPPs) lasing requires population inversion, it is inefficient and possesses poor spectral properties. We develop an inversion-less concept for a quantum plasmonic waveguide that exploits unidirectional superradiant SPP emission of radiation to produce intense coherent surface plasmon beams. Our scheme includes a resonantly driven cold atomic medium in a lossless dielectric situated above an ultra-low loss negative index metamaterial~(NIMM) layer. We propose generating unidirectional superradiant radiation of the plasmonic field within an atomic medium and a NIMM lay…
Correlated polarization dependences between surface-enhanced resonant Raman scattering and plasmon resonance elastic scattering showing spectral uncorrelation to each other
We derive envelope equations which generate the Maxwell-Lorentz model and describe the interaction of optical pulses with plasmonic oscillations in metal nanoparticle composites. A family of solitary wave solutions is found which is analogous to self-induced transparency in Maxwell-Bloch. The evolution of incident optical pulses is studied numerically as are the collision dynamics of the solitary waves. These simulations reveal that the collision dynamics vary from near perfectly elastic to highly radiative depending on the relative phase of the initial pulses.
The physical mechanism underlying scattering properties of matter wave gap-solitons by linear optical lattice defects is investigated. The occurrence of repeated reflection, transmission and trapping regions for increasing strengths of an optical lattice defect are shown to be due to impurity modes inside the defect potential with chemical potentials and numbers of atoms matching corresponding quantities of an incoming gap-soliton. For gap-solitons with chemical potentials very close to band edges, the number of resonances observed in the scattering coincides with the number of bound states wh…
We present an analytic theory for the optical properties of ellipsoidal plasmonic particles covered by anisotropic molecular layers. The theory is applied to the case of a prolate spheroid covered by chromophores oriented parallel and perpendicular to the metal surface. For the case that the molecular layer resonance frequency is close to being degenerate with one of the particle plasmon resonances strong hybridization between the two resonances occur. Approximate analytic expressions for the hybridized resonance frequencies, their extinction cross section peak heights and widths are derived. …
We report on an experimental and numerical study of temporal Kerr cavity soliton dynamics in dispersion-managed fiber ring resonators. We find that dispersion management can significantly magnify the Kelly-like resonant radiation sidebands emitted by the solitons. Because of the underlying phase-matching conditions, the sideband amplitudes tend to increase with increasing pump-cavity detuning, ultimately limiting the range of detunings over which the solitons can exist. Our experimental findings show excellent agreement with numerical simulations.
The red shifted solitonic resonant radiation is a fascinating phase matching phenomenon that occurs when an optical pulse, launched in the normal dispersion regime of photonic crystal fiber, radiates across the zero dispersion wavelength. The formation of such phase-matched radiation is independent of the generation of any optical soliton and mainly governed by the leading edge of input pump which forms a shock front. The radiation is generated at the anomalous dispersion regime and found to be confined both in time and frequency domain. We experimentally investigate the formation of such radi…
A significant interest in combining plasmonics and magnetism at the nanoscale gains momentum in both photonics and magnetism sectors that are concerned with the resonant enhancement of light-magnetic-matter interaction in nanostructures. These efforts result in a considerable amount of literature, which is difficult to collect and digest in limited time. Furthermore, there is insufficient exchange of results between the two research sectors. Consequently, the goal of this review paper is to bridge this gap by presenting an overview of recent progress in the field of magneto-plasmonics from two…
We investigate existence and linear stability of coupled vortex solitons supported by cascaded four-wave mixing in a Raman active medium excited away from the resonance. We present a detailed analysis for the two- and three-component vortex solitons and demonstrate the formation of stable and unstable vortex solitons, and associated spatio-temporal helical beams, under the conditions of the simultaneous frequency and vortex comb generation.
Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at oblique incidence. We study the influence of the periodicity, the incidence angle and the direction of the linear input polarization on the second harmonic generation. Excitation of the surface lattice resonance either at the fundamental or second harmonic wavelength, achieved by varying the incidence angle, enhance the conversion efficiency. As a special ca…
We report a theoretical investigation of quadratic frequency combs in a dispersive second-harmonic generation cavity system. We identify different dynamical regimes and demonstrate that the same system can exhibit both bright and dark localized cavity solitons in the absence of a temporal walk-off.
Optical metasurfaces have great potential to form the platform for manipulation of surface waves. A plethora of advanced surface-wave phenomena utilizing negative refraction, self-collimation and channeling of 2D waves can be realized through on-demand engineering of dispersion properties of a periodic metasurface. In this letter, we report on the first-time direct experimental polarization-resolved measurement of dispersion of 2D optical plasmons supported by an anisotropic metasurface. We demonstrate that a subdiffractive array of strongly coupled resonant anisotropic plasmonic nanoparticles…
We compare the optical response of isolated nanowires, double-wire systems, and Pi-structures, and show that their radiation is well described in terms of their electric and magnetic dipole moments. We also show that both dielectric permittivity and magnetic permeability can be negative at optical and near infrared frequencies, and demonstrate the connection between the geometry of the system and its resonance characteristics. We conclude that plasmonic nanowires can be employed for developing novel negative-index materials. Finally, we demonstrate that it is possible to construct a nanowire-b…
We show that a temporal soliton can induce resonant radiation by three-wave mixing nonlinearities. This constitutes a new class of resonant radiation whose spectral positions are parametrically tunable. The experimental verification is done in a periodically poled lithium niobate crystal, where a femtosecond near-IR soliton is excited and resonant radiation waves are observed exactly at the calculated soliton phase-matching wavelengths via the sum- and difference-frequency generation nonlinearities. This extends the supercontinuum bandwidth well into the mid-IR to span 550-5000 nm and the mid-…
We report three-well, resonant-phonon depopulation terahertz quantum cascade lasers with semi-insulating surface-plasmon waveguides and reduced active region (AR) thicknesses. Devices with thicknesses of 10, 7.5, 6, and 5 μm are compared in terms of threshold current density, maximum operating temperature, output power and AR temperature. Thinner ARs are technologically less demanding for epitaxial growth and result in reduced electrical heating of devices. However, it is found that 7.5-μm-thick devices give the lowest electrical power densities at threshold, as they represent the optimal trad…
Pure solitons are for the first time distilled from the resonant continuous wave (CW) background in a fiber laser by utilizing nonlinear Fourier transform (NFT). It is identified that the soliton and the resonant CW background have different eigenvalue distributions in the nonlinear frequency domain. Similar to water distillation, we propose the approach of soliton distillation, by making NFT on a steady pulse generated from a fiber laser, then filtering out the eigenvalues of the resonant CW background in the nonlinear frequency domain, and finally recovering the soliton by inverse NFT (INFT)…
We present two complementary models to study stationary nonlinear solutions in one-dimensional plasmonic slot waveguides made of a finite-thickness nonlinear dielectric core surrounded by metal regions. The considered nonlinearity is of focusing Kerr type. In the first model, it is assumed that the nonlinear term depends only on the transverse component of the electric field and that the nonlinear refractive index change is small compared to the linear part of the refractive index. This first model allows us to describe analytically the field profiles in the whole waveguide using Jacobi ellipt…
Plasmonic metasurfaces represent a promising platform for enhancing light-matter interaction. Active control of the optical response of metasurfaces is desirable for applications such as beam-steering, modulators and switches, biochemical sensors, and compact optoelectronic devices. Here we use a plasmonic metasurface with two Fano resonances to enhance the interaction of infrared light with electrically controllable single layer graphene. It is experimentally shown that the narrow spectral width of these resonances, combined with strong light/graphene coupling, enables reflectivity modulation…
We address formation of stable dissipative surface solitons in the exciton-polariton condensate in one-dimensional array of microcavity pillars under the action of localized resonant pump acting in the edge resonator. We show that localization degree and peak amplitudes of surface solitons can be effectively controlled by the pump frequency and that the allowed energy gap of periodic structure determines the energy range, where surface solitons can form. One observes bistability at sufficiently large pump amplitudes and nonlinearity-induced shift of the position of resonance peak from the allo…
We propose that a weakly-coupled nonlinear dielectric waveguide -- surface-plasmon system can be formulated as a new type of Josephson junction. Such a system can be realized along a metal - dielectric interface where the dielectric medium hosts a nonlinear waveguide (e.g. fiber) for soliton propagation. We demonstrate that the system is in close analogy to the bosonic Josephson-Junction (BJJ) of atomic condensates at very low temperatures, yet exhibits different dynamical features. In particular, the inherently dynamic coupling parameter between soliton and surface-plasmon generates self-trap…
Nanomaterials capable of confining light are desirable for enhancing spectroscopies such as Raman scattering, infrared absorption, and nonlinear optical processes. Plasmonic superlattices have shown the ability to host collective resonances in the mid-infrared, but require stringent fabrication processes to create well-ordered structures. Here, we demonstrate how short-range-ordered Au nanoparticle multilayers on a mirror, self-assembled by a sub-nm molecular spacer, support collective plasmon-polariton resonances in the visible and infrared, continuously tunable beyond 11 $μ$m by simply varyi…
Spatio-temporal dynamics of singly resonant optical parametric oscillators with external seeding displays hexagonal, roll and honeycomb patterns, optical turbulence, rogue waves and cavity solitons. We derive appropriate mean-field equations with a sinc$^2$ nonlinearity and demonstrate that off-resonance seeding is necessary and responsible for the formation of complex spatial structures via self-organization. We compare this model with those derived close to the threshold of signal generation and find that back-conversion of signal and idler photons is responsible for multiple regions of spat…
Peculiar ring gap modes on the surface of disk close to the metallic thin film are excited in the visible light regime. We apply plasmon hybridization method to illustrate the ring gap modes arising from the interaction between localized disk plasmons and continuum surface plasmons, which cannot be easily excited by the plane wave with polarization parallel to the film interface. In the coupled system, the hybrid modes energy and the surface charge distribution of nanoparticle are investigated both in simulation and hybridization method, showing consistence with each other. The excitation of r…
