We propose a probe based on nuclear relaxation and Knight shift measurements for the Kondo scenario for the "0.7 feature" in semiconductor quantum point contact (QPC) devices. We show that the presence of a bound electron in the QPC would lead to a much higher rate of nuclear relaxation compared to nuclear relaxation through exchange of spin with conduction electrons. Furthermore, we show that the temperature dependence of this nuclear relaxation is very non-monotonic as opposed to the linear-T relaxation from coupling with conduction electrons. We present a qualitative analysis for the additional relaxation due to nuclear spin diffusion (NSD) and study the extent to which NSD affects the range of validity of our method. The conclusion is that nuclear relaxation, in combination with Knight shift measurements, can be used to verify whether the 0.7 feature is indeed due to the presence of a bound electron in the QPC.
We study nuclear relaxation in the presence of localized electrons in a two-dimensional electron gas in a disordered delta-doped semiconductor heterostructure and show that this method can reliably probe their magnetic interactions and possible long-range order. In contrast, we argue that transport measurements, the commonly employed tool, may not sometimes distinguish between spatial disorder and long-range order. We illustrate the utility of using the nuclear relaxation method to detect long-range order by analyzing a recent proposal made on the basis of transport measurements, on the sponta…
Atomic contacts made of ferromagnetic metals present zero-bias anomalies in the differential conductance due to the Kondo effect. These systems provide a unique opportunity to perform a statistical analysis of the Kondo parameters in nanostructures since a large number of contacts can be easily fabricated using break-junction techniques. The details of the atomic structure differ from one contact to another so a large number of different configurations can be statistically analyzed. Here we present such a statistical analysis of the Kondo effect in atomic contacts made from the ferromagnetic t…
It is demonstrated theoretically that the circularly polarized irradiation of two-dimensional electron systems can induce the localized electron states which antiferromagnetically interact with conduction electrons, resulting in the Kondo effect. Conditions of experimental observation of the effect are discussed for semiconductor quantum wells.
Decoherence of the Kondo Singlet via a Quantum Point Contact Detector
研究了电容耦合量子点接触探测器对量子点晶体管近藤单态电荷测量的影响。通过对量子点单重态基态的变分分析，结合耦合系统的密度矩阵公式，我们证明了量子点接触处的透射/反射系数的相敏探测和幅敏探测都破坏了相干Kondo单重态.我们认为，退相干率的相位敏感分量可以解释Avinun-Kalish { \em et al.}（Phys. Rev. Lett. { \bf 92}，156801（2004））。我们还讨论了量子点接触探测器的散粒噪声和量子点的退相干的相关性。
Spin exchange between a single-electron charged quantum dot and itinerant electrons leads to an emergence of Kondo correlations. When the quantum dot is driven resonantly by weak laser light, the resulting emission spectrum allows for a direct probe of these correlations. In the opposite limit of vanishing exchange interaction and strong laser drive, the quantum dot exhibits coherent oscillations between the single-spin and optically excited states. Here, we show that the interplay between strong exchange and non-perturbative laser coupling leads to the formation of a new nonequilibrium quantu…
We use a low-temperature scanning tunneling microscope to study the interplay between the Kondo effect of a single-atom contact and a spin current. To this end, a nickel tip is coated by a thick layer of copper and brought into contact with a single Co atom adsorbed on a Cu(100) surface. We show that upon contact the Kondo resonance of Co is spin split and attribute the splitting to the spin current produced by the nickel tip and flowing across the copper spacer. A quantitative line shape analysis indicates that the spin polarization of the junction amounts up to 18%, but decreases when a pris…
Iron, cobalt and nickel are archetypal ferromagnetic metals. In bulk, electronic conduction in these materials takes place mainly through the $s$ and $p$ electrons, whereas the magnetic moments are mostly in the narrow $d$-electron bands, where they tend to align. This general picture may change at the nanoscale because electrons at the surfaces of materials experience interactions that differ from those in the bulk. Here we show direct evidence for such changes: electronic transport in atomic-scale contacts of pure ferromagnets (iron, cobalt and nickel), despite their strong bulk ferromagneti…
A low-temperature scanning tunneling microscope was employed to study the differential conductance in an atomic junction formed by an adsorbed Co atom on a Cu(100) surface and a copper-covered tip. A zero-bias anomaly (ZBA) reveals spin scattering off the Co atom, which is assigned to a Kondo effect. The ZBA exhibits a characteristic asymmetric lineshape when electrons tunnel between tip and sample, while upon the tip-Co contact it symmetrizes and broadens. Through density functional theory calculations and the non-equilibrium non-crossing approximation we show that the lineshape broadening is…
Quantum point contacts exhibit mysterious conductance anomalies in addition to well known conductance plateaus at multiples of 2e^2/h. These 0.7 and zero-bias anomalies have been intensively studied, but their microscopic origin in terms of many-body effects is still highly debated. Here we use the charged tip of a scanning gate microscope to tune in situ the electrostatic potential of the point contact. While sweeping the tip distance, we observe repetitive splittings of the zero-bias anomaly, correlated with simultaneous appearances of the 0.7 anomaly. We interpret this behaviour in terms of…
We analyze the full counting statistics (FCS) of quantum dots in the Kondo regime contacted by normal and superconducting leads or an STM tip. To describe the Kondo resonance we use an effective model for the quantum dot in the Kondo regime in combination with the FCS for tunneling contacts calculated using the Hamiltonian approach. We show that the situation of weak coupling to the superconducting electrode in the case of superconductor gap being larger than the Kondo resonance width can be easily handled and verify the method by comparing our theoretical predictions to experimental data. Thi…
We investigate the effects induced by spin polarization in the contacts attached to a serial double quantum dot. The polarization generates effective magnetic fields and suppresses the Kondo effect in each dot. The super-exchange interaction ($J_{\mathrm{AFM}}$), tuned by the inter-dot tunnelling rate $t$, can be used to compensate the effective fields and restore the Kondo resonance when the contact polarizations are aligned. As a consequence, the direction of the spin conductance can be controlled and even reversed using electrostatic gates alone. Furthermore, we study the associated two-imp…
The size-effect of Kondo-scattering in nanometer-sized metallic point contacts is measured with the simplified, mechanically-controlled break-junction technique for CuMn alloy of different Mn concentrations: 0.017; 0.035; and 0.18 ($\pm$0.017) at.\%. The results are compared with our previous publication on nominally 0.1 at.\% CuMn alloy \cite{1,2}. The increase of width of the Kondo resonance and enhanced ratio of Kondo-peak intensity to electron-phonon scattering intensity is observed for contacts with sizes smaller than 10 $nm$. From the comparison of electron-phonon scattering intensity fo…
Emergence of a symmetry-broken Chern insulator near a moiré Kondo breakdown
Shanghai Jiao Tong University（上海交通大学）；Cornell University（康奈尔大学）；Kavli Institute at Cornell for Nanoscale Science（康奈尔纳米科学卡弗里研究所）；Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；Tsung-Dao Lee Institute, Shanghai Jiao Tong University（上海交通大学李政道研究所）；National Institute for Materials Science（国立材料研究所）；Hefei National Laboratory（合肥国家实验室）；Max Planck Institute for the Structure and Dynamics of Matter（马克斯·普朗克物质结构动力学研究所）
The nonlinear conductance observed in a quantum point contact is theoretically reproduced for the entire range of applied bias. The single-impurity Anderson model with two reservoirs at different chemical potentials is studied for a sequential change of the gate voltage. The imbalance in the left and right Kondo coupling strength is introduced by the displacement of the Kondo impurity by the electric field produced in the constriction of quantum point contact. We reveal the origin of the side peaks and study the behavior of the height and width of the zero-bias anomaly.
The Kondo effect is the many-body screening of a local spin by a cloud of electrons at very low temperature. It has been proposed as an explanation of the zero-bias anomaly in quantum point contacts where interactions drive a spontaneous charge localization. However, the Kondo origin of this anomaly remains under debate, and additional experimental evidence is necessary. Here we report on the first phase-sensitive measurement of the zero-bias anomaly in quantum point contacts using a scanning gate microscope to create an electronic interferometer. We observe an abrupt shift of the interference…
We consider effects of magnetic field on the thermopower and thermoconductance of a single-electron transistor based on a quantum dot strongly coupled to one of the leads by a single-mode quantum point contact. We show appearance of two new energy scales: T_{min} ~ |r|^2 E_C(B/B_C)^2 depending on a ratio of magnetic field B and the field B_C corresponding to a full polarization of point contact and T_{max} ~ |r|^2 E_C depending on a reflection amplitude r and charging energy E_C. We predict that the behavior of thermoelectric coefficients is consistent with the Fermi-liquid theory at temperatu…
The current $I$ through nickelocene molecules and its noise are measured with a low temperature scanning tunneling microscope on a Cu(100) substrate. Density functional theory calculations and many-body modeling are used to analyze the data. During contact formation, two types of current evolution are observed, an abrupt jump to contact and a smooth transition. These data along with conductance spectra ($dI/dV$) recorded deep in the contact range are interpreted in terms of a transition from a spin-1 to a spin-1/2 state that is Kondo screened. Many-body calculations show that the smooth transi…
We theoretically study the nonequilibrium thermoelectric transport properties of a strongly-correlated molecule (or quantum dot) embedded in a tunnel junction. Assuming that the coupling of the molecule to the contacts is asymmetric, we determine the nonlinear current driven by the voltage and temperature gradients by using the perturbation theory. However, the subsystem consisting of the molecule strongly coupled to one of the contacts is solved by using the numerical renormalization group method, which allows for accurate description of Kondo correlations. We study the temperature gradient a…
Linear conductance below $2e^2/h$ shows resonance peaks in highly asymmetric quantum point contacts (QPCs). As the channel length increases, the number of peaks also increases. At the same time, differential conductance exhibits zero bias anomalies (ZBAs) in correspondence with every other peak in the linear conductance. This even odd effect, observable in the longer channels, is consistent with the formation of quasi-localized states within the QPC. In rare cases, triple peaks are observed, indicating the formation of a spin one Kondo effect when the electron filling number is even. Changing …
Kondo physics in nonequilibrium interacting nanoscale devices is an attractive fundamental many-particle phenomenon with a rich potential for applications. Due to enormous complexity its clear and flexible theory is still highly desirable. We develop a physically transparent analytical theory capable to correctly describe the Kondo effect in strongly interacting systems at temperatures close to and above the Kondo temperature. We derive a nonequilibrium Keldysh field theory valid for a system with any finite electron-electron interaction which is much stronger than the coupling of the system t…
Scaling laws and universality are often associated with systems exhibiting emergent phenomena possessing a characteristic energy scale. We report nonequilibrium transport measurements on two different types of single-molecule transistor (SMT) devices in the Kondo regime. The conductance at low bias and temperature adheres to a scaling function characterized by two parameters. This result, analogous to that reported recently in semiconductor dots with Kondo temperatures two orders of magnitude lower, demonstrates the universality of this scaling form. We compare the extracted values of the scal…
The nonlinear conductance of semiconductor heterostructures and single molecule devices exhibiting Kondo physics has recently attracted attention. We address the observed sample dependence of the measured steady state transport coefficients by considering additional electronic contributions in the effective low-energy model underlying these experiments that are absent in particle-hole symmetric setups. A novel version of the superperturbation theory of Hafermann et al. in terms of dual fermions is developed, which correctly captures the low-temperature behavior. We compare our results with the…
We elaborate on the recently introduced concept of reentrant Kondo effect in quantum impurities/dots coupled to hybrid metal-semiconductor contacts [G.~Diniz {\em et al.}, Phys. Rev. B {\bf 101}, 125115 (2020)]. By noticing the equivalence of the originally suggested semiconducting arrangement to an analogous three-terminal quantum dot setup with a normal and two phase-biased superconducting leads introduced in our recent work [Phys. Rev. B {\bf 103}, 035419 (2021)], we put this effect into a new physical context, which enables us a fresh look on the problem. First, we identify the superconduc…
In this Letter we investigate the properties of a quantum impurity model in the presence of additional many-body interactions between mobile carriers. The fundamental question which is addressed here is how the interactions in the charge and spin sectors of an itinerant system affect the quantum impurity physics in the vicinity of the intermediate coupling fixed point. To illustrate the general answer to this question we discuss a two-channel charge Kondo circuit model. We show that the electron-electron interactions resulting in the formation of a massive spin mode in an itinerant electron su…
The Kondo effect of a Co atom on Cu(100) was investigated with a low-temperature scanning tunneling microscope using a monoatomically sharp nickel tip. Upon a tip-Co contact, the differential conductance spectra exhibit a spin-split asymmetric Kondo resonance. The computed ab initio value of the exchange coupling is too small to suppress the Kondo effect, but sufficiently large to produce the splitting observed. A quantitative analysis of the line shape using the numerical renormalization group technique indicates that the junction spin polarization is weak.
We consider electromechanical properties of a single-electronic device consisting of movable quantum dot attached to a vibrating cantilever, forming a tunnel contact with a non-movable source electrode. We show that the resonance Kondo tunneling of electrons amplify exponentially the strength of nanoelectromechanical (NEM) coupling in such device and makes the latter to be insensitive to mesoscopic fluctuations of electronic levels in a nano-dot. It is also shown that the study of Kondo-NEM phenomenon provides an additional (as compared with a standard conductance measurements in a non-mechani…
We investigate the effect of contact geometry on the instantaneous thermoelectric response of a quantum dot pushed suddenly into the Kondo regime via a gate voltage using time dependent non-crossing approximation and linear response Onsager relations. We utilize graphene and metal contacts for this purpose. Instantaneous thermopower displays sinusoidal oscillations whose frequency is proportional to the energy separation between the van Hove singularity in the contact density of states and Fermi level for both cases regardless of the asymmetry factor at the onset of Kondo timescale. The amplit…
We study the conductance of an electron interferometer formed in a two dimensional electron gas between a nanostructured quantum contact and the charged tip of a scanning gate microscope. Measuring the conductance as a function of the tip position, thermally induced rings may be observed in addition to Fabry-Pérot interference fringes spaced by half the Fermi wavelength. If the contact is made of a quantum dot opened in the middle of a Kondo valley, we show how the location of the rings allows to measure by electron interferometry the magnetic moment of the dot above the Kondo temperature.
The impact of semiconductor surface roughness on the electrical and thermal contact resistances and thermoEMF of thermoelectric material (TEM)-metal transient contact layer is studied theoretically. The distribution of hollows and humps on the rough surface is simulated by the truncated Gaussian distribution. The impact of distribution parameters on the electrical contact resistance and thermoEMF of thermoelectric material-metal contact is studied.
We have investigated break junctions of normal non-magnetic metals as well as ferromagnets at low temperatures. The point contacts with radii 0.15 - 15 nm showed zero-bias anomalies which can be attributed to Kondo scattering at a single Kondo impurity at the contact or to the switching of a single conducting channel. The Kondo temperatures derived from the width of the anomalies varied between 10 and 1000 K. These results agree well with literature data on atomic-size contacts of the ferromagnets as well as with spear-anvil type contacts on a wide variety of metals.
The method of microcontact spectroscopy is used to study alloys with magnetic impurities CuMn and CuFe in the range of concentrations 0.01-1 at.%. Minima or maxima (so-called zero-bias anomalies) were observed in the microcontact spectra of these alloys at voltages ~ 1 mV. The Lande g-factor for the Mn impurity in a Cu matrix was determined from the splitting of the minimum of the zero-bias anomaly in a magnetic field. The quantitative calculations carried out agree well with theory and permit determining both the important geometric contact parameter <K> i.e., the averaged geometric form fact…
A multiscale simulation approach is developed to simulate the contact transport properties between semimetal to a monolayer two-dimensional (2D) transition metal dichalcogenide (TMDC) semiconductor. The results elucidate the mechanisms for low contact resistance between semimetal and TMDC semiconductor contacts from a quantum transport perspective. The simulation results compare favorably with recent experiments. Furthermore, the results show that the contact resistance of a Bismuth-MoS2 contact can be further reduced by engineering the dielectric environment and doping the TMDC material to <1…
