We study electronic transport through a magnetic molecule with an intrinsic spin $S$ coupled to two magnetic electrodes, in the incoherent regime. The molecule is modeled as a single resonant level with large Coulomb repulsion (no double occupancy). The molecular spin is isotropic and it interacts with the electronic spin through an exchange interaction. Using an alternative method to the usual master equation approach, we are able to obtain analytical formulas for various physical quantities of interest, such as the mean current and the current fluctuations, but also the mean value of $J_z$ -the $z$ component of the total spin on the molecule- and its fluctuations. This allows us to understand how the electronic current between the magnetized electrodes can control the polarization of the molecular spin. We observe in particular that the fluctuations of $J_z$ reach unexpectedly high values.
Magnetic resonance and microwave resistance modulation in van der Waals colossal-magnetoresistance material
Institute for Solid State Physics, The University of Tokyo(东京大学固体物理研究所);Department of Physics and Astronomy, The University of Manchester(曼彻斯特大学物理与天文学系)
Colossal Magnetoresistance and Phonon Driven Exchange Dynamics in Eu$_5$Sn$_2$As$_6$
University of Tokyo(东京大学);University of California, Berkeley(加州大学伯克利分校);Lawrence Berkeley National Laboratory(劳伦斯伯克利国家实验室);National High Magnetic Field Laboratory, Los Alamos National Laboratory(洛斯阿拉莫斯国家实验室国家高磁场实验室);Molecular Foundry, Lawrence Berkeley National Laboratory(劳伦斯伯克利国家实验室分子发现中心);Physikalisch-Technische Bundesanstalt(德国物理技术联邦研究院)