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arXiv 2101.07595cond-mat.mes-hallcond-mat.mtrl-scicond-mat.str-el
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阶梯状单层石墨烯的室温巨磁电阻效应

Room-temperature colossal magnetoresistance in terraced single-layer graphene

J. X. Hu, J. Gou, M. Yang, G. J. Omar, J. Y. Tan, S. W. Zeng, Y. P. Liu, K. Han, Z. S. Lim, Z. Huang, A. T. S. Wee, A. Ariando

摘要:

无序感生磁电阻效应在低垂直磁场下是二次的,在高垂直磁场下是线性的。这种效应在技术上很有吸引力,特别是在二维(2D)材料如石墨烯中,因为它在具有纳米级空间分辨率的磁传感器中提供了潜在的应用。然而,这是一个很大的挑战,实现基于这种效应的石墨烯磁传感器,因为在控制的空间分布的无序和提高MR灵敏度在单层制度的困难。在这里,我们报告了一个高达5,000%的室温巨大MR在9 T的梯形单层石墨烯。通过层压单层石墨烯的阶梯衬底上,如TiO 2终止SrTiO 3,我们证明了一个普遍的一个数量级的增强MR相比,传统的单层石墨烯设备。引人注目的是,即使在约1012 cm-2的高载流子密度下,在阶梯石墨烯中也实现了>1,000%的巨大MR。对单层石墨烯在各种氧化物和非氧化物基阶梯表面上的MR的系统研究表明,阶梯结构是驱动MR增强的主导因素。我们的研究结果开辟了一条新的路线,定制的二维材料的物理性能的工程应变通过一个梯田基板。

英文摘要:

Disorder-induced magnetoresistance (MR) effect is quadratic at low perpendicular magnetic fields and linear at high fields. This effect is technologically appealing, especially in the two-dimensional (2D) materials such as graphene, since it offers potential applications in magnetic sensors with nanoscale spatial resolution. However, it is a great challenge to realize a graphene magnetic sensor based on this effect because of the difficulty in controlling the spatial distribution of disorder and enhancing the MR sensitivity in the single-layer regime. Here, we report a room-temperature colossal MR of up to 5,000% at 9 T in terraced single-layer graphene. By laminating single-layer graphene on a terraced substrate, such as TiO2 terminated SrTiO3, we demonstrate a universal one order of magnitude enhancement in the MR compared to conventional single-layer graphene devices. Strikingly, a colossal MR of >1,000% was also achieved in the terraced graphene even at a high carrier density of ~1012 cm-2. Systematic studies of the MR of single-layer graphene on various oxide- and non-oxide-based terraced surfaces demonstrate that the terraced structure is the dominant factor driving the MR enhancement. Our results open a new route for tailoring the physical property of 2D materials by engineering the strain through a terraced substrate.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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