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arXiv 0704.0902cond-mat.str-el
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金属VO2中绝缘相的有效能带结构与强动力学关联

Effective band-structure in the insulating phase versus strong dynamical correlations in metallic VO2

Jan M. Tomczak, Ferdi Aryasetiawan, Silke Biermann

摘要:

使用一般的分析连续计划集群动力学平均场计算,我们分析了实频自能,动量分辨谱函数,和单粒子激发的金属和绝缘相的VO2。虽然前者的动力学相关性和寿命效应阻止了准粒子的描述,后者的激发允许一个有效的能带结构。我们构建了一个依赖于轨道的,但静态的单粒子势,再现了完整的多体光谱。然而,基态远远超出了静态的单粒子描述。这幅新出现的图像对绝缘体的性质这一长达十年之久的问题给出了一个重要的答案,我们将其描述为“多体佩尔斯”状态。

英文摘要:

Using a general analytical continuation scheme for cluster dynamical mean field calculations, we analyze real-frequency self-energies, momentum-resolved spectral functions, and one-particle excitations of the metallic and insulating phases of VO2. While for the former dynamical correlations and lifetime effects prevent a description in terms of quasi-particles, the excitations of the latter allow for an effective band-structure. We construct an orbital-dependent, but static one-particle potential that reproduces the full many-body spectrum. Yet, the ground state is well beyond a static one-particle description. The emerging picture gives a non-trivial answer to the decade-old question of the nature of the insulator, which we characterize as a ``many-body Peierls'' state.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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