We discuss a simple scheme for preparing atoms and molecules in an arbitrary preselected coherent superposition of quantum states. The technique, which we call fractional stimulated Raman adiabatic passage ({\it f-STIRAP}), is based upon (incomplete) adiabatic population transfer between an initial state $ψ_1$ and state $ψ_3$ through an intermediate state $ψ_2$. As in STIRAP, the Stokes pulse arrives before the pump pulse, but unlike STIRAP, the two pulses terminate simultaneously while maintaining a constant ratio of amplitudes. The independence of f-STIRAP from details of pulse shape and pulse area makes it the analog of conventional STIRAP in the creation of coherent superpositions of states. We suggest a smooth realization of f-STIRAP which requires only two laser pulses (which can be derived from a single laser) and at the same time ensures the automatic fulfillment of the asymptotic conditions at early and late times. Furthermore, we provide simple analytic estimates of the robustness of f-STIRAP against variations in the pulse intensity, the pulse delay, and the intermediate-state detuning, and discuss its possible extension to multistate systems.
Schemes for creation of N particle entangled Greenberger-Horne-Zeilinger (GHZ) states are important for understanding multi-particle non-classical correlations. Here, a theoretical scheme for creation of a multi-particle GHZ state implemented on a target ensemble of N, $Λ$ three-level Rydberg atoms and a single Rydberg atom as a control using Stimulated Raman Adiabatic Passage (STIRAP) is presented. We work in the Rydberg blockade regime for the ensemble atoms induced due to excitation of the control atom to a high lying Rydberg level. It is shown that using STIRAP, atoms from one ground state…
We consider the problem of the implementation of Stimulated Raman Adiabatic Passage (STIRAP) processes in degenerate systems, with a view to be able to steer the system wave function from an arbitrary initial superposition to an arbitrary target superposition. We examine the case a $N$-level atomic system consisting of $ N-1$ ground states coupled to a common excited state by laser pulses. We analyze the general case of initial and final superpositions belonging to the same manifold of states, and we cover also the case in which they are non-orthogonal. We demonstrate that, for a given initial…
We experimentally demonstrate composite stimulated Raman adiabatic passage (CSTIRAP), which combines the concepts of composite pulse sequences and adiabatic passage. The technique is applied for population transfer in a rare-earth doped solid. We compare the performance of CSTIRAP with conventional single and repeated STIRAP, either in the resonant or the highly detuned regime. In the latter case, CSTIRAP improves the peak transfer efficiency and robustness, boosting the transfer efficiency substantially compared to repeated STIRAP. We also propose and demonstrate a universal version of CSTIRA…
Stimulated Raman adiabatic passage (STIRAP) describes adiabatic population transfer between two states coherently coupled via a mediating state that remains unoccupied. This renders STIRAP robust against loss in the mediating state, leading to profound applications in atomic- and molecular-beam research, trapped-ion physics, superconducting circuits, other solid-state systems, optics, in entanglement generation and qubit operations. STIRAP in optomechanics has been considered for optical frequency conversion where a mechanical mode provides the mediating state. Given the advances of optomechan…
We introduce and analyze theoretically a procedure that combines slow adiabatic STIRAP manipulation with short nonadiabatic Rabi pulses to produce any desired three-level state in a qutrit system. In this protocol, the fast pulses create superpositions between the ground state and the first excited state, while the slow pulses transfer an arbitrary population to the second excited state via stimulated Raman adiabatic passage (STIRAP). We demonstrate high-fidelity quantum control of the level populations and phases and we characterize the errors incurred under the breakdown of adiabaticity. In …
We suggest a way to produce higher-energy superposition states in a circular system of quantum wells. This is inspired by a link to convergence results for geometric transformations of polygons using circulant Hermitian matrices.
The evolution of a measured system and an experimental apparatus is presented in an unified form. Conditions under which the state of such a total system forms, evaluates and declines from a superposition of states are defined. The problem of definite outcomes in the quantum-mechanical measurement theory is considered.
We recently proposed a scheme for the creation of coherent superpositions of vortex states in Bose-Einstein condensates (BEC) using orbital angular momentum (OAM) states of light [Phys. Rev. Lett. 95, 173601 (2005)]. Here we discuss further technical details of the proposal, provide alternative, time-reversal-symmetric scheme for transfer of a superposition of OAM states of light to the BEC via a procedure analogous to the traditional STimulated Raman Adiabatic Passage (STIRAP) technique, and discuss an alternative trap configuration conducive for sustaining large charge vortices. Superpositio…
We present a method for the controlled and robust generation of spatial superposition states of single atoms in micro-traps. Using a counter-intuitive positioning sequence for the individual potentials and appropriately chosen trapping frequencies, we show that it is possible to selectively create two different orthogonal superposition states, which can in turn be used for quantum information purposes.
We propose and analyze a scheme for "on demand" creation of coherent superposition of meta-stable states in a tripod-structured atom using frequency-chirped laser pulses. Negligible excitation of the atoms during the creation of the superposition states is a priority in our consideration. The underlying physics of the scheme is explained using the formalism of adiabatic states. By numerically solving master equation for the density matrix operator, we analyze the influence of the spontaneous decay and transverse relaxation on the efficiency of the creation of superposition states. We show that…
We propose a novel protocol for the creation of macroscopic quantum superposition (MQS) states based on a measurement of a non-monotonous function of a quantum collective variable. The main advantage of this protocol is that it does not require switching on and off nonlinear interactions in the system. We predict this protocol to allow the creation of multiatom MQS by measuring the number of atoms coherently outcoupled from a two-component (spinor) Bose-Einstein condensate.
We consider how macroscopic quantum superpositions may be created from arrays of Bose-Einstein condensates. We study a system of three condensates in Fock states, all with the same number of atoms and show that this has the form of a highly entangled superposition of different quasi-momenta. We then show how, by partially releasing these condensates and detecting an interference pattern where they overlap, it is possible to create a macroscopic superposition of different relative phases for the remaining portions of the condensates. We discuss methods for confirming these superpositions.
We consider the creation of superpositions of macroscopically distinct states by a completely-positive (CP) operation on a subsystem. We conclude that the subsystem on which the CP operation acts must be macroscopically large if the success probability of the CP operation does not vanish in the thermodynamic limit. In order to obtain this conclusion, we show two inequalities each of which represents a trade-off relation among the magnitude of an indicator for superpositions of macroscopically distinct states, the success probability of a CP operation, and the volume of the subsystem on which t…
We present a straightforward scheme for creating macroscopic superpositions of different superfluid flow states of Bose-Einstein condensates trapped in optical lattices. This scheme has the great advantage that all the techniques required are achievable with current experiments. Furthermore, the relative difficulty of creating cats scales favorably with the size of the cat. This means that this scheme may be well-suited to creating superpositions involving large numbers of particles. Such states may have interesting technological applications such as making quantum-limited measurements of angu…
We propose a scheme for creating atomic coherent superpositions via stimulated Raman adiabatic passage in a Lambda-type system where the final state has twofold levels. In the employ of a control field, the presence of double dark states leads to two arbitrary coherent superposition states with equal amplitude but inverse relative phase without the condition of multi-photon resonance. In particular, two orthogonal maximal coherent superposition states are created when the control field is resonant with the transition of the twofold levels. This scheme can also be extended to manifold Lambda-ty…
The principle of superposition is a key ingredient for quantum mechanics. A recent work [M. Oszmaniec et al., Phys. Rev. Lett. 116, 110403 (2016)] has shown that a quantum adder that deterministically generates a superposition of two unknown states is forbidden. Here we propose a probabilistic approach for creating a superposition state of two arbitrary states encoded in two three-dimensional cavities. Our implementation is based on a three-level superconducting transmon qubit dispersively coupled to two cavities. Numerical simulations show that high-fidelity generation of the superposition of…
We consider an adiabatic population transfer process that resembles the well established stimulated Raman adiabatic passage (STIRAP). In our system, the states have nonzero angular momentums $J$, therefore, the coupling laser fields induce transitions among the magnetic sublevels of the states. In particular, we discuss the possibility of creating coherent superposition states in a system with coupling pattern $J=0\Leftrightarrow J=1$ and $J=1\Leftrightarrow J=2$. Initially, the system is in the J=0 state. We show that by two delayed, overlapping laser pulses it is possible to create any final…
We analyze single particle coherence and interference in the presence of particle loss and derive an inequality that relates the preservation of coherence, the creation of superposition with the vacuum, and the degree of particle loss. We find that loss channels constructed using linear optics form a special subclass. We suggests a generalized spectroscopy where, in analogy with the absorption spectrum, we measure a "coherence loss spectrum" and a "superposition creation spectrum". The theory is illustrated with examples.
As one of the most intriguing intrinsic properties of quantum world, quantum superposition provokes great interests in its own generation. Oszmaniec [Phys. Rev. Lett. 116, 110403 (2016)] have proven that though a universal quantum machine that creates superposition of arbitrary two unknown states is physically impossible, a probabilistic protocol exists in the case of two input states have nonzero overlaps with the referential state. Here we report a heralded quantum machine realizing superposition of arbitrary two unknown photonic qubits as long as they have nonzero overlaps with the horizont…
Nonlinear dynamics of establishment of electron-hole coherent superpositions states in graphene by multiphoton resonant excitation of interband transitions in laser fields is considered. The single-particle time dependent density matrix for such a quantized system is calculated in the multiphoton resonant approximation. The dependence of Rabi oscillations of Fermi-Dirac sea in graphene on the time, momentum, and photon number at multiphoton laser-excitation is analyzed.
The superposition principle is one of the landmarks of quantum mechanics. The importance of quantum superpositions provokes questions about the limitations that quantum mechanics itself imposes on the possibility of their generation. In this work we systematically study the problem of creation of superpositions of unknown quantum states. First, we prove a no-go theorem that forbids the existence of a universal probabilistic quantum protocol producing a superposition of two unknown quantum states. Secondly, we provide an explicit probabilistic protocol generating a superposition of two unknown …
This work investigates the effect of phonon coupling on the transfer of population and creation of coherence using variant of stimulated Raman adiabatic passage (STIRAP) known as \emph{fractional} stimulated Raman adiabatic passage (FSTIRAP). The study is based on the Liouville equation, which is solved numerically in the adiabatic limit. Although the phonon is assumed to be coupled only to the intermediate state, it is coupled to the other two states by dipolar system-environment interaction, inducing phonon coupling to the other states which are not directly in contact with the phonon. At ze…
Adiabatic techniques using multi-level systems have recently been generalised from the optical case to settings in atom optics, solid state and even classical electrodynamics. The most well known example of these is the so called STIRAP process, which allows transfer of a particle between different states with large fidelity. Here we generalise and examine this process for an atomic centre-of-mass state with a non-trivial phase distribution and show that even though dark state dynamics can be achieved for the atomic density, the phase dynamics will still have to be considered as a dynamical pr…
We study a coherent superposition of field annihilation and creation operator acting on continuous variable systems and propose its application for quantum state engineering. Specifically, it is investigated how the superposed operation transforms a classical state to a nonclassical one, together with emerging nonclassical effects. We also propose an experimental scheme to implement this elementary coherent operation and discuss its usefulness to produce an arbitrary superposition of number states involving up to two photons.
We consider the simultaneous propagation of a pair of Raman-resonant, frequency-modulated (chirped) laser pulses in an optically thick medium, modeled by an ensemble of $Λ$-atoms. A self-organization ('matching`) effect is shown for the chirped pulse pair, which leads to a quasi-lossless propagation. Furthermore, we demonstrate that a well-defined coherent superposition of the atomic ground states and, correspondingly, a coherence is robustly created in the medium that can be controlled by amplitudes of the laser pulses. The proposed scheme can be applied to substantially increase the efficien…
Mesoscopic quantum superpositions, or Schrödinger cat states, are widely studied for fundamental investigations of quantum measurement and decoherence as well as applications in sensing and quantum information science. The generation and maintenance of such states relies upon a balance between efficient external coherent control of the system and sufficient isolation from the environment. Here we create a variety of cat states of a single trapped atom's motion in a harmonic oscillator using ultrafast laser pulses. These pulses produce high fidelity impulsive forces that separate the atom into …
We propose an experimental scheme to generate, in a heralded fashion, arbitrary quantum superpositions of two-mode optical states with a fixed total photon number $n$ based on weakly squeezed two-mode squeezed state resources (obtained via weak parametric down conversion), linear optics, and photon detection. Arbitrary $d$-level (qudit) states can be created this way where $d=n+1$. Furthermore, we experimentally demonstrate our scheme for $n=2$. The resulting qutrit states are characterized via optical homodyne tomography. We also discuss possible extensions to more than two modes concluding t…
We investigate a Landau-Zener (LZ) transition process modeled by a quantum two-level system (TLS) coupled to a photon mode when the bias energy is varied linearly in time. The initial state of the photon field is assumed to be a superposition of coherent states, leading to a more intricate LZ transition. Applying the rotating-wave approximation (RWA), analytical results are obtained revealing the enhancement of the LZ probability by increasing the average photon number. We also consider the creation of entanglement and the change of photon statistics during the LZ process. Without the RWA, we …
We provide a scheme for the generation of entangled number states of Bose-Einstein condensates in multiple wells with cyclic pairwise connectivity. The condensate ground state in a multiple well trap can self-evolve, when phase engineered with specific initial phase differences between the neighboring wells, to a macroscopic superposition state with controllable entanglement -- to multiple well generalization of double well NOON states. We demonstrate through numerical simulations the creation of entangled states in three and four wells and then explore the creation of "larger" entangled state…
We study two ions confined in a Penning trap. We show that electronically highly excited states exist in which an electron is delocalized among the two ions forming a giant molecule of several micrometer size. At energies close to the top of the Coulomb barrier these molecular states can be regarded as superpositions of Rydberg states of individual ions. We illuminate the possibility to observe coherent charge transfer between the ions. Beyond a critical principal quantum number the electron can coherently tunnel through the Coulomb barrier to an adjacent doubly charged ion. The tunneling occu…
A procedure is discussed for creating coherent superpositions of motional states of ion strings. The motional states are across the structural transition linear-zigzag, and their coherent superposition is achieved by means of spin-dependent forces, such that a coherent superposition of the electronic states of one ion evolves into an entangled state between the chain's internal and external degrees of freedom. It is shown that the creation of such an entangled state can be revealed by performing Ramsey interferometry with one ion of the chain.
We show a surprising link between experimental setups to realize high-dimensional multipartite quantum states and Graph Theory. In these setups, the paths of photons are identified such that the photon-source information is never created. We find that each of these setups corresponds to an undirected graph, and every undirected graph corresponds to an experimental setup. Every term in the emerging quantum superposition corresponds to a perfect matching in the graph. Calculating the final quantum state is in the complexity class #P-complete, thus cannot be done efficiently. To strengthen the li…
We propose a fast and efficient technique to create classes of highly entangled states of trapped ions, such as arbitrary Dicke states and superpositions of them, e.g. NOON states. The ions are initialized in the phonon ground state and are addressed globally with a composite pulse that is resonant with the first motional sideband. The technique operates on comparatively short time scales, as resonant interactions allow one to use the minimum laser pulse area. The number of single pulses from the composite sequence is equal to the number of ions, thus the implementation complexity grows only l…
NOON states (states of the form $|N>_{a}|0>_{b}+|0>_{a}|N>_{b}$ where $a$ and $b$ are single particle states) have been used for predicting violations of hidden-variable theories (Greenberger-Horne-Zeilinger violations) and are valuable in metrology for precision measurements of phase at the Heisenberg limit. We show theoretically how the use of two Fock state/Bose-Einstein condensates as sources in a modified Mach Zender interferometer can lead to the creation of the NOON state in which $a$ and $b$ refer to arms of the interferometer and $N$ is the total number of particles in the two condens…
Quantum state manipulation with gates based on geometric phases acquired during cyclic operations promises inherent fault-tolerance and resilience to local fluctuations in the control parameters. Here we create a general non-Abelian and non-adiabatic holonomic gate acting in the $(\ket{0},\ket{2})$ subspace of a three-level transmon fabricated in a fully coplanar design. Experimentally, this is realized by simultaneously coupling the first two transitions by microwave pulses with amplitudes and phases defined such that the condition of parallel transport is fulfilled. We demonstrate the creati…
An interferometric scheme for the creation of momentum superposition states of mechanical oscillators, using a quantum mirror kicked by free photons is analyzed. The scheme features ultra-fast preparation with immediate detection and should allow for the observation of signatures of momentum superpositions in a massive macroscopic system at non-zero temperatures. It is robust against thermalized initial states, displacement and movement, mirror imperfections, and the measurements' back-actions.
Recently, intensely driven laser-matter interactions have been used to connect the fields of strong laser field physics with quantum optics by generating non-classical states of light. Here, we make a further key step and show the potential of strong laser fields for generating controllable high-photon-number coherent-state superpositions. This has been achieved by using two of the most prominent strong-laser induced processes: high-harmonic generation and above-threshold ionization. We show how the obtained coherent-state superpositions change from an optical Schrödinger "cat" state to a "kit…
We propose a method to create "spin cat states", i.e. macroscopic superpositions of coherent spin states, in Bose-Einstein condensates using the Kerr nonlinearity due to atomic collisions. Based on a detailed study of atom loss, we conclude that cat sizes of hundreds of atoms should be realistic. The existence of the spin cat states can be demonstrated by optical readout. Our analysis also includes the effects of higher-order nonlinearities, atom number fluctuations, and limited readout efficiency.
We study the quantum dynamics of a symmetric nanomechanical graphene resonator with degenerate flexural modes. Applying voltage pulses to two back gates, flexural vibrations of the membrane can be selectively actuated and manipulated. For graphene, nonlinear response becomes important already for amplitudes comparable to the magnitude of zero point fluctuations. We show, using analytical and numerical methods, that this allows for creation of cat-like superpositions of coherent states as well as superpositions of coherent cat-like non-product states.
Promising access to high-speed quantum networks relies on the creation of high-dimensional entangled memories that provide quantum communication with higher capacity of noisy quantum channels, thereby reducing the transmission time of information. Yet, the distribution of multidimensional entanglement between remote memory nodes is still faintly investigated. We propose an experimentally feasible protocol of deterministic generation of high-dimensional entanglement between distant multi-level atoms confined in high-finesse optical cavities and driven by laser pulses. Three-dimensional entangle…
We explore the possibility to entangle an excitonic two-level system in a semiconductor quantum dot (QD) with a cavity defined on a photonic crystal by sweeping the cavity frequency across its resonance with the exciton transition. The dynamic cavity detuning is established by a radio frequency surface acoustic wave (SAW). It induces Landau-Zener (LZ) transitions between the excitonic and the photonic degrees of freedom and thereby creates a superposition state. We optimize this scheme by using tailored Fourier-synthesized SAW pulses with up to five harmonics. The theoretical study is performe…
The spontaneous creation and persistence of ground-state coherence in an ensemble of intracavity Rb atoms has been observed as a quantum beat. Our system realizes a quantum eraser, where the detection of a first photon prepares a superposition of ground-state Zeeman sublevels, while detection of a second erases the stored information. Beats appear in the time-delayed photon-photon coincidence rate (intensity correlation function). We study the beats theoretically and experimentally as a function of system parameters, and find them remarkably robust against perturbations such as spontaneous emi…
In the presence of conservation laws, superpositions of eigenstates of the corresponding conserved quantities cannot be generated by quantum dynamics. Thus, any such coherence represents a potentially valuable resource of asymmetry, which can be used, for example, to enhance the precision of quantum metrology or to enable state transitions in quantum thermodynamics. Here we ask if such superpositions, already present in a reference system, can be broadcast to other systems, thereby distributing asymmetry indefinitely at the expense of creating correlations. We prove a no-go theorem showing tha…
States in quantum field theory (QFT) are represented by many-particle wave functions, such that a state describing n particles depends on n spacetime positions. Since a general state is a superposition of states with different numbers of particles, the wave function lives in the configuration space identified with a product of an infinite number of 4-dimensional Minkowski spacetimes. The squared absolute value of the wave function is interpreted as the probability density in the configuration space, from which the standard probabilistic predictions of QFT can be recovered. Such a formulation a…
Non-local mass superpositions and optical clock interferometry in atomic ensemble quantum networks
University of Innsbruck（因斯布鲁克大学）；Institute for Quantum Optics and Quantum Information of the Austrian Academy of Sciences（奥地利科学院量子光学和量子信息研究所）；Leibniz Universität Hannover（汉诺威莱布尼茨大学）；JILA, NIST and Department of Physics, University of Colorado（科罗拉多大学JILA、美国国家标准与技术研究院及物理系）；Center for Theory of Quantum Matter, University of Colorado（科罗拉多大学量子物质理论中心）
We report on the creation, observation and optimization of superposition states of cold atoms. In our experiments, rubidium atoms are prepared in a magneto-optical trap and later, after switching off the trapping fields, Faraday rotation of a weak probe beam is used to characterize atomic states prepared by application of appropriate light pulses and external magnetic fields. We discuss the signatures of polarization and alignment of atomic spin states and identify main factors responsible for deterioration of the atomic number and their coherence and present means for their optimization, like…
