The problem of quantizing the radiation field inside a nonlinear dielectric is studied. Based on the quantization of radiation in a linear dielectric which includes absorption and dispersion, we extend the theory in order to treat also nonlinear optical processes. We derive propagation equations in space and time for the quantized radiation field including the effects of linear absorption and dispersion as well as nonlinear optical effects. As a special case we derive the propagation equation of a narrow-frequency band light pulse in a Kerr medium.
Canonical quantization of electromagnetic field inside the time--spatially dispersive inhomogeneous dielectrics is presented. Interacting electromagnetic and matter excitation fields create the closed system, Hamiltonian of which may be diagonalized by generalized polariton transformation. Resulting dispersion relations coincide with the classical ones obtained by the solution of wave equation, the corresponding mode decomposition is, however, orthogonal and complete in the enlarged Hilbert space.
The quantization of the electromagnetic field in a three-dimensional inhomogeneous dielectric medium with losses is carried out in the framework of a damped-polariton model with an arbitrary spatial dependence of its parameters. The equations of motion for the canonical variables are solved explicitly by means of Laplace transformations for both positive and negative time. The dielectric susceptibility and the quantum noise-current density are identified in terms of the dynamical variables and parameters of the model. The operators that diagonalize the Hamiltonian are found as linear combinati…
By modeling a dielectric medium with two independent reservoirs, i.e., electric and magnetic reservoirs, the electromagnetic field is quantized in a linear dielectric medium consistently. A Hamiltonian is proposed from which using the Heisenberg equations, not only the Maxwell equations but also the structural equations can be obtained. Using the Laplace transformation, the wave equation for the electromagnetic vector potential is solved in the case of a homogeneous dielectric medium. Some examples are considered showing the applicability of the model to both absorptive and nonabsorptive diele…
We present a Gupta-Bleuler quantization scheme for the electromagnetic field in time-dependent dielectric media. Starting from the Maxwell equations, a generalization of the Lorentz gauge condition adapted to time varying dielectrics is derived. Using this gauge, a Gupta-Bleuler approach to quantize all polarizations of the radiation field and the corresponding constraint condition are introduced. This new approach is different from the quantized electromagnetic field in vacuum in the sense that here the contributions of unphysical photons cannot be thoroughly eliminated, which further lead to…
A quantum damped-polariton model is constructed for an inhomogeneous anisotropic linear dielectric with arbitrary dispersion in space and time. The model Hamiltonian is completely diagonalized by determining the creation and annihilation operators for the fundamental polariton modes as specific linear combinations of the basic dynamical variables. Explicit expressions are derived for the time-dependent operators describing the electromagnetic field, the dielectric polarization and the noise term in the latter. It is shown how to identify bath variables that generate the dissipative dynamics of…
Recently two methods have been developed for the quantization of the electromagnetic field in general dispersing and absorbing linear dielectrics. The first is based upon the introduction of a quantum Langevin current in Maxwell's equations [T. Gruner and D.-G. Welsch, Phys. Rev. A 53, 1818 (1996); Ho Trung Dung, L. Knöll, and D.-G. Welsch, Phys. Rev. A 57, 3931 (1998); S. Scheel, L. Knöll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)], whereas the second makes use of a set of auxiliary fields, followed by a canonical quantization procedure [A. Tip, Phys. Rev. A 57, 4818 (1998)]. We show that…
A quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive and absorbing dielectric medium is developed. The classical Maxwell equations with spatially varying and Kramers-Kronig consistent permittivity are regarded as operator-valued field equations, introducing additional current- and charge-density operator fields in order to take into account the noise associated with the dissipation in the medium. It is shown that the equal-time commutation relations between the fundamental electromagnetic fields $\hat …
An ad hoc quantization scheme for the electromagnetic field in a weakly dispersive, transparent dielectric leads to the definition of canonical and kinetic forms for the momentum of the electromagnetic field in a dispersive medium. The canonical momentum is uniquely defined as the operator that generates spatial translations in a uniform medium, but the quantization scheme suggests two possible choices for the kinetic momentum operator, corresponding to the Abraham or the Minkowski momentum in classical electrodynamics. Another implication of this procedure is that a wave packet containing a s…
It has very recently been suggested that asymmetric coupling of electromagnetic fields to thermal reservoirs under nonequilibrium conditions can produce unexpected oscillatory behavior in the local photon statistics in layered structures. Better understanding of the predicted phenomena could enable useful applications related to thermometry, noise filtering, and enhancing optical interactions. In this work we briefly review the field quantization and study the local steady state temperature distributions in optical cavities formed of lossless and lossy media to show that also local field tempe…
Starting from a Lagrangian, the electromagnetic field is quantized in the presence of a body rotating along its axis of symmetry. Response functions and fluctuation-dissipation relations are obtained. A general formula for rotational friction and power radiated by a rotating dielectric body is obtained in terms of the dyadic Green's tensor. Hamiltonian is determined and possible generalizations are discussed. As an example, the rotational friction and power radiated by a spherical dielectric in the vicinity of a semi-infinite dielectric plane is obtained and discussed in some limiting cases.
We show that in the presence of free charge carriers the definition of the frequency-dependent dielectric permittivity requires additional regularization. As an example, the dielectric permittivity of the Drude model is considered and its time-dependent counterpart is derived and analyzed. The respective electric displacement cannot be represented in terms of the standard Fourier integral. The regularization procedure allowing to circumvent these difficulties is suggested. For purpose of comparison it is shown that the frequency-dependent dielectric permittivity of insulators satisfies all rig…
By a generalization of the Hopfield model, we construct a microscopic Lagrangian describing a dielectric medium with dispersion and dissipation. This facilitates a well-defined and unambiguous $\textit{ab initio}$ treatment of quantum electrodynamics in such media, even in time-dependent backgrounds. As an example, we calculate the number of photons created by switching on and off dissipation in dependence on the temporal switching function. This effect may be stronger than quantum radiation produced by variations of the refractive index $Δn(t)$ since the latter are typically very small and yi…
There are several possible applications of quantum electrodynamics in dielectric media which require a quantum description for the electromagnetic field interacting with matter fields. The associated quantum models can refer to macroscopic electromagnetic fields or, in alternative, to mesoscopic fields (polarization fields) describing an effective interaction between electromagnetic field and matter fields. We adopt the latter approach, and focus on the Hopfield model for the electromagnetic field in a dielectric dispersive medium in a framework in which space-time dependent mesoscopic paramet…
In this paper we will present a quantization method for SPP (Surface Plasmon Polariton) based on Green's tensor method, which is applied usually for quantization of EM-field in various dielectric media. This method will be applied for a semi-infinite structure, which contains metal and dielectric regions with one interface. Moreover, by introducing the quantized SPP, we will investigate the SPP propagation in the attenuating and amplifying systems. We will also consider two modes of SPP, i.e., coherent and squeezed states, and finally compare the propagation of these modes in the amplifying me…
We study the Casimir pressure for a dielectric-diamagnetic cylinder subject to light velocity conservation and with a dispersion law analogous to Sellmeir's rule. Similarities to and differences from the spherical case are pointed out.
The electromagnetic field is canonically quantized in the presence of a linear, dispersive and dissipative medium that is in uniform motion. Specifically we calculate the change in the normal modes of the coupled matter-field system and find a Hamiltonian that contains negative energy normal modes. We interpret these modes as the origin of phenomena such as quantum friction, and find that a detector initially in its ground state and coupled to the electromagnetic field in the vicinity of, or within a uniformly moving medium has a non-zero probability of excitation at T=0K.
We study the Brownian motion of a charged test particle driven by quantum electromagnetic fluctuations in the vacuum region near a non-dispersive and non-absorbing dielectric half-space and calculate the mean squared fluctuations in the velocity of the test particle. Our results show that a nonzero susceptibility of the dielectrics has its imprints on the velocity dispersions of the test particles. The most noteworthy feature in sharp contrast to the case of an idealized perfectly conducting interface is that the velocity dispersions in the parallel directions are no longer negative and does n…
Recently a quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive, and absorbing dielectric medium has been developed and applied to a system consisting of two infinite half-spaces with a common planar interface (H.T. Dung, L. Knoell, and D.-G. Welsch, Phys. Rev. A 57, in press). Here we show that the scheme, which is based on the classical Green-tensor integral representation of the electromagnetic field, applies to any inhomogeneous medium. For this purpose we prove that the fundamental equal-time commut…
Modeling a nonlinear anisotropic magnetodielectric medium with spatial-temporal dispersion by two continuum collections of three dimensional harmonic oscillators, a fully canonical quantization of the electromagnetic field is demonstrated in the presence of such a medium. Some coupling tensors of various ranks are introduced that couple the magnetodielectric medium with the electromagnetic field. The polarization and magnetization fields of the medium are defined in terms of the coupling tensors and the oscillators modeling the medium. The electric and magnetic susceptibility tensors of the me…
As a quantum analog of Cherenkov radiation, an inertial photon detector moving through a medium with constant refractive index $n$ may perceive the electromagnetic quantum fluctuations as real photons if its velocity $v$ exceeds the medium speed of light $c/n$. For dispersive Hopfield type media, we find this Ginzburg effect to extend to much lower $v$ because the phase velocity of light is very small near the medium resonance. In this regime, however, dissipation effects become important. Via an extended Hopfield model, we present a consistent treatment of quantum fluctuations in dispersive a…
By modeling a linear polarizable and magnetizable medium (magneto-dielectric) with two quantum fields, namely E and M, electromagnetic field is quantized in such a medium consistently and systematically. A Hamiltonian is proposed from which, using the Heisenberg equations, Maxwell and constitutive equations of the medium are obtained. For a homogeneous medium, the equation of motion of the quantum vector potential, $\vec{A}$, is derived and solved analytically. Two coupling functions which describe the electromagnetic properties of the medium are introduced. Four examples are considered showin…
Electromagnetic field quantization in the presence of two semi-infinite dielectrics with moving interface is investigated in $1+1$-dimensional space-time. The moving interface is modeled for small displacements and the field equation is solved perturbatively. Input-output relations and spectral distribution of emitted photons are obtained and the effect of small transitions trough the interface discussed.
Modeling an anisotropic spatially and temporarily dispersive magnetodielectric medium by two independent collections of three dimensional vector fields, we demonstrate a fully canonical quantization of electromagnetic field in the presence of such a medium. Two tensor fields which couple the electromagnetic field with the medium and have an important role in this quantization method are introduced. The electric and magnetic polarization fields of the medium naturally are concluded in terms of the coupling tensors and the dynamical variables modeling the magnetodielectric medium. In Heisenberg …
By modeling a linear, anisotropic and inhomogeneous magnetodielectric medium with two independent set of harmonic oscillators, electromagnetic field is quantized in such a medium. The electric and magnetic polarizations of the medium are expressed as linear combinations of the ladder operators describing the magnetodielectric medium. The Maxwell and the constitutive equations of the medium are obtained as the Heisenberg equations of the total system. The electric and magnetic susceptibilities of the medium are obtained in terms of the tensors coupling the medium with the electromagnetic field.…
The universal analytic expressions in the limit of low temperatures (short separations) are obtained for the free energy, entropy and pressure between the two parallel plates made of any dielectric. The analytical proof of the Nernst heat theorem in the case of dispersion forces acting between dielectrics is provided. This permitted us to formulate the stringent thermodynamical requirement that must be satisfied in all models used in the Casimir physics.
A recently developed technique for the system--and--bath quantization of open optical cavities is applied to three resonator geometries: A one dimensional dielectric, a Fabry--Perot resonator, and a dielectric disk. The system--and--bath Hamiltonian for these geometries is derived starting from Maxwell's equations and employed to compute the electromagnetic fields, the resonances, and the cavity gain factors. Exact agreement is found with standard quantization methods based on a modes--of--the--universe description. Our analysis provides a microscopic justification for the system--and--bath qu…
The Hamiltonian of a polariton model for an inhomogeneous linear absorptive dielectric is diagonalized by means of Fano's diagonalization method. The creation and annihilation operators for the independent normal modes are explicitly found as linear combinations of the canonical operators. The coefficients in these combinations depend on the tensorial Green function that governs the propagation of electromagnetic waves through the dielectric. The time-dependent electromagnetic fields in the Heisenberg picture are given in terms of the diagonalizing operators. These results justify the phenomen…
Quantization of Polaritons Confined in Dielectric Structures
Institute of Physics Polish Academy of Sciences（波兰科学院物理研究所）；Center for Theoretical Physics, Polish Academy of Sciences（波兰科学院理论物理中心）；Institute of Physics, Lodz University of Technology（罗兹理工大学物理研究所）；Institute of Experimental Physics, Faculty of Physics, University of Warsaw（华沙大学物理学院实验物理研究所）
On the basis of general theoretical results developed previously in JETP 112, 246 (2011) we analyze the atomic polarization created by weak monochromatic light in an optically thick, dense and cold atomic ensemble. We show that the amplitude of the polarization averaged over a uniform random atomic distribution decreases exponentially beyond the boundary regions. The phase of this polarization increases linearly with increasing penetration into the medium. On these grounds, we determine numerically the wavelength of the light in the dense atomic medium, its extinction coefficient, and the comp…
A simple approach is proposed for the quantization of the electromagnetic field in nonlinear and inhomogeneous media. Given the dielectric function and nonlinear susceptibilities, the Hamiltonian of the electromagnetic field is determined completely by this quantization method. From Heisenberg's equations we derive Maxwell's equations for the field operators. When the nonlinearity goes to zero, this quantization method returns to the generalized canonical quantization procedure for linear inhomogeneous media [Phys. Rev. A, 43, 467, 1991]. The explicit Hamiltonians for the second-order and thir…
Boundary-dependent radiative corrections that modify the magnetic moment of an electron near a dielectric or conducting surface are investigated. Normal-mode quantization of the electromagnetic field and perturbation theory applied to the Dirac equation for a charged particle in a weak magnetic field yields a general formula for the magnetic moment correction in terms of any choice of electromagnetic mode functions. For two particular models, a non-dispersive dielectric and an undamped plasma, it is shown that, by using contour integration techniques over a complex wave vector, this can be sim…
The quantization of plasmons has been analyzed mostly under the assumption of an infinite-sized bulk medium interacting with the electromagnetic field. We reformulate it for finite-size media, such as metallic or dielectric nano-structures, highlighting sharp differences. By diagonalizing the Hamiltonian by means of a Lippmann-Schwinger equation, we show the contribution of two sets of bosonic operators, one stemming from medium fluctuations, and one from the electromagnetic field. The results apply to general models including dissipative and dispersive responses.
We study the quantum properties of the electromagnetic field in optical cavities coupled to an arbitrary number of escape channels. We consider both inhomogeneous dielectric resonators with a scalar dielectric constant $ε({\bf r})$ and cavities defined by mirrors of arbitrary shape. Using the Feshbach projector technique we quantize the field in terms of a set of resonator and bath modes. We rigorously show that the field Hamiltonian reduces to the system--and--bath Hamiltonian of quantum optics. The field dynamics is investigated using the input--output theory of Gardiner and Collet. In the c…
Using the Green function approach to the problem of quantization of the phenomenological Maxwell theory, the propagation of quantized radiation through dispersive and absorptive multilayer dielectric plates is studied. Input--output relations are derived, with special emphasis on the determination of the quantum noise generators associated with the absorption of radiation inside the dielectric matter. The input--output relations are used to express arbitrary correlation functions of the outgoing field in terms of correlation functions of the incoming field and those of the noise generators. To…
The dispersion interaction between two point-like particles confined in a dielectric slab between two plates of another dielectric medium is studied within a continuum (Lifshitz) theory. The retarded (Casimir-Polder) interaction at large inter-particle distances is found to be strongly enhanced as the mismatch between the dielectric permittivities of the two media is increased. The large-distance interaction is multiplied due to confinement by a factor of $(33γ^{5/2}+13γ^{-3/2})/46$ at zero temperature, and by $(5γ^2+γ^{-2})/6$ at finite temperature, $γ=\ein(0)/\eout(0)$ being the ratio betwee…
We present a Lagrangian-Hamiltonian formalism of a moving dielectric sphere interacting with radiation fields. By including the interaction up to the first order in the speed of the sphere, we derive the Hamiltonian and perform quantization of both the field and the mechanical motion of the sphere. In particular, we show how independent degrees of freedom can be consistently identified under the generalized radiation gauge via instantaneous mode projection. Our Hamiltonian indicates the form of coupling due to velocity-dependent interactions beyond adiabatic approximation. In addition, the Ham…
We investigate the dispersion relations of TE resonances in different graphene-dielectric structures. Previous work has shown that when a graphene layer is brought into contact with a dielectric material, a gap can appear in its electric band structure. This allows for the formation of TE-plasmons with unusual dispersion relations. In addition, if the dielectric has a finite thickness, graphene strongly modifies the behavior of the waveguiding modes by introducing dissipation above a well-defined cutoff frequency thus providing the possibility of mode filtering. This cutoff and the properties …
This article is provides an introduction to the quantum theory of optics in nonlinear dielectric media. We begin with a short summary of the classical theory of nonlinear optics, that is nonlinear optics done with classical fields. We then discuss the canonical formalism for fields and its quantization. This is applied to quantizing the electromagnetic field in free space. The definition of a nonclassical state of the electromagnetic field is presented, and several examples are examined. This is followed by a brief introduction to entanglement in the context of field modes. The next task is th…
We present a canonical quantization of macroscopic electrodynamics. The results apply to inhomogeneous media with a broad class of linear magneto-electric responses which are consistent with the Kramers-Kronig and Onsager relations. Through its ability to accommodate strong dispersion and loss, our theory provides a rigorous foundation for the study of quantum optical processes in structures incorporating metamaterials, provided these may be modeled as magneto-electric media. Previous canonical treatments of dielectric and magneto-dielectric media have expressed the electromagnetic field opera…
The quantization of optical fields in vacuum has been known for decades, but extending the field quantization to lossy and dispersive media in nonequilibrium conditions has proven to be complicated due to the position-dependent electric and magnetic responses of the media. In fact, consistent position-dependent quantum models for the photon number in resonant structures have only been formulated very recently and only for dielectric media. Here we present a general position-dependent quantized fluctuational electrodynamics (QFED) formalism that extends the consistent field quantization to desc…
Fast, large area patterning of arbitrary structures down to the nanometre scale is of great interest for a range of applications including the semiconductor industry, quantum electronics, nanophotonics and others. It was recently proposed that nanometre-resolution mask lithography can be realised by sending metastable helium atoms through a binary holography mask consisting of a pattern of holes. However, these first calculations were done using a simple scalar wave approach, which did not consider the dispersion force interaction between the atoms and the mask material. To access the true pot…
Despite suggestions to the contrary, we show in this paper that the usual dispersive form of the electromagnetic energy must be used to derive the Lifshitz force between parallel dielectric media. This conclusion follows from the general form of the quantum vacuum energy, which is the basis of the multiple-scattering formalism. As an illustration, we explicitly derive the Lifshitz formula for the interaction between parallel dielectric semispaces, including dispersion, starting from the expression for the total energy of the system. The issues of constancy of the energy between parallel plates…
We have recently developed a position-dependent quantization scheme for describing the ladder and effective photon-number operators associated with the electric field to analyze quantum optical energy transfer in lossy and dispersive dielectrics [Phys. Rev. A, 89, 033831 (2014)]. While having a simple connection to the thermal balance of the system, these operators only described the electric field and its coupling to lossy dielectric bodies. Here we extend this field quantization scheme to include the magnetic field and thus to enable description of the total electromagnetic field and discuss…
Dispersion forces such as van der Waals forces between two microscopic particles, the Casimir--Polder forces between a particle and a macroscopic object or the Casimir force between two dielectric objects are well studied in vacuum. However, in realistic situations the interacting objects are often embedded in an environmental medium. Such a solvent influences the induced dipole interaction. With the framework of macroscopic quantum electrodynamics, these interactions are mediated via an exchange of virtual photons. Via this method the impact of a homogeneous solvent medium can be expressed as…
