By modeling a dielectric medium with two independent reservoirs, i.e., electric and magnetic reservoirs, the electromagnetic field is quantized in a linear dielectric medium consistently. A Hamiltonian is proposed from which using the Heisenberg equations, not only the Maxwell equations but also the structural equations can be obtained. Using the Laplace transformation, the wave equation for the electromagnetic vector potential is solved in the case of a homogeneous dielectric medium. Some examples are considered showing the applicability of the model to both absorptive and nonabsorptive dielectrics.
Canonical quantization of electromagnetic field inside the time--spatially dispersive inhomogeneous dielectrics is presented. Interacting electromagnetic and matter excitation fields create the closed system, Hamiltonian of which may be diagonalized by generalized polariton transformation. Resulting dispersion relations coincide with the classical ones obtained by the solution of wave equation, the corresponding mode decomposition is, however, orthogonal and complete in the enlarged Hilbert space.
The quantization of the electromagnetic field in a three-dimensional inhomogeneous dielectric medium with losses is carried out in the framework of a damped-polariton model with an arbitrary spatial dependence of its parameters. The equations of motion for the canonical variables are solved explicitly by means of Laplace transformations for both positive and negative time. The dielectric susceptibility and the quantum noise-current density are identified in terms of the dynamical variables and parameters of the model. The operators that diagonalize the Hamiltonian are found as linear combinati…
The problem of quantizing the radiation field inside a nonlinear dielectric is studied. Based on the quantization of radiation in a linear dielectric which includes absorption and dispersion, we extend the theory in order to treat also nonlinear optical processes. We derive propagation equations in space and time for the quantized radiation field including the effects of linear absorption and dispersion as well as nonlinear optical effects. As a special case we derive the propagation equation of a narrow-frequency band light pulse in a Kerr medium.
We present a Gupta-Bleuler quantization scheme for the electromagnetic field in time-dependent dielectric media. Starting from the Maxwell equations, a generalization of the Lorentz gauge condition adapted to time varying dielectrics is derived. Using this gauge, a Gupta-Bleuler approach to quantize all polarizations of the radiation field and the corresponding constraint condition are introduced. This new approach is different from the quantized electromagnetic field in vacuum in the sense that here the contributions of unphysical photons cannot be thoroughly eliminated, which further lead to…
A quantum damped-polariton model is constructed for an inhomogeneous anisotropic linear dielectric with arbitrary dispersion in space and time. The model Hamiltonian is completely diagonalized by determining the creation and annihilation operators for the fundamental polariton modes as specific linear combinations of the basic dynamical variables. Explicit expressions are derived for the time-dependent operators describing the electromagnetic field, the dielectric polarization and the noise term in the latter. It is shown how to identify bath variables that generate the dissipative dynamics of…
Recently two methods have been developed for the quantization of the electromagnetic field in general dispersing and absorbing linear dielectrics. The first is based upon the introduction of a quantum Langevin current in Maxwell's equations [T. Gruner and D.-G. Welsch, Phys. Rev. A 53, 1818 (1996); Ho Trung Dung, L. Knöll, and D.-G. Welsch, Phys. Rev. A 57, 3931 (1998); S. Scheel, L. Knöll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)], whereas the second makes use of a set of auxiliary fields, followed by a canonical quantization procedure [A. Tip, Phys. Rev. A 57, 4818 (1998)]. We show that…
A quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive and absorbing dielectric medium is developed. The classical Maxwell equations with spatially varying and Kramers-Kronig consistent permittivity are regarded as operator-valued field equations, introducing additional current- and charge-density operator fields in order to take into account the noise associated with the dissipation in the medium. It is shown that the equal-time commutation relations between the fundamental electromagnetic fields $\hat …
A new mathematical and computational technique for calculating quantum vacuum expectation values of energy and momentum densities associated with electromagnetic fields in bounded domains containing inhomogeneous media is discussed. This technique is illustrated by calculating the mode contributions to the difference in the vacuum force expectation between opposite ends of an inhomogeneous dielectric non-dispersive medium confined to a perfectly conducting rigid box.
An ad hoc quantization scheme for the electromagnetic field in a weakly dispersive, transparent dielectric leads to the definition of canonical and kinetic forms for the momentum of the electromagnetic field in a dispersive medium. The canonical momentum is uniquely defined as the operator that generates spatial translations in a uniform medium, but the quantization scheme suggests two possible choices for the kinetic momentum operator, corresponding to the Abraham or the Minkowski momentum in classical electrodynamics. Another implication of this procedure is that a wave packet containing a s…
It has very recently been suggested that asymmetric coupling of electromagnetic fields to thermal reservoirs under nonequilibrium conditions can produce unexpected oscillatory behavior in the local photon statistics in layered structures. Better understanding of the predicted phenomena could enable useful applications related to thermometry, noise filtering, and enhancing optical interactions. In this work we briefly review the field quantization and study the local steady state temperature distributions in optical cavities formed of lossless and lossy media to show that also local field tempe…
The quantization of the electromagnetic field in vacuum is presented without reference to lagrangean quantum field theory. The equal time commutators of the fields are calculated from basic principles. A physical discussion of the commutators suggest that the electromagnetic fields are macroscopic emergent properties of more fundamental physical system: the photons.
A simple approach is proposed for the quantization of the electromagnetic field in nonlinear and inhomogeneous media. Given the dielectric function and nonlinear susceptibilities, the Hamiltonian of the electromagnetic field is determined completely by this quantization method. From Heisenberg's equations we derive Maxwell's equations for the field operators. When the nonlinearity goes to zero, this quantization method returns to the generalized canonical quantization procedure for linear inhomogeneous media [Phys. Rev. A, 43, 467, 1991]. The explicit Hamiltonians for the second-order and thir…
On the example of stationary states of a system consisting of an atom and a quantized electromagnetic field (the Jaynes-Cummings model in free space), it is shown that the physical characteristics of the system (as the energy and the probability distribution of finding the center of mass of the atom) explicitly depend on the choice of the basis of quantization of the electromagnetic field. Therefore, the secondary quantization procedure is not independent of the choice of the quantization basis in the interaction of the field with the material medium.
Starting from a Lagrangian, the electromagnetic field is quantized in the presence of a body rotating along its axis of symmetry. Response functions and fluctuation-dissipation relations are obtained. A general formula for rotational friction and power radiated by a rotating dielectric body is obtained in terms of the dyadic Green's tensor. Hamiltonian is determined and possible generalizations are discussed. As an example, the rotational friction and power radiated by a spherical dielectric in the vicinity of a semi-infinite dielectric plane is obtained and discussed in some limiting cases.
The Hamiltonian of a polariton model for an inhomogeneous linear absorptive dielectric is diagonalized by means of Fano's diagonalization method. The creation and annihilation operators for the independent normal modes are explicitly found as linear combinations of the canonical operators. The coefficients in these combinations depend on the tensorial Green function that governs the propagation of electromagnetic waves through the dielectric. The time-dependent electromagnetic fields in the Heisenberg picture are given in terms of the diagonalizing operators. These results justify the phenomen…
Mathematical Foundation for Quantum Computing of Electromagnetic Wave Propagation in Dielectric Media
Plasma Science and Fusion Center Massachusetts Institute of Technology（麻省理工学院等离子体科学与聚变中心）；School of Electrical and Computer Engineering National Technical University of Athens（雅典国立技术大学电气与计算机工程学院）；Department of Physics College of William & Mary（威廉玛丽学院物理系）
We study the scattering of the quantized electromagnetic field from a linear, dispersive dielectric using the scattering formalism for quantum fields. The medium is modeled as a collection of harmonic oscillators with a number of distinct resonance frequencies. This model corresponds to the Sellmeir expansion, which is widely used to describe experimental data for real dispersive media. The integral equation for the interpolating field in terms of the in field is solved and the solution used to find the out field. The relation between the in and out creation and annihilation operators is found…
It has been found, that free electromagnetic (EM) field in restricted volume (typical experimental case) consists of two independent and equally possible components with different parity under spatial inversion transformations. Either of the two components indicated represents the system of also two independent and equally possible fields, which are even and uneven under time reversal transformations. The rules for local quantization of EM-field in Minkowski space are obtained.
We present a quantization procedure for the electromagnetic field in a circular cylindrical cavity with perfectly conducting walls, which is based on the decomposition of the field. A new decomposition procedure is proposed; all vector mode functions satisfying the boundary conditions are obtained with the help of this decomposition. After expanding the quantized field in terms of the vector mode functions, it is possible to derive the Hamiltonian for this quantized system.
It is currently believed that light quantum or the quantization of light energy is beyond classical physics and the picture of wave-particle duality, which was criticized by Einstein but attracted a number of experimental researches, is necessary for the description of light. We show in this paper, however, that the quantization of light energy in vacuum, which is the same as that in quantum electrodynamics, can be derived directly from the classical electromagnetic theory through the consideration of statistics based on classical physics. Therefore, the quantization of energy is an intrinsic …
By introducing a suitable Lagrangian, a canonical quantization of the electromagnetic field in the presence of a non-dispersive bi-anisotropic inhomogeneous magnetodielectric medium is investigated. A tensor projection operator is defined and the commutation relation between the vector potential and its canonically conjugate variable is written in terms of the projection operator. The quantization method is generalized in the presence of the atomic systems. The spontaneous emission of a two-level atom located in a non-dispersive anisotropic megnetodielectric medium is studied.
A bi-anisotropic magnetodielectric medium is modeled by two independent set of three dimensional harmonic oscillators .A fully canonical quantization of electromagnetic field is demonstrated in the presence of a bi-anisotropic magnetodielectric medium. The electric and magnetic polarization fields of the medium are obtained in terms of the dynamical variable modeling the medium. The Heisenberg equations of the system are solved for a multilayer bi-anisotropic magnetodielectric medium.
A canonical relativistic formulation is introduced to quantize electromagnetic field in the presence of a polarizable and magnetizable moving medium. The medium is modeled by a continuum of four vectors in a phenomenological way. The covariant wave equation for the vector potential and the covariant constitutive equation of the medium are obtained as the Euler- Lagrange equations using the Lagrangian of the total system. A tensor of the third rank which couples the electromagnetic field with the medium is introduced and the susceptibility tensor of the medium is obtained in terms of the coupli…
There are several possible applications of quantum electrodynamics in dielectric media which require a quantum description for the electromagnetic field interacting with matter fields. The associated quantum models can refer to macroscopic electromagnetic fields or, in alternative, to mesoscopic fields (polarization fields) describing an effective interaction between electromagnetic field and matter fields. We adopt the latter approach, and focus on the Hopfield model for the electromagnetic field in a dielectric dispersive medium in a framework in which space-time dependent mesoscopic paramet…
We consider an approach in which the usual wave function in the quadrature representation of mode j of the electromagnetic field is further quantized to produce a field operator. Since the electromagnetic field is already second quantized, this corresponds to an additional or third quantization. The third-quantization approach can be used to perform certain quantum optics calculations in the Heisenberg picture that could only be performed in the Schrodinger picture when using the conventional second-quantized theory. This approach also allows an interesting generalization of quantum optics and…
A general theory of the interaction of the quantized electromagnetic field with atoms in the presence of dispersing and absorbing dielectric bodies of given Kramers--Kronig consistent permittivities is developed. It is based on a source-quantity representation of the electromagnetic field, in which the electromagnetic-field operators are expressed in terms of a continuous set of fundamental bosonic fields via the Green tensor of the classical problem. Introducing scalar and vector potentials, the formalism is extended in order to include in the theory the interaction of the quantized electroma…
Very recently we present a theory [Wei-long She, Chin. Phys. 14, 2514(2005); Online: http://www.jop.org/journals/cp; http://arxiv.org/abs/quant-ph/0512097] to show that the quantization of light energy in vacuum can be derived directly from classical electromagnetic theory through the consideration of statistics based on classical physics and reveal that the quantization of energy is an intrinsic property of light as a classical electromagnetic wave and has no need of being related to particles. In this theory a key concept of stability of statistical distribution was involved. Here is a note …
In this paper we will present a quantization method for SPP (Surface Plasmon Polariton) based on Green's tensor method, which is applied usually for quantization of EM-field in various dielectric media. This method will be applied for a semi-infinite structure, which contains metal and dielectric regions with one interface. Moreover, by introducing the quantized SPP, we will investigate the SPP propagation in the attenuating and amplifying systems. We will also consider two modes of SPP, i.e., coherent and squeezed states, and finally compare the propagation of these modes in the amplifying me…
A gauge invariant quantization in a closed integral form is developed over a linear phase space endowed with an inhomogeneous Faraday electromagnetic tensor. An analog of the Groenewold product formula (corresponding to Weyl ordering) is obtained via a membrane magnetic area, and extended to the product of N symbols. The problem of ordering in quantization is related to different configurations of membranes: a choice of configuration determines a phase factor that fixes the ordering and controls a symplectic groupoid structure on the secondary phase space. A gauge invariant solution of the qua…
The eletromagnetic field in a linear absorptive dielectric medium, is quantized in the framework of the damped polarization model. A Hamiltonian containing a reservoir with continuous degrees of freedom, is proposed. The reservoir minimally interacts with the dielectric polarization and the electromagnetic field. The Lagevin-Schrodinger equation is obtained as the equation of motion of the polarization field. The radiation reaction electromagnetic field is considered. For a homogeneous medium, the equations of motion are solved using the Laplace transformation method.
Modeling an anisotropic spatially and temporarily dispersive magnetodielectric medium by two independent collections of three dimensional vector fields, we demonstrate a fully canonical quantization of electromagnetic field in the presence of such a medium. Two tensor fields which couple the electromagnetic field with the medium and have an important role in this quantization method are introduced. The electric and magnetic polarization fields of the medium naturally are concluded in terms of the coupling tensors and the dynamical variables modeling the magnetodielectric medium. In Heisenberg …
We present a quantization scheme for the electromagnetic field interacting with atomic systems in the presence of dispersing and absorbing magnetodielectric media, including left-handed material having negative real part of the refractive index. The theory is applied to the spontaneous decay of a two-level atom at the center of a spherical free-space cavity surrounded by magnetodielectric matter of overlapping band-gap zones. Results for both big and small cavities are presented, and the problem of local-field corrections within the real-cavity model is addressed.
Based on calculations involving an idealized boundary condition, it has long been assumed that the stress on a spherical conducting shell is repulsive. We use the more realistic case of a Drude dielectric to show that the stress is attractive, matching the generic behavior of Casimir forces in electromagnetism. We trace the discrepancy between these two cases to interactions between the electromagnetic quantum fluctuations and the dielectric material.
Analogous to Landau quantization related to a neutral particle possessing an electric quadrupole moment, we generalize such Landau quantization to include position-dependent mass (PDM) neutral particles. Using cylindrical coordinates, the exact solvability of PDM neutral particles with an electric quadrupole moment moving in electromagnetic fields is reported. The interaction between the electric quadrupole moment of a PDM neutral particle and a magnetic field in the absence of an electric field is analyzed for two different radial cylindrical PDM settings. Next, two particular cases of radial…
Modeling a nonlinear anisotropic magnetodielectric medium with spatial-temporal dispersion by two continuum collections of three dimensional harmonic oscillators, a fully canonical quantization of the electromagnetic field is demonstrated in the presence of such a medium. Some coupling tensors of various ranks are introduced that couple the magnetodielectric medium with the electromagnetic field. The polarization and magnetization fields of the medium are defined in terms of the coupling tensors and the oscillators modeling the medium. The electric and magnetic susceptibility tensors of the me…
By modeling a linear, anisotropic and inhomogeneous magnetodielectric medium with two independent set of harmonic oscillators, electromagnetic field is quantized in such a medium. The electric and magnetic polarizations of the medium are expressed as linear combinations of the ladder operators describing the magnetodielectric medium. The Maxwell and the constitutive equations of the medium are obtained as the Heisenberg equations of the total system. The electric and magnetic susceptibilities of the medium are obtained in terms of the tensors coupling the medium with the electromagnetic field.…
The electromagnetic field in an anisotropic and inhomogeneous magnetodielectric is quantized by modelling the medium with two independent quantum fields. Some coupling tensors coupling the electromagnetic field with the medium are introduced. Electric and magnetic polarizations are obtained in terms of the ladder operators of the medium and the coupling tensors explicitly. Using a minimal coupling scheme for electric and magnetic interactions, the Maxwell equations and the constitutive equations of the medium are obtained. The electric and magnetic susceptibility tensors of the medium are calc…
We derive expressions for the quantum electromagnetic field in a dispersive and dissipative dielectric medium, treating the medium as a continuum. We compare the Langevin approach with the Fano diagonalization procedure for the coupled system composed of the electromagnetic field, the dielectric medium, and the reservoir. In particular, we show that the quantized electric and magnetic fields obtained in both methods have exactly the same form. More generally, in thermal equilibrium, correlation functions computed in both methods are identical.
By modeling a linear polarizable and magnetizable medium (magneto-dielectric) with two quantum fields, namely E and M, electromagnetic field is quantized in such a medium consistently and systematically. A Hamiltonian is proposed from which, using the Heisenberg equations, Maxwell and constitutive equations of the medium are obtained. For a homogeneous medium, the equation of motion of the quantum vector potential, $\vec{A}$, is derived and solved analytically. Two coupling functions which describe the electromagnetic properties of the medium are introduced. Four examples are considered showin…
The derivation of Casimir forces between dielectrics can be simplified by ignoring absorption, calculating energy changes due to displacements of the dielectrics, and only then admitting absorption by allowing permittivities to be complex. As a first step towards a better understanding of this situation we consider in this paper the model of a dielectric as a collection of oscillators, each of which is coupled to a reservoir giving rise to damping and Langevin forces on the oscillators and a noise polarization acting as a source of a fluctuating electromagnetic (EM) field in the dielectric. Th…
The electromagnetic field is canonically quantized in the presence of a linear, dispersive and dissipative medium that is in uniform motion. Specifically we calculate the change in the normal modes of the coupled matter-field system and find a Hamiltonian that contains negative energy normal modes. We interpret these modes as the origin of phenomena such as quantum friction, and find that a detector initially in its ground state and coupled to the electromagnetic field in the vicinity of, or within a uniformly moving medium has a non-zero probability of excitation at T=0K.
Recently a quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive, and absorbing dielectric medium has been developed and applied to a system consisting of two infinite half-spaces with a common planar interface (H.T. Dung, L. Knoell, and D.-G. Welsch, Phys. Rev. A 57, in press). Here we show that the scheme, which is based on the classical Green-tensor integral representation of the electromagnetic field, applies to any inhomogeneous medium. For this purpose we prove that the fundamental equal-time commut…
Light in a dielectric medium moves slower than in vacuum. The corresponding electromagnetic field equations are then no longer invariant under ordinary Lorentz transformations, but only under such transformations corresponding to this reduced velocity. Based on this physical symmetry, an effective theory for low-energy electromagnetic phenomena in dielectrics is constructed. It has none of the problems of the old formulations of Minkowski and Abraham. Dispersion in the optical regime and the Kerr effect arise in a natural way from higher order interaction terms. The effective field theory is q…
We consider the electric and magnetic field fluctuations in the vacuum state in the region external to a half-space filled with a homogeneous non-dissipative dielectric. We discuss an appropriate limit to an ideal metal and concentrate our interest on the renormalized field fluctuations, or equivalently to renormalized electric and magnetic energy densities, in the proximity of the dielectric-vacuum interface. We show that surface divergences of field fluctuations arise at the interface in an appropriate ideal conductor limit, and that our limiting procedure allows to discuss in detail their s…
The stress tensor for the quantized electromagnetic field is calculated in the region between a pair of dispersive, dielectric half-spaces. This generalizes the stress tensor for the Casimir energy to the case where the boundaries have finite reflectivity. We also include the effects of finite temperature. This allows us to discuss the circumstances under which the weak energy condition and the null energy condition can be violated in the presence of finite reflectivity and finite temperature.
Electromagnetic Casimir stresses are of relevance to many technologies based on mesoscopic devices such as MEMS embedded in dielectric media, Casimir induced friction in nano-machinery, micro-fluidics and molecular electronics. Computation of such stresses based on cavity QED generally require numerical analysis based on a regularization process. A new scheme is described that has the potential for wide applicability to systems involving realistic inhomogeneous media. From a knowledge of the spectrum of the stationary modes of the electromagnetic field the scheme is illustrated by estimating n…
A general, exact formula is derived for the expectation value of the electromagnetic energy density of an inhomogeneous absorbing and dispersive dielectric medium in thermal equilibrium, assuming that the medium is well approximated as a continuum. From this formula we obtain the formal expression for the Casimir force density. Unlike most previous approaches to Casimir effects in which absorption is either ignored or admitted implicitly through the required analytic properties of the permittivity, we include dissipation explicitly via the coupling of each dipole oscillator of the medium to a …
Quantization of Polaritons Confined in Dielectric Structures
Institute of Physics Polish Academy of Sciences（波兰科学院物理研究所）；Center for Theoretical Physics, Polish Academy of Sciences（波兰科学院理论物理中心）；Institute of Physics, Lodz University of Technology（罗兹理工大学物理研究所）；Institute of Experimental Physics, Faculty of Physics, University of Warsaw（华沙大学物理学院实验物理研究所）
We determine the commutation relations satisfied by the quantized electromagnetic field in the presence of macroscopic dielectrics and conductors, with arbitrary dispersive and dissipative properties. We consider in detail the case of two plane-parallel material slabs, separated by an empty gap, and we show that at all points in the empty region between the slabs, including their surfaces, the electromagnetic fields always satisfy free-field canonical equal-time commutation relations. This result is a consequence of general analyticity and fall-off properties at large frequencies satisfied by …
Quantization of electromagnetic fields is investigated in the framework of stochastic variational method (SVM). Differently from the canonical quantization, this method does not require canonical form and quantization can be performed directly from the gauge invariant Lagrangian. The gauge condition is used to choose dynamically independent variables. We verify that, in the Coulomb gauge condition, SVM result is completely equivalent to the traditional result. On the other hand, in the Lorentz gauge condition, SVM quantization can be performed without introducing the indefinite metric. The tem…
In the framework of the canonical quantization of the electromagnetic field, we impose as primary condition on the dynamics the positive definiteness of the energy spectrum. This implies that (Glauber) coherent states have to be considered for the longitudinal and the scalar photon fields. As a result we obtain that the relation holds which in the traditional approach is called the Gupta-Bleuler condition. Gauge invariance emerges as a property of the physical states. The group structure of the theory is recognized to be the one of $SU(2) \otimes SU(1,1)$.
The microscopic theory of the Casimir effect in the dielectric is studied in the framework when absorption is realized via a reservoir modeled by a set of oscillators with continuously distributed frquencies with the aim to see if the effects depend on the form of interaction with the reservoir. A simple case of the one-dimensional dielectric between two metallic plates is considered. Two possible models are investigated, the direct interaction of the electromagnetic field with the reservoir and indirect interaction via an intermediate oscillator imitating the atom. It is found that with the s…
Quantum-statistical effects occur during the propagation of electromagnetic (EM) waves inside the dielectric media or metamaterials, which include a large class of nanophotonic and plasmonic waveguides with dissipation and noise. Exploiting the formal analogy between the Schrodinger equation and the Maxwell equations for dielectric linear media, we rigorously derive the effective Hamiltonian operator which describes such propagation. This operator turns out to be essentially non-Hermitian in general, and pseudo-Hermitian in some special cases. Using the density operator approach for general no…
We develop a framework that provides a few-mode master equation description of the interaction between a single quantum emitter and an arbitrary electromagnetic environment. The field quantization requires only the fitting of the spectral density, obtained through classical electromagnetic simulations, to a model system involving a small number of lossy and interacting modes. We illustrate the power and validity of our approach by describing the population and electric field dynamics in the spontaneous decay of an emitter placed in a complex hybrid plasmonic-photonic structure.
