We propose and demonstrate a method for measuring the spectral density matrix of a single photon pulse. The method is based on registering Hong-Ou-Mandel interference between photon to be measured and a pair of attenuated and suitably delayed laser pulses described by a known spectral amplitude. The density matrix is retrieved from a two-dimensional interferogram of coincidence counts. The method has been implemented for a type-I downconversion source, pumped by ultrashort laser pulses. The experimental results agree well with a theoretical model which takes into account the temporal as well as spatial effects in the source.
In a macroscopic realm, in which photons are too many for being counted by any photon counting detector, photon statistics can be measured by using detectors simply endowed with linear response. We insert one of such detectors in a conventional photon-counting apparatus, which returns a voltage every time the detector responds to light by generating a number of elementary charges via its primary photo-detection process. We only assume that, when a single charge is photo-generated, the probability density of the voltages is a distribution that is narrow with respect to its mean value. Under thi…
We have investigated the excitation-power dependence of polarization-entangled photon-pairs generated from a CuCl single crystal using biexciton resonant hyper-parametric scattering. The measured two-photon polarization density matrix which corresponds to the two-photon polarization state changes with increasing the excitation power. The evaluation of the tangle and the linear entropy obtained from the measured density matrix indicates that the two-photon polarization density matrix can be expressed as the mixed state of an ideal state and a totally mixed state, and the mixture ratio of the to…
The measurement of photon-number statistics of fields composed of photon pairs, generated in spontaneous parametric down-conversion and detected by an intensified CCD camera is described. Final quantum detection efficiencies, electronic noises, finite numbers of detector pixels, transverse intensity spatial profiles of the detected beams as well as losses of single photons from a pair are taken into account in a developed general theory of photon-number detection. The measured data provided by an iCCD camera with single-photon detection sensitivity are analyzed along the developed theory. Join…
We present the general structure of two-photon S matrix for a waveguide coupled to a local quantum system that supports multiple ground states. The presence of the multiple ground states results in a non-commutative aspect of the system with respect to the exchange of the orders of photons. Consequently, the two-photon S matrix significantly differs from the standard form as described by the cluster decomposition principle in the quantum field theory.
For one-mode and multimode light, the photon-number tomograms of Gaussian quantum states are explicitly calculated in terms of multivariable Hermite polynomials. Positivity of the tomograms is shown to be necessary condition for positivity of the density matrix.
We introduce an effective numerical method of density matrix determination of fiber coupled single photon generated in process of spontaneous parametric down conversion in type I non-collinear configuration. The presented theory has been successfully applied in case of source exploited in Phys. Rev. Lett. 99, 123601 (2007) to demonstrate the experimental characterization of spectral state of single photon.
One-photon and two-photon wavepackets of entangled two-photon states in spontaneous parametric down-conversion (SPDC) fields are calculated and measured experimentally. For type-II SPDC, measured one-photon and two-photon wavepackets agree well with theory. For type-I SPDC, the measured one-photon wavepacket agree with the theory. However, the two-photon wavepacket is much bigger than the expected value and the visibility of interference is low. We identify the sources of this discrepancy as the spatial filtering of the two-photon bandwidth and non-pair detection events caused by the detector …
We consider state reconstruction from the measurement statistics of phase space observables generated by photon number states. The results are obtained by inverting certain infinite matrices. In particular, we obtain reconstruction formulas, each of which involves only a single phase space observable.
Coherent photon-emitter interfaces offer a way to mediate efficient nonlinear photon-photon interactions, much needed for quantum information processing. Here we experimentally study the case of a two-level emitter, a quantum dot, coupled to a single optical mode in a nanophotonic waveguide. We carry out few-photon transport experiments and record the statistics of the light to reconstruct the scattering matrix elements of 1- and 2-photon components. This provides direct insight to the complex nonlinear photon interaction that contains rich many-body physics.
We show how one can deterministically generate photonic matrix product states with high bond and physical dimensions with an atomic array if one has access to a Rydberg-blockade mechanism. We develop both a quantum gate and an optimal control approach to universally control the system and analyze the photon retrieval efficiency of atomic arrays. Comprehensive modeling of the system shows that our scheme is capable of generating a large number of entangled photons. We further develop a multi-port photon emission approach that can efficiently distribute entangled photons into free space in sever…
We propose and demonstrate a method for measuring the joint spectrum of photon pairs via Fourier spectroscopy. The biphoton spectral intensity is computed from a two-dimensional interferogram of coincidence counts. The method has been implemented for a type-I downconversion source using a pair of common-path Mach-Zender interferometers based on Soleil compensators. The experimental results agree well with calculated frequency correlations that take into account the effects of coupling into single-mode fibers. The Fourier method is advantageous over scanning spectrometry when detectors exhibit …
We study and exactly solve the two-photon and k-photon Jaynes-Cummings models by using a novelty algebraic method. This algebraic method is based on the Pauli matrices realization and the tilting transformation of the $SU(2)$ group and let us diagonalize the Hamiltonian of these models by properly choosing the coherent state parameters of the transformation. Finally, we explicitly obtain the energy spectrum and eigenfunctions for each model.
BosonSampling is a well-defined scheme for demonstrating quantum supremacy with photons in near term. Although relying only on multi-photon interference in nonadaptive linear-optical networks, it is hard to simulate classically. Here we study BosonSampling using matrix product states, a powerful method from quantum many-body physics. This method stores the instantaneous quantum state during the evolution of photons in the optical quantum circuit, which allows us to reveal the dynamical features of single photons in BosonSampling devices, such as entanglement entropy growth. We show the flexibl…
We provide a simple analytic relation which connects the density operator of the radiation field with the number probabilities. The problem of experimentally "sampling" a general matrix elements is studied, and the deleterious effects of nonunit quantum efficiency in the detection process are analyzed showing how they can be reduced by using the squeezing technique. The obtained result is particulary useful for intracavity field reconstruction states.
Quantum spectroscopy was performed using the frequency-entangled broadband photon pairs generated by spontaneous parametric down-conversion. An absorptive sample was placed in front of the idler photon detector, and the frequency of signal photons was resolved by a diffraction grating. The absorption spectrum of the sample was measured by counting the coincidences, and the result is in agreement with the one measured by a conventional spectrophotometer with a classical light source.
Adiabatic passage techniques allow the generation of single photons which are very long compared to the typical detector time resolution. Therefore the detection time of a photon can be measured within the duration of the single-photon wavepacket. As a consequence, two-photon interference can be investigated in a time-resolved manner, i.e., the coincidence rate can be measured as a function of the time between photodetections. The theoretical analysis shows that this method not only gives information about the duration of single photons, but also about their coherence time. Here we discuss how…
We present a first-principles approach to electronic many-body systems strongly coupled to cavity modes in terms of matter-photon one-body reduced density matrices. The theory is fundamentally non-perturbative and thus captures not only the effects of correlated electronic systems but accounts also for strong interactions between matter and photon degrees of freedom. We do so by introducing a higher-dimensional auxiliary system that maps the coupled fermion-boson system to a dressed fermionic problem. This reformulation allows us to overcome many fundamental challenges of density-matrix theory…
Probabilities of photon counts at the output of a multiport optical device are generalised for optical sources of arbitrary quantum states in partially distinguishable optical modes. For the single-mode photon sources, the generating function for the probabilities is a linear combination of the matrix permanents of positive semi-definite Hermitian matrices, where each Hermitian matrix is a Hadamard product of a submatrix of the multiport matrix and a Hermitian matrix describing partial distinguishability. For the multi-mode sources the generating function is given by an integral of the Husimi …
Multiphoton interference effects can be measured with a single detector when two input photons are temporally well separated when compared with the dead time of the single-photon avalanche detector. Here we experimentally demonstrate that the Hong-Ou-Mandel interference effect can be observed with a single non-photon-number resolving detector via a time-delayed coincidence measurement of successive electrical signals from the detector. The two-photon interference experiment is performed by utilizing temporally well-separated pairwise weak coherent pulses and the interference fringes are succes…
We investigate the formation of photon bound states in a system of interacting photons inside nanoscale wires. The photons interact through the exchange of vibrational modes induced along the waveguide mainly due to radiation pressure. The problem of many-body photons is treated in using the formalism of contour Green's functions under the T-matrix approximation. The complex pole of the T-matrix is a signature for the appearance of photon-molecules. The analysis of such singularity provides the critical temperature at which the T-matrix approximation breaks down and photon-molecules appear. Fo…
We study a quantum system of coupled oscillators subject to a periodic excitation of its parameters. Using Floquet-Lyapunov theory we derive the linear integrals of motion of the system and relate their covariance matrix to that for the canonical observables. The operator integrals allows us to construct the intelligent (minimum uncertainty) states of the system and the corresponding photon-added states. We found explicit expressions for the wavefunction, Wigner function and covariance matrix of these states.
The experiments of multi-photon entanglements have been made by some groups, including Pan's group (Ref.[2],[3],[5]). Obviously, the increase number of the photon would cause a dramatically increase in the dimension of the measurement matrix, which result in a great consumption of time in the measurements. From a practical view, we wish to gain the most information through as little measurements as possible for the multi-photon entanglements. The low rank matrix recovery (LRMR) provides such a possibility to resolve all the issues of the measurement matrix based on less data. In this paper, we…
The indistinguishability of successively generated photons from a single quantum emitter is most commonly measured using two-photon interference at a beam splitter. Whilst for sources excited in the pulsed regime the measured bunching of photons reflects the full wavepacket indistinguishability of the emitted photons, for continuous wave (cw) excitation the inevitable dependence on detector timing resolution and driving strength obscures the underlying photon interference process. Here we derive a method to extract the photon indistinguishability from cw measurements by considering the relevan…
We devise a multiphoton interferometry scheme for sampling a quadratic function of a specific immanant for any submatrix of a unitary matrix and its row permutations. The full unitary matrix describes a passive, linear interferometer, and its submatrix is used when photons enter in and are detected at subsets of possible input and output channels. Immanants are mathematical constructs that interpolate between the permanent and determinant; contrary to determinants and permanents, which have meaningful physical applications, immanants are devoid of physical meaning classically but here are show…
We investigate the use of correlated photon pair sources for the improved quantum-level detection of a target in the presence of a noise background. Photon pairs are generated by spontaneous four-wave mixing, one photon from each pair (the herald) is measured locally while the other (the signal) is sent to illuminate the target. Following diffuse reflection from the target, the signal photons are detected by a receiver and non-classical timing correlations between the signal and herald are measured in the presence of a configurable background noise source. Quantum correlations from the photon …
We have measured the photon statistics of pump and probe beams after interaction with Rb atoms in a situation of Electromagnetically Induced Transparency. Both fields present super-poissonian statistics and their intensities become correlated, in good qualitative agreement with theoretical predictions in which both fields are treated quantum-mechanically. The intensity correlations measured are a first step towards the observation of entanglement between the fields.
We study two-photon scattering in a one-dimensional coupled resonator arrays (CRA) by a two-level system (TLS), which is localized as a quantum controller. The $S$-matrix is analytically calculated for various two-photon scattering processes by TLS, e.g., one photon is confined by TLS to form a bound state while the other is in the scattering state. It is discovered from the poles of the $S$-matrix that there exist two kinds of three-body bound states for describing two bound photons localized around TLS.
High visibility on-chip quantum interference among indistinguishable single-photons from multiples sources is a key prerequisite for integrated linear optical quantum computing. Resonant enhancement in micro-ring resonators naturally enables brighter, purer and more indistinguishable single-photon production without any tight spectral filtering. The indistinguishability of heralded single-photons from multiple micro-ring resonators has not been measured in any photonic platform. Here, we report on-chip indistinguishability measurements of heralded single-photons generated from independent micr…
We provide a systematic treatment of $N$-photon transport in a waveguide coupled to a local system, using the input-output formalism. The main result of the paper is a general connection between the $N$-photon S matrix and the Green functions of the local system. We also show that the computation can be significantly simplified, by exploiting the connectedness structure of both the S matrix and the Green function, and by computing the Green function using an effective Hamiltonian that involves only the degrees of freedom of the local system. We illustrate our formalism by computing $N$-photon …
Linear optical circuits of growing complexity are playing an increasing role in emerging photonic quantum technologies. Individual photonic devices are typically described by a unitary matrix containing amplitude and phase information, the characterisation of which is a key task. We present a constructive scheme to retrieve the unitary matrix describing an arbitrary linear optical device using data obtained from one-photon and two-photon ensembles. The scheme is stable on the arbitrarily increasable length scale of the photon packet and independent of photon loss at input and output ports of t…
We theoretically investigate the joint photodetection probabilities of the biexciton-exciton cascade in single semiconductor quantum dots and analytically derive the density matrix and the Bell's inequalities of the entangled state. Our model includes different mechanisms that may spoil or even destroy entanglement such as dephasing, energy splitting of the relay excitonic states and incoherent population exchange between these relay levels. We explicitly relate the fidelity of entanglement to the dynamics of these processes and derive a threshold for violation of Bell's inequalities. Applied …
We demonstrate a large grid of individually addressable superconducting single photon detectors on a single chip. Each detector element is fully integrated into an independent waveguide circuit with custom functionality at telecom wavelengths. High device density is achieved by fabricating the nanowire detectors in traveling wave geometry directly on top of silicon-on-insulator waveguides. Our superconducting single-photon detector matrix includes detector designs optimized for high detection efficiency, low dark count rate and high timing accuracy. As an example, we exploit the high timing re…
Photon number resolving detectors can be highly useful for studying the statistics of multi-photon quantum states of light. In this work we study the counts statistics of different states of light measured on multiplexed on-off detectors. We put special emphasis on artificial nonclassical features of the statistics obtained. We show new ways to derive analytical formulas for counts statistics and their moments. Using our approach we are the first to derive statistics moments for multi-mode thermal states measured on multiplexed on-off detectors. We use them to determine empirical Mandel parame…
The one- and two-photon scattering matrix S is obtained analytically for a one-dimensional waveguide and a point-like scatterer with N excited levels (generalized V -type atom). We argue that the two-photon scattering matrix contains sufficient information to distinguish between different level structures which are equivalent for single-photon scattering, such as a V -atom with N = 2 excited levels and two two-level systems. In particular, we show that the scattering with the V -type atom exhibits a destructive interference effect leading to two-photon Coupled-Resonator-Induced Transparency, w…
We developed a time-dependent density-matrix model to study photon-assisted (PA) electron transport in quantum cascade lasers. The Markovian equation of motion for the density matrix in the presence of an optical field is solved for an arbitrary field amplitude. Level-broadening terms emerge from microscopic Hamiltonians and supplant the need for empirical parameters that are often employed in related approaches. We show that, in quantum cascade lasers with diagonal design, photon resonances have a pronounced impact on electron dynamics around and above the lasing threshold, an effect that ste…
We generalize an approach for description of multi-photon experiments with multi-port unitary linear optical devices, initiated in \textit{Phys. Rev. A \textbf{89}, 022333 (2014)} for the case of single photons in mixed spectral states, to arbitrary (multi-photon) input and arbitrary photon detectors. We give a physical interpretation of a non-negative definite Hermitian matrix, the matrix of a quadratic form giving output probabilities, as the partial indistinguishability matrix. We show that output probabilities are \textit{always} given in terms of the matrix permanents of the Hadamard prod…
In this work we discuss the emergence of approximate causality in a general setup from waveguide QED -i.e. a one-dimensional propagating field interacting with a scatterer. We prove that this emergent causality translates into a structure for the N-photon scattering matrix. Our work builds on the derivation of a Lieb-Robinson-type bound for continuous models and for all coupling strengths, as well as on several intermediate results, of which we highlight (i) the asymptotic independence of space-like separated wave packets, (ii) the proper definition of input and output scattering states, and (…
The balanced homodyne detection as a readout scheme of gravitational-wave detectors is carefully examined, which specifies the directly measured quantum operator in the detection. This specification is necessary to apply the quantum measurement theory to gravitational-wave detections. We clarify the contribution of vacuum fluctuations to the noise spectral density without using the two-photon formulation. We found that the noise spectral density in the two-photon formulation includes vacuum fluctuations from the main interferometer but does not includes those from the local oscillator which de…
Despite the enormous technological interest in micro and nanolasers, surprisingly, no class-B quantum density-matrix model is available to date, capable of accurately describing coherence and photon correlations within a unified theory. In class-B lasers $-$applicable for most solid-state lasers at room temperature$-$, the macroscopic polarization decay rate is larger than the cavity damping rate which, in turn, exceeds the upper level population decay rate. Here we carry out a density-matrix theoretical approach for generic class-B lasers, and provide closed equations for the photonic and ato…
We study the generation of correlated photon pairs and heralded single photons via strongly non-degenerate spontaneous four-wave mixing (SFWM) in a series of identical micro-/nano fibers (MNF). Joint spectral intensity of the biphoton field generated at the wavelength of about 880 nm and 1310 nm has been measured under excitation by 100 ps laser pulses demonstrating good agreement with the theoretical prediction. The measured zero-time second-order autocorrelation function was about 0.2 when the emission rate of the heralded photons was of 4 Hz. The MNF-based source perfectly matches standard …
The microwave properties of a crystalline sapphire dielectric whispering gallery mode resonator have been measured at very low excitation strength (E/hf=1) and low temperatures (T = 30 mK). The measurements were sensitive enough to observe saturation due to a highly detuned electron spin resonance, which limited the loss tangent of the material to about 2e-8 measured at 13.868 and 13.259 GHz. Small power dependent frequency shifts were also measured which correspond to an added magnetic susceptibility of order 1e-9. This work shows that quantum limited microwave resonators with Q-factors > 1e8…
The quantum version of Google PageRank has recently been investigated by various groups and shown to be quadratically faster in time than the classical PageRank algorithm. In this paper we propose the implementation of Quantum PageRank by a stochastic quantum walk of correlated photons in a photonic waveguide lattice, where we allow the density matrix to evolve according to the Lindblad-Kossakowski master equation. This yields a stationary state, the diagonal of whose density matrix gives the page ranking.
We designed, fabricated, and measured superconducting nanowire single-photon detectors (SSPDs) with low filling factor which achieve high system detection efficiency (SDE) and counting rate simultaneously. Numerical simulation reveals that high optical absorptance is possible in SSPDs even for low filing factor by tuning the device design. The SDEs of fabricated 18-50% filling factor SSPDs were measured systematically, and all SSPDs showed high SDEs of 61-80% and the lowest 18% filling factor SSPD achieved a high SDE of 69%.
The second order photon correlation g^(2)(tau) of a chaotic optical-feedback semiconductor laser is precisely measured using a Hanbury Brown-Twiss interferometer. The accurate g^(2)(tau) with non-zero delay time is obtained experimentally from the photon pair time interval distribution through a ninth-order self-convolution correction. The experimental results agree well with the theoretical analysis. The relative error of g^(2)(tau) is no more than 0.005 within 50 ns delay time. The bunching effect and coherence time of the chaotic laser are measured via the precise photon correlation techniq…
