We show how one can deterministically generate photonic matrix product states with high bond and physical dimensions with an atomic array if one has access to a Rydberg-blockade mechanism. We develop both a quantum gate and an optimal control approach to universally control the system and analyze the photon retrieval efficiency of atomic arrays. Comprehensive modeling of the system shows that our scheme is capable of generating a large number of entangled photons. We further develop a multi-port photon emission approach that can efficiently distribute entangled photons into free space in several directions, which can become a useful tool in future quantum networks.
We propose a novel scheme for high fidelity photonic controlled phase gates using Rydberg blockade in an ensemble of atoms in an optical cavity. The gate operation is obtained by first storing a photonic pulse in the ensemble and then scattering a second pulse from the cavity, resulting in a phase change depending on whether the first pulse contained a single photon. We show that the combination of Rydberg blockade and optical cavities effectively enhances the optical non-linearity created by the strong Rydberg interaction and thereby reduces the requirements for photonic quantum gates. The re…
We consider the propagation of photons in a gas of Rydberg atoms under conditions of electromagnetically induced transparency, where they form strongly interacting massive particles, termed Rydberg polaritons. Depending on the strength of the van der Waals-type interactions of the atoms either bunching or anti-bunching of photons can be observed when driving the atoms off-resonantly. The bunching is associated with the formation of bound states. We employ a Green's function approach and numerical wave-function simulations to analyze the conditions for the creation and the dynamics of these pho…
We present the experimental demonstration of interaction induced enhancement in Rydberg excitation or Rydberg anti-blockade in thermal atomic vapor. We have used optical heterodyne detection technique to measure Rydberg population due to two-photon excitation to the Rydberg state. The anti-blockade peak which doesn't satisfy the two-photon resonant condition is observed along with the usual two-photon resonant peak which can't be explained using the model with non-interacting three-level atomic system. A model involving two interacting atoms is formulated for thermal atomic vapor using the dre…
We demonstrate Rabi flopping of small numbers of $\rm{^{87}Rb}$ atoms between ground and Rydberg states with $n\le 43$. Coherent population oscillations are observed for single atom flopping, while the presence of two or more atoms decoheres the oscillations. We show that these observations are consistent with van der Waals interactions of Rydberg atoms.
We study the atom-photon quantum interface with intracavity Rydberg-blocked atomic ensemble where the ground-Rydberg transition is realized by two-photon transition. Via theoretical analysis, we report our recent findings of the Jaynes-Cummings model on optical domain and robust atom-photon quantum gate enabled by this platform. The requirement on the implementation is mild which includes an optical cavity of moderately high finesse, typical alkali atoms such as Rb or Cs and the condition that cold atomic ensemble is well within the Rydberg blockade radius. The analysis focuses on the atomic e…
We propose a scheme for realizing quantum repeaters with Rydberg-blockade coupled atomic ensembles, based on a recently proposed collective encoding strategy. Rydberg-blockade mediated two-qubit gates and efficient cooperative photon emission are employed to create ensemble-photon entanglement. Thanks to deterministic entanglement swapping operations via Rydberg-based two-qubit gates, and to the suppression of multi-excitation errors by the blockade effect, the entanglement distribution rate of the present scheme is higher by orders of magnitude than the rates achieved by other ensemble-based …
We study the interaction of two photons in a Rydberg atomic ensemble under the condition of electromagnetically induced transparency, combining a semi-classical approach for pulse propagation and a complete quantum treatment for quantum state evolution. We find that the blockade regime is not suitable for implementing photon-photon cross-phase modulation due to pulse absorption and dispersion. However, approximately ideal cross-phase modulation can be realized based on relatively weak interactions, with counter-propagating and transversely separated pulses.
We study the excitation dynamics of Rydberg atoms in a one-dimensional lattice with periodic boundary conditions where the atomic Rydberg states are resonantly excited from the electronic ground state. Our description of the corresponding dynamics is numerically exact within the perfect blockade regime, i.e. no two atoms in a given range can be excited. The time-evolution of the mean Rydberg density, density-density correlations as well as entanglement properties are analyzed in detail. We demonstrate that the short time dynamics is universal and dominated by quantum phenomena, while for large…
We propose and analyze a quantum repeater architecture in which Rydberg blocked atomic ensembles inside optical cavities are linked by optical fibers. Entanglement generation, swapping and purification are achieved through collective laser manipulations of the ensembles and photon transmission. Successful transmission and storage of entanglement are heralded by ionization events rather than by photon detection signal used in previous proposals. We demonstrate how the high charge detection efficiency allows for a shortened average entanglement generation time, and we analyze an implementation o…
We propose a protocol to realize atomic nonadiabatic holonomic quantum computation (NHQC) with two computational atoms and an auxiliary atom. Dynamics of the system is analyzed in the regime of Rydberg blockade, and robust laser pulses are designed via reverse engineering, so that quantum gates can be easily realized with high fidelities. In addition, we also study the evolution suffering from dissipation with a master equation. The result indicates that decays of atoms can be heralded by measuring the state of the auxiliary atom, and nearly perfect unitary evolution can be obtained if the aux…
The dipole blockade of multiple Rydberg excitations in mesoscopic atomic ensembles allows the implementation of various quantum information tasks using collective states of cold, trapped atoms. Precise coherent manipulations of the collective ground and single Rydberg excitation states of an atomic ensemble requires the knowledge of the number of atoms with small uncertainty. We present an efficient method to acquire such information by interrogating the atomic ensemble with resonant pulses while monitoring the resulting Rydberg excitations. We show that after several such steps accompanied by…
We investigate electromagnetically induced transparency (EIT) and Autler-Townes (AT) splitting in Rydberg rubidium atoms for a six-level excitation scheme. In this six-level system, one radio-frequency field simultaneously couples to two high-laying Rydberg states and results in interesting atomic spectra observed in the EIT lines. We present experimental results for several excitation parameters. We also present two theoretical models for this atomic system, where these two models capture different aspects of the observed spectra. One is a six-level model used to predict dominant spectral fea…
We report on the experimental observation of non-trivial three-photon correlations imprinted onto initially uncorrelated photons through interaction with a single Rydberg superatom. Exploiting the Rydberg blockade mechanism, we turn a cold atomic cloud into a single effective emitter with collectively enhanced coupling to a focused photonic mode which gives rise to clear signatures in the connected part of the three-body correlation function of the out-going photons. We show that our results are in good agreement with a quantitative model for a single, strongly coupled Rydberg superatom. Furth…
Strong resonant dipole-dipole interactions in flexible Rydberg aggregates enable the formation of exciton pulses, the interplay of atomic motion and electronic excitation transfer which feature high fidelity entanglement transport. Here, we demonstrate the coherent splitting of such pulses into two modes, which induce strongly different atomic motion, leading to clear signatures of nonadiabatic effects in atomic density profiles. The mechanism exploits local nonadiabatic effects at a conical intersection, turning them from a decoherence source into an asset. The conical intersection is a conse…
A scheme is proposed to prepare squeezed states and Schrödinger cat-like states of the collective spin degrees of freedom associated with a pair of ground states in an atomic ensemble. The scheme uses an effective Jaynes-Cummings interaction which can be provided by excitation of the atoms to Rydberg states and an effective J_x interaction implemented by a resonant Raman coupling between the atomic ground states. Both dynamical evolution with a constant Hamiltonian and with adiabatic variation of the two interaction terms are studied. We show that by the application of further resonant laser f…
We study the dynamics of up to two Rydberg excitations and the correlation growth in a chain of atoms coupled to a photonic crystal waveguide. In this setup, an excitation can hop from one atom to another via exponentially decaying exchange interactions mediated by the waveguide. An initially localized excitation undergoes a continuous-time quantum walk for short-range hopping, and for long-range, it experiences quasi-localization. Besides that, the inverse participation ratio reveals a super-ballistic diffusion of the excitation in short times, whereas, at a long time, it becomes ballistic. F…
Strong interaction between two single photons is a long standing and important goal in quantum photonics. This would enable a new regime of nonlinear optics and unlock several applications in quantum information science, including photonic quantum gates and deterministic Bell-state measurements. In the context of quantum networks, it would be important to achieve interactions between single photons from independent photon pairs storable in quantum memories. So far, most experiments showing nonlinearities at the single-photon level have used weak classical input light. Here, we demonstrate the …
We study optical bistable behavior of a Rydberg electromagnetically-induced transparency (EIT) atomic medium in a unidirectional optical ring-cavity. Due to strong van del Waal (vdW) interactions between the atoms, both optical nonlinear dispersion and nonlinear absorption coefficients are enhanced substantially. Under the condition of two-photon on resonance, we show that probe one-photon detuning can change the phase of the third order nonlinearity coefficient, which tunes the character of the optical bistability within different ratios of dispersive and absorptive types. This enables the si…
We propose an efficient quantum repeater architecture with mesoscopic atomic ensembles, where the Rydberg blockade is employed for deterministic local entanglement generation, entanglement swapping and entanglement purification. Compared with conventional atomic-ensemble-based quantum repeater, the entanglement distribution rate is improved by up to two orders of magnitude with the help of the deterministic Rydberg gate. This new quantum repeater scheme is robust and fast, and thus opens up a new way for practical long-distance quantum communication.
We study radial wave packets produced by short-pulsed laser fields acting on Rydberg atoms, using analytical tools from supersymmetry-based quantum-defect theory. We begin with a time-dependent perturbative calculation for alkali-metal atoms, incorporating the atomic-excitation process. This provides insight into the general wave packet behavior and demonstrates agreement with conventional theory. We then obtain an alternative analytical description of a radial wave packet as a member of a particular family of squeezed states, which we call radial squeezed states. By construction, these have c…
We study resonant optical excitations of strongly-interacting Rydberg states of atoms in the presence of relaxations. We employ the quantum stochastic (Monte Carlo) wavefunctions to simulate the dissipative dynamics of tens of atoms in two-dimensional lattices. We show that under typical experimental conditions involving slow Rydberg state decay and sizable relaxation of atomic coherences, on the time scale of several microseconds the atomic ensemble approaches a stationary state in which much of the quantum correlations between the atoms have decayed away. The steady state, however, exhibits …
We apply reservoir engineering to construct a thermal environment with controllable temperature in an ultracold atomic Rydberg system. A Boltzmann distribution of the system's eigenstates is produced by optically driving a small environment of ultracold atoms, which is coupled to a photonic continuum through spontaneous emission. This technique provides a useful tool for quantum simulation of dynamics coupled to a thermal environment. Additionally, we demonstrate that pure eigenstates, such as Bell states, can be prepared in the Rydberg atomic system using this method.
We study the propagation of Rydberg slow light polaritons through an atomic medium for intermediate interactions. Then, the dispersion relation for the polaritons is well described by the slow light velocity alone, which allows for an analytical solution for arbitrary shape of the atomic cloud. We demonstrate the connection of Rydberg polaritons to the behavior of a conventional Kerr nonlinearity for weak interactions, and determine the leading quantum corrections for increasing interactions. We propose an experimental setup which allows one to measure the effective two-body interaction potent…
We investigated the Autler-Townes splitting produced by microwave transitions between atomic Rydberg states explored by optical spectroscopy from the ground electronic state. The laser-atom Hamiltonian describing the double irradiation of such a multilevel system is analysed on the basis of the Morris-Shore transformation. The application of this transformation to the microwave-dressed atomic system allows the identification of bright, dark, and spectator states associated with different configurations of atomic states and microwave polarisation. We derived synthetic spectra that show the main…
We describe a novel method for producing Greenberger-Horne-Zeilinger states in cold atoms coupled to a superconducting coplanar cavity. In the proposed scheme, atoms interact between each other by virtual photon exchange via a cavity mode. These interactions cause an asymmetric Rydberg blockade mechanism that suppresses simultaneous excitations into different atomic Rydberg levels, thus forcing all atoms to occupy the same Rydberg state. This mechanism has effect even if the atoms are separated by distances of the order of millimeters. The atomic populations are transferred adiabatically from …
The combination of electromagnetically induced transparency (EIT) with the nonlinear interaction between Rydberg atoms provides an effective interaction between photons. In this paper, we investigate the storage of optical pulses as collective Rydberg atomic excitations in a cold atomic ensemble. By measuring the dynamics of the stored Rydberg polaritons, we experimentally demonstrate that storing a probe pulse as Rydberg polaritons strongly enhances the Rydberg mediated interaction compared to the slow propagation case. We show that the process is characterized by two time scales. At short st…
Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary Rydberg excitation becomes unlikely leading to the Rydberg blockade effect. In a related effect, off-resonant coupling of light to Rydberg states of atoms contributes to the Rydberg anti-blockade effect where the Rydberg interaction creates a resonant condition that promotes a secondary excitation in a Rydberg atomic gas. Here, we study the light-matter interact…
We review methods for coherently controlling Rydberg quantum states of atomic ensembles using Adiabatic Rapid Passage and Stimulated Raman Adiabatic Passage. These methods are commonly used for population inversion in simple two-level and three-level systems. We show that adiabatic techniques allow us to control population and phase dynamics of complex entangled states of mesoscopic atomic ensembles for quantum information processing with Rydberg atoms. We also propose several schemes of single-qubit and two-qubit gates based on adiabatic passage, Rydberg blockade and Förster resonances in Ryd…
We demonstrate the storage and retrieval of an on-demand single photon generated by a collective Rydberg excitation in an ultra-low noise Raman quantum memory located in a different cold atomic ensemble. We generate single photons on demand by exciting a cold cloud of Rubidium atoms off resonantly to a Rydberg state, with a generation probability up to 15 $\%$ per trial. We then show that the single photons can be stored and retrieved with an efficiency of 21 $\%$ and a noise floor of $p_n= 2.3(3) \times 10^{-4}$ per trial in the Raman quantum memory. This leads to a signal-to-noise ratio rang…
With a resonant amplitude-modulation field on two Rydberg atoms, we propose a Rydberg antiblockade (RAB) regime, where the Rabi oscillation between collective ground and excited states is induced. A controlled-Z gate can be yielded through a Rabi cycle. Further, several common issues of the RAB gates are solved by modifying the parameter relation. The gate fidelity and the gate robustness against the control error are enhanced with a shaped pulse. The requirement of control precision of the Rydberg-Rydberg interaction strength is relaxed. In addition, the atomic excitation is restrained and th…
We propose and analyze a scheme for realizing the quantum reflection of single photons in a cold Rydberg atomic gas via electromagnetically induced transparency, by which a deep and tunable attractive potential well can be prepared by using stored gate photons. Such a scheme is promising for designing dispersion-type single-photon switches, and may be taken as a quantum device for observing the wave and particle natures of photons simultaneously.
We show that optical spectroscopy of Rydberg states can provide accurate {\em in situ} thermometry at room-temperature. Transitions from a metastable state to Rydberg states with principal quantum numbers of 25 to 30 have 200 times larger fractional frequency sensitivities to blackbody radiation than the Strontium clock transition. We demonstrate that magic wavelength lattices exist for both Strontium and Ytterbium transitions between the metastable and Rydberg states. Frequency measurements of Rydberg transitions with $10^{-16}$ accuracy provide $10 \, \mathrm{mK}$ resolution and yield a blac…
We present and analyze a simple model to illustrate the possibility of Rydberg state control by means of a moving guided electron. Specifically, we consider alkali metal atoms whose valence electron is initially prepared in a Rydberg s-state and investigate state changes induced by the interaction with the nearby passing electron. We analyze the dependence of the atomic final state, obtained after the passage, on the electron's momentum. We identify experimentally accessible parameter regimes and discuss the experimental feasibility of the proposed scheme. We furthermore discuss the possibilit…
We report on the observation of Rabi oscillations to a Rydberg state on a timescale below one nanosecond in thermal rubidium vapor. We use a bandwidth-limited pulsed excitation and observe up to 6 full Rabi cycles within a pulse duration of ~ 4 ns. We find good agreement between the experiment and numerical simulations based on a surprisingly simple model. This result shows that fully coherent dynamics with Rydberg states can be achieved even in thermal atomic vapor thus suggesting small vapor cells as a platform for room temperature quantum devices. Furthermore the result implies that previou…
We calculate interspecies Rydberg-Rydberg interaction strengths for the heavy alkalis Rb and Cs. The presence of strong Förster resonances makes interspecies coupling a promising approach for long range entanglement generation. We also provide an overview of the strongest Förster resonances for Rb-Rb and Cs-Cs using different principal quantum numbers for the two atoms. We show how interspecies coupling can be used for high fidelity quantum non demolition state measurements with low crosstalk in qubit arrays.
We investigate the indistinguishability of single photons retrieved from collective Rydberg excitations in cold atomic ensembles. The Rydberg spin waves are created either by off resonant two-photon excitation to the Rydberg state or by Rydberg electromagnetically induced transparency. To assess the indistinguishability of the generated single photons, we perform Hong-Ou-Mandel experiments between the single photons and weak coherent states of light. We analyze the indistinguishability of the single photons as a function of the detection window and for photons generated by off-resonant excitat…
We demonstrate $|W\rangle$ state encoding of multi-atom ensemble qubits. Using optically trapped Rb atoms the $T_2$ coherence time is 2.6(3) ms for $\bar N=7.6$ atoms and scales approximately inversely with the number of atoms. Strong Rydberg blockade between two ensemble qubits is demonstrated with a fidelity of $0.89(1)$ and a fidelity of $\sim \hspace{-.05cm}1.0$ when postselected on control ensemble excitation. These results are a significant step towards deterministic entanglement of atomic ensembles.
We present a review of quantum computation with neutral atom qubits. After an overview of architectural options and approaches to preparing large qubit arrays we examine Rydberg mediated gate protocols and fidelity for two- and multi-qubit interactions. Quantum simulation and Rydberg dressing are alternatives to circuit based quantum computing for exploring many body quantum dynamics. We review the properties of the dressing interaction and provide a quantitative figure of merit for the complexity of the coherent dynamics that can be accessed with dressing. We conclude with a summary of the cu…
Versatile controllability of interactions in ultracold atomic and molecular gases has now reached an unprecedented era where quantum correlations and unconventional many-body phases can be studied with no corresponding analogs in solid state systems. Recent experiments in Rydberg atomic gases have achieved exquisite control over non-local interactions, allowing novel quantum phases unreachable with the usual local interactions in atomic systems. Here, we study Rydberg dressed atomic fermions in a three dimensional optical lattice predicting the existence of hitherto unheard-of exotic mixed top…
We propose a robust localization of the highly-excited Rydberg atoms, interacting with doughnut-shaped optical vortices. Compared with the earlier standing-wave (SW)-based localization methods, a vortex beam can provide an ultrahigh-precision two-dimensional localization solely in the zero-intensity center, within a confined excitation region down to the nanometer scale. We show that the presence of the Rydberg-Rydberg interaction permits counter-intuitively much stronger confinement towards a high spatial resolution when it is partially compensated by a suitable detuning. In addition, applyin…
