We study the quantum dynamics of a material wavepacket bouncing off a modulated atomic mirror in the presence of a gravitational field. We find the occurrence of coherent accelerated dynamics for atoms. The acceleration takes place for certain initial phase space data and within specific windows of modulation strengths. The realization of the proposed acceleration scheme is within the range of present day experimental possibilities.
The interaction of quantum objects lies at the heart of fundamental quantum physics and is key to a wide range of quantum information technologies. Photon-quantum-emitter interactions are among the most widely studied. Two-qubit interactions are generally simplified into two quantum objects in static well-defined states . In this work we explore a fundamentally new dynamic type of spin-photon interaction. We demonstrate modulation of a coherent narrowband wavepacket with another truly quantum object, a quantum dot with ground state spin degree of freedom. What results is a quantum modulation o…
Accelerating non-spreading wavepackets in nonrelativistic free particle system, with probability distribution having an Airy function profile, were discovered by Berry and Balazs (1979), and have been subsequently realised in several optical experiments. It is shown that these wavepackets are actually Perelomov coherent states. It is found that the Galilean invariance of the Schrodinger equation plays a key role in making these states unique and giving rise to their unusual propagation properties.
We present a fully quantum model for the excitation of a bound electron based on the free-electron bound-electron resonant interaction (FEBERI) scheme. The bound electron is modeled as a quantum two-level system (TLS) at any initial quantum (qubit) state, and the free electron is presented as a pre-shaped quantum electron wavepacket (QEW). In the case that the QEW is short or modulated at optical frequency, the TLS quantum state may be coherently controlled with multiple modulation-correlated QEWs. For this case, we derive the transition probability of the TLS due to interaction with a multi-p…
We study the dynamics of an Airy wavepacket moving in a one-dimensional lattice potential. In contrast to the usual case of propagation in a continuum, for which such a wavepacket experiences a uniform acceleration, the lattice bounds its velocity, and so the acceleration cannot continue indefinitely. Instead, we show that the wavepacket's motion is described by relativistic equations of motion, which surprisingly, arise naturally from evolution under the standard non-relativistic Schrödinger equation. The presence of the lattice potential allows the wavepacket's motion to be controlled by mea…
We investigate the interplay between gravity and the quantum coherence present in the state of a pulse of light propagating in curved spacetime. We first introduce an operational way to distinguish between the overall shift in the pulse wavepacket and its genuine deformation after propagation. We then apply our technique to quantum states of photons that are coherent in the frequency degree of freedom, as well as to states of completely incoherent light. We focus on Gaussian profiles and frequency combs and find that the quantum coherence initially present can enhance the deformation induced b…
Coherent electron displacement is a conventional strategy for processing quantum information, as it enables to interconnect distinct sites in a network of atoms. The efficiency of the processing relies on the precise control of the mechanism, which has yet to be established. Here, we theoretically demonstrate a new route to drive the electron displacement on a timescale faster than that of the dynamical distortion of the electron wavepacket by utilizing attosecond single-cycle pulses. The characteristic feature of these pulses relies on a vast momentum transfer to an electron, leading to its d…
The application of a matrix-based reconstruction protocol for obtaining Molecular Frame (MF) photoelectron angular distributions (MFPADs) from laboratory frame (LF) measurements (LFPADs) is explored. Similarly to other recent works on the topic of MF reconstruction, this protocol makes use of time-resolved LF measurements, in which a rotational wavepacket is prepared and probed via photoionization, followed by a numerical reconstruction routine; however, in contrast to other methodologies, the protocol developed herein does not require determination of photoionization matrix elements, and cons…
Do the wavepacket-size of free-electron wavefunction and its history have physical effect in its interaction with light? Here we answer this problem by analyzing a QED model, considering both spontaneous and stimulated emission of quantized radiation field. For coherent radiation (Glauber state), we confirm that stimulated emission/absorption of photons has a dependence on wavepacket size that decays when it exceeds the interacting radiation wavelength, consistently and complementarily with Schrodinger equation analysis of wavepacket acceleration in classical electromagnetic field. Furthermore…
In the foundation of quantum mechanics, the spatial dimensions of electron wavepacket are understood only in terms of an expectation value - the probability distribution of the particle location. One can still inquire how the quantum electron wavepacket size affects a physical process. Here we address the fundamental physics problem of particle-wave duality and the measurability of a free electron quantum wavepacket. Our analysis of stimulated radiative interaction of an electron wavepacket, accompanied by numerical computations, reveals two limits. In the quantum regime of long wavepacket siz…
The usual concepts of topological physics, such as the Berry curvature, cannot be applied directly to non-Hermitian systems. We show that another object, the quantum metric, which often plays a secondary role in Hermitian systems, becomes a crucial quantity near exceptional points in non-Hermitian systems, where it diverges in a way that fully controls the description of wavepacket trajectories. The quantum metric behaviour is responsible for a constant acceleration with a fixed direction, and for a non-vanishing constant velocity with a controllable direction. Both contributions are independe…
Here we present a semiclassical analysis of spontaneous and stimulated radiative emission from unmodulated and optically-modulated electron quantum wavepackets. We show that the radiative emission/absorption and corresponding deceleration/acceleration of the wavepackets depend on the controllable 'history-dependent' wavepacket size. The characteristics of the radiative interaction when a wavepacket of size (duration) is short relative to the radiation wavelength, are close to the predictions of the classical point-particle modeling. On the other hand, in the long-sized wavepacket limit, the in…
The last two decades experimentally affirmed the quantum nature of free electron wavepackets by the rapid development of transmission electron microscopes into ultrafast, quantum-coherent systems. In particular, ultrafast electron pulses can be generated and timed to interact with optical near-fields, yielding coherent exchange of the quantized photon energy between the relativistic electron wavepacket and the light field. So far, all experiments have been restricted to the physically-confining bounds of transmission electron microscopes, with their small, millimeter-sized sample chambers. In …
Interference of two photons at a beamsplitter is at the core of many quantum photonic technologies, such as quantum key distribution or linear-optics quantum computing. Observing high-visibility interference is challenging because of the difficulty of realizing indistinguishable single-photon sources. Here, we perform a two-photon interference experiment using phase-randomized weak coherent states with different mean photon numbers. We place a tight upper bound on the expected coincidences for the case when the incident wavepackets contain single photons, allowing us to observe the Hong-Ou-Man…
Attosecond four-wave mixing spectroscopy using an XUV pulse and two noncollinear near-infrared pulses is employed to measure Rydberg wavepacket dynamics resulting from extreme ultraviolet excitation of a 3s electron in atomic argon into a series of autoionizing 3s-1np Rydberg states around 29 eV. The emitted signals from individual Rydberg states exhibit oscillatory structure and persist well beyond the expected lifetimes of the emitting Rydberg states. These results reflect substantial contributions of longer-lived Rydberg states to the four wave mixing emission signals of each individually d…
Recording molecular movies on ultrafast timescales has been a longstanding goal for unravelling detailed information about molecular dynamics. We present the direct experimental recording of very-high-resolution and -fidelity molecular movies over more than one-and-a-half periods of the laser-induced rotational dynamics of carbonylsulfide (OCS) molecules. Utilising the combination of single-quantum-state selection and an optimised two-pulse sequence to create a tailored rotational wavepacket, an unprecedented degree of field-free alignment, $\langle \cos^{2}{θ_{2D}}\rangle=0.96$ ($\langle \cos…
We derive semiclassical equations of motion for an accelerated wavepacket in a two-band system. We show that these equations can be formulated in terms of the static band geometry described by the quantum metric. We consider the specific cases of the Rashba Hamiltonian with and without a Zeeman term. The semiclassical trajectories are in full agreement with the ones found by solving the Schrödinger equation. This formalism successfully describes the adiabatic limit and the anomalous Hall effect traditionally attributed to Berry curvature. It also describes the opposite limit of coherent band s…
Fundamental quantum electrodynamical (QED) processes such as spontaneous emission and electron-photon scattering encompass a wealth of phenomena that form one of the cornerstones of modern science and technology. Conventionally, calculations in QED and in other field theories assume that incoming particles are single-momentum states. The possibility that coherent superposition states, i.e. "shaped wavepackets", will alter the result of fundamental scattering processes is thereby neglected, and is instead assumed to sum to an incoherent (statistical) distribution in the incoming momentum. Here,…
In this article, we present a unified reciprocal quantum electrodynamics (QED) formulation of quantum light-matter interaction. For electron-light interactions, we bridge the underlying theories of Photon-Induced Near-field Electron Microscopy (PINEM), Laser-induced Particle Accelerators and radiation sources, such as Free Electron Laser (FEL), transition radiation and Smith-Purcell effect. We demonstrate an electron-photon spectral reciprocity relation between the electron energy loss/gain and the radiation spectra. This "Acceleration/Radiation Correspondence" (ARC) conserves the electron-ene…
Optical Neural Networks from Coherent Transient Dynamics in Waveguide QED
School of Physics, Sun Yat-sen University（中山大学物理学院）；Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education, Hunan Normal University（湖南师范大学低维量子结构与量子控制教育部重点实验室）；Center for Quantum Computing, RIKEN（理化学研究所量子计算中心）；Department of Physics, University of Michigan（密歇根大学物理系）；State Key Laboratory of Optoelectronic Materials and Technologies, Sun Yat-sen University（中山大学光电材料与技术国家重点实验室）
