I. Novikova, Y. Xiao, D. F. Phillips, R. L. Walsworth
We study experimentally the effect of diffusion of Rb atoms on Electromagnetically Induced Transparency (EIT) in a buffer gas vapor cell. In particular, we find that diffusion of atomic coherence in-and-out of the laser beam plays a crucial role in determining the EIT resonance lineshape and the stored light lifetime.
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With atomic spontaneously generated coherence (SGC), we propose a novel scheme to coherently control the atom--photon momentum entanglement through atomic internal coherence. A novel phenomena of ``phase entanglement in momentum'' is proposed, and we found, under certain conditions, that super--high degree of momentum entanglement can be produced with this scheme.
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We have experimentally demonstrated the enhancement of coherent Raman scattering in Rb atomic vapor by exciting atomic coherence with fractional stimulated Raman adiabatic passage. Experimental results are in good agreement with numerical simulations. The results support the possibility of increasing the sensitivity of CARS by preparing atomic or molecular coherence using short pulses.
There is generally no obvious evidence in any direct relation between photon blockade and atomic coherence. Here instead of only illustrating the photon statistics, we show an interesting relation between the steady-state photon blockade and the atomic coherence by designing a weakly driven cavity QED system with a two-level atom trapped. It is shown for the first time that the maximal atomic coherence has a perfect correspondence with the optimal photon blockade. The negative effects of the strong dissipations on photon statistics, atomic coherence and their correspondence are also addressed.…
The second-order susceptibility which vanishes in the electric-dipole approximation for an atom is induced by the spontaneously generated coherence. The spontaneously generated coherence considered in a lambda-type atomic system causes an indirect coupling between the lower two levels which acts equivalently as a DC-field and therefore makes possible the existence of second-order susceptibility.
The entanglement of two dipole-coupled atoms with nondegenerate two-photon transitions interacting with two-mode field in lossless cavity has been investigated. It shows that the entanglement is dependent on the initial atomic states. The possibility of considerable growth of atomic entanglement due atomic coherence and dipole-dipole interaction is shown in the case of great mean values of thermal photons.
We present a convenient and efficient way to exchange and distribute multipartite entangled state via atomic coherence induced by electromagnetically induced transparency (EIT) in an atomic ensemble. By using the EIT-based nondegenerate four-wave mixing processes, the generation, exchange, and distribution of light-light, atom-light, and atom-atom multipartite entanglement can be achieved in a deterministic way with only coherent light fields. This EIT-induced atomic coherence acts as a quantum information processor and has the function of quantum beam splitter, quantum frequency converter, qu…
A symmetric four-level closed-loop $\diamondsuit$ type (the diamond structure) atomic system driven by four coherent optical fields is investigated. The system shows rich quantum interference and coherence features. When symmetry of the system is broken, interesting phenomena such as single and double dark resonances appear. As a result, the double electromagnetically induced transparency effect is generated, which will facilitate the implementation of quantum phase gate operation.
We present a quantum interference approach to preserve coherence in the external states of an atom trapped in an optical lattice. We show that this is possible by suitably choosing the initial state of the atom. We demonstrate this in context of decoherence due to spontaneous emission in an one-dimensional optical double-well lattice.
The electric field in a lossless, regularly-pumped micromaser with injected atomic coherence can undergo a period 2 oscillations in the steady state. The field changes its value after a single atom passes through the micromaser cavity, but returns to its original value after a second atom travels through. We give a simple explanation for this phenomenon in terms of tangent and cotangent states. We also examine the effect of cavity damping on this steady state.
Following the method of Victor V. Kozlov et al.[PhysRevA. 74. 063829],we inspect the coherence induced by incoherent pump and spontaneous decay process in $Λ$ type three-level atomic system with degenerated lower duplicate levels. The system shows a coherent population trapping state and multi-steady states characteristic in different conditions. Interestingly, two kinds of steady states generated by the system in different sets of pumping and decaying parameters, the "singlet" state and the "triplet" state, exhibit stable or unstable characteristics under the action of pumping field and vacuu…
Complementarity of which-path information in induced and stimulated coherences via four-wave mixing process from warm Rb atomic ensemble
本研究通过双路径干涉仪和两个四波混频原子系综，建立了诱导与受激相干性中干涉可见度、并发性和可预测性的互补关系，并区分了量子与经典行为。
We propose a scheme via three-level cascade atoms to entangle two optomechanical oscillators as well as two-mode fields. We show that two movable mirrors and two-mode fields can be entangled even for bad cavity limit. We also study entanglement of the output two-mode fields in frequency domain. The results show that the frequency of the mirror oscillation and the injected atomic coherence affect the output entanglement of the two-mode fields.
We utilize the generation of large atomic coherence to enhance the resonant nonlinear magneto-optic effect by several orders of magnitude, thereby eliminating power broadening and improving the fundamental signal-to-noise ratio. A proof-of-principle experiment is carried out in a dense vapor of Rb atoms. Detailed numerical calculations are in good agreement with the experimental results. Applications such as optical magnetometry or the search for violations of parity and time reversal symmetry are feasible.
We investigate the quantum properties of fields generated by resonantly enhanced wave mixing based on atomic coherence in Raman systems. We show that such a process can be used for generation of pairs of Stokes and anti-Stokes fields with nearly perfect quantum correlations, yielding almost complete (i.e. 100%) squeezing without the use of a cavity. We discuss the extension of the wave mixing interactions into the domain of a few interacting light quanta.
Effect of spontaneously generated coherence on left-handedness in a degeneracy atomic system
研究四能级Y型近简并原子系统中SGC对左手性的调控作用，表明强SGC可实现负介电常数与负磁导率、增强折射率并抑制吸收。
We demonstrate fast and accurate control of the evolution of collective atomic coherences in an Erbium doped solid using external electric fields. This is achieved by controlling the inhomogeneous broadening of Erbium ions emitting at 1536 nm using an electric field gradient and the linear Stark effect. The manipulation of atomic coherence is characterized with the collective spontaneous emission (optical free induction decay) emitted by the sample after an optical excitation, which does not require any previous preparation of the atoms. We show that controlled dephasing and rephasing of the a…
The photon spectrum in macrocoherent atomic de-excitation via radiative emission of neutrino pairs (RENP) has been proposed as a sensitive probe of the neutrino mass spectrum, capable of competing with conventional neutrino experiments. In this paper we revisit this intriguing possibility, presenting an alternative method for inducing large coherence in a target based on adiabatic techniques. More concretely, we propose the use of a modified version of Coherent Population Return (CPR), namely double CPR, that turns out to be extremely robust with respect to the experimental parameters, and cap…
Four-wave mixing in resonant atomic vapors based on maximum coherence induced by Stark-chirped rapid adiabatic passage (SCRAP) is investigated theoretically. We show the advantages of a coupling scheme involving maximum coherence and demonstrate how a large atomic coherence between a ground and an highly excited state can be prepared by SCRAP. Full analytic solutions of the field propagation problem taking into account pump field depletion are derived. The solutions are obtained with the help of an Hamiltonian approach which in the adiabatic limit permits to reduce the full set of Maxwell-Bloc…
The evolution of the quantum wave packet describing an atom trapped in the surface-tip junction of the scanning tunneling microscope is investigated by using the time-dependent Schroedinger equation, and by a quasi-classical Hamiltonian approach. The estimates concern a Xe atom in a biased double-well junction potential. The exact treatment shows that quantum coherence oscillations of the metastable ground state may occur at particular resonant values of the bias voltage. The effect of decoherence by partial localization is studied within the quasi-classical frame.
For a transition $F_e=0\leftrightarrow F_g=1$ driven by a linearly polarized light and probed by a circularly light, quantum coherence effects are investigated. Due to the coherence between the drive Rabi frequency and Zeeman splitting, electromagnetically induced transparency, electromagnetically induced absorption, and the transition from positive to negative dispersion are obtained, as well as the populations coherently oscillating in a wide spectral region. At the zero pump-probe detuning, the subluminal and superluminal light propagation is predicted. Finally, coherent population trapping…
Quantum coherence measures in entangled atomic systems
本研究探讨了相对论加速对纠缠原子系统中量子相干度量的影响，分析了不同情景下相干性的变化规律。
We consider N identical two-level atoms coupled to an optical cavity, which is coherently driven by an external field. In the limit of small atomic excitation, the reflection and transmission coefficients for both fields and intensities are calculated analytically. In addition, the frequency content of the cavity field and hence also the emission spectrum of the cavity is determined. It is discussed in particular how individual collisional dephasing and common atomic energy-level fluctuations prevent the cavity field from being in a coherent state, which in turn affects the outgoing fields.
We report a prolonged coherence time of the collective spin wave of a thermal 87Rb atomic ensemble in a paraffin coated cell. The spin wave is prepared through a stimulated Raman Process. The long coherence time time is achieved by prolonging the lifetime of the spins with paraffin coating and minimize dephasing with optimal experimental configuration. The observation of the long time delayed-stimulated Stokes signal in the writing process suggests the prolonged lifetime of the prepared spins; a direct measurement of the decay of anti-Stokes signal in the reading process shows the coherence ti…
Multipartite entanglement plays an important role in quantum information processing and quantum metrology. Here, the dressing-energy-level-cascaded (DELC) four-wave mixing (FWM) processes are proposed to generate all-optical controlled multipartite entanglement within a single device. The entanglement characteristics of the produced states of light are characterized by applying the Duan criterion and the positivity under partial transposition criterion. Moreover, by using an internal dressing field to modulate atomic coherence, multiple quantum coherent channels of FWM are simultaneously const…
We investigate the dynamical behavior of the atom-photon entanglement in a V-type three-level quantum system using the atomic reduced entropy. It is shown that an atom and photons are entangled at the steady-state; however disentanglement can also be achieved in an especial condition. It is demonstrated that in the presence of quantum interference induced by spontaneous emission, the reduced entropy and the atom-photon entanglement are phase-dependent. Non-stationary solution is also obtained when the quantum interference due to the spontaneous emission is completely included.
An isotropic medium, having magnetic sublevels, when subjected to a magnetic field or an electromagnetic field can induce anisotropy in the medium; and as a result the plane of polarization of the probe field can rotate. Therefore the rotation due to the magnetic field alone, can be {\em controlled efficiently} with use of a coherent field. We show, using a control field, significant enhancement of the magneto-optical rotation and demonstrate the possibility of realizing {\em magneto-optical switch}.
In contrast to the traditional Spontaneous Generated Coherence (SGC), Field Generated Coherence (FGC)-based atomic scheme is presented for spontaneous emission cancellation. It is easy to achieve externally controllable experimental trapping condition in this 4-field-driven 5-level atomic system. Consequently, due to the FGC the decay from the central dressed \emph{bare-energy-state} of the set of upper three closely spaced hyperfine decaying states of Sodium D2 line is completely cancelled under the trapping condition, exhibiting a novel phenomenon of a \textit{dark bare-energy-state}% . Exte…
We investigate scaling of work and efficiency of a photonic Carnot engine with the number of quantum coherent resources. Specifically, we consider a generalization of the "phaseonium fuel" for the photonic Carnot engine, which was first introduced as a three-level atom with two lower states in a quantum coherent superposition by [M. O. Scully, M. Suhail Zubairy, G. S. Agarwal, and H. Walther, Science {\bf 299}, 862 (2003)], to the case of $N+1$ level atoms with $N$ coherent lower levels. We take into account atomic relaxation and dephasing as well as the cavity loss and derive a coarse grained…
Quantum coherence and interference effects in atomic and molecular physics has been extensively studied due to intriguing counterintuitive physics and potential important applications. Here we present one such application of using quantum coherence to generate and enhance gain in extreme ultra-violet(XUV)(@58.4nm in Helium) and infra-red(@794.76nm in Rubidium) regime of electromagnetic radiation. We show that using moderate external coherent drive, a substantial enhancement in the energy of the lasing pulse can be achieved under optimal conditions. We also discuss the role of coherence. The pr…
We investigate the evolution of a Zeeman coherence grating induced in a cold atomic cesium sample in the presence of an external magnetic field. The gratings are created in a three-beam light storage configuration using two quasi-collinear writing laser pulses and reading with a counterpropagating pulse after a variable time delay. The phase conjugated pulse arising from the atomic sample is monitored. Collapses and revivals of the retrieved pulse are observed for different polarizations of the laser beams and for different directions of the applied magnetic field. While magnetic field inhomog…
Spontaneous emission can create coherences in a multilevel atom having close lying levels, subject to the condition that the atomic dipole matrix elements are non-orthogonal. This condition is rarely met in atomic systems. We report the possibility of bypassing this condition and thereby creating coherences by letting the atom with orthogonal dipoles to interact with the vacuum of a pre-selected polarized cavity mode rather than the free space vacuum. We derive a master equation for the reduced density operator of a model four level atomic system, and obtain its analytical solution to describe…
In spontaneous emission an atom in an excited state undergoes a transition to the ground state and emits a single photon. Associated with the emission is a change of the atomic momentum due to photon recoil. Photon emission can be modified close to surfaces and in cavities. For an ion, localized in front of a mirror, coherence of the emitted resonance fluorescence has been reported. In free space experiments demonstrated that spontaneous emission destroys motional coherence. Here we report on motional coherence created by a single spontaneous emission event close to a mirror surface. The coher…
Two-mode squeezing and entanglement is obtained in a atom-cavity system cosisting a three-level atom and a two-mode cavity with driving laser fields. Here non-resonatn dressed-state transitions between the cavity modes and atom are used to get the effective Hamiltonian.
We report an ultrafast and efficient way to create the maximum coherence between the two lower states in a -like atomic systems, driven by two nonlinearly chirped few-cycle pulses. The phenomenon of coherent population trapping and electromagnetically induced population transfer are investigated by solving the appropriate density matrix equations without invoking the rotating wave approximation. The robustness of the scheme for maximum coherence against the variation of the laser parameters are tested numerically. We also demonstrate that the proposed scheme could be used to obtain complete po…
We present a detailed analysis of coherence creation in a four level double lambda-like atomic system using a train of ultra-short few-cycle Gaussian pulses. The effect of the Doppler broadening has been analyzed. It is possible to create high coherence across all the velocity groups in the atomic ensemble using pulses with low repetition frequency. The accumulation of coherence at different radial locations within the atomic beam cross-section as a function of the number of pulses in the train is also reported. We find that pulse train with lower repetition frequencies are able to generate hi…
Bright, entangled multiphoton sources based on atom photon interactions are an essential requirement in the realization of several quantum information and quantum computation schemes based on photonic quantum systems. Here, we experimentally demonstrate a four photon polarization entangled GHZ state obtained from Doppler broadened atomic ensembles of 87Rb atoms. Owing to collective two photon coherence in the Doppler broadened cascade-type atomic system, our setup enables the generation of robust four photon GHZ states with a fidelity of 0.82 and a measured four photon average coincidence rate…
The role of spontaneous emission in the interaction between a two-level atom and a pumped micro-cavity in the strong coupling regime is discussed in this paper. Especially, using a quantum Monte-Carlo simulation, we investigate atomic spatial coherence. It is found that atomic spontaneous emission destroys the coherence between neighboring lattice sites, while the cavity decay does not. Furthermore, our computation of the spatial coherence function shows that the in-site locality is little affected by the cavity decay, but greatly depends on the cavity pump amplitude.
The coherent manipulation of the atomic matter waves is of great interest both in science and technology. In order to study how an atom optic device alters the coherence of an atomic beam, we consider the quantum lens proposed by Averbukh et al [1] to show the discrete nature of the electromagnetic field. We extend the analysis of this quantum lens to the study of another essentially quantum property present in the focusing process, i.e., the atom-field entanglement, and show how the initial atomic coherence and purity are affected by the entanglement. The dynamics of this process is obtained …
We study the quantum coherence properties of a finite sized atomic condensate using a toy-model and the thin spectrum model formalism. The decoherence time for a condensate in the ground state, nominally taken as a variational symmetry breaking state, is investigated for both zero and finite temperatures. We also consider the lifetimes for Bogoliubov quasi-particle excitations, and contrast them to the observability window determined by the ground state coherence time. The lifetimes are shown to exhibit a general characteristic dependence on the temperature, determined by the thin spectrum acc…
We demonstrate $|W\rangle$ state encoding of multi-atom ensemble qubits. Using optically trapped Rb atoms the $T_2$ coherence time is 2.6(3) ms for $\bar N=7.6$ atoms and scales approximately inversely with the number of atoms. Strong Rydberg blockade between two ensemble qubits is demonstrated with a fidelity of $0.89(1)$ and a fidelity of $\sim \hspace{-.05cm}1.0$ when postselected on control ensemble excitation. These results are a significant step towards deterministic entanglement of atomic ensembles.
Quantum technologies are built on the power of coherent superposition. Atomic coherence is typically generated from optical coherence, most often via Rabi oscillations. However, canonical coherent states of light create imperfect resources; a fully-quantized description of "$\tfracπ{2}$ pulses" shows that the atomic superpositions generated remain entangled with the light. We show that there are quantum states of light that generate coherent atomic states perfectly, with no residual atom-field entanglement. These states can be found for arbitrarily short times and approach slightly-number-sque…
We demonstrate coupling of light resonant to transition between two excited states of rubidium and long-lived ground-state atomic coherence. In our proof-of-principle experiment a non-linear process of four-wave mixing is used to achieve light emission proportional to independently prepared ground-state atomic coherence. Strong correlations between stimulated Raman scattering light heralding generation of ground-state coherence and the four-wave mixing signal are measured and shown to survive the storage period, which is promising in terms of quantum memory applications. The process is charact…
Squeezing of atomic resonance fluorescence is shown to be optimized by a properly designed environment, which can be realized by a quasi-resonant cavity. Optimal squeezing is achieved if the atomic coherence is maximized, corresponding to a pure atomic quantum state. The atomic-state purification is achieved by the backaction of the cavity field on the atom, which increases the atomic coherence and decreases the atomic excitation. For realistic cavities, the coupling of the atom to the cavity field yields a purity of the atomic state of more than 99%. The fragility of squeezing against dephasi…
We report on the storage of orbital angular momentum of light in a cold ensemble of cesium atoms. We employ Bragg diffraction to retrieve the stored optical information impressed into the atomic coherence by the incident light fields. The stored information can be manipulated by an applied magnetic field and we were able to observe collapses and revivals due to the rotation of the stored atomic Zeeman coherence for times longer than 15 $μs$.
We propose a model to study the coherence and entanglement resulting from the interaction of a finite-size atomic ensemble with degenerate counter-propagating field modes of a high-Q ring cavity. Our approach applies to an arbitrary number of atoms N and includes the spatial variation of the field throughout the ensemble. We report several new interesting aspects of coherence and entangled behavior that emerge when the size of the atomic ensemble is not taken to the thermodynamic limit of N>>1. Under such conditions, it is found that the counter-propagating cavity modes, although in the thermo…
The method of perturbative expansion of master equation is employed to study the dissipative properties of system and of atom in the two-photon Jaynes-Cummings model (JCM) with degenerate atomic levels. The numerical results show that the degeneracy of atomic levels prolongs the period of entanglement between the atom and the field. The asymptotic value of atomic linear entropy is apparently increased by the degeneration. The amplitude of local entanglement and disentanglement is suppressed. The better the initial coherence property of the degenerate atom, the larger the coherence loss.
We present a scheme for two-dimensional (2D) atom localization in a three-level atomic system. The scheme is based on quantum coherence via classical standing wave fields between the two excited levels. Our results show that conditional position probability is significantly phase dependent of the applied field and frequency detuning of spontaneously emitted photons. We obtain a single localization peak having probability close to unity by manipulating the control parameters. The effect of atomic level coherence on the sub-wavelength localization has also been studied. Our scheme may be helpful…
Left handness in a four-level atomic system
本文提出利用四能级密集原子系统中的量子相干实现同时负介电常数和负磁导率，拓展了左手法性在更宽频率带的应用潜力。
We propose a scheme able to generate on demand a steady-state entanglement between two non-degenerate cavity modes. The scheme relies on the interaction of the cavity modes with driven two or three-level atoms which act as a coupler to build entanglement between the modes. We show that in the limit of a strong driving, crucial for the generation of entanglement between the modes is to imbalance populations of the dressed states of the driven atomic transition. In the case of a three-level V-type atom, we find that a stationary entanglement can be created on demand by tuning the Rabi frequency …
We demonstrate an atom localization scheme based on monitoring of the atomic coherences. We consider atomic transitions in a Lambda configuration where the control field is a standing wave field. The probe field and the control field produce coherence between the two ground states. We show that this coherence has the same fringe pattern as produced by a Fabry-Perot interferometer and thus measurement of the atomic coherence would localize the atom. Interestingly enough the role of the cavity finesse is played by the ratio of the intensities of the pump and probe. This is in fact the reason for…
The subtle and fundamental issue of indistinguishability and interference between independent pathways to the same target state is examined in the context of coherent control of atomic and molecular processes, with emphasis placed on possible "which-way" information due to quantum entanglement established in the quantum dynamics. Because quantum interference between independent pathways to the same target state occurs only when the independent pathways are indistinguishable, it is first shown that creating useful coherence (as defined in the paper) between nondegenerate states of a molecule fo…
The exactly analytical solutions for the dynamics of the dissipative three-level V-type and $Λ$-type atomic systems in the vacuum Lorentzian environments are presented. Quantum interference phenomenon between the two transitions in V-type atomic system is studied and the intuitive interference conditions are derived. For the dissipative $Λ$-type atomic system, we demonstrate that the similar quantum interference phenomenon does not exist. Finally, we study the dynamical evolution of quantum Fisher information, quantum entanglement and quantum coherence for the V-type atomic system. We find tha…
We report on the observation of the coherent enhancement of the return probability ("enhanced return to the origin" , ERO) in a periodically kicked cold-atom gas. By submitting an atomic wave packet to a pulsed, periodically shifted laser standing wave, we induce an oscillation of ERO in time and explain it in terms of a periodic, reversible dephasing in the weak-localization interference sequences responsible for ERO. Monitoring the temporal decay of ERO, we exploit its quantum coherent nature to quantify the decoherence rate of the atomic system.
Developing an analytical theory for atomic coherence driven by ultrashort laster pulses has proved to be challenging due to the breakdown of the rotating wave approximation (RWA). In this paper, we present an approximate, closed-form solution to the Schrodinger equation that describes a two-level atom under the excitation of a far-off-resonance, few-cycle pulse of arbitrary shape without invoking the RWA. As an example of its applicability, an analytical solution for Gaussian pulses is explicitly given. Comparisons with numerical solutions validate the accuracy our solution within the scope of…
We consider finite sized atomic systems with varying number of particles which have dipolar interactions among them and also under the collective driving and dissipative effect of thermal photon environment. Focusing on the simple case of two atoms, we investigate the impact of different parameters of the model on the coherence contained in the system. We observe that even though the system is initialized in a completely incoherent state, it evolves to a state with a finite amount of coherence and preserve that coherence in the long-time limit in the presence of thermal photons. We propose a n…
We present experimental observations of interference between an atomic spin coherence and an optical field in a Λ-type gradient echo memory. The interference is mediated by a strong classical field that couples a weak probe field to the atomic coherence through a resonant Raman transition. Interference can be observed between a prepared spin coherence and another propagating optical field, or between multiple Λ transitions driving a single spin coherence. In principle, the interference in each scheme can yield a near unity visibility.
Thermal vapor quantum battery based on collective atomic spins
本文基于热碱金属蒸气中的集体原子自旋集体实现室温量子电池，通过直接测量单位元演化的极值内部能量确定电池容量，并验证了相干与非相干贡献的分解。
Interference effects in quantum transitions, giving rise to amplification without inversion, optical transparency and to enhancements in nonlinear optical frequency conversions are considered. Review of the relevant early theoretical and experimental results is given. The role of relaxation processes, spontaneous cascade of polarizations, local field effects, Doppler-broadening, as well as specific features of the interference in the spectral continuum are discussed.
We study phase-sensitive amplification of electromagnetically induced transparency in a warm ${}^{85}$Rb vapor wherein a microwave driving field couples the two lower-energy states of a Λ energy-level system thereby transforming into a Δ system. Our theoretical description includes effects of ground-state coherence decay and temperature effects. In particular, we demonstrate that driving-field-enhanced electromagnetically induced transparency is robust against significant loss of coherence between ground states. We also show that for specific field intensities, a threshold rate of ground-state…
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