We study the driven tunneling of a one-dimensional charged particle confined to a rectangular double-well. The numerical simulation of the Schrödinger equation based on the Cranck-Nicholson finite-difference scheme, shows that the modulation of the amplitude of the external field may result in the parametric resonance. The latter is accompanied by the breakdown of the quasi-periodic motion characteristic of the usual driven tunneling, and the emergence of an irregular dynamics. We describe the above breakdown with the occupation probability for the ground state of the unperturbed system, and make the visualization of the irregular dynamics with the help of Shaw-Takens' reconstruction of the state-space. Both approaches agree as to the values of the resonant frequency for the parametric excitation. Our results indicate that the shape of the laser pulse could be essential for generating chaotic tunneling.
The interplay between chaotic tunneling and dynamical localization in mixed phase space is investigated. Semiclassical analysis using complex classical orbits reveals that tunneling through torus regions and transport in chaotic regions are not independent processes, rather they are strongly correlated and described by complex orbits with both properties. This predicts a phenomenon analogous to the quantum suppression of classical diffusion: chaotic tunneling is suppressed as a result of dynamical localization in chaotic regions. This hypothesis is confirmed by numerical experiments where the …
In generic Hamiltonian systems tori of regular motion are dynamically separated from regions of chaotic motion in phase space. Quantum mechanically these phase-space regions are coupled by dynamical tunneling. We introduce a semiclassical approach based on complex paths for the prediction of dynamical tunneling rates from regular tori to the chaotic region. This approach is demonstrated for the standard map giving excellent agreement with numerically determined tunneling rates.
We derive a prediction of dynamical tunneling rates from regular to chaotic phase-space regions combining the direct regular-to-chaotic tunneling mechanism in the quantum regime with an improved resonance-assisted tunneling theory in the semiclassical regime. We give a qualitative recipe for identifying the relevance of nonlinear resonances in a given $\hbar$-regime. For systems with one or multiple dominant resonances we find excellent agreement to numerics.
Quantum tunneling in the presence of chaos is analyzed, focusing especially on the interplay between quantum tunneling and dynamical localization. We observed flooding of potentially existing tunneling amplitude by adding noise to the chaotic sea to attenuate the destructive interference generating dynamical localization. This phenomenon is related to the nature of complex orbits describing tunneling between torus and chaotic regions. The tunneling rate is found to obey a perturbative scaling with noise intensity when the noise intensity is sufficiently small and then saturate in a large noise…
It is known that the ponderomotive potential from the laser electron interaction behaves like a static potential that scatters off electrons. We have investigated the process of the electron tunneling the ponderomotive potential by using the nonperturbative quantum electrodynamic approach with a modified Gaussian quantized laser field. The results show that the ponderomotive tunneling is significantly larger than the tunneling of a static potential of the same profile. The tunneled electron is discrete in energy spectrum and spatial diffraction as the result of multiphoton processes. A resonan…
We derive a formula predicting dynamical tunneling rates from regular states to the chaotic sea in systems with a mixed phase space. Our approach is based on the introduction of a fictitious integrable system that resembles the regular dynamics within the island. For the standard map and other kicked systems we find agreement with numerical results for all regular states in a regime where resonance-assisted tunneling is not relevant.
We review the fictitious integrable system approach which predicts dynamical tunneling rates from regular states to the chaotic region in systems with a mixed phase space. It is based on the introduction of a fictitious integrable system that resembles the regular dynamics within the regular island. We focus on the direct regular-to-chaotic tunneling process which dominates, if nonlinear resonances within the regular island are not relevant. For quantum maps, billiard systems, and optical microcavities we find excellent agreement with numerical rates for all regular states.
We revisit the problem of laser-induced suppression of quantum dynamical tunneling in a model system studied by Kilin et al. [Phys. Rev. Lett. 76 (1996) 3297]. This quantum system consists of a ground state symmetric double-well potential which is coupled by a strong laser field to an excited state asymmetric double-well potential. By analyzing the assumptions used in their analysis we show that the suppression of quantum dynamical tunneling can be explained with the use of dark and bright states of the system. We also generalize the system and the conditions for suppression of quantum tunneli…
We investigate dynamical tunneling in many dimensional systems using a quasi-periodically modulated kicked rotor, and find that the tunneling rate from the torus to the chaotic region is drastically enhanced when the chaotic states become delocalized as a result of the Anderson transition. This result strongly suggests that amphibious states, which were discovered for a one-dimensional kicked rotor with transporting islands [L. Hufnagel et al., Phys. Rev. Lett. 89, 154101 (2002)], quite commonly appear in many dimensional systems.
We study a model for frustrated tunneling ionization using ultrashort laser pulses. The model is based on the strong field approximation and it employs the saddle point approximation to predict quasiclassical trajectories that are captured on Rydberg states. We present a classification of the saddle-point solutions and explore their behavior as functions of angular momentum of the final state, as well as the carrier--envelope phase (CEP) of the laser pulse. We compare the final state population computed by the model to results obtained by numerical propagation of the time-dependent Schrödinger…
Using quantum computers to simulate polyatomic reaction dynamics has an exponential advantage in the amount of resources needed over classical computers. Here we demonstrate an exact simulation of the dynamics of the laser-driven isomerization reaction of asymmetric malondialdehydes. We discretize space and time, decompose the Hamiltonian operator according to the number of qubits and use Walsh-series approximation to implement the quantum circuit for diagonal operators. We observe that the reaction evolves by means of a tunneling mechanism through a potential barrier and the final state is in…
In this paper, we investigate tunneling of conduction band electrons in a system of an asymmetric double quantum dot which interacts with an environment. First, we consider the case in which the system only interacts with the environment and demonstrate that as time goes to infinity they both reach an equilibrium, which is expected, and there is always a maximum and minimum for the populations of the states of the system. Then we investigate the case in which an external resonant optical pulse (a laser) is applied to the system interacting with the environment. However, in this case for differ…
It is now common practice to solve the Schrödinger equation to estimate the tunneling current between two metal electrodes at specified potentials, or the transmission through a potential barrier by assuming an incident, reflected, and transmitted wave. However, we suggest that these methods may not be appropriate for nanoscale circuits. The electron man-free path may be as long as 68.2 nm in metallic elements so we consider the possibility that quantum effects may occur throughout a nanoscale circuit, including the connections. Analytical methods are presented for modeling the coherent transf…
We derive the photocount statistics of the radiation emitted from a chaotic laser resonator in the regime of single-mode lasing. Random spatial variations of the resonator eigenfunctions lead to strong mode-to-mode fluctuations of the laser emission. The distribution of the mean photocount over an ensemble of modes changes qualitatively at the lasing transition, and displays up to three peaks above the lasing threshold.
We develop the semiclassical method of complex trajectories in application to chaotic dynamical tunneling. First, we suggest a systematic numerical technique for obtaining complex tunneling trajectories by the gradual deformation of the classical ones. This provides a natural classification of the tunneling solutions. Second, we present a heuristic procedure for sorting out the least suppressed trajectory. As an illustration, we apply our technique to the process of chaotic tunneling in a quantum mechanical model with two degrees of freedom. Our analysis reveals rich dynamics of the system. At…
In the spectrum of systems showing chaos-assisted tunneling, three-state crossings are formed when a chaotic singlet intersects a tunnel doublet. We study the dissipative quantum dynamics in the vicinity of such crossings. A harmonically driven double well coupled to a bath serves as a model. Markov and rotating-wave approximations are introduced with respect to the Floquet spectrum of the time-dependent central system. The resulting master equation is integrated numerically. We find various types of transient tunneling, determined by the relation of the level width to the inherent energy scal…
Coherent control of chaotic molecular systems, using laser-assisted alignment of sulphur dioxide (SO$_2$) molecules in the presence of a static electric field as an example, is considered. Conditions for which the classical version of this system is chaotic are established, and the quantum and classical analogs are shown to be in very good correspondence. It is found that the chaos present in the classical system does not impede the alignment, neither in the classical nor the quantum system. Using the results of numerical calculations, we suggest that laser-assisted alignment is stable against…
Mode-mode coupling theory is presented for the resonant pumping via dynamical tunneling processes in a deformed microcavity. From the steady-state solution of the coupled differential equations of chaotic modes and a high-Q regular mode, pumping efficiency is obtained as a function of pump detuning, coupling constants and decay rates of the involved modes. We show that the pump-excited chaotic modes as a whole can be regarded as a single pump mode with an effective decay rate and an effective coupling constant with the regular mode. We also show that the decay rate of the regular mode is enhan…
We theoretically study the effect of atomic nonlinearity on the tunneling time in the case of an atomic Bose-Einstein condensate (BEC) traversing the laser-induced potential barrier. The atomic nonlinearity is controlled to appear only in the region of the barrier by employing the Feshbach resonance technique to tune interatomic interaction in the tunneling process. Numerical simulation shows that the atomic nonlinear effect dramatically changes the tunneling behavior of the BEC matter wave packet, and results in the violation of Hartman effect and the occurrence of negative tunneling time.
Atoms, propagating across a detuned standing laser wave, can be scattered in a chaotic way even in the absence of spontaneous emission and any modulation of the laser field. Spontaneous emission masks the effect in some degree, but the Monte Carlo simulation shows that it can be observed in real experiments by the absorption imaging method or depositing atoms on a substrate. The effect of chaotic scattering is explained by a specific behavior of the dipole moments of atoms crossing the field nodes and is shown to depend strongly on the value of the atom-laser detuning.
We study the motion of a cold atom in a frequency-modulated standing laser wave. If the detuning between the atomic electronic transition and the field is large, the atom moves in a modulated optical potential demonstrating known classical nonlinear effects such as chaos and nonlinear resonances. If the atom-field detuning is small, then two optical potentials emerge in the system, and the atom performs Landau-Zener (LZ) tunnelings between them. It is a radically non-classical behavior. However, we show that classical nonlinear structures in system's phase space (KAM-tori and chaotic layers) s…
The ignition of Quantum Cascade Lasers can occur from a state of oscillating fie ld domains. Here, the interplay between lasing and the kinetics of traveling dom ain boundaries provides complex oscillation scenarios. We analyze our numerical findings in detail for a device operating at terahertz frequencies and manifest chaotic evolution by positive Lyapunov exponents. This shows that these importan t devices can exhibit chaotic behavior even without periodic driving, which need s to be taken into account in their design.
The Schwinger limit refers to longitudinal electric fields that are sufficiently strong to "polarize the vacuum" into electron-positron pairs by a tunneling mechanism. Laser fields are transverse electromagnetic fields for which the Schwinger limit has no relevance. Longitudinal and transverse fields are fundamentally different because of the different values of the F^{μν}F_{μν} Lorentz invariant that characterizes the fields. One aspect of this difference is the zero-frequency limit, that exists for longitudinal fields, but is ill-defined for transverse fields. The goal of approaching the Sch…
The photon statistics and bunching of a semiconductor laser with external optical feedback are investigated experimentally and theoretically. In a chaotic regime, the photon number distribution is measured and undergoes a transition from Bose-Einstein distribution to Poisson distribution with increasing the mean photon number. The second order degree of coherence decreases gradually from 2 to 1. Based on Hanbury Brown-Twiss scheme, pronounced photon bunching is observed experimentally for various injection currents and feedback strengths, which indicates the randomness of the associated emissi…
We present a detailed study of the gaussian laser propagation through a dielectric system composed by two right angle prisms. We investigate the transition between the spatial coherence limit, which exhibits wave-like properties and for which the resonance phenomenon can be seen, and the decoherence limit, which exhibits particle-like properties and for which the multiple diffusion occurs. We also analyze the tunneling at critical angles. In our numerical analysis, we shall use BK7 and Fused Silica prisms and a gaussian He-Ne laser with a wavelength of 632.8 nm and beam waists of 2 mm and 200 …
Radiation from a chaotic cavity filled with gain medium is considered. A set of coupled equations describing the photon density and the population of gain medium is proposed and solved. The spectral distribution and fluctuations of the radiation are found. The full noise is a result of a competition between positive correlations of photons with equal frequencies (due to stimulated emission and chaotic scattering) which increase fluctuations, and a suppression due to interaction with a gain medium which leads to negative correlations between photons. The latter effect is responsible for a prono…
The tunneling ionization of an electron from a p-state in a highly charged ion in the relativistic regime is investigated in a linearly polarized strong laser field. In contrast to the case of an s-state, the tunneling ionization from the p-state is spin asymmetric. We have singled out two reasons for the spin asymmetry: first, the difference of the electron energy Zeeman splitting in the bound state and during tunneling, and second, the relativistic momentum shift along the laser propagation direction during the under-the barrier motion. Due to the latter, those states are predominantly ioniz…
The second order photon correlation g^(2)(tau) of a chaotic optical-feedback semiconductor laser is precisely measured using a Hanbury Brown-Twiss interferometer. The accurate g^(2)(tau) with non-zero delay time is obtained experimentally from the photon pair time interval distribution through a ninth-order self-convolution correction. The experimental results agree well with the theoretical analysis. The relative error of g^(2)(tau) is no more than 0.005 within 50 ns delay time. The bunching effect and coherence time of the chaotic laser are measured via the precise photon correlation techniq…
The tunneling dynamics in relativistic strong-field ionization is investigated with the aim to develop an intuitive picture for the relativistic tunneling regime. We demonstrate that the tunneling picture applies also in the relativistic regime by introducing position dependent energy levels. The quantum dynamics in the classically forbidden region features two time scales, the typical time that characterizes the probability density's decay of the ionizing electron under the barrier (Keldysh time) and the time interval which the electron spends inside the barrier (Eisenbud-Wigner-Smith tunneli…
The tunneling model of ionization applies only to longitudinal fields: quasistatic electric fields that do not propagate. Laser fields are transverse: plane wave fields that possess the ability to propagate. Although there is an approximate connection between the effects of longitudinal and transverse fields in a useful range of frequencies, that equivalence fails completely at very low frequencies. Insight into this breakdown is given by an examination of radiation pressure, which is a unique transverse-field effect whose relative importance increases rapidly as the frequency declines. Radiat…
Classically allowed transport is shown to compete with quantum tunneling during the ionization of atoms by ultrashort and intense laser pulses, despite Keldysh parameters smaller than unity. This is done by comparing exact probability densities with the ones obtained from purely classical propagation using the Truncated Wigner Approximation. Not only is classical transport capable of moving trajectories away from the core, but it can also furnish ionization probabilities of the same order as the quantum ones for intensities currently employed in experiments. Our results have implications rangi…
We observe Wannier-Stark localization in curved photonic lattices, realized using arrays of evanescently coupled optical waveguides. By correctly tuning the strength of inter-site coupling in the lattice, we observe that Wannier-Stark states become increasingly localized, and eventually fully localized to one site, as the curvature of the lattice is increased. We then demonstrate that tunneling can be successfully restored in the lattice by applying a sinusoidal modulation to the lattice position, an effect that is a direct analogue of photon-assisted tunneling. This precise tuning of the tunn…
The electron dynamics in the classically forbidden region during relativistic tunnel-ionization is investigated. The classical forbidden region in the relativistic regime is identified by defining a gauge invariant total energy operator. Introducing position dependent energy levels inside the tunneling barrier, we demonstrate that the relativistic tunnel-ionization can be well described by a one-dimensional intuitive picture. This picture predicts that, in contrast to the well-known nonrelativistic regime, the ionized electron wave packet arises with a momentum shift along the laser's propagat…
Time-delay signature (TDS) suppression of semiconductor lasers with external optical feedback is necessary to ensure the security of chaos-based secure communications. Here we numerically and experimentally demonstrate a technique to effectively suppress the TDS of chaotic lasers using quantum noise. The TDS and dynamical complexity are quantified using the autocorrelation function and normalized permutation entropy at the feedback delay time, respectively. Quantum noise from quadrature fluctuations of vacuum state is prepared through balanced homodyne measurement. The effects of strength and …
A random-matrix theory is presented for the linewidth of a laser cavity in which the radiation is scattered chaotically. The linewidth is enhanced above the Schawlow-Townes value by the Petermann factor K, due to the non-orthogonality of the cavity modes. The factor K is expressed in terms of a non-Hermitian random matrix and its distribution is calculated exactly for the case that the cavity is coupled to the outside via a small opening. The average of K is found to depend non-analytically on the area of the opening, and to greatly exceed the most probable value.
Tunneling of a particle through a potential barrier remains one of the most remarkable quantum phenomena. Owing to advances in laser technology, electric fields comparable to those electrons experience in atoms are readily generated and open opportunities to dynamically investigate the process of electron tunneling through the potential barrier formed by the superposition of both laser and atomic fields. Attosecond-time and angstrom-space resolution of the strong laser-field technique allow to address fundamental questions related to tunneling, which are still open and debated: Which time is s…
Tunneling ionization of an atom in ultrashort laser pulses is considered. When the driving laser pulse is switched-on and -off with a steep slope, the photoelectron momentum distribution (PMD) shows an edge-effect because of the photoelectron diffraction by the time-slit of the pulse. The trivial diffraction pattern of the edge effect consisting of fast oscillations in the PMD disguises in the deep nonadiabatic regime the physically more interesting features in the spectrum which originate from the photoelectron dynamics. We point out the precise conditions how to avoid this scenario experimen…
We present a novel experimental technique that can differentiate unequivocally between chaotic light and coherent light with amplitude fluctuations, and thus permits to characterize unambiguously the output of a laser. This technique consists of measuring the second-order intensity cross-correlation at the outputs of an unbalanced Michelson interferometer. It is applied to a chaotic light source and to the output of a semiconductor nanolaser whose "standard" intensity correlation function above-threshold displays values compatible with a mixture of coherent and chaotic light. Our experimental …
Tunneling between two classically disconnected regular regions can be strongly affected by the presence of a chaotic sea in between. This phenomenon, known as chaos-assisted tunneling, gives rise to large fluctuations of the tunneling rate. Here we study chaos-assisted tunneling in the presence of Anderson localization effects in the chaotic sea. Our results show that the standard tunneling rate distribution is strongly modified by localization, going from the known Cauchy distribution in the ergodic regime to a log-normal distribution in the strongly localized case. We develop an analytical s…
We investigate the liberation of an atomic electron by a linearly polarized single-cycle near-infrared laser pulse having a peak intensity that ensures tunneling. Based on phase space analysis and energy distribution in the instantaneous potential, we reveal the importance of quantum interference between tunneling and over-the-barrier pathways of escape. Tunneling is blurred both in space and time, and the contribution of tunneling at the mean energy is almost negligible. We suggest and justify improved initial conditions for a classical particle approximation of strong-field ionization, based…
Photo-induced transition probabilities in graphene are studied theoretically from the viewpoint of Floquet theory. Conduction band populations are computed for a strongly, periodically driven graphene sheet under linear, circular, and elliptic polarization. Features of the momentum spectrum of excited quasi-particles can be directly related to the avoided crossing of the Floquet quasi-energy levels. In particular, the impact of the ellipticity and the strength of the laser excitation on the avoided crossing structure -- and on the resulting transition probabilities -- is studied. It is shown t…
We report temperature-dependent current-voltage (I - V - T) and output light power-voltage or current (P - V - T) or (P - I - T) characteristics of 1550 nm tunneling injection quantum dot (TI QD) laser diodes. Experimental data is accompanied by physical models that distinguish between different current flow and light emission mechanisms for different applied voltages and temperature ranges. Three exponential regimes in the I - V characteristics were identified for low bias levels where no optical radiation takes place. At the lowest bias levels, the diffusion-recombination mechanism based on …
Group-theoretical approach is applied to study behavior of lossless two-level atoms in a standing-wave laser field. Due to the recoil effect, the internal and external atomic degrees of freedom become coupled. The internal dynamics is described quantum mechanically in terms of the SU(2) group parameters. The evolution operator is found in an explicit way after solving a single ODE for one of the group parameters. The translational motion in a standing wave is governed by the classical Hamilton equations which are coupled to the SU(2) group equations. It is shown that the full set of equations …
We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The net photoionization undergoes an optimal enhancement when a broadband chaotic field is added to the weak laser pulse. The enhanced ionization is analyzed using time-resolved wavepacket evolution and the population dynamics of the atomic levels. We elucidate the enhancement produced by spectrally-shaped chaotic fields of two different classes, one with a tuna…
