We derive the photocount statistics of the radiation emitted from a chaotic laser resonator in the regime of single-mode lasing. Random spatial variations of the resonator eigenfunctions lead to strong mode-to-mode fluctuations of the laser emission. The distribution of the mean photocount over an ensemble of modes changes qualitatively at the lasing transition, and displays up to three peaks above the lasing threshold.
A general relationship is presented between the statistics of thermal radiation from a random medium and its scattering matrix S. Familiar results for black-body radiation are recovered in the limit S to 0. The mean photocount is proportional to the trace of 1-SS^dagger, in accordance with Kirchhoff's law relating emissivity and absorptivity. Higher moments of the photocount distribution are related to traces of powers of 1-SS^dagger, a generalization of Kirchhoff's law. The theory can be applied to a random amplifying medium (or "random laser") below the laser threshold, by evaluating the Bos…
Highly degenerate chaotic radiation has a Gaussian density matrix and a large occupation number of modes $f $. If it is passed through a weakly transmitting barrier, its counting statistics is close to Poissonian. We show that a second identical barrier, in series with the first, drastically modifies the statistics. The variance of the photocount is increased above the mean by a factor $f$ times a numerical coefficient. The photocount distribution reaches a limiting form with a Gaussian body and highly asymmetric tails. These are general consequences of the combination of weak transmission and…
We study fluctuations of the number of photocounts measured by an ideal photodetector illuminated by light scattered in an amplifying disordered medium, below the threshold for random lasing. We show that the variance of fluctuations and their correlation function carry information about fluctuating properties of the medium. A direct link is established between the fluctuations of the number of photocounts due to the amplified spontaneous emission (ASE) and the dimensionless conductance g of the medium. Our results suggest a possibility of probing amplifying disordered media by analyzing stati…
We compute the statistics of thermal emission from systems in which the radiation is scattered chaotically, by relating the photocount distribution to the scattering matrix - whose statistical properties are known from random-matrix theory. We find that the super-Poissonian noise is that of a black body with a reduced number of degrees of freedom. The general theory is applied to a disordered slab and to a chaotic cavity, and is extended to include amplifying as well as absorbing systems. We predict an excess noise of amplified spontaneous emission in a random laser below the laser threshold.
Radiation from a chaotic cavity filled with gain medium is considered. A set of coupled equations describing the photon density and the population of gain medium is proposed and solved. The spectral distribution and fluctuations of the radiation are found. The full noise is a result of a competition between positive correlations of photons with equal frequencies (due to stimulated emission and chaotic scattering) which increase fluctuations, and a suppression due to interaction with a gain medium which leads to negative correlations between photons. The latter effect is responsible for a prono…
Coherent control of chaotic molecular systems, using laser-assisted alignment of sulphur dioxide (SO$_2$) molecules in the presence of a static electric field as an example, is considered. Conditions for which the classical version of this system is chaotic are established, and the quantum and classical analogs are shown to be in very good correspondence. It is found that the chaos present in the classical system does not impede the alignment, neither in the classical nor the quantum system. Using the results of numerical calculations, we suggest that laser-assisted alignment is stable against…
A random-matrix theory is presented for the linewidth of a laser cavity in which the radiation is scattered chaotically. The linewidth is enhanced above the Schawlow-Townes value by the Petermann factor K, due to the non-orthogonality of the cavity modes. The factor K is expressed in terms of a non-Hermitian random matrix and its distribution is calculated exactly for the case that the cavity is coupled to the outside via a small opening. The average of K is found to depend non-analytically on the area of the opening, and to greatly exceed the most probable value.
Atoms, propagating across a detuned standing laser wave, can be scattered in a chaotic way even in the absence of spontaneous emission and any modulation of the laser field. Spontaneous emission masks the effect in some degree, but the Monte Carlo simulation shows that it can be observed in real experiments by the absorption imaging method or depositing atoms on a substrate. The effect of chaotic scattering is explained by a specific behavior of the dipole moments of atoms crossing the field nodes and is shown to depend strongly on the value of the atom-laser detuning.
We study the driven tunneling of a one-dimensional charged particle confined to a rectangular double-well. The numerical simulation of the Schrödinger equation based on the Cranck-Nicholson finite-difference scheme, shows that the modulation of the amplitude of the external field may result in the parametric resonance. The latter is accompanied by the breakdown of the quasi-periodic motion characteristic of the usual driven tunneling, and the emergence of an irregular dynamics. We describe the above breakdown with the occupation probability for the ground state of the unperturbed system, and m…
The ignition of Quantum Cascade Lasers can occur from a state of oscillating fie ld domains. Here, the interplay between lasing and the kinetics of traveling dom ain boundaries provides complex oscillation scenarios. We analyze our numerical findings in detail for a device operating at terahertz frequencies and manifest chaotic evolution by positive Lyapunov exponents. This shows that these importan t devices can exhibit chaotic behavior even without periodic driving, which need s to be taken into account in their design.
The second order photon correlation g^(2)(tau) of a chaotic optical-feedback semiconductor laser is precisely measured using a Hanbury Brown-Twiss interferometer. The accurate g^(2)(tau) with non-zero delay time is obtained experimentally from the photon pair time interval distribution through a ninth-order self-convolution correction. The experimental results agree well with the theoretical analysis. The relative error of g^(2)(tau) is no more than 0.005 within 50 ns delay time. The bunching effect and coherence time of the chaotic laser are measured via the precise photon correlation techniq…
The photon statistics and bunching of a semiconductor laser with external optical feedback are investigated experimentally and theoretically. In a chaotic regime, the photon number distribution is measured and undergoes a transition from Bose-Einstein distribution to Poisson distribution with increasing the mean photon number. The second order degree of coherence decreases gradually from 2 to 1. Based on Hanbury Brown-Twiss scheme, pronounced photon bunching is observed experimentally for various injection currents and feedback strengths, which indicates the randomness of the associated emissi…
A theory for the photon statistics of a random laser is presented. Noise is described by Langevin operators, where both fluctuations of the electromagnetic field and of the medium are included. The theory is valid for all lasers with small outcoupling when the laser cavity is large compared to the wavelength of the radiation. The theory is applied to a chaotic laser cavity with a small opening. It is known that a large number of modes can be above threshold simultaneously in such a cavity. It is shown the amount of fluctuations is increased compared to the Poissonian value by an amount that de…
Time-delay signature (TDS) suppression of semiconductor lasers with external optical feedback is necessary to ensure the security of chaos-based secure communications. Here we numerically and experimentally demonstrate a technique to effectively suppress the TDS of chaotic lasers using quantum noise. The TDS and dynamical complexity are quantified using the autocorrelation function and normalized permutation entropy at the feedback delay time, respectively. Quantum noise from quadrature fluctuations of vacuum state is prepared through balanced homodyne measurement. The effects of strength and …
We present a novel experimental technique that can differentiate unequivocally between chaotic light and coherent light with amplitude fluctuations, and thus permits to characterize unambiguously the output of a laser. This technique consists of measuring the second-order intensity cross-correlation at the outputs of an unbalanced Michelson interferometer. It is applied to a chaotic light source and to the output of a semiconductor nanolaser whose "standard" intensity correlation function above-threshold displays values compatible with a mixture of coherent and chaotic light. Our experimental …
Group-theoretical approach is applied to study behavior of lossless two-level atoms in a standing-wave laser field. Due to the recoil effect, the internal and external atomic degrees of freedom become coupled. The internal dynamics is described quantum mechanically in terms of the SU(2) group parameters. The evolution operator is found in an explicit way after solving a single ODE for one of the group parameters. The translational motion in a standing wave is governed by the classical Hamilton equations which are coupled to the SU(2) group equations. It is shown that the full set of equations …
We study dissipative transport of spontaneously emitting atoms in a 1D standing-wave laser field in the regimes where the underlying deterministic Hamiltonian dynamics is regular and chaotic. A Monte Carlo stochastic wavefunction method is applied to simulate semiclassically the atomic dynamics with coupled internal and translational degrees of freedom. It is shown in numerical experiments and confirmed analytically that chaotic atomic transport can take the form either of ballistic motion or a random walking with specific statistical properties. The character of spatial and momentum diffusion…
Coherent motion of cold atoms in a standing-wave field is interpreted as a propagation in two optical potentials. It is shown that the wave-packet dynamics can be either regular or chaotic with transitions between these potentials after passing field nodes. Manifestations of de Broglie-wave chaos are found in the behavior of the momentum and position probabilities and the Wigner function. The probability of those transitions depends on the ratio of the squared detuning to the Doppler shift and is large in that range of the parameters where the classical motion is shown to be chaotic.
We investigate the influence of the photon statistics on the excitation dynamics of a single two level system. A single semiconductor quantum dot represents the two level system and is resonantly excited either with coherent laser light, or excited with chaotic light, with photon statistics corresponding to that of thermal radiation. Experimentally, we observe a reduced absorption cross-section under chaotic excitation in the steady-state. In the transient regime, the Rabi oscillations observable under coherent excitation disappear under chaotic excitation. Likewise, in the emission spectrum t…
The qualitative nature (i.e. integrable vs. chaotic) of the translational dynamics of a three-level atom in an optical lattice is shown to be controllable by varying the relative laser phase of two standing wave lasers. Control is explained in terms of the nonadiabatic transition between optical potentials and the corresponding regular to chaotic transition in mixed classical-quantum dynamics. The results are of interest to both areas of coherent control and quantum chaos.
We demonstrate experimentally a new form of induced transparency, i.e., chaos-induced transparency, in a slightly deformed microcavity which support both continuous chaotic modes and discrete regular modes with Q factors exceeding 3X?10^7. When excited by a focused laser beam, the induced transparency in the transmission spectrum originates from the destructive interference of two parallel optical pathways: (i) directly refractive excitation of the chaotic modes, and (ii) excitation of the ultra-high-Q regular mode via chaos-assisted dynamical tunneling mechanism coupling back to the chaotic m…
Dielectric resonators are open systems particularly interesting due to their wide range of applications in optics and photonics. In a recent paper [PRE, vol. 78, 056202 (2008)] the trace formula for both the smooth and the oscillating parts of the resonance density was proposed and checked for the circular cavity. The present paper deals with numerous shapes which would be integrable (square, rectangle, and ellipse), pseudo-integrable (pentagon) and chaotic (stadium), if the cavities were closed (billiard case). A good agreement is found between the theoretical predictions, the numerical simul…
