The evolution of a Raman coupled three-level lambda atom with two quantized cavity modes is studied in the large detuning case; i.e. when the upper atomic level can be adiabatically eliminated. Particularly the situation when the two modes are prepared in initial coherent or squeezed states, with a large average number of photons, is investigated. It is found that the atom, after specific interaction times, disentangles from the two modes, leaving them, in certain cases, in entangled Schrodinger cat states. These disentanglement times can be controlled by adjusting the ratio between average numbers of photons in the two modes. It is also shown how this effective model may be used for implementing quantum information processing. Especially it is demonstrated how to generate various entangled states, such as EPR- and GHZ-states, and quantum logic operations, such as the control-not and the phase-gate.
Quantum entanglement of particles is regarded as a fundamental character in quantum information, in which quantum state should be given for whole system instead of independently describing single particle. Constructing quantum memory of photonic entanglement is essential for realizing quantum networks, which had been performed previously by many memory protocols. Of which Raman quantum memory gives advantages in broadband and high-speed properties, resulting in huge potential in quantum network and quantum computation. However, Raman quantum memory of photonic polarised entanglement is a chall…
The dynamics of a cascaded system that consists of two atom-cavity subsystems is studied by using the quantum trajectory method. Considering the two atom-cavity subsystems driven by a Raman interaction, analytical solutions are obtained. Subsequently, the entanglement evolution between the two atoms is studied, and it is shown that the entanglement can be stored by switching off the Raman coupling. By monitoring the radiation field, the entanglement between the two atoms can be enhanced.
We examine the theoretical limits of the generation of entanglement in a damped coupled ion-cavity system using jump-based feedback. Using Raman transitions to produce entanglement between ground states reduces the necessary feedback bandwidth, but does not improve the overall effect of the spontaneous emission on the final entanglement. We find that the fidelity of the resulting entanglement will be limited by the asymmetries produced by vibrations in the trap, but that the concurrence remains above 0.88 for realistic ion trap sizes.
The existence of higher order entanglement in the stimulated and spontaneous Raman processes is established using the perturbative solutions of the Heisenberg equations of motion for various field modes that are obtained using the Sen-Mandal technique and a fully quantum mechanical Hamiltonian that describes the stimulated and spontaneous Raman processes. Specifically, the perturbative Sen-Mandal solutions are exploited here to show the signature of the higher order two-mode and multi-mode entanglement. In some special cases, we have also observed higher order entanglement in the partially spo…
We propose a scheme of generating and verifying mesoscopic-level entanglement between two atomic ensembles using non-resonant stimulated Raman scattering. Entanglement can be generated by direct detection or balanced homodyne detection of the Stokes fields from the two cells, after they interfere on a beam splitter. The entanglement of the collective atomic fields can be transferred to the anti-Stokes fields in a readout process. By measuring the operator moments of the anti-Stokes fields, we can verify the presence of entanglement. We model the effects of practical factors such as Stokes fiel…
It has now been possible to prepare chain of ions in an entangled state and thus question arises --- how the optical properties of a chain of entangled ions differ from say a chain of independent particles. We investigate nonlinear optical processes in such chains. We explicitly demonstrate the possibility of entanglement produced super Raman scattering. Our results in contrast to Dicke's work on superradiance are applicable to stimulated processes and are thus free from the standard complications of multimode quantum electrodynamics. Our results suggest the possibility of similar enhancement …
We address an experimental scheme to analyze the optical bistability and the entanglement of two movable mirrors coupled to a two-mode laser inside a doubly resonant cavity. With this aim we investigate the master equations of the atom-cavity subsystem in conjunction with the quantum Langevin equations that describe the interaction of the mirror cavity. The parametric amplification-type coupling induced by the two-photon coherence on the optical bistability of the intracavity mean photon numbers is found and investigated. Under this condition, the optical intensities exhibit bistability for al…
Making use of the Rydberg blockade, we generate entanglement between two atoms individually trapped in two optical tweezers. In this paper we detail the analysis of the data and show that we can determine the amount of entanglement between the atoms in the presence of atom losses during the entangling sequence. Our model takes into account states outside the qubit basis and allows us to perform a partial reconstruction of the density matrix describing the two atom state. With this method we extract the amount of entanglement between pairs of atoms still trapped after the entangling sequence an…
We discuss theoretically quantum interface between light and a spin polarized ensemble of atoms with the spin >= 1 based on an off-resonant Raman scattering. We present the spectral theory of the light-atoms interaction and show how particular spectral modes of quantum light couple to spatial modes of the extended atomic ensemble. We show how this interaction can be used for quantum memory storage and retrieval and for deterministic entanglement protocols. The proposed protocols are attractive due to their simplicity since they involve just a single pass of light through atoms without the need…
The operator solution of a completely quantum mechanical Hamiltonian of the Raman processes is used here to investigate the possibility of obtaining intermodal entanglement between different modes involved in the Raman processes (e.g. pump mode, Stokes mode, vibration (phonon) mode and anti-Stokes mode). Intermodal entanglement is reported between a) pump mode and anti-Stokes mode, b) pump mode and vibration (phonon) mode c) Stokes mode and vibration phonon mode, d) Stokes mode and anti-stokes mode in the stimulated Raman processes for the variation of the phase angle of complex eigenvalue $α_…
We show that an absolute coherent phase of a laser can be used to manipulate the entanglement of photon pairs of two-photon laser. Our focus is on the generation of a continuous source of entangled photon pairs in the double $Λ$ (or Raman) scheme. We study the dependence of steady state entanglement on the phase and laser parameters. We obtain a relationship between entanglement and two-photon correlation. We derive conditions that give steady state entanglement for the Raman-EIT scheme and use it to identify region of steady state macroscopic entanglement. No entanglement is found for the dou…
We introduce a scheme for creating continuous variable entanglement between an atomic beam and an optical field, by using squeezed light to outcouple atoms from a BEC via a Raman transition. We model the full multimode dynamics of the atom laser beam and the squeezed optical field, and show that with appropriate two-photon detuning and two-photon Rabi frequency, the transmitted light is entangled in amplitude and phase with the outcoupled atom laser beam. The degree of entanglement is controllable via changes in the two-photon Rabi frequency of the outcoupling process.
Entanglement and Optical Nonreciprocity in spontaneous Raman Scattering
Max Planck Institute for the Structure and Dynamics of Matter（马克斯·普朗克物质结构与动力学研究所）；University of Hamburg（汉堡大学）；The Hamburg Centre for Ultrafast Imaging（汉堡超快成像中心）
A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes are coherent) and chaotic scattering (where initial phonon mode is chaotic and all the other modes are coherent) are studied. Nonclassical character of Raman process is observed by means of intermodal entanglement, single mode and intermodal squeezing of vacuum fluctuations, sub-shot noise and wave variances. Joint photon-phonon number and integrated-intensi…
We analyze quantum entanglement of Stokes light and atomic electronic polarization excited during single-pass, linear-regime, stimulated Raman scattering in terms of optical wave-packet modes and atomic-ensemble spatial modes. The output of this process is confirmed to be decomposable into multiple discrete, bosonic mode pairs, each pair undergoing independent evolution into a two-mode squeezed state. For this we extend the Bloch-Messiah reduction theorem, previously known for discrete linear systems (S. L. Braunstein, Phys. Rev. A, vol. 71, 055801 (2005)). We present typical mode functions in…
In this article, non-classical properties of Raman modes are investigated. The original goal, actually, is to identify how and by which method we can induce non-classicality in Raman modes. We introduce a plasmonic system in which Raman dye molecules are buried between two shells of the plasmonic materials similar to onion-like core/shell nanoparticle. This system is excited by the entangled photons, followed by analyzing its dynamics of motion using the Heisenberg-Langevin equations by which the time evolution of the signal-idler mode and Raman modes are derived. Interestingly, the entangled …
We introduce and study the concept of a reversible transfer of the quantum state of two internally-translationally entangled fragments, formed by molecular dissociation, to a photon pair. The transfer is based on intracavity stimulated Raman adiabatic passage and it requires a combination of processes whose principles are well established.
We investigate the steady-state photon-number squeezing and quantum entanglement in a network of nondegenerate optical parametric oscillators (NOPOs). We treat each NOPO with Shen's Raman laser model, whose lasing mode provides a photon-number-squeezed state. Two dissipatively coupled NOPOs satisfy Hillery-Zubairy's $HZ1$ entanglement criterion if they are pumped far above the threshold and the dissipative coupling is sufficiently larger than the NOPO cavity loss.
We propose a direct, coherent coupling scheme that can create massively entangled states of Bose-Einstein condensed atoms. Our idea is based on an effective interaction between two atoms from coherent Raman processes through a (two atom) molecular intermediate state. We compare our scheme with other recent proposals for generation of massive entanglement of Bose condensed atoms.
We present a scheme to realise the basic two-quibit logic gates such as quantum phase gate and controlle-NOT gate using a detuned optical cavity interacting with a three-level Raman system. We discuss the role of Stark shifts which are as important as the terms leading to two-photon transition. The operation of the proposed logic gates involves metastable states of the atom and hence is not affected by spontaneous emission. These ideas can be extended to produce multiparticle entanglement.
Phase-locking governs the phase noise in classical clocks through effects described in precise mathematical terms. We seek here a quantum counterpart of these effects by working in a finite Hilbert space. We use a coprimality condition to define phase-locked quantum states and the corresponding Pegg-Barnett type phase operator. Cyclotomic symmetries in matrix elements are revealed and related to Ramanujan sums in the theory of prime numbers. The employed mathematical procedures also emphasize the isomorphism between algebraic number theory and the theory of quantum entanglement
In spontaneous Raman process in atomic cell at high gain, both the Stokes field and the accompanying collective atomic excitation (atomic spin wave) are coherent. We find that, due to the spontaneous nature of the process, the phases of the Stokes field and the atomic spin wave change randomly from one realization to another but are anti-correlated. The phases of the atomic ensembles are read out via another Raman process at a later time, thus realizing phase memory in atoms. The observation of phase correlation between the Stokes field and the collective atomic excitations is an important ste…
A perturbative analytic operator solution of a completely quantum mechanical Hamiltonian of multi-photon pump non-degenerate hyper-Raman process is obtained. It is shown that the obtained solution is general in nature as the solutions of non-degenerate hyper-Raman and stimulated Raman processes can be obtained as special cases of the present solution. The analytic solutions obtained here are used to investigate the nonclassical properties of the different modes in the stimulated, spontaneous and partially spontaneous multi-photon pump non-degenerate hyper-Raman processes. The nonclassical natu…
We propose a new avenue towards distillation of quantum entanglement that is implemented by directly passing the entangled qubits through a mode-matched filter. This approach can be applied to a common class of entanglement impurities appearing in photonic systems where the impurities inherently occupy different spatiotemporal modes than the entangled qubits. As a specific application, we show that our method can be used to significantly purify the telecom-band entanglement generated via the Kerr nonlinearity in single-mode fibers where a substantial amount of Raman-scattering noise is concomi…
We propose a scheme employing quantum-reservoir engineering to controllably entangle the internal states of two atoms trapped in a high finesse optical cavity. Using laser and cavity fields to drive two separate Raman transitions between metastable atomic ground states, a system is realized corresponding to a pair of two-state atoms coupled collectively to a squeezed reservoir. Phase-sensitive reservoir correlations lead to entanglement between the atoms, and, via local unitary transformations and adjustment of the degree and purity of squeezing, one can prepare entangled mixed states with any…
We demonstrate a novel way to efficiently and very robust create an entanglement between an atomic and a photonic qubit. A single laser beam is used to excite one atomic ensemble and two different spatial modes of scattered Raman fields are collected to generate the atom-photon entanglement. With the help of build-in quantum memory, the entanglement still exists after 20.5 $μ$s storage time which is further proved by the violation of CHSH type Bell's inequality. Our entanglement procedure is the building block for a novel robust quantum repeater architecture [Zhao et al, Phys. Rev. Lett. 98, 2…
Large-scale quantum information processing networks will most probably require the entanglement of distant systems that do not interact directly. This can be done by performing entangling gates between standing information carriers, used as memories or local computational resources, and flying ones, acting as quantum buses. We report the deterministic entanglement of two remote transmon qubits by Raman stimulated emission and absorption of a traveling photon wavepacket. We achieve a Bell state fidelity of 73 %, well explained by losses in the transmission line and decoherence of each qubit.
We present a quantum electrodynamical model involving nitrogen-vacancy centers coupled to a whispering-gallery mode cavity. Two schemes are considered to create W state and Bell state, respectively. One of the schemes makes use of the Raman transition with the cavity field virtually excited; The other enables the Bell state preparation and quantum information transfer by virtue of dark state evolution and adiabatic passage, which is tolerant to ambient noise and experimental parameter fluctuations. We justify our schemes by considering the experimental feasibility and challenge using currently…
Entanglement is at the core of quantum information processing and may prove essential for quantum speed-up. Inspired by both theoretical and experimental studies of spin-momentum coupling in systems of ultra-cold atoms, we investigate the entanglement between the spin and momentum degrees of freedom of an optically trapped BEC of $^{87}$Rb atoms. We consider entanglement that arises due to the coupling of these degrees of freedom induced by Raman and radio-frequency fields and examine its dependence on the coupling parameters by evaluating von Neumann entropy as well as concurrence as measures…
We study the effects of arbitrary laser pulse excitations on quantum correlation, entanglement and the role of quantum noise. The transient quantities are computed exactly using a method that provides exact solutions of the Langevin field operators for photon pairs produced by a double Raman atom driven by laser pulses. Short pulses with appropriate chirping, delay and/or detuning can generate broadband photon pairs and yield results that provide insights on how to generate very large nonclassical correlation. We find that short pulses are not favorable for entanglement. The quantity was previ…
Quantum entanglement between distant qubits is an important feature of quantum networks. Distribution of entanglement over long distances can be enabled through coherently interfacing qubit pairs via photonic channels. Here, we report the realization of optically generated quantum entanglement between electron spin qubits confined in two distant semiconductor quantum dots. The protocol relies on spin-photon entanglement in the trionic $Λ$-system and quantum erasure of the Raman-photon path. The measurement of a single Raman photon is used to project the spin qubits into a joint quantum state w…
We report the generation of entanglement between two individual $^{87}$Rb atoms in hyperfine ground states $|F=1,M=1>$ and $|F=2,M=2>$ which are held in two optical tweezers separated by 4 $μ$m. Our scheme relies on the Rydberg blockade effect which prevents the simultaneous excitation of the two atoms to a Rydberg state. The entangled state is generated in about 200 ns using pulsed two-photon excitation. We quantify the entanglement by applying global Raman rotations on both atoms. We measure that 61% of the initial pairs of atoms are still present at the end of the entangling sequence. These…
We discuss a technique and a material system that enable the controlled realization of quantum entanglement between spin-wave modes of electron ensembles in two spatially separated pieces of semiconductor material. The approach uses electron ensembles in GaAs quantum wells that are located inside optical waveguides. Bringing the electron ensembles in a quantum Hall state gives selection rules for optical transitions across the gap that can selectively address the two electron spin states. Long-lived superpositions of these electron spin states can then be controlled with a pair of optical fiel…
We present a study of the quantum properties of two light fields used to parametric four-wave mixing in a Raman-type atomic system. The system realizes an effective Hamiltonian of beamsplitter type coupling between the light fields, which allows to control squeezing and amplitude distribution of the light fields, as well as realizing their entanglement. The scheme can be feasibly applied to engineer the quantum properties of two single-mode light fields in properly chosen input states.
We propose a method for quantum state transfer from one atom laser beam to another via an intermediate optical field, using Raman incoupling and outcoupling techniques. Our proposal utilises existing experimental technologies to teleport macroscopic matter waves over potentially large distances without shared entanglement.
Recently, a new method, which can significantly speed up adiabatic quantum state transfer by using dressed states, was proposed by Baksic \emph{et~al.} [Phys. Rev. Lett. \textbf{116}, 230503 (2016)]. Assisted by quantum Zeno dynamics, we develop this dressed-state method to achieve shortcuts to complete and fractional stimulated Raman adiabatic passage for speeding up adiabatic two-atom quantum state transfer and maximum entanglement generation, respectively. By means of some numerical simulations, we determine the parameters used in the scheme which can guarantee the feasibility and efficienc…
Entanglement between a single photon and a matter qubit is an indispensable resource for quantum repeater and quantum networks. With atomic ensembles, the entanglement creation probability is typically very low to inhibit high-order events. In this paper, we propose and experimentally realize a scheme which creates atom-photon entanglement with an intrinsic efficiency of 50%. We make use of Rydberg blockade to generate two collective excitations, lying in separate internal states. By introducing the momentum degree of freedom for the excitations, and interfering them via Raman coupling, we ent…
We propose a robust deterministic scheme to generate entanglement at high fidelity without the need of photodetectors even for quantum bits, qubits, with extremely poor optically active states. Our protocol employs stimulated Raman adiabatic passage for population transfer without actually exciting the system. Furthermore, it is found to be effective even if the environmental decoherence rate is of the same order of magnitude as the atom--photon coupling frequency. Our scheme holds potential to solve entanglement generation problems, e.g., in distributed quantum computing.
We propose using spontaneous Raman scattering from an optically driven Bose-Einstein condensate as a source of atom-photon pairs whose internal states are maximally entangled. Generating entanglement between a particle which is easily transmitted (the photon) and one which is easily trapped and coherently manipulated (an ultracold atom) will prove useful for a variety of quantum-information related applications. We analyze the type of entangled states generated by spontaneous Raman scattering and construct a geometry which results in maximum entanglement.
Universidade Federal de São Carlos（圣卡洛斯联邦大学）；Institute for Quantum Optics and Quantum Information, Austrian Academy of Sciences（奥地利科学院量子光学与量子信息研究所）；Stockholm University（斯德哥尔摩大学）；California Institute of Technology（加州理工学院）；Université Côte d’Azur（蔚蓝海岸大学）；CNRS, Institut de Physique de Nice（法国国家科学研究中心尼斯物理研究所）
We propose a scheme to dissipatively produce steady-state entanglement in a two-qubit system, via an interaction with a bosonic mode. The system is driven into a stationary entangled state, while we compensate the mode dissipation by injecting energy via a coherent pump field. We also present a scheme which allows us to adiabatically transfer all the population to the desired entangled state. The dynamics leading to the entangled state in these schemes can be understood in analogy with electromagnetically induced transparency (EIT) and stimulated Raman adiabatic passage (STIRAP), respectively.
We propose a mechanism of ground-state blockade between two $N$-type Rydberg atoms in virtue of Rydberg-antiblockade effect and Raman transition. Inspired by the quantum Zeno effect, the strong Rydberg antiblockade interaction plays a role in frequently measuring one ground state of two, leading to a blockade effect for double occupation of the corresponding quantum state. By encoding the logic qubits into the ground states, we efficiently avoid the spontaneous emission of the excited Rydberg state, and maintain the nonlinear Rydberg-Rydberg interaction at the same time. As applications, we di…
Raman process is used for generation of nonclassical states and subsequent applications due to its simplicity. In view of the experimental feasibility of the off-resonant Raman process at single photon level useful in long distance quantum communication and quantum memory, we perform here a detailed study of possibility of generation of nonclassical states under off-resonance conditions. Specifically, we have studied nonclassicality in the off-resonant Raman process with the help of a characteristic function written using more general solution than the conventional short-time solution under co…
We show how one can prepare three-qubit entangled states like W states, Greenberger-Horne-Zeilinger states as well as two-qutrit entangled states using the multiatom two-mode entanglement. We propose a technique of preparing such a multi-particle entanglement using stimulated Raman adiabatic passage. We consider a collection of three-level atoms in $Λ$ configuration simultaneously interacting with a resonant two-mode cavity for this purpose. Our approach permits a variety of multiparticle extensions.
Solid state quantum emitters have shown strong potential for applications in quantum information, but spectral inhomogeneity of these emitters poses a significant challenge. We address this issue in a cavity-quantum dot system by demonstrating cavity-stimulated Raman spin flip emission. This process avoids populating the excited state of the emitter and generates a photon that is Raman shifted from the laser and enhanced by the cavity. The emission is spectrally narrow and tunable over a range of at least 125 GHz, which is two orders of magnitude greater than the natural linewidth. We obtain t…
The sources, which generate atom-photon quantum correlations or entanglement based on quantum memory, are basic blocks for building quantum repeaters (QRs). For achieving highly entanglement-generation rates in ensemble-based QRs, spatial-, temporal- and spectral-multimode memories are needed. The previous temporal-multimode memories are based on rephrasing mechanisms in inhomogeneous-broadened media. Here, by applying a train of multi-direction write pulses into a homogeneous-broadened atomic ensemble to induce Duan-Lukin-Cirac-Zoller-like Raman processes, we prepare up to 19 pairs of modes, …
It was shown in [T. Morimae, Phys. Rev. A {\bf81}, 060307(R) (2010)] that the gate fidelity of an inaccurate one-way quantum computation is upper bounded by a decreasing function of the amount of entanglement in the register. This means that a strong entanglement causes the low gate fidelity in the one-way quantum computation with inaccurate measurements. In this paper, we derive similar entanglement-fidelity relations for the inaccurate ancilla-driven quantum computation. These relations again imply that a strong entanglement in the register causes the low gate fidelity in the ancilla-driven …
We argue that entanglement is the essential non-classical ingredient which provides the computational speed-up in quantum algorithms as compared to algorithms based on the processes of classical physics.
Adiabatic quantum computation provides an alternative approach to quantum computation using a time-dependent Hamiltonian. The time evolution of entanglement during the adiabatic quantum search algorithm is studied, and its relevance as a resource is discussed.
We show that universal quantum computation can be achieved in the standard pure-state circuit model while, at any time, the entanglement entropy of all bipartitions is small---even tending to zero with growing system size. The result is obtained by showing that a quantum computer operating within a small region around the set of unentangled states still has universal computational power, and by using continuity of entanglement entropy. In fact an analogous conclusion applies to every entanglement measure which is continuous in a certain natural sense, which amounts to a large class. Other exam…
We present a scheme to realize a deterministic solid state source of time-bin entangled photon pairs using cavity-assisted stimulated Raman adiabatic passage (STIRAP) in a single quantum dot. The quantum dot is embedded inside a semiconductor cavity, and the interaction of a coherent superposition of two temporally separated input pulses and the cavity mode leads to a two-photon Raman transition, which produces a time-bin entangled photon pair through the biexciton-exciton cascade. We show that the entanglement of the generated state can be measured using triple coincidence detection, and the …
Efficient interfaces between photons and quantum emitters form the basis for quantum networks and enable nonlinear optical devices operating at the single-photon level. We demonstrate an integrated platform for scalable quantum nanophotonics based on silicon-vacancy (SiV) color centers coupled to nanoscale diamond devices. By placing SiV centers inside diamond photonic crystal cavities, we realize a quantum-optical switch controlled by a single color center. We control the switch using SiV metastable orbital states and verify optical switching at the single-photon level by using photon correla…
