The dynamics of a cascaded system that consists of two atom-cavity subsystems is studied by using the quantum trajectory method. Considering the two atom-cavity subsystems driven by a Raman interaction, analytical solutions are obtained. Subsequently, the entanglement evolution between the two atoms is studied, and it is shown that the entanglement can be stored by switching off the Raman coupling. By monitoring the radiation field, the entanglement between the two atoms can be enhanced.
We theoretically show that bright six-partite continuous-variable entanglement can be generated using cascaded four-wave mixing effects of third-order nonlinearity atomic systems above threshold. The six-partite continuous-variable entanglement among the six cavity fields with different frequencies is analyzed by applying optimized inseparability criteria proposed by Van Loock and Furusawa.
We present a cascaded system consisting of three non-degenerate optical parametric amplifiers (NOPAs) for the generation and the enhancement of quantum entanglement of continuous variables. The entanglement of optical fields produced by the first NOPA is successively enhanced by the second and the third NOPAs from -5.3 $dB$ to -8.1 $dB$ below the quantum noise limit. The dependence of the enhanced entanglement on the physical parameters of the NOPAs and the reachable entanglement limitation for a given cascaded NOPA system are calculated. The calculation results are in good agreement with the …
We analyse a nonlinear optical system which uses cascaded nonlinearities to produce both second and fourth harmonic outputs from an input field at the fundamental frequency. Using fully quantum equations of motion, we show that the system produces quadrature squeezed outputs which exhibit bipartite entanglement, EPR-steering, and asymmetric steering across a two octave frequency range.
The dynamics of a cascaded system that consists of two atom-cavity subsystems is studied by using the quantum trajectory method. Unwanted losses are included, such as photon absorption and scattering by the cavity mirrors and spontaneous emission of the atoms. Considering an initially excited two-level atom in the source subsystem, analytical solutions are obtained. The entanglement evolution is studied for the two atoms and for the two intracavity fields.
We compare the bipartite entanglement and EPR-steering properties of the two different schemes which produce third harmonic optical fields from an input field at the fundamental frequency. The first scheme uses second harmonic cascaded with sum-frequency generation while the second uses triply degenerate four-wave mixing, also known as direct third harmonic generation. We examine and compare the two schemes in both the travelling wave and intra-cavity configurations. We find that both schemes produce continuous-variable bipartite entanglement and EPR-steering. The direct scheme produces a grea…
We propose a scheme to unconditionally entangle the internal states of atoms trapped in separate high finesse optical cavities. The scheme uses the technique of quantum reservoir engineering in a cascaded cavity QED setting, and for ideal (lossless) coupling between the cavities generates an entangled pure state. Highly entangled states are also shown to be possible for realizable cavity QED parameters and with nonideal coupling.
We theoretically investigate the spectral entanglement of a multiphoton source generated from the cascade emissions in the cascaded cold atomic ensembles.\ This photon source is highly directional, guaranteed under the four-wave mixing condition, and is also highly frequency-correlated due to finite driving pulse durations and superradiant decay constants.\ We utilize Schmidt decomposition to study the bipartite entanglement of the biphoton states projected from the multiphoton ones.\ This entropy of entanglement can be manipulated by controlling the driving parameters and superradiant decay r…
We study the entanglement distillation in continuous variable systems when a photon replacement protocol is employed. A cascaded protocol is studied and we find that the resultant entanglement increases by increasing the number of repetitions. Interestingly, the entanglement enhancement is not sensitive to the asymmetry of the protocol and gives the same result for any arrangement in the absence of loss. The non-Gaussianity of the outcome state is also studied and it is found that the non-Gaussianity of the state dramatically depends on the experimental arrangements. By providing practical inf…
Stable sources of entangled photons are important requirements for quantum communications. In recent years, cascaded downconversion has been demonstrated as an effective method of directly producing three-photon entanglement. However, to produce polarization entanglement these sources have until now relied on intricate active phase stabilization schemes, thus limiting their robustness and usability. In this work, we present a completely phase-stable source of three-photon entanglement in the polarization degree of freedom. With this source, which is based on a cascade of two pair sources based…
In this paper, we propose a scheme for generating steady-state entanglement of remote micromechanical oscillators in unidirectionally-coupled cavities. For the system of two mechanical oscillators, we show that when two cavity modes in each cavity are driven at red- and blue-detuned sidebands, respectively, a stationary two-mode squeezed vacuum state of the two mechanical oscillators can be generated with the help of the cavity dissipation. The degree of squeezing is controllable by adjusting the relative strength of the pump lasers. Our calculations also show that the achieved mechanical enta…
Quantum entanglement of particles is regarded as a fundamental character in quantum information, in which quantum state should be given for whole system instead of independently describing single particle. Constructing quantum memory of photonic entanglement is essential for realizing quantum networks, which had been performed previously by many memory protocols. Of which Raman quantum memory gives advantages in broadband and high-speed properties, resulting in huge potential in quantum network and quantum computation. However, Raman quantum memory of photonic polarised entanglement is a chall…
We examine the theoretical limits of the generation of entanglement in a damped coupled ion-cavity system using jump-based feedback. Using Raman transitions to produce entanglement between ground states reduces the necessary feedback bandwidth, but does not improve the overall effect of the spontaneous emission on the final entanglement. We find that the fidelity of the resulting entanglement will be limited by the asymmetries produced by vibrations in the trap, but that the concurrence remains above 0.88 for realistic ion trap sizes.
The existence of higher order entanglement in the stimulated and spontaneous Raman processes is established using the perturbative solutions of the Heisenberg equations of motion for various field modes that are obtained using the Sen-Mandal technique and a fully quantum mechanical Hamiltonian that describes the stimulated and spontaneous Raman processes. Specifically, the perturbative Sen-Mandal solutions are exploited here to show the signature of the higher order two-mode and multi-mode entanglement. In some special cases, we have also observed higher order entanglement in the partially spo…
We studied the quantum correlation between the photon pairs generated by biexciton cascade decays of self-assembled quantum dots, and determined the temperature behavior associated with so-called sudden change of the quantum correlation. The relationship between the fine structure splitting and the sudden change temperature is also provided. Our study indicates that this correlation behavior sudden change temperature is independent on the back ground noise in the system and far lower than entanglement sudden death temperature, therefore it should be easier to observe the phenomenon of correlat…
Cascaded Rydberg antiblockade: Multi-atom excitation dynamics and entanglement
School of Physics, Zhengzhou University（郑州大学物理学院）；School of Physics, Anhui University（安徽大学物理学院）；School of Electronics and Information, Zhengzhou University of Light Industry（郑州轻工业大学电子与信息工程学院）；Institute of Quantum Materials and Physics, Henan Academy of Science（河南省科学院量子材料与物理研究所）
We propose a scheme of generating and verifying mesoscopic-level entanglement between two atomic ensembles using non-resonant stimulated Raman scattering. Entanglement can be generated by direct detection or balanced homodyne detection of the Stokes fields from the two cells, after they interfere on a beam splitter. The entanglement of the collective atomic fields can be transferred to the anti-Stokes fields in a readout process. By measuring the operator moments of the anti-Stokes fields, we can verify the presence of entanglement. We model the effects of practical factors such as Stokes fiel…
It has now been possible to prepare chain of ions in an entangled state and thus question arises --- how the optical properties of a chain of entangled ions differ from say a chain of independent particles. We investigate nonlinear optical processes in such chains. We explicitly demonstrate the possibility of entanglement produced super Raman scattering. Our results in contrast to Dicke's work on superradiance are applicable to stimulated processes and are thus free from the standard complications of multimode quantum electrodynamics. Our results suggest the possibility of similar enhancement …
We analyse the output quantum tripartite correlations from an intracavity nonlinear optical system which uses cascaded nonlinearities to produce both second and fourth harmonic outputs from an input field at the fundamental frequency. Using fully quantum equations of motion, we investigate two parameter regimes and show that the system produces tripartite inseparability, entanglement and EPR steering, with the detection of these depending on the correlations being considered.
The cascade-emitted biphotons generated from the alkali metal atomic ensembles are an excellent entanglement resource which enables long-distance quantum communication. The communication of quantum information between distant locations can be realized by utilizing the low-loss telecom bandwidth in the upper transition of the cascaded photons in a fiber-based quantum network. Meanwhile, the infrared photon from the lower transition of this highly directional and frequency-correlated biphoton can be created under the four-wave mixing process and can be stored locally as a collective spin wave. H…
In this paper, we demonstrate the generation of high-performance entangled photon-pairs in different degrees of freedom from a single piece of fiber pigtailed periodically poled LiNbO$_3$ (PPLN) waveguide. We utilize cascaded second-order nonlinear optical processes, i.e. second-harmonic generation (SHG) and spontaneous parametric down conversion (SPDC), to generate photon-pairs. Previously, the performance of the photon pairs is contaminated by Raman noise photons from the fiber pigtails. Here by integrating the PPLN waveguide with noise rejecting filters, we obtain a coincidence-to-accidenta…
The preparation of light pulses with well-defined quantum properties requires precise control at the individual photon level. Here, we demonstrate exact and controlled multi-photon subtraction from incoming light pulses. We employ a cascaded system of tightly confined cold atom ensembles with strong, collectively enhanced coupling of photons to Rydberg states. The excitation blockade resulting from interactions between Rydberg atoms limits photon absorption to one per ensemble and engineered dephasing of the collective excitation suppresses stimulated re-emission of the photon. We experimental…
The cascaded biphoton state generated from a cold atomic ensemble presents one of the strongly correlated resources that can preserve and relay quantum information. Under the four-wave mixing condition, the emitted signal and idler photons from the upper and lower excited states become highly correlated in their traveling directions and entangled in continuous frequency spaces. In this system, we theoretically study the spectral compression of the biphoton source using an external cavity and show the reduction in its frequency entanglement entropy. This indicates, respectively, an improved lig…
We address an experimental scheme to analyze the optical bistability and the entanglement of two movable mirrors coupled to a two-mode laser inside a doubly resonant cavity. With this aim we investigate the master equations of the atom-cavity subsystem in conjunction with the quantum Langevin equations that describe the interaction of the mirror cavity. The parametric amplification-type coupling induced by the two-photon coherence on the optical bistability of the intracavity mean photon numbers is found and investigated. Under this condition, the optical intensities exhibit bistability for al…
Making use of the Rydberg blockade, we generate entanglement between two atoms individually trapped in two optical tweezers. In this paper we detail the analysis of the data and show that we can determine the amount of entanglement between the atoms in the presence of atom losses during the entangling sequence. Our model takes into account states outside the qubit basis and allows us to perform a partial reconstruction of the density matrix describing the two atom state. With this method we extract the amount of entanglement between pairs of atoms still trapped after the entangling sequence an…
We discuss theoretically quantum interface between light and a spin polarized ensemble of atoms with the spin >= 1 based on an off-resonant Raman scattering. We present the spectral theory of the light-atoms interaction and show how particular spectral modes of quantum light couple to spatial modes of the extended atomic ensemble. We show how this interaction can be used for quantum memory storage and retrieval and for deterministic entanglement protocols. The proposed protocols are attractive due to their simplicity since they involve just a single pass of light through atoms without the need…
We study the dissipative dynamics and the formation of entangled states in driven cascaded quantum networks, where multiple systems are coupled to a common unidirectional bath. Specifically, we identify the conditions under which emission and coherent reabsorption of radiation drives the whole network into a pure stationary state with non-trivial quantum correlations between the individual nodes. We illustrate this effect in more detail for the example of cascaded two-level systems, where we present an explicit preparation scheme that allows one to tune the whole network through "bright" and "…
We show that an absolute coherent phase of a laser can be used to manipulate the entanglement of photon pairs of two-photon laser. Our focus is on the generation of a continuous source of entangled photon pairs in the double $Λ$ (or Raman) scheme. We study the dependence of steady state entanglement on the phase and laser parameters. We obtain a relationship between entanglement and two-photon correlation. We derive conditions that give steady state entanglement for the Raman-EIT scheme and use it to identify region of steady state macroscopic entanglement. No entanglement is found for the dou…
The evolution of a Raman coupled three-level lambda atom with two quantized cavity modes is studied in the large detuning case; i.e. when the upper atomic level can be adiabatically eliminated. Particularly the situation when the two modes are prepared in initial coherent or squeezed states, with a large average number of photons, is investigated. It is found that the atom, after specific interaction times, disentangles from the two modes, leaving them, in certain cases, in entangled Schrodinger cat states. These disentanglement times can be controlled by adjusting the ratio between average nu…
The operator solution of a completely quantum mechanical Hamiltonian of the Raman processes is used here to investigate the possibility of obtaining intermodal entanglement between different modes involved in the Raman processes (e.g. pump mode, Stokes mode, vibration (phonon) mode and anti-Stokes mode). Intermodal entanglement is reported between a) pump mode and anti-Stokes mode, b) pump mode and vibration (phonon) mode c) Stokes mode and vibration phonon mode, d) Stokes mode and anti-stokes mode in the stimulated Raman processes for the variation of the phase angle of complex eigenvalue $α_…
We introduce a scheme for creating continuous variable entanglement between an atomic beam and an optical field, by using squeezed light to outcouple atoms from a BEC via a Raman transition. We model the full multimode dynamics of the atom laser beam and the squeezed optical field, and show that with appropriate two-photon detuning and two-photon Rabi frequency, the transmitted light is entangled in amplitude and phase with the outcoupled atom laser beam. The degree of entanglement is controllable via changes in the two-photon Rabi frequency of the outcoupling process.
We analyze quantum entanglement of Stokes light and atomic electronic polarization excited during single-pass, linear-regime, stimulated Raman scattering in terms of optical wave-packet modes and atomic-ensemble spatial modes. The output of this process is confirmed to be decomposable into multiple discrete, bosonic mode pairs, each pair undergoing independent evolution into a two-mode squeezed state. For this we extend the Bloch-Messiah reduction theorem, previously known for discrete linear systems (S. L. Braunstein, Phys. Rev. A, vol. 71, 055801 (2005)). We present typical mode functions in…
Experimental results from the generation of Raman sidebands using optical vortices are presented. By generating two sets of sidebands originating from different locations in a Raman active crystal, one set containing optical orbital angular momentum and the other serving as a reference, a Young's double slit experiment was simultaneously realized for each sideband. The interference between the two sets of sidebands was used to determine the helicity and topological charge in each order. Topological charges in all orders were found to be discrete and follow selection rules predicted by a cascad…
Entanglement and Optical Nonreciprocity in spontaneous Raman Scattering
Max Planck Institute for the Structure and Dynamics of Matter（马克斯·普朗克物质结构与动力学研究所）；University of Hamburg（汉堡大学）；The Hamburg Centre for Ultrafast Imaging（汉堡超快成像中心）
A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes are coherent) and chaotic scattering (where initial phonon mode is chaotic and all the other modes are coherent) are studied. Nonclassical character of Raman process is observed by means of intermodal entanglement, single mode and intermodal squeezing of vacuum fluctuations, sub-shot noise and wave variances. Joint photon-phonon number and integrated-intensi…
We analyze the stabilizability of entangled two-mode Gaussian states in three benchmark dissipative models: local damping, dissipators engineered to preserve two-mode squeezed states, and cascaded oscillators. In the first two models, we determine principal upper bounds on the stabilizable entanglement, while in the last model, arbitrary amounts of entanglement can be stabilized. All three models exhibit a tradeoff between state entanglement and purity in the entanglement maximizing limit. Our results are derived from the Hamiltonian-independent stabilizability conditions for Gaussian systems.…
Quantum entanglement is an integral part of quantum optics and has been exploited in areas such as computation, cryptography and metrology. The entanglement between photons can be present in various degrees of freedom (DOFs), and even the simplest bi-partite systems can occupy a large Hilbert space. Therefore, it is desirable to exploit this multi-dimensional space for various quantum applications by fully controlling the properties of the entangled photons in multiple DOFs. While current entangled-photon sources are capable of generating entanglement in one or more DOFs, there is currently a …
We theoretically investigate the stability of a two cascaded cavity optomechanical system with optical parametric amplifiers (OPAs) inside the two coupled cavities, and study the steady-state entanglement between two distant mechanical resonators. We show that the parameter regime where the system is unstable without OPAs, such as relatively high laser intensity and blue detuning, can be exploited to build the steady-state mechanical entanglement by modulating the parametric gain. The application of OPAs is helpful to preserve the mechanical entanglement suffered from the dissipation at some f…
In this article, non-classical properties of Raman modes are investigated. The original goal, actually, is to identify how and by which method we can induce non-classicality in Raman modes. We introduce a plasmonic system in which Raman dye molecules are buried between two shells of the plasmonic materials similar to onion-like core/shell nanoparticle. This system is excited by the entangled photons, followed by analyzing its dynamics of motion using the Heisenberg-Langevin equations by which the time evolution of the signal-idler mode and Raman modes are derived. Interestingly, the entangled …
We report an experimental demonstration of entanglement swapping over two quantum stages. By successful realizations of two cascaded photonic entanglement swapping processes, entanglement is generated and distributed between two photons, that originate from independent sources and do not share any common past. In the experiment we use three pairs of polarization entangled photons and conduct two Bell-state measurements (BSMs) one between the first and second pair, and one between the second and third pair. This results in projecting the remaining two outgoing photons from pair 1 and 3 into an …
We introduce and study the concept of a reversible transfer of the quantum state of two internally-translationally entangled fragments, formed by molecular dissociation, to a photon pair. The transfer is based on intracavity stimulated Raman adiabatic passage and it requires a combination of processes whose principles are well established.
We propose a direct, coherent coupling scheme that can create massively entangled states of Bose-Einstein condensed atoms. Our idea is based on an effective interaction between two atoms from coherent Raman processes through a (two atom) molecular intermediate state. We compare our scheme with other recent proposals for generation of massive entanglement of Bose condensed atoms.
We present a scheme to realise the basic two-quibit logic gates such as quantum phase gate and controlle-NOT gate using a detuned optical cavity interacting with a three-level Raman system. We discuss the role of Stark shifts which are as important as the terms leading to two-photon transition. The operation of the proposed logic gates involves metastable states of the atom and hence is not affected by spontaneous emission. These ideas can be extended to produce multiparticle entanglement.
The process of cascaded downconversion and sum-frequency generation inside an optical cavity has been predicted to be a potential source of three-mode continuous-variable entanglement. When the cavity is pumped by two fields, the threshold properties have been analysed, showing that these are more complicated than in well-known processes such as optical parametric oscillation. When there is only a single pumping field, the entanglement properties have been calculated using a linearised fluctuation analysis, but without any consideration of the threshold properties or critical operating points …
We present a first-principles theoretical analysis of the entanglement of two superconducting qubits in spatially separated microwave cavities by a sequential (cascaded) probe of the two cavities with a coherent mode, that provides a full characterization of both the continuous measurement induced dynamics and the entanglement generation. We use the SLH formalism to derive the full quantum master equation for the coupled qubits and cavities system, within the rotating wave and dispersive approximations, and conditioned equations for the cavity fields. We then develop effective stochastic maste…
In spontaneous Raman process in atomic cell at high gain, both the Stokes field and the accompanying collective atomic excitation (atomic spin wave) are coherent. We find that, due to the spontaneous nature of the process, the phases of the Stokes field and the atomic spin wave change randomly from one realization to another but are anti-correlated. The phases of the atomic ensembles are read out via another Raman process at a later time, thus realizing phase memory in atoms. The observation of phase correlation between the Stokes field and the collective atomic excitations is an important ste…
We propose to realize the two-mode continuous-variable entanglement of microwave photons in an electro-optic system, consisting of two superconducting microwave resonators and one or two optical cavities filled with certain electro-optic medium. The cascaded and parallel schemes realize such entanglement via coherent control on the dynamics of the system, while the dissipative dynamical scheme utilizes the reservoir-engineering approach and exploits the optical dissipation as a useful resource. We show that, for all the schemes, the amount of entanglement is determined by the ratio of the effe…
We propose schemes for the unconditional preparation of a two-mode squeezed state of effective bosonic modes realized in a pair of atomic ensembles interacting collectively with optical cavity and laser fields. The scheme uses Raman transitions between stable atomic ground states and under ideal conditions produces pure entangled states in the steady state. The scheme works both for ensembles confined within a single cavity and for ensembles confined in separate, cascaded cavities.
Entanglement between distant massive mechanical oscillators is of particular interest in quantum-enabled devices due to its potential applications in distributed quantum information processing. Here we propose how to achieve nonreciprocal remote entanglement between two spatially separated mechanical oscillators within a cascaded optomechanical configuration, where the two optomechanical resonators are indirectly coupled through a telecommunication fiber. We show that by selectively spinning the optomechanical resonators, one can break the time reversal symmetry of this compound system via Sag…
The generation of entanglement between disparate physical objects is a key ingredient in the field of quantum technologies, since they can have different functionalities in a quantum network. Here we propose and analyze a generic approach to steady-state entanglement generation between two oscillators with different temperatures and decoherence properties coupled in cascade to a common unidirectional light field. The scheme is based on a combination of coherent noise cancellation and dynamical cooling techniques for two oscillators with effective masses of opposite signs, such as quasi-spin an…
We propose a scheme employing quantum-reservoir engineering to controllably entangle the internal states of two atoms trapped in a high finesse optical cavity. Using laser and cavity fields to drive two separate Raman transitions between metastable atomic ground states, a system is realized corresponding to a pair of two-state atoms coupled collectively to a squeezed reservoir. Phase-sensitive reservoir correlations lead to entanglement between the atoms, and, via local unitary transformations and adjustment of the degree and purity of squeezing, one can prepare entangled mixed states with any…
