We report correlation and cross-correlation measurements of photons emitted under continuous wave excitation by a single II-VI quantum dot (QD) grown by molecular-beam epitaxy. A standard technique of microphotoluminescence combined with an ultrafast photon correlation set-up allowed us to see an antibunching effect on photons emitted by excitons recombining in a single CdTe/ZnTe QD, as well as cross-correlation within the biexciton ($X_{2}$)-exciton ($X$) radiative cascade from the same dot. Fast microchannel plate photomultipliers and a time-correlated single photon module gave us an overall temporal resolution of 140 ps better than the typical exciton lifetime in II-VI QDs of about 250ps.
We predict dominating cooperative two-photon emission from two quantum dots coupled with a single mode photonic crystal cavity. The cooperative two photon emission occurs when excitons in two off-resonantly coupled quantum dots decay simultaneously. The interaction with common cavity field leads to cavity induced two-photon emission which is strongly inhibited by electron phonon coupling. The interaction with common phonon bath produces phonon induced two-photon emission which increases on increasing temperature. For identical quantum dots cavity induced two-photon emission is negligible but p…
We investigate the effects of a low frequency (acoustic) phonon bath on the dynamics of a quantum dot modelled as a cascade three-level system. We show that the phonon bath appears to the upper transition of the cascade system as a broadband reservoir of inverted rather than conventional harmonic oscillators. The action of the annihilation and creation operators of the inverted oscillator are interchanges relative to those of the usual harmonic oscillator that it serves as a linear amplifier to the system, and thereby gives rise to unusual features in the dynamics of the quantum dot. We find t…
Quantum dots embedded in photonic nanostructures have in recent years proven to be a very powerful solid-state platform for quantum optics experiments. The combination of near-unity radiative coupling of a single quantum dot to a photonic mode and the ability to eliminate decoherence processes imply that an unprecedented light-matter interface can be obtained. As a result, high-cooperativity photon-emitter quantum interfaces can be constructed opening a path-way to deterministic photonic quantum gates for quantum-information processing applications. In the present manuscript, I review current …
Single photon emitters are indispensable to photonic quantum technologies. Here we demonstrate waveform-controlled high-purity single photons from room-temperature colloidal quantum dots. The purity of the single photons does not vary with the excitation power, thereby allowing the generation rate to be increased without compromising the single-photon quality.
Semiconductor quantum dots, as promising solid-state platform, have exhibited deterministic photon pair generation with high polarization entanglement f\textcompwordmark idelity for quantum information applications. However, due to temporal correlation from inherently cascaded emission, photon indistinguishability is limited, which restricts their potential scalability to multi-photon experiments. Here, by utilizing quantum interferences to decouple polarization entanglement from temporal correlation, we improve multi-photon entanglement f\textcompwordmark idelity from $(58.7\pm 2.2)\%$ to $(7…
We observe the unconventional photon blockade effect in quantum dot cavity QED, which, in contrast to conventional photon blockade, operates in the weak coupling regime. A single quantum dot transition is simultaneously coupled to two orthogonally polarized optical cavity modes, and by careful tuning of the input and output state of polarization, the unconventional photon blockade effect is observed. We find a minimum second-order correlation $g^{(2)}(0)\approx0.37$ which corresponds to $g^{(2)}(0)\approx0.005$ when corrected for detector jitter, and observe the expected polarization dependenc…
Tho-photon Rabi oscillations hold potential for quantum computing and quantum information processing, because during a Rabi cycle a pair of entangled photons may be created. We theoretically investigate the onset of this phenomenon in a heterodimer comprising a semiconductor quantum dot strongly coupled to a metal nanoparticle. Two-photon Rabi oscillations in this system occur due to a coherent two-photon process involving the ground-to-biexciton transition in the quantum dot. The presence of a metal nanoparticle nearby the quantum dot results in a self-action of the quantum dot via the metal …
Polarized cross-correlation spectroscopy on a quantum dot charged with a single hole shows the sequential emission of photons with common circular polarization. This effect is visible without magnetic field, but becomes more pronounced as the field along the quantization axis is increased. We interpret the data in terms of electron dephasing in the X+ state caused by the Overhauser field of nuclei in the dot. We predict the correlation timescale can be increased by accelerating the emission rate with cavity-QED.
We propose methods for realization of continuous two photon source using coherently pumped quantum dot embedded inside a photonic crystal cavity. We analyze steady state population in quantum dot energy levels and field inside the cavity mode. We find conditions for population inversion in coherently pumped and incoherently pumped quantum dot. We show that squeezing in the output for two two photon laser is not visible using coherent as well as incoherent pump. We discuss effect of phonon coupling using recently developed polaron transformed master equation at low temperatures. We also propose…
We exploit the nonlinearity arising from the spin-photon interaction in an InAs quantum dot to demonstrate phase shifts of scattered light pulses at the single-photon level. Photon phase shifts of close to 90 degrees are achieved using a charged quantum dot in a micropillar cavity. We also demonstrate a photon phase switch by using a spin-pumping mechanism through Raman transitions in an in-plane magnetic field. The experimental findings are supported by a theoretical model which explores the dynamics of the system. Our results demonstrate the potential of quantum dot-induced nonlinearities fo…
We perform extended numerical studies to maximize the overall photon coupling efficiency of fiber-coupled quantum dot single-photon sources emitting in the near-infrared and telecom regime. Using the finite element method, we optimize the photon extraction and fiber-coupling efficiency of quantum dot single-photon sources based on micromesas, microlenses, circular Bragg grating cavities and micropillars. The numerical simulations which consider the entire system consisting of the quantum dot source itself, the coupling lens, and the single-mode fiber yield overall photon coupling efficiencies …
Charged quantum dots containing an electron or hole spin are bright solid-state qubits suitable for quantum networks and distributed quantum computing. Incorporating such quantum dot spin into a photonic crystal cavity creates a strong spin-photon interface, in which the spin can control a photon by modulating the cavity reflection coefficient. However, previous demonstrations of such spin-photon interfaces have relied on quantum dots that are charged randomly by nearby impurities, leading to instability in the charge state, which causes poor contrast in the cavity reflectivity. Here we demons…
The spontaneous emission rate of a quantum dot coupled to a structured photonic reservoir is determined by the frequency dependence of its local density of photon states. Through phonon-dressing, a breakdown of Fermi's golden rule can occur for certain photonic structures whose photon decay time become comparable to the longitudinal acoustic phonon decay times. We present a polaron master equation model to calculate the photoluminescence intensity from a coherently excited quantum dot coupled to a structured photonic reservoir. We consider examples of a semiconductor microcavity and a coupled …
The electro-optic, acousto-optic and nonlinear properties of lithium niobate make it a highly versatile material platform for integrated quantum photonic circuits. A prerequisite for quantum technology applications is the ability to efficiently integrate single photon sources, and to guide the generated photons through ad-hoc circuits. Here we report the integration of quantum dots in monolayer WSe2 into a Ti in-diffused lithium niobate directional coupler. We investigate the coupling of individual quantum dots to the waveguide mode, their spatial overlap, and the overall efficiency of the hyb…
In this note we present some results concerning photon blockade and antibunching in a system consisting of a quantum dot embedded in a microcavity. We give analytic conditions for resonant and non-resonant photon blockade, valid for small values of the external pump amplitude. Starting from these results, we discuss the quantum states characteristics of the system within a master equation formalism and highlight quantities like stationary second order correlations both static and dynamic and one-photon purity.
A semiconductor quantum dot can generate highly coherent and indistinguishable single photons. However, intrinsic semiconductor dephasing mechanisms can reduce the visibility of two-photon interference. For an electron in a quantum dot, a fundamental dephasing process is the hyperfine interaction with the nuclear spin bath. Here we directly probe the consequence of the fluctuating nuclear spins on the elastic and inelastic scattered photon spectra from a resident electron in a single dot. We find the nuclear spin fluctuations lead to detuned Raman scattered photons which are distinguishable fr…
Colloidal quantum dots have garnered active research interest as quantum emitters due to their robust synthesis process and straightforward integration with nanophotonic platforms. However, obtaining indistinguishable photons from the colloidal quantum dots at room temperature is fundamentally challenging because they suffer from an extremely large dephasing rate. Here we propose an experimentally feasible method of obtaining indistinguishable single photons from an incoherently pumped solution-processed colloidal quantum dot coupled to a system of nanocavities. We show that by coupling a coll…
Universal properties of entangled many-body states are controlled by their symmetry and quantum fluctuations. By magnetic-field tuning of the spin-orbital degeneracy in a Kondo-correlated quantum dot, we have modified quantum fluctuations to directly measure their influence on the many-body properties along the crossover from $SU(4)$ to $SU(2)$ symmetry of the ground state. High-sensitive current noise measurements combined with the non-equilibrium Fermi liquid theory clarify that the Kondo resonance and electron correlations are enhanced as the fluctuations, measured by the Wilson ratio, incr…
In this letter, we present a detailed, all optical study of the influence of different excitation schemes on the indistinguishability of single photons from a single InAs quantum dot. For this study, we measure the Hong-Ou-Mandel interference of consecutive photons from the spontaneous emission of an InAs quantum dot state under various excitation schemes and different excitation conditions and give a comparison.
