Physical processes that could facilitate coherent control of light propagation are now actively explored. In addition to fundamental interest, these efforts are stimulated by possibilities to develop, for example, a quantum memory for photonic states. At the same time, controlled localization and storage of photonic pulses may allow novel approaches to manipulate light via enhanced nonlinear optical processes. Recently, Electromagnetically Induced Transparency (EIT) was used to reduce the group velocity of propagating light pulses and to reversibly map propagating light pulses into stationary spin excitations in atomic media. Here we describe and experimentally demonstrate a novel technique in which light propagating in a medium of Rb atoms is converted into an excitation with localized, stationary electromagnetic energy, which can be held and released after a controllable interval. Our method creates pulses of light with stationary envelopes bound to an atomic spin coherence, raising new possibilities for photon state manipulation and non-linear optical processes at low light levels.
We present a detailed theoretical description of the generation of stationary light pulses by standing wave electromagnetically induced transparency in media comprised of stationary atoms. We show that, contrary to thermal gas media, the achievable storage times are limited only by the ground state dephasing rate of the atoms, making such media ideally suited for nonlinear optical interactions between stored pulses. Furthermore, we find significant quantitative and qualitative differences between the two types of media, which are important for quantum information processing schemes involving s…
We show that the recently demonstrated technique for generating stationary pulses of light [Nature {\bf 426}, 638 (2003)] can be extended to localize optical pulses in all three spatial dimensions in a resonant atomic medium. This method can be used to dramatically enhance the nonlinear interaction between weak optical pulses. In particular, we show that an efficient Kerr-like interaction between two pulses can be implemented as a sequence of several purely linear optical processes. The resulting process may enable coherent interactions between single photon pulses.
We present a detailed analysis of the recently demonstrated technique to generate quasi-stationary pulses of light [M. Bajcsy {\it et al.}, Nature (London) \textbf{426}, 638 (2003)] based on electromagnetically induced transparency. We show that the use of counter-propagating control fields to retrieve a light pulse, previously stored in a collective atomic Raman excitation, leads to quasi-stationary light field that undergoes a slow diffusive spread. The underlying physics of this process is identified as pulse matching of probe and control fields. We then show that spatially modulated contro…
We present a theoretical treatment of electromagnetically induced transparency and light storage using standing wave coupling fields in a medium comprised of stationary atoms, such as an ultra cold atomic gas or a solid state medium. We show that it is possible to create stationary pulses of light which have a qualitatively different behavior than in the case of a thermal gas medium, offering greater potential for quantum information processing applications.
We show the pulse matching phenomenon can be obtained in the general multi-level system with electromagnetically induced transparency (EIT). For this we find a novel way to create tightly localized stationary pulses by using counter-propagating pump fields. The present process is a spatial compression of excitation so that it allows us to shape and further intensify the localized stationary pulses, without using standing waves of pump fields or spatially modulated pump fields.
We describe a technique for generating pulses of light with controllable photon numbers, propagation direction, timing, and pulse shapes. The technique is based on preparation of an atomic ensemble in a state with a desired number of atomic spin excitations, which is later converted into a photon pulse. Spatio-temporal control over the pulses is obtained by exploiting long-lived coherent memory for photon states and electromagnetically induced transparency (EIT) in an optically dense atomic medium. Using photon counting experiments we observe generation and shaping of few-photon sub-Poissonian…
The stationary light pulse (SLP) refers to a zero-group-velocity optical pulse in an atomic ensemble prepared by two counter-propagating driving fields. Despite the uniqueness of an optical pulse trapped within an atomic medium without a cavity, observations of SLP so far have been limited to trapping a single optical pulse due to the stringent SLP phase-matching condition, and this has severely hindered the development of SLP-based applications. In this paper, we first show theoretically that the SLP process in fact supports two phase-matching conditions and we then utilize the result to expe…
We investigate the dynamics of a single two-level atom, which interacts with pulses propagating in two spatial-modes (right and left) and frequency-continuum. Using Heisenberg equations of motion, we present the explicit analytical derivations and general formalisms for atomic excitation with two spatial-mode multi-photon pulses in both Fock state and coherent state. Based on those formalisms, we show that perfect atomic excitation by single photon Fock state pulse can only be realized when it is rising-exponentially shaped in the even-mode---a balanced superposition of the two spatial-modes. …
We investigate the problem of propagation of three-component resonant light pulses with adiabatically varying amplitudes through a medium consisting of atoms with the tripod level configuration. By means of both analytic and numerical methods we found the two modes of shape-preserving pulse propagation. The pulse propagation velocity is found to be either equal to the speed of light or significantly slowed down, depending on a particular propagation mode.
We have observed the ultraslow propagation of matched pulses in nondegenerate four-wave mixing in a hot atomic vapor. Probe pulses as short as 70 ns can be delayed by a tunable time of up to 40 ns with little broadening or distortion. During the propagation, a probe pulse is amplified and generates a conjugate pulse which is faster and separates from the probe pulse before getting locked to it at a fixed delay. The precise timing of this process allows us to determine the key coefficients of the susceptibility tensor. The presence of gain in this system makes this system very interesting in th…
We derive composite pulse sequences that achieve high-fidelity excitation of two-state systems in an optically dense, inhomogeneously broadened ensemble. The composite pulses are resistant to distortions due to the back-action of the medium they propagate in and are able to create high-fidelity inversion to optical depths $αz>10$. They function well with smooth pulse shapes used for coherent control of optical atomic transitions in quantum computation and communication. They are an intermediary solution between single $π$-pulse excitation schemes and adiabatic passage schemes, being far more e…
We have studied stationary and quasi-stationary signal light pulses in cold lambda-type atomic media driven by counterpropagating control laser fields at the condition of electromagnetically induced transparency. By deriving a dispersion relation we present spectral and temporal properties of the signal light pulse and a significant influence of atomic decoherence on the coupled stationary light pulses for spatial splitting. Finally we discuss quasi-stationary light pulse evolution characterized by frozen spatial spreading for a robust coherent control of slow light pulses.
We present an analysis of atomic diffraction due to the interaction of an atomic beam with a pair of Gaussian light pulses. We derive a simple analytical expression for the populations in different diffraction orders. The validity of the obtained solution extends beyond the Raman-Nath regime, where the kinetic energy associated with different diffraction peaks is neglected, into the so-called channeling regime where accurate analytical expressions have not previously been available for the diffraction. Comparison with experimental results and exact numerical solutions demonstrate the validity …
We discuss stationary light created by a pair of counter-propagating control fields in Lambda-type atomic gases with electromagnetically induced transparency for the case of negligible Doppler broadening. In this case the secular approximation used in the discussion of stationary light in hot vapors is no longer valid. We discuss the quality of the effective light-trapping system and show that in contrast to previous claims it is finite even for vanishing ground-state dephasing. The dynamics of the photon loss is in general non exponential and can be faster or slower than in hot gases.
We report on the generation of pulses of a low-frequency squeezed vacuum with noise suppression >2 dB below the standard quantum limit in a hot resonant 87 Rb vapor with polarization self-rotation. We demonstrate the possibility to precisely control the temporal profile of the squeezed noise quadrature by applying a calibrated longitudinal magnetic field, without degrading the maximum amount of squeezing.
We present a time-dependent perturbative approach adapted to the treatment of intense pulsed interactions. We show there is a freedom in choosing secular terms and use it to optimize the accuracy of the approximation. We apply this formulation to a unitary superconvergent technique and improve the accuracy by several orders of magnitude with respect to the Magnus expansion.
The robustness of an atomic fountain interferometer with respect to variations in the initial velocity of the atoms and deviations from the optimal pulse amplitude is examined. We numerically simulate the dynamics of an interferometer in momentum space with a maximum separation of $20 \hbar k$ and map out the expected signal contrast depending on the variance of the initial velocity distribution and the value of the laser field amplitude. We show that an excitation scheme based on rapid adiabatic passage significantly enhances the expected signal contrast compared to the commonly used scheme c…
We show how two circular polarization components of a linearly polarized pulse, propagating through a coherently driven dilute atomic vapor, can be well resolved in time domain by weak measurement. Slower group velocity of one of the components due to electromagnetically induced transparency leads to a differential group delay between the two components. For low number density, this delay may not be large enough to temporally resolve the two components. We show how this can be enhanced in terms of mean time of arrival of the output pulse through a post-selected polarizer. We demonstrate the id…
We describe the interaction of two two-level atoms in free space with propagating modes of the quantized electromagnetic field, using the time-dependent Heisenberg-Langevin method. For single- photon pulses, we consider the effect of the pulse's spatial and temporal profiles on the atomic excitation. In particular, we find the ideal shape for a pulse to put exactly one excitation in any desired state of the bi-atomic system. Furthermore, we analyze the differences in the atomic dynamics between the cases of Fock state pulses and coherent state pulses.
New technologies providing tight focusing lens and mirrors with large numerical apertures and electro-optic modulation of single photons are now available for the investigation of photon-atom interactions without a cavity. From the theoretical side, new models must be developed which take into account the intrinsic open system aspect of the problem as well as details about atomic relative positions and temporal (spectral) features of the pulses. In this paper, we investigate the generation of nonclassical correlations between two atoms in free space interacting with a quantized pulse containin…
We have considered theoretically the feasibility of the broadband quantum memory based on the resonant tripod-type atomic configuration. In this case, the writing of a signal field is carried out simultaneously into two channels, and characterized by an excitation of two spin waves of the atomic ensemble. With simultaneous read out from both channels quantum properties of the original signal are mapped on the retrieval pulse no worse than in the case of memory based on Lambda-type atomic configuration. At the same time new possibilities are opened up for manipulation of quantum states associat…
We study the suppression of noise-induced phase decoherence in a single atomic qubit by employing pulse sequences. The atomic qubit is composed of a single neutral atom in a far-detuned optical dipole trap and the phase decoherence may originate from the laser intensity and beam pointing fluctuations as well as magnetic field fluctuations. We show that suitable pulse sequences may prolongate the qubit coherence time substantially as comparing to the conventional spin echo pulse.
When ensembles of atoms interact with coherent light fields a great many interesting and useful effects can be observed. In particular, the group velocity of the coherent fields can be modified dramatically. Electromagnetically induced transparency is perhaps the best known example, giving rise to very slow light. Careful tuning of the optical fields can also produce stored light where a light field is mapped completely into a coherence of the atomic ensemble. In contrast to stored light, in which the optical field is extinguished, stationary light is a bright field of light with a group veloc…
We present a quantum manipulation of a traveling light pulse using double atomic coherence for two-color stationary light and quantum frequency conversion. The quantum frequency conversion rate of the traveling light achieved by the two-color stationary light phenomenon is near unity. We theoretically discuss the two-color stationary light for the frequency conversion process in terms of pulse area, energy transfer and propagation directions. The resulting process may apply the coherent interactions of a weak field to nonlinear quantum optics such as quantum nondemolition measurement.
We investigate the dispersion relations for light coupled to one-dimensional ensembles of atoms with different level schemes. The unifying feature of all the considered setups is that the forward and backward propagating quantum fields are coupled by the applied classical drives such that the group velocity can vanish in an effect known as "stationary light". We derive the dispersion relations for all the considered schemes, highlighting the important differences between them. Furthermore, we show that additional control of stationary light can be obtained by treating atoms as discrete scatter…
We report on the first observation of stationary light pulses and narrowband light storage inside a hollow-core photonic crystal fiber. Laser-cooled atoms were first loaded into the fiber core providing strong light-matter coupling. Light pulses were then stored in a collective atomic excitation using a single control laser beam. By applying a second counterpropagating control beam, a light pulse could be brought to a standstill. Our work paves the way towards the creation of strongly-correlated many-body systems with photons and applications in the field of quantum information processing.
Efficient photon-photon interaction is one of the key elements for realizing quantum information processing. The interaction, however, must often be mediated through an atomic medium due to the bosonic nature of photons, and the interaction time, which is critically linked to the efficiency, depends on the properties of the atom-photon interaction. While the electromagnetically induced transparency effect does offer the possibility of photonic quantum memory, it does not enhance the interaction time as it fully maps the photonic state to an atomic state. The stationary light pulse (SLP) effect…
A dynamic quantum control of three-color lights in an optically dense medium is presented. We discuss how effectively to stop traveling three-color light pulses in the medium by using three control laser fields at near resonant transitions satisfying electromagnetically induced transparency. This opens a door to the quantum coherent control of multiple traveling light pulses for quantum memory and quantum switching, which are essential components in multi-party quantum optical communications.
We study the interaction of two photons in a Rydberg atomic ensemble under the condition of electromagnetically induced transparency, combining a semi-classical approach for pulse propagation and a complete quantum treatment for quantum state evolution. We find that the blockade regime is not suitable for implementing photon-photon cross-phase modulation due to pulse absorption and dispersion. However, approximately ideal cross-phase modulation can be realized based on relatively weak interactions, with counter-propagating and transversely separated pulses.
We analyze the nonlinear dynamics of atomic dark states in Lambda configuration that interact with light at exact resonance. We found a generalization of shape-preserving pulses [R. Grobe, F. T. Hioe, and J. H. Eberly, Phys. Rev. Lett. 73, 3183 (1994)] and show that the condition for adiabaticity of the atomic dynamics is never violated, as long as spontaneous emission is negligible.
We investigate theoretically the optical properties of an atomic gas which has been cooled by the laser cooling method velocity-selective coherent population trapping. We demonstrate that the application of a weak laser pulse gives rise to a backscattered pulse, which is a direct signal for the entanglement in the atomic system, and which leads to single-particle entanglement on the few-photon level. If the pulse is applied together with the pump lasers, it also displays the phenomenon of electromagnetically induced transparency. We suggest that the effect should be observable in a gas of Rubi…
Nonlinear effects in pulse propagation through a medium consisting of four-level double-$Λ$-type systems are studied theoretically. We apply three continous-wave driving fields and a pulsed probe field such that they form a closed interaction loop. Due to the closed loop and the finite frequency width of the probe pulses the multiphoton resonance condition cannot be fulfilled, such that a time-dependent analysis is required. By identifying the different underlying physical processes we determine the parts of the solution relevant to calculate the linear and nonlinear response of the system. We…
Uniting Quantum Processing Nodes of Cavity-coupled Ions with Rare-earth Quantum Repeaters Using Single-photon Pulse Shaping Based on Atomic Frequency Comb
We present experimental evidence that light storage, i.e. the controlled release of a light pulse by an atomic sample dependent on the past presence of a writing pulse, is not restricted to small group velocity media but can also occur in a negative group velocity medium. A simple physical picture applicable to both cases and previous light storage experiments is discussed.
We investigate lensing and waveguiding properties of an atomic Bose-Einstein condensate for ultraslow pulse generated by electromagnetically induced transparency method. We show that a significant time delay can be controllably introduced between the lensed and guided components of the ultraslow pulse. In addition, we present how the number of guided modes supported by the condensate and the focal length can be controlled by the trap parameters or temperature.
Strong resonant dipole-dipole interactions in flexible Rydberg aggregates enable the formation of exciton pulses, the interplay of atomic motion and electronic excitation transfer which feature high fidelity entanglement transport. Here, we demonstrate the coherent splitting of such pulses into two modes, which induce strongly different atomic motion, leading to clear signatures of nonadiabatic effects in atomic density profiles. The mechanism exploits local nonadiabatic effects at a conical intersection, turning them from a decoherence source into an asset. The conical intersection is a conse…
We discuss a simple scheme for preparing atoms and molecules in an arbitrary preselected coherent superposition of quantum states. The technique, which we call fractional stimulated Raman adiabatic passage ({\it f-STIRAP}), is based upon (incomplete) adiabatic population transfer between an initial state $ψ_1$ and state $ψ_3$ through an intermediate state $ψ_2$. As in STIRAP, the Stokes pulse arrives before the pump pulse, but unlike STIRAP, the two pulses terminate simultaneously while maintaining a constant ratio of amplitudes. The independence of f-STIRAP from details of pulse shape and pul…
We consider propagation of a probe pulse in an atomic medium characterized by a combined tripod and Lambda ($Λ$) atom-light coupling scheme. The scheme involves three atomic ground states coupled to two excited states by five light fields. It is demonstrated that dark states can be formed for such an atom-light coupling. This is essential for formation of the electromagnetically induced transparency (EIT) and slow light. In the limiting cases the scheme reduces to conventional $Λ$- or $N$-type atom-light couplings providing the EIT or absorption, respectively. Thus the atomic system can experi…
We present a general model for an atomic memory using ultra-short pulses of light, which allows both spatial and temporal multimode storage. The process involves the storage of a faint quantum light pulse into the spin coherence of the ground state of Lambda-type 3-level atoms, in the presence of a strong driving pulse. Our model gives a full description of the evolution of the field and of the atomic coherence in space and time throughout the writing and the read-out processes. It is valid for any frequency detuning, from the resonant case to the Raman case, and allows a detailed optimization…
The eigenstate problem of the Jaynes-Cummings model on the basis of complete Hamiltonian, including the center-of -mass kinetic energy operator, is treated. The energy spectrum and wave functions in standing-wave (SW)- and counterpropagating waves (CPW)- cases are calculated and compared with each other. It is shown that in CPW-case i) the atomic momentum distribution is asymmetric and somewhat narrower in general; ii) the concept of quasimomentum is not applicable and instead the ordinary momentum concerns the problem; iii) atomic and photonic state distributions are self-consistent, and, in …
We consider a medium of multilevel atomic systems interacting with radiation pulses. A relatively simple technique of analytic calculations is proposed, which allows revealing all necessary conditions (with sufficient conditions to be checked separately) imposed on the interaction parameters, for which the mean dipole moment of a multilevel atomic medium vanishes, i.e., the medium becomes transparent via adiabatic interaction. The proposed technique is based on the method of quasienergies and illustrated for three- and five-level atomic systems. The necessary conditions for the propagation len…
Some recent theoretical studies have tended to employ analytically-continuous {\em gaussian}, or infinite-bandwidth step pulses to examine tunneling process. The stationary phase method is often employed to this aim. However, {\em gaussian} functions do not have a well-defined front, such that their speed of propagation becomes ambiguous. Also, infinite bandwidth signals cannot propagate through any real physical medium (whose transfer function is therefore finite) without pulse distortion, which also leads to ambiguities in determining propagation velocity during the tunneling process. In thi…
We develop the theory of an optical quantum memory protocol based on the three pulse photon echo (PE) in an optically dense medium with controlled reversible inhomogeneous broadening (CRIB). The wave-function of the retrieved photon echo field is derived explicitly as a function of an arbitrary input Data light field. The storage and retrieval of time-bin qubit states based on the described quantum memory is discussed, and it is shown that the memory allows to measure the path length difference in an imbalanced interferometer using short light pulses.
Dynamic control of a weak quantum probe light pulse for the generation and quantum manipulations of a stationary multi-color (MC-) light field in a resonant coherent atomic medium using electromagnetically induced transparency is proposed. The manipulations have been analyzed based on the analytical solution of the adiabatic limit in the evolution of MC-light fields resulting from interaction of the slow probe light with the new fields generated in the nondegenerate multi-wave mixing scheme. We have found a critical stopping condition for the MC-light fields where the group velocity of light s…
We demonstrate broadband laser cooling of atomic ions in an rf trap using ultrafast pulses from a modelocked laser. The temperature of a single ion is measured by observing the size of a time-averaged image of the ion in the known harmonic trap potential. While the lowest observed temperature was only about 1 K, this method efficiently cools very hot atoms and can sufficiently localize trapped atoms to produce near diffraction-limited atomic images.
We extend the theory of quantum light memory in atomic ensemble of Lambda type atoms with considering lower levels coherence decay rate and one and two-photon detunings from resonances in low intensity and adiabatic passage limit. We obtain that with considering these parameters, that there will be a considerable decay of probe pulse and stored information; also, we obtain that the group velocity of probe (light) pulse and its amplitude does not tend to zero by turning off the control field. We propose a method to keep the probe pulse in small values in turn off time of control field and to re…
In contrast to the free-space evolution of an atom governed by a multi-mode interaction with the surrounding electromagnetic vacuum, the evolution of a cavity-QED system can be characterized by just three parameters, (i) atom-cavity coupling strength g, (ii) cavity relaxation rate κ, and (iii) atomic decay rate into the non-cavity modes γ. In the case of an atom inserted into a planar resonator with an input beam coupled from the outside, it has been shown by Koshino [Phys. Rev. A 73, 053814 (2006)] that these three parameters are determined not only by the atom and cavity characteristics, but…
We study the process of squeezing of an ensemble of cold atoms in a pulsed optical lattice. The problem is treated both classically and quantum-mechanically under various thermal conditions. We show that a dramatic compression of the atomic density near the minima of the optical potential can be achieved with a proper pulsing of the lattice. Several strategies leading to the enhanced atomic squeezing are suggested, compared and optimized.
We present a detailed analysis of coherence creation in a four level double lambda-like atomic system using a train of ultra-short few-cycle Gaussian pulses. The effect of the Doppler broadening has been analyzed. It is possible to create high coherence across all the velocity groups in the atomic ensemble using pulses with low repetition frequency. The accumulation of coherence at different radial locations within the atomic beam cross-section as a function of the number of pulses in the train is also reported. We find that pulse train with lower repetition frequencies are able to generate hi…
Here we discuss an effect of dephasing induced by a weak gravitational field on the collective radiation dynamics of an atomic system in timed single-photon Dicke states. We show that a photon absorbed by the stationary system of randomly placed stationary atoms is no longer spontaneously emitted in the direction of the impinging photon. Gravity leads to broadening of the angular distribution of emission.
We study theoretically the dipole radiation of a hydrogen atom driven by an intense sub-cycle pulse. The time-dependent Schrödinger equation for the system is solved by ab initio calculation to obtain the dipole response. Remarkably, a narrowband emission lasting longer than the driving pulse appears at a frequency just above the ionization threshold. An additional calculation using the strong field approximation also recovers this emission, which suggests that it corresponds to the oscillation of nearly-bound electrons that behave similarly to Rydberg electrons. The predicted phenomenon is un…
We report a detailed investigation on the generation of pulse pairs during the readout of a coherence grating stored in a cold atomic ensemble. The pulse shapes and the split of the retrieved energy between the two pulses are studied as a function of the relative intensities of the two reading fields, and a minimum is observed for the total retrieved energy. We introduce a simplified analytical theory for the process, considering a three-level atomic system, which explains all the most striking experimental features.
We study the dynamics of a two-level system driven by an off-resonant few-cycle pulse which has a phase jump $ϕ$ at $t=t_{0}$, in contrast to many cycle pulses, under non rotating-wave approximation (NRWA). We give a closed form analytical solution for the evolution of the probability amplitude $|C_{a} (t)|$ for the upper level. Using the appropriate pulse parameters like phase-jump $ϕ$, jump time $t_{0}$, pulse width $τ$, frequency $ν$ and Rabi frequency $Ω_{0}$ the population transfer, after the pulse is gone, can be optimized and for the pulse considered here, enhancement of $10^{6}-10^{8}$…
We analyse the experiment by Hultgren et al. [Phys. Rev. A {\bf 87}, 031404 (2013)] on orbital alignment and quantum beats in coherently excited atomic fine-structure manifolds produced by short-pulse laser photodetachment of C$^-$, Si$^-$ and Ge$^-$ negative ions, and derive a formula that describes the beats. Analysis of the experimental data enables us to extract the non-coherent background contribution for each species, and indicates the need for a full density matrix treatment of the problem.
We present a new scheme of compact atomic gravimeter based on atom interferometry. Atoms are maintained against gravity using a sequence of coherent accelerations performed by the Bloch oscillations technique. We demonstrate a sensitivity of 4.8$\times 10^{-8}$ with an integration time of 4 min. Combining this method with an atomic elevator allows to measure the local gravity at different positions in the vacuum chamber. This method can be of relevance to improve the measurement of the Newtonian gravitational constant $G$.
The propagation of a weak optical pulse through an atomic system in closed $Λ$ configuration is investigated in which the hyper fine levels are coupled by a microwave pulse. Under three photon resonance condition, it is observed that the probe pulse shape gets cloned by the shape of the microwave pulse along propagation through the medium. The temporal position of the probe pulse is dragged to that of the microwave pulse. A simple expression for the linear susceptibility of the medium for the corresponding transition is derived in the Fourier domain. From the numerical analysis of dynamics usi…
