Sympathetic cooling of $^9Be^+$ and $^{24}Mg^+$ for quantum logic
M. D. Barrett, B. DeMarco, T. Schaetz, D. Leibfried, J. Britton, J. Chiaverini, W. M. Itano, B. Jelenkovic, J. D. Jost, C. Langer, T. Rosenband, D. J. Wineland
We demonstrate the cooling of a two species ion crystal consisting of one $^9Be^+$ and one $^{24}Mg^+$ ion. Since the respective cooling transitions of these two species are separated by more than 30 nm, laser manipulation of one ion has negligible effect on the other even when the ions are not individually addressed. As such this is a useful system for re-initializing the motional state in an ion trap quantum computer without affecting the qubit information. Additionally, we have found that the mass difference between ions enables a novel method for detecting and subsequently eliminating the effects of radio frequency (RF) micro-motion.
We sympathetically cool a trapped 112Cd+ ion by directly Doppler-cooling a 114Cd+ ion in the same trap. This is the first demonstration of optically addressing a single trapped ion being sympathetically cooled by a different species ion. Notably, the experiment uses a single laser source, and does not require strong focusing. This paves the way toward reducing decoherence in an ion trap quantum computer based on Cd+ isotopes.
Sympathetic cooling of a Fermi gas with a buffer gas of bosonic atoms is an efficient way to achieve quantum degeneracy in Fermi systems. However, all attempts to use this method for cooling ions until recently were ineffective because of the unremovable ion `"micromotion" in electromagnetic Paul traps, which prevents the realization of a number of hot projects with cold atom-ion systems. In this regard, we propose a new efficient method for sympathetic cooling of ions: the use for this purpose of cold buffer atoms in the region of atom-ion confinement-induced resonances (CIRs) [V.S. Melezhik,…
We analyze the dynamics and steady state of a linear ion array when some of the ions are continuously laser cooled. We calculate the ions' local temperature measured by its position fluctuation under various trapping and cooling configurations, taking into account background heating due to the noisy environment. For a large system, we demonstrate that by arranging the cooling ions evenly in the array, one can suppress the overall heating considerably. We also investigate the effect of different cooling rates and find that the optimal cooling efficiency is achieved by an intermediate cooling ra…
We demonstrate sympathetic cooling of a 43Ca+ trapped-ion "memory" qubit by a 40Ca+ "coolant" ion near the ground state of both axial motional modes, whilst maintaining coherence of the qubit. This is an essential ingredient in trapped-ion quantum computers. The isotope shifts are sufficient to suppress decoherence and phase shifts of the memory qubit due to the cooling light which illuminates both ions. We measure the qubit coherence during 10 cycles of sideband cooling, finding a coherence loss of 3.3% per cooling cycle. The natural limit of the method is O(0.01%) infidelity per cooling cycl…
One limit to the fidelity of quantum logic operations on trapped ions arises from heating of the ions' collective modes of motion. Sympathetic cooling of the ions during the logic operations may eliminate this source of errors. We discuss benefits and drawbacks of this proposal, and describe possible experimental implementations. We also present an overview of trapped-ion dynamics in this scheme.
We have cooled a two-ion-crystal to the ground state of its collective modes of motion. Laser cooling, more specific resolved sideband cooling is performed sympathetically by illuminating only one of the two $^{40}$Ca$^+$ ions in the crystal. The heating rates of the motional modes of the crystal in our linear trap have been measured, and we found them considerably smaller than those previously reported by Q. Turchette {\em et. al.} Phys. Rev. A 61, 063418 (2000) in the case of trapped $^9$Be$^+$ ions. After the ground state is prepared, coherent quantum state manipulation of the atomic popula…
We discuss fast frictionless cooling techniques in the framework of sympathetic cooling of cold atomic mixtures. It is argued that optimal cooling of an atomic species - in which the deepest quantum degeneracy regime is achieved - may be obtained by means of sympathetic cooling with another species whose trapping frequency is dynamically changed to maintain constancy of the Lewis-Riesenfeld adiabatic invariant. Advantages and limitations of this cooling strategy are discussed, with particular regard to the possibility of cooling Fermi gases to a deeper degenerate regime.
A promising route to novel quantum technologies are hybrid quantum systems, which combine the advantages of several individual quantum systems. We have realized a hybrid atomic-mechanical experiment consisting of a SiN membrane oscillator cryogenically precooled to 500 mK and optically coupled to a cloud of laser cooled Rb atoms. Here, we demonstrate active feedback cooling of the oscillator to a minimum mode occupation of n = 16 corresponding to a mode temperature of T = 200 μK. Furthermore, we characterize in detail the coupling of the membrane to the atoms by means of sympathetic cooling. B…
We present a complete theory for laser cooling of a macroscopic radio-frequency LC electrical circuit by means of an optoelectromechanical system, consisting of an optical cavity dispersively coupled to a nanomechanical oscillator, which is in turn capacitively coupled to the LC circuit of interest. We determine the optimal parameter regime where the LC resonator can be cooled down to its quantum ground state, which requires a large optomechanical cooperativity, and a larger electromechanical cooperativity. Moreover, comparable optomechanical and electromechanical coupling rates are preferable…
Sympathetic cooling of an atomic Fermi gas by a Bose gas is studied by solution of the coupled quantum Boltzmann equations for the confined gas mixture. Results for equilibrium temperatures and relaxation dynamics are presented, and some simple models developed. Our study illustrate that a combination of sympathetic and forced evaporative cooling enables the Fermi gas to be cooled to the degenerate regime where quantum statistics, and mean field effects are important. The influence of mean field effects on the equilibrium spatial distributions is discussed qualitatively.
We discuss the coupling of the motion of two ion species in separate Penning traps via a common tank circuit. The enhancement of the coupling assisted by the tank circuit is demonstrated by an avoided crossing behavior measurement of the motional modes of two coupled ions. We propose an intermittent laser cooling method for sympathetic cooling and provide a theoretical description. The technique enables tuning of the coupling strength between two ion species in separate traps and thus allows for efficient sympathetic cooling of an arbitrary type of single ion for high-precision Penning-trap ex…
Modular mixed-species ion-trap networks are a promising framework for scalable quantum information processing, where one species acts as a memory qubit and another as a communication qubit. This architecture requires high-fidelity mixed-species entangling gates to transfer information from communication to memory qubits through their collective motion. We investigate the character of the motional modes of a mixed-species ion chain for entangling operations and also sympathetic cooling. We find that the laser power required for high-fidelity entangling gates based on transverse modes is at leas…
We propose a new way for sympathetic cooling of ions in an electromagnetic Paul trap: it implies the use for this purpose of cold buffer atoms in the region of atom-ion confinement-induced resonance (CIR). The problem is that the unavoidable micromotion of the ion and the long-range nature of its interaction with the environment of colder atoms in a hybrid atomic-ion trap prevent its sympathetic cooling. We show that the destructive effect of ion micromotion on its sympathetic cooling can however be suppressed in the vicinity of the atom-ion CIR. The origin of this is the "fermionization" of t…
Cooling the center-of-mass motion of levitated nanoparticles provides a route to quantum experiments at mesoscopic scales. Here we demonstrate three-dimensional sympathetic cooling and detection of the center-of-mass motion of a levitated silica nanoparticle. The nanoparticle is electrostatically coupled to a feedback-cooled particle while both particles are trapped in the same Paul trap. We identify two regimes, based on the strength of the cooling: in the first regime, the sympathetically cooled particle thermalizes with the directly cooled one, while in the second regime, the sympatheticall…
We show, both experimentally and theoretically, that sympathetic cooling of $^{87}$Rb atoms in the $|F=2,m_F=2>$ state by evaporatively cooled atoms in the $|F=1,m_F=-1>$ state can be precisely controlled to produce dual or single condensate in either state. We also study the thermalization rate between two species. Our model renders a quantitative account of the observed role of the overlap between the two clouds and points out that sympathetic cooling becomes inefficient when the masses are very different. Our calculation also yields an analytical expression of the thermalization rate for a …
Sympathetic cooling of trapped ions has become an indispensable tool for quantum information processing and precision spectroscopy. In the simplest situation a single Doppler-cooled ion sympathetically cools another ion which typically has a different mass. We analytically investigate the effect of the mass ratio of such an ion crystal on the achievable temperature limit in the presence of external heating. As an example, we show that cooling of a single Al+ with Be+, Mg+ and Ca+ ions provides similar results for heating rates typically observed in ion traps, whereas cooling ions with a larger…
It is shown that the translational degrees of freedom of a large variety of molecules, from light diatomic to heavy organic ones, can be cooled sympathetically and brought to rest (crystallized) in a linear Paul trap. The method relies on endowing the molecules with an appropriate positive charge, storage in a linear radiofrequency trap, and sympathetic cooling. Two well--known atomic coolant species, ${}^9{\hbox{Be}}^+$ and ${}^{137}{\hbox{Ba}}^+$, are sufficient for cooling the molecular mass range from 2 to 20,000 amu. The large molecular charge required for simultaneous trapping of heavy m…
Sympathetic Cooling of Levitated Optomechanics through Nonreciprocal Coupling
Center for Quantum Technology Research and Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurements (MOE), School of Physics, Beijing Institute of Technology（北京理工大学物理学院量子技术研究中心及先进光电子量子架构与测量教育部重点实验室）
We use electromagnetically induced transparency (EIT) laser cooling to cool motional modes of a linear ion chain. As a demonstration, we apply EIT cooling on $^{24}Mg^+$ ions to cool the axial modes of a $^9Be^+$ - $^{24}Mg^+$ ion pair and a $^9Be^+$ - $^{24}Mg^+$ - $^{24}Mg^+$ - $^9Be^+$ ion chain, thereby sympathetically cooling the $^{9}$Be$^{+}$ ions. Compared to previous implementations of conventional Raman sideband cooling, we achieve approximately an order-of-magnitude reduction in the duration required to cool the modes to near the ground state and significant reduction in required la…
Cold molecular ions are promising candidates in various fields ranging from precision spectroscopy and test of fundamental physics to ultra-cold chemistry. Control of internal and external degrees of freedom is a prerequisite for many of these applications. Motional ground state cooling represents the starting point for quantum logic-assisted internal state preparation, detection, and spectroscopy protocols. Robust and fast cooling is crucial to maximize the fraction of time available for the actual experiment. We optimize the cooling rate of ground state cooling schemes for single $^{25}\math…
We present and derive analytic expressions for a fundamental limit to the sympathetic cooling of ions in radio-frequency traps using cold atoms. The limit arises from the work done by the trap electric field during a long-range ion-atom collision and applies even to cooling by a zero-temperature atomic gas in a perfectly compensated trap. We conclude that in current experimental implementations this collisional heating prevents access to the regimes of single-partial-wave atom-ion interaction or quantized ion motion. We determine conditions on the atom-ion mass ratio and on the trap parameters…
Efficient cooling of trapped charged particles is essential to many fundamental physics experiments, to high-precision metrology, and to quantum technology. Until now, sympathetic cooling has required close-range Coulomb interactions, but there has been a sustained desire to bring laser-cooling techniques to particles in macroscopically separated traps, extending quantum control techniques to previously inaccessible particles such as highly charged ions, molecular ions and antimatter. Here we demonstrate sympathetic cooling of a single proton using laser-cooled Be+ ions in spatially separated …
Long range polarization forces between ions and neutral atoms result in large elastic scattering cross sections, e.g., 10^6 a.u. for Na+ on Na or Ca+ on Na at cold and ultracold temperatures. This suggests that a hybrid ion-neutral trap should offer a general means for significant sympathetic cooling of atomic or molecular ions. We present SIMION 7.0 simulation results concerning the advantages and limitations of sympathetic cooling within a hybrid trap apparatus, consisting of a linear rf Paul trap concentric with a Na magneto-optical trap (MOT). This paper explores the impact of various heat…
We report the trapping of ultracold neutral $ \text{Rb}$ atoms and $ \text{Ba}^+ $ ions in a common optical potential in absence of any radiofrequency (RF) fields. We prepare $ \text{Ba}^+ $ at $ 370 ~ μK $ and demonstrate efficient sympathetic cooling by $100 ~ μK $ after one collision. Our approach is currently limited by the $ \text{Rb}$ density and related three-body losses, but it overcomes the fundamental limitation in RF traps set by RF-driven, micromotion-induced heating. It is applicable to a wide range of ion-atom species, and may enable novel ultracold chemistry experiments and comp…
Sympathetic cooling with ultracold atoms and atomic ions enables ultralow temperatures in systems where direct laser or evaporative cooling is not possible. It has so far been limited to the cooling of other microscopic particles, with masses up to $90$ times larger than that of the coolant atom. Here we use ultracold atoms to sympathetically cool the vibrations of a Si$_3$N$_4$ nanomembrane, whose mass exceeds that of the atomic ensemble by a factor of $10^{10}$. The coupling of atomic and membrane vibrations is mediated by laser light over a macroscopic distance and enhanced by placing the m…
We report a detailed investigation on near-ground state cooling of one and two trapped atomic ions. We introduce a simple sideband cooling method for confined atoms and ions, using RF radiation applied to bare ionic states in a static magnetic field gradient, and demonstrate its application to ions confined at secular trap frequencies, $ω_z \approx 2π\times 117 $kHz. For a single \ybplus ion, the sideband cooling cycle reduces the average phonon number, $\left\langle\,n\,\right\rangle$ from the Doppler limit to $\left\langle\,n\,\right\rangle =$ 0.30(12). This is in agreement with the theoreti…
We investigate the dynamics of an ion sympathetically cooled by another laser-cooled ion or small ion crystal. To this end, we develop simple models of the cooling dynamics in the limit of weak Coulomb interactions. Experimentally, we create a two-ion crystal of Ca$^+$ and Al$^+$ by photo-ionization of neutral atoms produced by laser ablation. We characterize the velocity distribution of the laser-ablated atoms crossing the trap by time-resolved fluorescence spectroscopy. We observe neutral atom velocities much higher than the ones of thermally heated samples and find as a consequence long sym…
Current experimental efforts to test the fundamental CPT symmetry with single (anti-)protons are progressing at a rapid pace but are hurt by the nonzero temperature of particles and the difficulty of spin state detection. We describe a laser-based and quantum logic inspired approach to single (anti-)proton cooling and state detection.
We discuss a sympathetic cooling strategy that can successfully mitigate fermion-hole heating in a dilute atomic Fermi-Bose mixture and access the temperature regime in which the fermions behave as a Fermi liquid. We introduce an energy-based formalism to describe the temperature dynamics with which we study a specific and promising mixture composed of 6Li and 87Rb. Analyzing the harmonically trapped mixture, we find that the favourable features of this mixture are further enhanced by using different trapping frequencies for the two species.
Cooling a range of molecules to ultracold temperatures (<1 mK) is a difficult but important challenge in molecular physics and chemistry. Collective cavity cooling of molecules is a promising method that does not rely on molecular energy level and thus can be applied to all molecules in principle. However, the initial lack of cold molecules leads to the difficulty in its experimental implementation. We show that efficient collective sympathetic cooling of molecules to sub-mK temperatures using a large ensemble of atoms within a cavity is feasible. This approach is a new type of sympathetic coo…
Isotope-selective Ion Trapping via Sympathetic Cooling using a Surface-Electrode Trap with a Hole for Collimated Atomic Loading
Graduate School of Engineering Science, Osaka University（大阪大学工学研究科）；Institute for Integrated Radiation and Nuclear Science, Kyoto University（京都大学辐射核科学综合研究所）；National Institute of Information and Communications Technology（信息通信研究机构）；Center of Quantum Information and Quantum Biology, Osaka University（大阪大学量子信息与量子生物学中心）
Quantum theory of electrically levitated nanoparticle-ion systems: Motional dynamics and sympathetic cooling
Institute for Theoretical Physics and Vienna Center for Quantum Science and Technology, Technical University of Vienna（维也纳大学理论物理研究所与维也纳量子科学与技术中心）；Institut für Experimentalphysik, Universität Innsbruck（因斯布鲁克大学实验物理研究所）
Precision optical spectroscopy of exotic ions reveals accurate information about nuclear properties such as charge radii and magnetic and quadrupole moments. Thorium ions exhibit unique nuclear properties with high relevance for testing symmetries of nature. We report loading and trapping of single $^{232}$Th$^+$ ions in a linear Paul trap, embedded into and sympathetically cooled by small crystals of trapped $^{40}$Ca$^+$ ions. Trapped Th ions are identified in a non-destructive manner from the voids in the laser-induced Ca fluorescence pattern emitted by the crystal, and alternatively, by me…
We reported the realization of a $^{174}\mathrm{Yb}^+$-$^{113}\mathrm{Cd}^+$ bi-species Coulomb crystal comprising $^{174}\mathrm{Yb}^+$ ions as coolant and verified its potential for application as a $^{113}\mathrm{Cd}^+$ microwave frequency standard employing sympathetic cooling.The two species of massive ions stably trapped in a Paul trap make up this large two-component crystal. The $^{113}\mathrm{Cd}^+$ ions are trapped in the center, which reduces considerably RF heating and excess micromotion to which the $^{113}\mathrm{Cd}^+$ ions are subjected. Under this scheme, the uncertainty due t…
Sympathetic cooling is the process of energy exchange between a system and a colder bath. We investigate this fundamental process in an atom-ion experiment where the system is composed of a single ion, trapped in a radio-frequency Paul trap, and prepared in a coherent state of ~200 K and the bath is an ultracold cloud of atoms at μK temperature. We directly observe the sympathetic cooling dynamics with single-shot energy measurements during one, to several, collisions in two distinct regimes. In one, collisions predominantly cool the system with very efficient momentum transfer leading to cool…
We propose a scheme to actively cool the fundamental flexural (out-of-plane) mode of a graphene sheet via vacuum forces. Our setup consists in a cold atom cloud placed close to a graphene sheet at distances of a few micrometers. The atoms couple to the graphene membrane via Casimir-Polder forces. By deriving a self-consistent set of equations governing the dynamics of the atomic gas and the flexural modes of the graphene, we show to be possible to cool graphene from room temperatures by actively (laser) cooling an atomic gas. By choosing the right set of experimental parameter we are able to c…
A mixed system of cooled and trapped, ions and atoms, paves the way for ion assisted cold chemistry and novel many body studies. Due to the different individual trapping mechanisms, trapped atoms are significantly colder than trapped ions, therefore in the combined system, the strong binary ion$-$atom interaction results in heat flow from ions to atoms. Conversely, trapped ions can also get collisionally heated by the cold atoms, making the resulting equilibrium between ions and atoms intriguing. Here we experimentally demonstrate, Rubidium ions (Rb$^+$) cool in contact with magneto-optically …
Current precision experiments with single (anti)protons to test CPT symmetry progress at a rapid pace, but are complicated by the need to cool particles to sub-thermal energies. We describe a cryogenic Penning-trap setup for $^9$Be$^+$ ions designed to allow coupling of single (anti)protons to laser-cooled atomic ions for sympathetic cooling and quantum logic spectroscopy. We report on trapping and laser cooling of clouds and single $^9$Be$^+$ ions. We discuss prospects for a microfabricated trap to allow coupling of single (anti)protons to laser-cooled $^9$Be$^+$ ions for sympathetic laser co…
Thermalization of a system in the presence of a heat bath has been the subject of many theoretical investigations especially in the framework of solid-state physics. In this setting, the presence of a large bandwidth for the frequency distribution of the harmonic oscillators schematizing the heat bath is crucial, as emphasized in the Caldeira-Leggett model. By contrast, ultracold gases in atomic traps oscillate at well-defined frequencies and therefore seem to lie outside the Caldeira-Leggett paradigm. We introduce interaction Hamiltonians which allow us to adapt the model to an atomic physics…
We predict concurrent selforganisation and cooling of multispecies ensembles of laser-illuminated polarisable particles within a high-Q cavity mode. Resonant collective scattering of laser light into the cavity creates optical potentials which above a threshold pump power transforms a homogeneous particle distribution to a crystalline order for all constituents. Adding extra particles of any mass and temperature always lowers the pump power required for selfordering and allows to concurrently trap atoms, for which high phase-space densities are readily available, in combination with many other…
Simulating computationally intractable many-body problems on a quantum simulator holds great potential to deliver insights into physical, chemical, and biological systems. While the implementation of Hamiltonian dynamics within a quantum simulator has already been demonstrated in many experiments, the problem of initialization of quantum simulators to a suitable quantum state has hitherto remained mostly unsolved. Here, we show that already a single dissipatively driven auxiliary particle can efficiently prepare the quantum simulator in a low-energy state of largely arbitrary Hamiltonians. We …
We study from the point of view of quantum logic the properties of the collective oscillations of a linear chain of ions trapped in a linear Paul trap and composed of two ion species. We discuss extensively sympathetic cooling of the chain and the effect of anharmonicity on laser-cooling and quantum-information processing.
We demonstrate key multi-qubit quantum logic primitives in a dual-species trapped-ion system based on $^{40}$Ca+ and $^{88}$Sr+ ions, using two optical qubits with quantum-logic-control frequencies in the red to near-infrared range. With all ionization, cooling, and control wavelengths in a wavelength band similar for the two species and centered in the visible, and with a favorable mass ratio for sympathetic cooling, this pair is a promising candidate for scalable quantum information processing. Same-species and dual-species two-qubit gates, based on the Moelmer-Soerensen interaction and perf…
It is shown that a two-qubit phase gate and SWAP operation between ground states of cold trapped ions can be realised in one step by simultaneously applying two laser fields. Cooling during gate operations is possible without perturbing the computation and the scheme does not require a second ion species for sympathetic cooling. On the contrary, the cooling lasers even stabilise the desired time evolution of the system. This affords gate operation times of nearly the same order of magnitude as the inverse coupling constant of the ions to a common vibrational mode.
We provide a comprehensive theoretical framework for describing the dynamics of a single trapped ion interacting with a neutral buffer gas, thus extending our previous studies on buffer-gas cooling of ions beyond the critical mass ratio [B. Höltkemeier et al., Phys. Rev. Lett. 116, 233003 (2016)]. By transforming the collisional processes into a frame, where the ion's micromotion is assigned to the buffer gas atoms, our model allows one to investigate the influence of non-homogeneous buffer gas configurations as well as higher multipole orders of the radio-frequency trap in great detail. Depen…
We discuss laser-based and quantum logic inspired cooling and detection methods amenable to single (anti-)protons. These would be applicable e.g. in a g-factor based test of CPT invariance as currently pursued within the BASE collaboration. Towards this end, we explore sympathetic cooling of single (anti-)protons with atomic ions as suggested by Heinzen and Wineland (1990).
Storage lifetime and capacity are two important factors to characterize the performance of a quantum memory. Here we report the stable trapping of above 200 ions in a cryogenic setup, and demonstrate the combination of the multi-qubit capacity and long storage lifetime by measuring the coherence time of randomly chosen ions to be on the order of hundreds of milliseconds. We apply composite microwave pulses to manipulate qubit states globally for efficient characterization of different storage units simultaneously, and we compare the performance of the quantum memory with and without the sympat…
Ultra-high sensitivity detection of quantum-scale displacements in cavity optomechanics optimises the combined errors from measurement back-action and imprecisions from incoming quantum noises. This sets the well-known Standard Quantum Limit (SQL). Normal quantum cavity optomechanics allows cooling and detection of a single degree of freedom, along the cavity axis. However, a recent breakthrough that allows quantum ground-state cooling of levitated nanoparticles [Delic et al, arxiv:1911.04406], is uniquely 3D in character, with coupling along the $x$, $y$ and $z$ axes. We investigate current e…
We discuss a hybrid quantum system where a dielectric membrane situated inside an optical cavity is coupled to a distant atomic ensemble trapped in an optical lattice. The coupling is mediated by the exchange of sideband photons of the lattice laser, and is enhanced by the cavity finesse as well as the square root of the number of atoms. In addition to observing coherent dynamics between the two systems, one can also switch on a tailored dissipation by laser cooling the atoms, thereby allowing for sympathetic cooling of the membrane. The resulting cooling scheme does not require resolved sideb…
