The nonlinear photon-photon interaction mediated by a single two-level atom is studied theoretically based on a one-dimensional model of the field-atom interaction. This model allows us to determine the effects of an atomic nonlinearity on the spatiotemporal coherence of a two photon state. Specifically, the complete two photon output wave function can be obtained for any two photon input wave function. It is shown that the quantum interference between the components of the output state associated with different interaction processes causes bunching and anti-bunching in the two photon statistics. This theory may be useful for various applications in photon manipulation, e.g. quantum information processing using photonic qubits, quantum nondemolition measurements, and the generation of entangled photons.
We present a direct measurement of the spatiotemporal coherence of parametric down-conversion in the range of negative group-velocity dispersion. In this case, the frequency-angular spectra are ring-shaped and temporal coherence is coupled to spatial coherence. Correspondingly, the lack of coherence due to spatial displacement can be compensated with the introduction of time delay. We show a simple technique, based on a modified Mach-Zehnder interferometer, which allowed us to measure time coherence and near-field space coherence simultaneously, with complete control of both variables. This te…
We develop a theoretical framework for the analysis of the quantum coherence of light emitted by two independent single-photon sources in an arbitrary environment. The theory provides design rules for the control of the degree of quantum coherence, in terms of classical quantities widely used in nanophotonics. As an important example, we derive generalized conditions to generate superradiant and subradiant states of the emitters, and demonstrate the ability of a structured environment to induce long-range quantum coherence. These results should have broad applications in quantum nanophotonics,…
Photon interference among distant quantum emitters is a promising method to generate large scale quantum networks. Interference is best achieved when photons show long coherence times. For the nitrogen-vacancy defect center in diamond we measure the coherence times of photons via optically induced Rabi oscillations. Experiments reveal a close to Fourier transform (i.e. lifetime) limited width of photons emitted even when averaged over minutes. The projected contrast of two-photon interference (0.8) is high enough to envisage the applications in quantum information processing. We report 12 and …
The correlations of the electrons field-emitted from a superconductor are fully analyzed, both in space and time. It is proposed that a coincidence experiment would reveal a positive correlation between the electrons emitted in opposite directions. The electrons can be entangled and can even violate Bell's inequality. The crucial role played by Andreev's process is scrutinized, analytical formulas are derived for the correlations, and the physics behind the phenomenon is clarified.
Addressing the correlation of Stokes-shifted photons emitted from two quantum emitters
Centro de Física de Materiales (CMF-MPC), CSIC-UPV/EHU（材料物理中心）；University of the Basque Country (UPV/EHU)（巴斯克大学）；Université de Bordeaux, LP2N（波尔多大学）；Institut d’Optique & CNRS, LP2N（光学研究所与法国国家科学研究中心）；Donostia International Physics Center (DIPC)（圣塞巴斯蒂安国际物理中心）；Université de Bordeaux, CNRS, LOMA, UMR 5798（波尔多大学）；Université de Strasbourg, CNRS, Institut de Physique et Chimie des Matériaux de Strasbourg, UMR 7504（斯特拉斯堡大学）；Ikerbasque, Basque Foundation for Science（伊克拉巴斯科，巴斯克科学基金会）
In the general framework of open quantum systems, we assess the impact of the pulse area on single and double quantum coherence (1QC and 2QC) signals extracted from fluorescence emitted by dilute thermal gases. We show that 1QC and 2QC signals are periodic functions of the pulse area, with distinctive features which reflect the particles' interactions via photon exchange, the polarizations of the laser pulses, and the observation direction.
We present a scheme for two-dimensional (2D) atom localization in a three-level atomic system. The scheme is based on quantum coherence via classical standing wave fields between the two excited levels. Our results show that conditional position probability is significantly phase dependent of the applied field and frequency detuning of spontaneously emitted photons. We obtain a single localization peak having probability close to unity by manipulating the control parameters. The effect of atomic level coherence on the sub-wavelength localization has also been studied. Our scheme may be helpful…
We investigate theoretically the quantum-coherence properties of the cathodoluminescence (CL) emission produced by a temporally modulated electron beam. Specifically, we consider the quantum-optical correlations of CL from electrons that are previously shaped by a laser field. The main prediction here is the presence of phase correlations between the emitted CL field and the electron-modulating laser, even though the emission intensity and spectral profile are independent of the electron state. In addition, the coherence of the CL field extends to harmonics of the laser frequency. Since electr…
Single photons produced by fundamentally dissimilar physical processes will in general not be indistinguishable. We show how photons produced from a quantum dot and by parametric down-conversion in a nonlinear crystal can be manipulated to be indistinguishable. The measured two-photon coalescence probability is 16%, and is limited by quantum-dot decoherence. Temporal filtering to the quantum dot coherence time and accounting for detector time response increases this to 61% while retaining 25% of the events. This technique can connect different elements in a scalable quantum network.
We report an electrically driven semiconductor single photon source capable of emitting photons with a coherence time of up to 400 ps under fixed bias. It is shown that increasing the injection current causes the coherence time to reduce and this effect is well explained by the fast modulation of a fluctuating environment. Hong-Ou-Mandel type two-photon interference using a Mach-Zehnder interferometer is demonstrated using this source to test the indistinguishability of individual photons by post-selecting events where two photons collide at a beamsplitter. Finally, we consider how improvement…
The squeezing spectrum of the fluorescence field emitted from a four-level atom in $J=1/2$ to $J=1/2$ configuration driven by two coherent fields is studied. We find that the squeezing properties of the fluorescence radiation are significantly influenced by the presence of vacuum-induced coherence in the atomic system. It is shown that such coherence induces spectral squeezing in phase quadratures of the fluorescence light for both weak and strong driving fields. The dependence of the squeezing spectrum on the relative phase of the driving fields is also investigated. Effects such as enhanceme…
We study C70 fullerene matter waves in a Talbot-Lau interferometer as a function of their temperature. While the ideal fringe visibility is observed at moderate molecular temperatures, we find a gradual degradation of the interference contrast if the molecules are heated before entering the interferometer. A method is developed to assess the distribution of the micro-canonical temperatures of the molecules in free flight. This way the heating-dependent reduction of interference contrast can be compared with the predictions of quantum theory. We find that the observed loss of coherence agrees q…
This paper reports a novel single mode source of narrow-band entangled photon pairs at telecom wavelengths under continuous wave excitation, based on parametric down conversion. For only 7 mW of pump power it has a created spectral radiance of 0.08 pairs per coherence length and a bandwidth of 10 pm (1.2 GHz). The effectively emitted spectral brightness reaches 3.9*10^5 pairs /(s pm). Furthermore, when combined with low jitter single photon detectors, such sources allow for the implementation of quantum communication protocols without any active synchronization or path length stabilization. A …
The resonance fluorescence of a four-level atom in J = 1/2 to J = 1/2 transition driven by two coherent fields is studied. We find that the incoherent fluorescence spectrum shows a direct indication of vacuum-induced coherence in the atomic system. We show that such coherence manifests itself via an enhancement or suppression of the spectral peaks in the $π$-polarized fluorescence. The effect of the relative phase of the driving fields on the spectral features is also investigated. We show that phase-dependent enhancement or suppression of the fluorescence peaks appears in the incoherent spect…
Coherence can be induced or stimulated in parametric down-conversion using two or three crystals when, for example, the idler modes of the crystals are aligned. Previous experiments with induced coherence [Phys. Rev. Lett. 114, 053601 (2015)] focused on which-path information and the role of vacuum fields in realizing complementarity via reduced visibility in single-photon interference. Here we describe experiments comparing induced and stimulated coherence. Different single-photon interference experiments were performed by blocking one of the pump beams in a three-crystal setup. Each counted …
We demonstrate fast and accurate control of the evolution of collective atomic coherences in an Erbium doped solid using external electric fields. This is achieved by controlling the inhomogeneous broadening of Erbium ions emitting at 1536 nm using an electric field gradient and the linear Stark effect. The manipulation of atomic coherence is characterized with the collective spontaneous emission (optical free induction decay) emitted by the sample after an optical excitation, which does not require any previous preparation of the atoms. We show that controlled dephasing and rephasing of the a…
Unitarity is a pillar of quantum theory. Nevertheless, it is also a source of several of its conceptual problems. We note that in a world where measurements are relational, as is the case in gravitation, quantum mechanics exhibits a fundamental level of loss of coherence. This can be the key to solving, among others, the puzzles posed by the black hole information paradox, the formation of inhomogeneities in cosmology and the measurement problem in quantum mechanics.
We identify an optical signature for detecting entanglement in experimental nanostructure systems comprising coupled excitonic qubits. This signature owes its strength to non-Markovian dynamical effects in the second-order temporal coherence function of the emitted radiation. We calculate autocorrelation and cross-correlation functions for both selective and collective light excitation, and prove that the coherence properties of the emitted light do indeed carry information about the entanglement of the initial multi-qubit state. We also show that this signature can survive in the presence of …
We investigate the nonlinear interaction between two photons in a single input pulse at an atomic two level nonlinearity. A one dimensional model for the propagation of light to and from the atom is used to describe the precise spatiotemporal coherence of the two photon state. It is shown that the interaction generates spatiotemporal entanglement in the output state similar to the entanglement observed in parametric downconversion. A method of generating photon pairs from coherent pump light using this quantum mechanical four wave mixing process is proposed.
Dicke superrandiance is a cooperative phenomenon which arises from the collective coupling of an ensemble of atoms to the electromagnetic radiation. Here we discuss the quantifying of quantum coherence for the Dicke model of superradiance in the mean-field approximation. We found the single-atom $l_1$-norm of coherence is given by the square root of the normalized average intensity of radiation emitted by the superradiant system. This validates quantum coherence as a useful figure of merit towards the understanding of superradiance phenomenon in the mean-field approach. In particular, this res…
The spatial coherence of an atomic wavepacket can be detected in the scattered photons, even when the center-of-mass motion is in the quantum coherent superposition of two distant, non-overlapping wave packets. Spatial coherence manifests itself in the power spectrum of the emitted photons, whose spectral components can exhibit interference fringes as a function of the emission angle. The contrast and the phase of this interference pattern provide information about the quantum state of the center of mass of the scattering atom.
We introduce a model of non-unitary quantum dynamics that exhibits infinitely long-lived discrete spatiotemporal order robust against any unitary or dissipative perturbation. Ergodicity is evaded by combining a sequence of projective measurements with a local feedback rule that is inspired by Toom's `North-East-Center' classical cellular automaton. The measurements in question only partially collapse the wavefunction of the system, allowing some quantum coherence to persist. We demonstrate our claims using numerical simulations of a Clifford circuit in two spatial dimensions which allows acces…
It is not widely appreciated that many subtleties are involved in the accurate measurement of intensity-correlated photons; even for the original experiments of Hanbury Brown and Twiss (HBT). Using a monolithic 4x4 array of single-photon avalanche diodes (SPADs), together with an off-chip algorithm for processing streaming data, we investigate the difficulties of measuring second-order photon correlations g2 in a wide variety of light fields that exhibit dramatically different correlation statistics: a multimode He-Ne laser, an incoherent intensity-modulated lamp-light source and a thermal lig…
A simplified theory for the wavepackets of the photons emitted during the read process of a quantum memory formed by cold atoms is provided. We arrive at analytical expressions for the single- and double-photon emissions, evidencing superradiant features in both cases. In the two-photon case, both photons are emitted in the same spatiotemporal mode, characterizing a superradiant emission of a Fock state of light with two excitations. Experiments confirm the theoretical predictions with a satisfactory agreement.
We have measured the 2-particle correlation function of atoms from a Bose--Einstein condensate participating in a superradiance process, which directly reflects the 2nd order coherence of the emitted light. We compare this correlation function with that of atoms undergoing stimulated emission. Whereas the stimulated process produces correlations resembling those of a coherent state, we find that superradiance, even in the presence of strong gain, shows a correlation function close to that of a thermal state, just as for ordinary spontaneous emission.
Recent developments in the coherent manipulation of electrons in ballistic conductors include the generation of time-periodic electrical currents involving one to few electronic excitations per period. However, using individual electrons as carrier of quantum information for flying qubit computation or quantum metrology applications calls for a general method to unravel the single-particle excitations embedded in a quantum electrical current and how quantum information is encoded within it. Here, we propose a general signal processing algorithm to extract the elementary single-particle states,…
In this paper, we investigate, phonon effects on the optical properties of a spherical quantum dot. For this purpose, we consider the interaction of a spherical quantum dot with classical and quantum fields while the exciton of quantum dot interacts with a solid state reservoir. We show that phonons strongly affect the Rabi oscillations and optical coherence on first picoseconds of dynamics. We consider the quantum statistics of emitted photons by quantum dot and we show that these photons are anti-bunched and obey the sub-Poissonian statistics. In addition, we examine the effects of detuning …
In spontaneous emission an atom in an excited state undergoes a transition to the ground state and emits a single photon. Associated with the emission is a change of the atomic momentum due to photon recoil. Photon emission can be modified close to surfaces and in cavities. For an ion, localized in front of a mirror, coherence of the emitted resonance fluorescence has been reported. In free space experiments demonstrated that spontaneous emission destroys motional coherence. Here we report on motional coherence created by a single spontaneous emission event close to a mirror surface. The coher…
We present the first calculation of coherent backscattering with inelastic scattering by saturated atoms. We consider the scattering of a quasi-monochromatic laser pulse by two distant atoms in free space. By restricting ourselves to scattering of two photons, we employ a perturbative approach, valid up to second order in the incident laser intensity. The backscattering enhancement factor is found to be smaller than two (after excluding single scattering), indicating a loss of coherence between the doubly scattered light emitted by both atoms. Since the undetected photon carries information ab…
Induced coherence in parametric down-conversion between two coherently pumped nonlinear crystals that share a common idler mode can be used as an imaging technique. Based on the interference between the two signal modes of the crystals, an image can be reconstructed. By obtaining an expression for the interference pattern that is valid in both the low- and the high-gain regimes of parametric down-conversion, we show how the coherence of the light emitted by the two crystals can be controlled. With our comprehensive analysis we provide deeper insight into recent discussions about the applicatio…
We examine quantum statistics of optical photons emitted from atomic ensembles which are classically driven and simultaneously coupled to a two-level atom via microwave photon exchange. Quantum statistics and correlations are analyzed by calculating second order coherence degree, von Neumann entropy, spin squeezing for multi-particle entanglement, as well as genuine two and three-mode entanglement parameters for steady state and non-equilibrium situations. Coherent transfer of population between the radiation modes and quantum state mapping between the two-level atom and the optical modes are …
Almost all novel observable phenomena in quantum optics are related to the quantum coherence. The coherence here is determined by the relative phase inside a state. Unfortunately, so far all the relevant experimental results in quantum optics are insensitive to the phase information of the coherent state. Lack of phase information may cause serious consequences in many problems in quantum optics. For example, an ensemble of two mode squeezed states is a classical ensemble if the phase in each state is totally random; but it is a non-classical ensemble if the phase in each state is fixed. As a …
Dicke superradiance, i.e., the enhanced spontaneous emission of coherent radiation, is often attributed to radiation emitted by synchronized dipoles coherently oscillating in phase. At the same time, Dicke derived superradiance assuming atoms in entangled Dicke states which do not display any dipole moment. To shed light on this apparent paradox, we study the intensity distribution arising from two identical two-level atoms prepared either in an entangled Dicke state or in a separable atomic state with non-vanishing dipole moment. We find that the two configurations produce similar far field i…
In theories with long-range forces like QED or perturbative gravity, only rates that include emitted soft radiation are non-vanishing. Independently of detector resolution, finite observables can only be obtained after integrating over the IR-component of this radiation. This integration can lead to some loss of quantum coherence. In this note, however, we argue that it should in general not lead to full decoherence. Based on unitarity, we suggest a way to define non-vanishing off-diagonal pieces of the IR-finite density matrix. For this IR-finite density matrix, we estimate the dependence of …
We theoretically and experimentally investigate quantum features of an interacting light-matter system from a multidisciplinary perspective, unifying approaches from semiconductor physics, quantum optics, and quantum information science. To this end, we quantify the amount of quantum coherence that results from the quantum superposition of Fock states, constituting a measure of the resourcefulness of the produced state for modern quantum protocols. As an archetypal example of a hybrid light-matter interface, we study a polariton condensate and implement a numerical model to predict its propert…
The detection of photocurrents is central to understanding and harnessing the interaction of light with matter. Although widely used, transport-based detection averages over spatial distributions and can suffer from low photocarrier collection efficiency. Here, we introduce a contact-free method to spatially resolve local photocurrent densities using a proximal quantum magnetometer. We interface monolayer MoS2 with a near-surface ensemble of nitrogen-vacancy centers in diamond and map the generated photothermal current distribution through its magnetic field profile. By synchronizing the photo…
We report on optical detection of a single photostable Ce3+ ion in an yttrium aluminium garnet (YAG) crystal and on its magneto-optical properties at room temperature. The quantum state of an electron spin of the emitting level of cerium ion in YAG can be initialized by circularly polarized laser pulse. Furthermore, its quantum state can be read out by observing temporal behaviour of circularly polarized fluorescence of the ion. This implies direct mapping of the spin quantum state of Ce3+ ion onto the polarization state of the emitted photon and represents one-way quantum interface between a …
Quantum correlations and coherence generated between two free spinless particles in the lattice, interacting with a common quantum phonon bath, are studied. The reduced density matrix is solved using the Markov approach. We show that the bath induces correlations between the particles. The coherence induced by the bath is studied, calculating off-diagonal elements of the density matrix, spatiotemporal dispersion, purity and quantum mutual information. We find a characteristic time-scale pointing out when this coherence is maximum. In addition, a Wigner-like distribution in the phase-space (lat…
A full quantum theory beyond the mean-field regime is developed for an exciton polariton condensate, to gain a complete understanding of quantum fluctuations. We find analytical solution for the polariton density matrix, showing the polariton nonlinearity causing fast relaxation correlated with the pump so as to yield the condensation at threshold. Increasing the pump intensity, a nonequilibrium phase transition towards the condensation of lower polaritons emerges, with a statistics transiting from a thermal, through a super-Poissonian and to a nonclassical distribution beyond the understandin…
We study the quantum entanglement of the quasiparticle pairs emitted by analogue black holes. We use a phenomenological description of the spectra in dispersive media to study the domains in parameter space where the final state is non-separable. In stationary flows, three modes are involved in each sector of fixed frequency, and not two as in homogeneous situations. The third spectator mode acts as an environment for the pairs, and the strength of the coupling significantly reduces the quantum coherence. The non-separability of the pairs emitted by white holes are also considered, and compare…
Numerous approaches to a quantum theory of gravity posit fundamental ontologies that exclude spacetime, either partially or wholly. This situation raises deep questions about how such theories could relate to the empirical realm, since arguably only entities localized in spacetime can ever be observed. Are such entities even possible in a theory without fundamental spacetime? How might they be derived, formally speaking? Moreover, since by assumption the fundamental entities can't be smaller than the derived (since relative size is a spatiotemporal notion) and so can't 'compose' them in any or…
The development of spectroscopic techniques able to detect and verify quantum coherence is a goal of increasing importance given the rapid progress of new quantum technologies, the advances in the field of quantum thermodynamics, and the emergence of new questions in chemistry and biology regarding the possible relevance of quantum coherence in biochemical processes. Ideally, these tools should be able to detect and verify the presence of quantum coherence in both the transient dynamics and the steady state of driven-dissipative systems, such as light-harvesting complexes driven by thermal pho…
Electric noise from metallic surfaces is a major obstacle towards quantum applications with trapped ions due to motional heating of the ions. Here, we discuss how the same noise source can also lead to pure dephasing of motional quantum states. The mechanism is particularly relevant at small ion-surface distances, thus imposing a new constraint on trap miniaturization. By means of a free induction decay experiment, we measure the dephasing time of the motion of a single ion trapped 50~$μ$m above a Cu-Al surface. From the dephasing times we extract the integrated noise below the secular frequen…
Engineering the impact of phonon dephasing on the coherence of a WSe$_{2}$ single-photon source via cavity quantum electrodynamics
Carl von Ossietzky University of Oldenburg（奥尔登堡卡尔·冯·奥西茨基大学）；University of Bremen（不来梅大学）；University of Michigan（密歇根大学）；Friedrich Schiller University Jena（耶拿弗里德里希·席勒大学）；Arizona State University（亚利桑那州立大学）；National Institute for Materials Science（日本国立材料研究所）
Coherent processing of quantum information and attosecond science had so far little in common. We here show that recent data in high harmonic emission reveal quantum information processing at the attosecond timescale. By observing the interference pattern created by the spatiotemporal overlap of photons emitted by two interfering electron paths we generate a photon Hadamard gate and thus erase the electron-trajectory information. This allows the measurement of the relative phase in electron-trajectory quantum superpositions and establishes the era of electron-photon quantum coherence and entan…
We consider a voltage-biased Josephson junction between two nanowires hosting Majorana zero modes which occur as topological protected zero-energy excitations at the junction. We show that two Majorana fermions localized at the junction, even though being neutral particles, interact with the electromagnetic field and generate coherent radiation similar to the conventional Josephson radiation. Within a semiclassical analysis of the radiation field, we find that the optical phase gets locked to the superconducting phase difference and that the radiation is emitted at half the Josephson frequency…
Accelerated charges emit electromagnetic radiation. According to classical electrodynamics if the charges move along sufficiently close trajectories they emit coherently, i.e., their emitted energy scales quadratically with their number rather than linearly. By investigating the emission by a two-electron wave packet in the presence of an electromagnetic plane wave within strong-field QED, we show that quantum effects deteriorate the coherence predicted by classical electrodynamics even if the typical quantum nonlinearity parameter of the system is much smaller than unity. We explain this resu…
We study the photonic interactions between two distant atoms which are coupled by an optical element (a lens or an optical fiber) focussing part of their emitted radiation onto each other. Two regimes are distinguished depending on the ratio between the radiative lifetime of the atomic excited state and the propagation time of a photon between the two atoms. In the two regimes, well below saturation the dynamics exhibit either typical features of a bad resonator, where the atoms act as the mirrors, or typical characteristics of dipole-dipole interaction. We study the coherence properties of th…
The fundamental process limiting the coherence of quantum-dot based single-photon sources is the interaction with phonons. We study the effect of phonon decoherence on the indistinguishability of single photons emitted from a quantum dot embedded in a suspended nanobeam waveguide. At low temperatures, the indistinguishability is limited by the coupling between the quantum dot and the fundamental vibrational modes of the waveguide and is sensitive to the quantum-dot position within the nanobeam cross-section. We show that this decoherence channel can be efficiently suppressed by clamping the wa…
To quantify quantum optical coherence requires both the particle- and wave-natures of light. For an ideal laser beam [1,2,3], it can be thought of roughly as the number of photons emitted consecutively into the beam with the same phase. This number, $\mathfrak{C}$, can be much larger than $μ$, the number of photons in the laser itself. The limit on $\mathfrak{C}$ for an ideal laser was thought to be of order $μ^2$ [4,5]. Here, assuming nothing about the laser operation, only that it produces a beam with certain properties close to those of an ideal laser beam, and that it does not have externa…
