We discuss level schemes of small quantum-dot turnstiles and their applicability in the production of entanglement in two-photon emission. Due to the large energy splitting of the single-electron levels, only one single electron level and one single hole level can be made resonant with the levels in the conduction band and valence band. This results in a model with nine distinct levels, which are split by the Coulomb interactions. We show that the optical selection rules are different for flat and tall cylindrically symmetric dots, and how this affects the quality of the entanglement generated in the decay of the biexciton state. The effect of charge carrier tunneling and of a resonant cavity is included in the model.
We discuss a mechanism for generating a maximum entangled state (GHZ) in a coupled quantum dots system, based on analytical techniques. The reliable generation of such states is crucial for implementing solid-state based quantum information schemes. The signature originates from a remarkably weak field pulse or a far off-resonance effects which could be implemented using technology that is currently being developed. The results are illustrated with an application to a specific wide-gap semiconductor quantum dots system, like Zinc Selenide (ZnSe) based quantum dots.
A practical source of high fidelity entangled photons is desirable for quantum information applications and exploring quantum physics. Semiconductor quantum dots have recently been shown to conveniently emit entangled light when driven electrically, however the fidelity was not optimal. Here we show that the fidelity is not limited by decoherence, but by coherent interaction with nuclei. Furthermore we predict that on 100μs timescales, strongly enhanced fidelities could be achieved. This insight could allow tailoring of quantum logic to operate using quantum dots in the fault tolerant regime.
The generation and long-haul transmission of highly entangled photon pairs is a cornerstone of emerging photonic quantum technologies, with key applications such as quantum key distribution and distributed quantum computing. However, a natural limit for the maximum transmission distance is inevitably set by attenuation in the medium. A network of quantum repeaters containing multiple sources of entangled photons would allow to overcome this limit. For this purpose, the requirements on the source's brightness and the photon pairs' degree of entanglement and indistinguishability are stringent. D…
We investigate how decoherence affects the entanglement established between two quantum dots in micro cavities, and propose a tomographic scheme able to measure the entangled state. The scheme we consider establishes the entanglement via the exchange and measurement of a photon. Making the realistic assumption of noise dominated by pure-dephasing processes, we find that the photon must be exchanged and measured on timescales shorter than the quantum dots' characteristic dephasing time for appreciable levels of entanglement to be achieved. The tomographic scheme is able to reconstruct the full …
Generation of polarization-entangled photons from quantum dots via the biexciton-exciton recombination cascade is complicated by the presence of an energy spitting between the intermediate excitonic levels, which severely degrades the quality of the entangled photon source. In this paper we present a novel, conceptually simple and straightforward proposal for restoring the entanglement of said source by applying a cascade of time-dependent operations on the emitted photons. This is in striking contrast with the techniques usually employed, that act on the quantum emitter itself in order to rem…
Multi-photon entangled states are a crucial resource for many applications in quantum information science. Semiconductor quantum dots offer a promising route to generate such states by mediating photon-photon correlations via a confined electron spin, but dephasing caused by the host nuclear spin environment typically limits coherence (and hence entanglement) between photons to the spin $T_2^*$ time of a few nanoseconds. We propose a protocol for the deterministic generation of multi-photon entangled states that is inherently robust against the dominating slow nuclear spin environment fluctuat…
We introduce a scalable photonic platform that enables efficient generation of entangled photon pairs from a semiconductor quantum dot. Our system, which is based on a self-aligned quantum dot-micro-cavity structure, erases the need for complex steps of lithography and nanofabrication. We experimentally show collection efficiency of 0.17 combined with a Purcell enhancement of up to 1.7 in the pair emission process. We harness the potential of our device to generate photon pairs entangled in time bin, reaching a fidelity of 0.84(5) with the maximally entangled state. The achieved pair collectio…
In this work we have proposed a scheme for generating $N$ qubit entangled states which can teleport an unknown state perfectly. By switching on the exchange interaction ($J$) between the qubits one can get the desired states periodically. A multi electron quantum dot can be a possible realization for generating such $N$ qubit states with high fidelity. In the limit of $N \to \infty$, there exists a unique time $t=\frac{1}{J}\cos^{-1}(-1/8)$ where the Hamiltonian dynamics gives the $N$ qubit state that can assist perfect teleportation. We have also discussed the effect of the nuclear spin envir…
With the assistance of a pair of Majorana fermions, we propose schemes to entangle two quantum dots by Lyapunov control in the charge and spin degrees of freedom. Four different schemes are considered, i.e., the teleportation scheme, the crossed Andreev reflection scheme, the intradot spin flip scheme, and the scheme beyond the intradot spin flip. We demonstrate that the entanglement can be generated by modulating the chemical potential of quantum dots with square pulses, which is easily realized in practice. In contrast to Lyapunov control, the preparation of entangled states by adiabatic pas…
The development of scalable sources of non-classical light is fundamental to unlock the technological potential of quantum photonics\cite{Kimble:Nat2008}. Among the systems under investigation, semiconductor quantum dots are currently emerging as near-optimal sources of indistinguishable single photons. However, their performances as sources of entangled-photon pairs are in comparison still modest. Experiments on conventional Stranski-Krastanow InGaAs quantum dots have reported non-optimal levels of entanglement and indistinguishability of the emitted photons. For applications such as entangle…
We show that excitons in coupled quantum dots are ideal candidates for reliable preparation of entangled states in solid-state systems. An optically controlled exciton transfer process is shown to lead to the generation of Bell and GHZ states in systems comprising two and three coupled dots, respectively. The strength and duration of selective light-pulses for producing maximally entangled states are identified by both analytic, and full numerical, solution of the quantum dynamical equations. Experimental requirements to build such entangled states are discussed.
Polarization-resolved single dot spectroscopy performed on (211)B InAs/GaAs quantum dots reveals that the fine structure splitting of the excitonic levels in these dots is much lower compared to the usual (100)-grown InAs dots. Time-resolved measurements confirm the high oscillator strength of these dots, and thus their good quantum efficiency at 4 K, comparable with that of (100) InAs/GaAs dots. Last, photon correlation measurements demonstrate single photon emission out of the excitonic optical transition of these dots. All these features make this novel dot system very promising for impleme…
We describe a mechanism for the production of polarisation-entangled microwaves using intra-band transitions in a pair of quantum dots. This proposal relies neither on spin-orbit coupling nor on control over electron-electron interactions. The quantum correlation of microwave polarisations is obtained from orbital degrees of freedom in an external magnetic field. We calculate the concurrence of emitted microwave photon pairs, and show that a maximally entangled Bell pair is obtained in the limit of weak inter-dot coupling.
We present a first measurement of photon polarization entanglement from the biexciton to ground state cascade of a single InAsP quantum dot embedded in an InP nanowire. We observe a fidelity of 0.76(2) to a reference maximally entangled state as well as a concurrence of 0.57(6).
Bell's inequality in three coupled quantum dots (QDs) within cavity QED, including Forster and exciton-phonon interactions, is investigated theoretically. For an initially entangled state, Bell's inequality is valid for certain times and violated for some other times. It is shown that the system moves from a product state to a entangled state and back again during it's time evolution.
An ideal source of entangled photon pairs combines the perfect symmetry of an atom with the convenient electrical trigger of light sources based on semiconductor quantum dots. We create a naturally symmetric quantum dot cascade that emits highly entangled photon pairs on demand. Our source consists of strain-free GaAs dots self-assembled on a triangular symmetric (111)A surface. The emitted photons strongly violate Bell's inequality and reveal a fidelity to the Bell state as high as 86 (+-2) % without postselection. This result is an important step towards scalable quantum-communication applic…
We investigate the generation of multipartite entangled state in a system of N quantum dots embedded in a microcavity and examine the emergence of genuine multipartite entanglement by three different characterizations of entanglement. At certain times of dynamical evolution one can generate multipartite entangled coherent exciton states or multiqubit $W$ states by initially preparing the cavity field in a superposition of coherent states or the Fock state with one photon, respectively. Finally we study environmental effects on multipartite entanglement generation and find that the decay rate f…
We study biexcitonic states in two tunnel-coupled semiconductor quantum dots and show that such systems provide the possibility to produce polarization- entangled photons or spin-entangled electrons that are spatially separated at production. We distinguish between the various spin configurations and calculate the low-energy biexciton spectrum using the Heitler-London approximation as a function of magnetic and electric fields. The oscillator strengths for the biexciton recombination involving the sequential emission of two photons are calculated. The entanglement of the photon polarizations r…
We report on exciton-acoustic-phonon coupling effects on the generation of exciton maximally entangled states in N=2 and 3 quantum dot systems. In particular, we address the question of the combined effect of laser pulses, appropriate for generating Bell and Greenberger-Horne-Zeilinger entangled states, together with decoherence mechanisms as provided by a phonon reservoir. By solving numerically the master equation for the optically driven exciton-phonon kinetics, we show that the generation of maximally entangled exciton states is preserved over a reasonable parameter window.
To generate entangled photon pairs via quantum dots (QDs), the exciton fine structure splitting (FSS) must be comparable to the exciton homogeneous line width. Yet in the (In,Ga)As/GaAs QD, the intrinsic FSS is about a few tens $μ$eV. To achieve photon entanglement, it is necessary to Cherry-pick a sample with extremely small FSS from a large number of samples, or to apply strong in-plane magnetic field. Using theoretical modeling of the fundamental causes of FSS in QDs, we predict that the intrinsic FSS of InAs/InP QDs is an order of magnitude smaller than that of InAs/GaAs dots, and better y…
More than 80 years passed since the first publication on entangled quantum states. In this period of time the concept of spookily interacting quantum states became an emerging field of science. After various experiments proving the existence of such non-classical states, visionary ideas were put forward to exploit entanglement in quantum information science and technology. These novel concepts have not yet come out of the experimental stage, mostly because of the lack of suitable, deterministic sources of entangled quantum states. Among many systems under investigation, semiconductor quantum d…
Equivalent-neighbor interactions of the conduction-band electron spins of quantum dots in the model of Imamoglu et al. [Phys. Rev. Lett. 83, 4204 (1999)] are analyzed. Analytical solution and its Schmidt decomposition are found and applied to evaluate how much the initially excited dots can be entangled to the remaining dots if all of them are initially disentangled. It is demonstrated that the perfect maximally entangled states (MES) can only be generated in the systems of up to 6 dots with a single dot initially excited. It is also shown that highly entangled states, approximating the MES wi…
A study of highly symmetric site-controlled Pyramidal In0.25Ga0.75As quantum dots (QDs) is presented. It is discussed that polarization-entangled photons can be also obtained from Pyramidal QDs of different designs from the one already reported in Juska et al. (Nat. Phot. 7, 527, 2013). Moreover, some of the limitations for a higher density of entangled photon emitters are addressed. Among these issues are (1) a remaining small fine-structure splitting and (2) an effective QD charging under non-resonant excitation conditions, which strongly reduce the number of useful biexciton-exciton recombi…
Tomographic analysis demonstrates that the polarization state of pairs of photons emitted from a biexciton decay cascade becomes entangled when spectral filtering is applied. The measured density matrix of the photon pair satisfies the Peres criterion for entanglement by more than 3 standard deviations of the experimental uncertainty and violates Bell's inequality. We show that the spectral filtering erases the ``which path'' information contained in the photons color and that the remanent information in the quantum dot degrees of freedom is negligible.
Entangled photon generation from semiconductor quantum dots via the biexciton-exciton cascade underlies various decoherence mechanisms related to the solid-state nature of the quantum emitters. So far, this has prevented the demonstration of nearly-maximally entangled photons without the aid of inefficient and complex post-selection techniques that are hardly suitable for quantum communication technologies. Here, we tackle this challenge using strain-tunable GaAs quantum dots driven under two-photon resonant excitation and with strictly-degenerate exciton states. We demonstrate experimentally …
The time evolution of entanglement for excitons in two quantum dots embedded in a single mode cavity is studied in a ``spin-boson'' regime. It is found that although with the dissipation from the boson mode, the excitons in the two quantum dots can be entangled by only modulating their energy bias $ε$ under the influence of external driving magnetic field. Initially, the two excitons are prepared in a pure separate state. When the time-dependent magnetic field is switched on, a highly entangled state is produced and maintained even in a very long time interval. The mechanism may be used to con…
We present a model of quantum teleportation protocol based on one-dimensional quantum dots system. Three quantum dots with three electrons are used to perform teleportation, the unknown qubit is encoded using one electron spin on quantum dot A, the other two dots B and C are coupled to form a mixed space-spin entangled state. By choosing the Hamiltonian for the mixed space-spin entangled system, we can filter the space (spin) entanglement to obtain pure spin (space) entanglement and after a Bell measurement, the unknown qubit is transfered to quantum dot B. Selecting an appropriate Hamiltonian…
We present a scheme to produce an entangled four-photon state from two pairs of entangled two-photon states. Such entangled four-photon states are equivalent to the quantum state of two maximally entangled spin-1 particles. The scheme can also be generated to prepare an entangled 2N-photon state from N pairs of entangled two-photon states. Such multi-photon states play a crucial role in fundamental tests of quantum mechanics versus local realism and in many quantum information and quantum computation schemes.
We show that the two-photon transition rates of quantum dots coupled to nanocavities are enhanced by up to 8 orders of magnitude relative to quantum dots in bulk host. We then propose how to take advantage of this enhancement to implement coherent quantum dot excitation by two-photon absorption, entangled photon pair generation by two-photon spontaneous emission, and single-photon generation at telecommunication wavelengths by two-photon stimulated and spontaneous emission.
We show how two qubits encoded in the orbital states of two quantum dots can be entangled or disentangled in a controlled way through their interaction with a weak electron current. The transmission/reflection spectrum of each scattered electron, acting as an entanglement mediator between the dots, shows a signature of the dot-dot entangled state. Strikingly, while few scattered carriers produce decoherence of the whole two-dots system, a larger number of electrons injected from one lead with proper energy is able to recover its quantum coherence. Our numerical simulations are based on a real-…
The scalability of quantum dot based non-classical light sources relies on the control over their dissimilar emission energies. Electric fields offer a promising route to tune the quantum dot emission energy through the quantum-confined Stark effect. However, electric fields have been mostly used for tuning the energy of single-photon emission from quantum dots, while electrical control over the energy of entangled-photon emission, which is crucial for building a solid-state quantum repeater using indistinguishable entangled photons, has not been realized yet. Here, we present a method to achi…
A scheme to distinguish entangled two-photon-polarization states (ETP) from two independent entangled one-photon-polarization states (EOP) is proposed. Using this scheme, the experimental generation of ETP by parametric down-conversion is confirmed through the anti-correlations between three orthogonal two-photon-polarization states. The estimated fraction of ETP among the correlated photon pairs is 37% in the present experimental setup.
We predict dominating cooperative two-photon emission from two quantum dots coupled with a single mode photonic crystal cavity. The cooperative two photon emission occurs when excitons in two off-resonantly coupled quantum dots decay simultaneously. The interaction with common cavity field leads to cavity induced two-photon emission which is strongly inhibited by electron phonon coupling. The interaction with common phonon bath produces phonon induced two-photon emission which increases on increasing temperature. For identical quantum dots cavity induced two-photon emission is negligible but p…
Quantum dot spin valves are characterized by exchange fields which induce spin precession and generate current spin resonances even in absence of spin splitting. Analogous effects have been studied in double quantum dots, in which the orbital degree of freedom, the pseudospin, replaces the spin in the valve configuration. We generalize, now, this setup to allow for arbitrary spin and orbital polarization of the leads, thus obtaining an even richer variety of current resonances, stemming from the precession dynamics of entangled spin and pseudospin. We observe for both vectors a delicate interp…
We theoretically study the generation of quantum correlations in a hybrid system composed by two interacting semiconductor quantum dots mediated by a metal nanoparticle and coupled to an external laser field. Interactions present in the hybrid system are treated using a semiclassical approximation except for the direct dipole-dipole interaction. We report the entanglement of formation, which gives information about entanglement quantum correlations, for continuous wave and pulsed driving applied fields. We have found that for proper values of the physical and geometrical parameters of the hybr…
The generation and storage of entangled photons play important roles in quantum information technique. Spontaneous Raman scattering (SRS) in atomic ensembles provides a promising method to generate entangled photons capable of storage. In the past experiments, a spin-wave-photon entangled state is produced via SRS in an atomic ensemble, with which a pair of entangled photons is obtained. Here, we report a scheme of simultaneously generating two spin-wave-photon entangled states in an atomic ensemble by collecting Stokes photons at two different directions. Based on the obtained two atom-photon…
New types of light fields localized in nanometer-sized regions of space were suggested and analyzed. The possibility of using these nanolocalized fields in atom optics for atom focusing and localization is discussed.
Single photon emitters are indispensable to photonic quantum technologies. Here we demonstrate waveform-controlled high-purity single photons from room-temperature colloidal quantum dots. The purity of the single photons does not vary with the excitation power, thereby allowing the generation rate to be increased without compromising the single-photon quality.
We propose a new scheme for solid-state photonic quantum computation in which trapped photons in optical cavities are taken as a quantum bit. Quantum gates can be realized by coupling the cavities with quantum dots through waveguides. The proposed scheme allows programmable and deterministic gate operations and the system can be scaled up to many quantum bits.
We extend entangled coincidence (ghost) imaging to fluorescent samples. Given the entangled photon correlation, one photon of the pair carries information on where the other photon has been absorbed and has produced fluorescence in a sample. Fluorescent molecules serve as ''detectors breaking'' the entanglement.
Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that allows the spectral shaping of entangled photons with high resolution. We evaluate its performances by detecting sum frequency generation in a non-linear crystal. The efficiency of the process is compared when performed with classical or entangled light.
The general concept of entangled photon holes is based on a correlated absence of photon pairs in an otherwise constant optical background. Here we consider the specialized case when this background is confined to two well-defined time bins, which allows the formation of time-bin entangled photon holes. We show that when the typical coherent state background is replaced by a true single-photon (Fock state) background, the basic time-bin entangled photon-hole state becomes equivalent to one of the time-bin entangled photon-pair states. We experimentally demonstrate these ideas using a parametri…
Semiconductor InAs/GaAs quantum dots grown by the Stranski-Krastanov method are among the leading candidates for the deterministic generation of polarization entangled photon pairs. Despite remarkable progress in the last twenty years, many challenges still remain for this material, such as the extremely low yield (<1% quantum dots can emit entangled photons), the low degree of entanglement, and the large wavelength distribution. Here we show that, with an emerging family of GaAs/AlGaAs quantum dots grown by droplet etching and nanohole infilling, it is possible to obtain a large ensemble (clo…
We present a concentration and purification scheme for nonmaximally entangled pure and mixed porization entangled state. We firstly show that two distant parties Alice and Bob first start with two shared but less entangled photon pure states to produce a four photon GHZ state, and then perform a 45 polarization measurement onto one of the two photons at each location such that the remaining two photon are projected onto a maximally entangled state. We further show the scheme also can be used to purify a class of mixed polarization-entangled state.
We report on the generation of time-bin entangled photon pairs from a semiconductor quantum dot via pulsed resonant biexciton generation. Based on theoretical modeling we optimized the duration of the excitation pulse to minimize the laser-induced dephasing and increase the biexciton-to-background single exciton occupation probability. This results in a high degree of entanglement with a concurrence of up to 0.78(6) and a 0.88(3) overlap with a maximally entangled state. Theoretical simulations also indicate a power dependent nature of the dephasing during the laser excitation that limits the …
State-of-the-art quantum key distribution systems are based on the BB84 protocol and single photons generated by lasers. These implementations suffer from range limitations and security loopholes, which require expensive adaptation. The use of polarization entangled photon pairs substantially alleviates the security threads while allowing for basically arbitrary transmission distances when embedded in quantum repeater schemes. Semiconductor quantum dots are capable of emitting highly entangled photon pairs with ultra-low multi-pair emission probability even at maximum brightness. Here we repor…
In addition to photon pairs entangled in polarization or other variables, quantum mechanics also allows optical beams that are entangled through the absence of the photons themselves. These correlated absences, or ``entangled photon holes'', can lead to counter-intuitive nonlocal effects analogous to those of the more familiar entangled photon pairs. Here we report an experimental observation of photon holes generated using quantum interference effects to suppress the probability that two photons in a weak laser pulse will separate at an optical beam splitter.
I show that the photon pairs used in experimental tests of quantum non-locality based on Bell's theorem are not in the entangled quantum state. The correct quantum state of the ``entangled'' photon pairs is suggested. Two experiments for testing this quantum state are proposed.
We show that fractional decay may be observable in experiments using quantum dots and photonic crystals with parameters that are currently achievable. We focus on the case of inverse opal photonic crystals and locate the position in the crystal where the effect is most pronounced. Furthermore, we quantify the influence of absorptive loss and show that it is a limiting but not prohibitive effect.
Semiconductor quantum dots, as promising solid-state platform, have exhibited deterministic photon pair generation with high polarization entanglement f\textcompwordmark idelity for quantum information applications. However, due to temporal correlation from inherently cascaded emission, photon indistinguishability is limited, which restricts their potential scalability to multi-photon experiments. Here, by utilizing quantum interferences to decouple polarization entanglement from temporal correlation, we improve multi-photon entanglement f\textcompwordmark idelity from $(58.7\pm 2.2)\%$ to $(7…
We demonstrate the on-demand emission of polarisation-entangled photon pairs from the biexciton cascade of a single InAs quantum dot embedded in a GaAs/AlAs planar microcavity. Improvements in the sample design blue shifts the wetting layer to reduce the contribution of background light in the measurements. Results presented show that >70% of the detected photon pairs are entangled. The high fidelity of the (|HxxHx>+|VxxVx>)/2^0.5 state that we determine is sufficient to satisfy numerous tests for entanglement. The improved quality of entanglement represents a significant step towards the real…
The quantum interference of entangled photons forms a key phenomenon underlying various quantum-optical technologies. It is known that the quantum interference patterns of entangled photon pairs can be reconstructed classically by the time-reversal method; however, the time-reversal method has been applied only to time-frequency-entangled two-photon systems in previous experiments. Here, for the first time, we apply the time-reversal method to the position-wavevector-entangled two-photon systems: the two-photon Young interferometer and the two-photon beam focusing system. We experimentally dem…
We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single…
An experimental scheme for concentrating entanglement in partially entangled photon pairs is proposed. In this scheme, two separated parties obtain one maximally entangled photon pair from previously shared two partially entangled photon pairs by local operations and classical communication. A practical realization of the proposed scheme is discussed, which uses imperfect photon detectors and spontaneous parametric down-conversion as a photon source. This scheme also works for purifying a class of mixed states.
We present an scheme to generate entangled state between two traveling modes for fixed number of photon, which is based on beam splitter transformation and conditional zero photon counters.
We show that electron recombination using positively charged excitons in single quantum dots provides an efficient method to transfer entanglement from electron spins onto photon polarizations. We propose a scheme for the production of entangled four-photon states of GHZ type. From the GHZ state, two fully entangled photons can be obtained by a measurement of two photons in the linear polarization basis, even for quantum dots with observable fine structure splitting for neutral excitons and significant exciton spin decoherence. Because of the interplay of quantum mechanical selection rules and…
