We report on the preparation and detection of entangled states between an electron spin 1/2 and a nuclear spin 1/2 in a molecular single crystal. These were created by applying pulses at ESR (9.5 GHz) and NMR (28 MHz) frequencies. Entanglement was detected by using a special entanglement detector sequence based on a unitary back transformation including phase rotation.
Recently, there have been significant developments to detect nuclear spins with an nitrogen vacancy (NV) center in diamond. However, due to the nature of the short range dipole-dipole interaction, it takes a long time to detect distant nuclear spins with the NV centers. Here, we propose a rapid detection of nuclear spins with an entanglement between the NV centers. We show that the necessary time to detect the nuclear spins with the entanglement is several orders of magnitude shorter than that with separable NV centers. Our result pave the way for new applications in nanoscale nuclear magnetic…
In this work, we experimentally created and characterized a class of qubit-ququart PPT (positive under partial transpose) entangled states using three nuclear spins on an nuclear magnetic resonance (NMR) quantum information processor. Entanglement detection and characterization for systems with a Hilbert space dimension $\ge 2 \otimes 3$ is nontrivial since there are states in such systems which are both PPT as well as entangled. The experimental detection scheme that we devised for the detection of qubit-ququart PPT entanglement was based on the measurement of three Pauli operators with high …
Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with standard techniques, no more than 8 nuclear spins have been resolved. Here we develop a method that improves significantly the ability to spectrally resolve nuclear spins and demonstrate its capabilities with detailed numerical simulations by using a nitrogen-vacancy (NV) centre as model system. Based on delayed entanglement control, a technique combining m…
We implement an embedding quantum simulator (EQS) in nuclear spin systems. The experiment consists of a simulator of up to three qubits, plus a single ancillary qubit, where we are able to efficiently measure the concurrence and the three-tangle of two-qubit and a three-qubit systems as they undergo entangling dynamics. The EQS framework allows us to drastically reduce the number of measurements needed for this task, which otherwise would require full-state reconstruction of the qubit system. Our simulator is built of the nuclear spins of 4 $^{13}C$ atoms in a molecule of trans-crotonic acid m…
We show that the two notions of entanglement: the maximum of the geometric measure of entanglement and the maximum of the nuclear norm is attained for the same states. We affirm the conjecture of Higuchi-Sudberry on the maximum entangled state of four qubits. We introduce the notion of d-density tensor for mixed d-partite states. We show that d-density tensor is separable if and only if its nuclear norm is $1$. We suggest an alternating method for computing the nuclear norm of tensors. We apply the above results to symmetric tensors. We give many numerical examples.
We obtain a compact analytical solution for the nonlinear equation for the nuclear spin dynamics in the central spin box model in the limit of many nuclear spins. The total nuclear spin component along the external magnetic field is conserved and the two perpendicular components precess or oscillate depending on the electron spin polarization, with the frequency, determined by the nuclear spin polarization. As applications of our solution, we calculate the nuclear spin noise spectrum and describe the effects of nuclear spin squeezing and many body entanglement in the absence of a system excita…
We compute the proton-neutron entanglement entropy in the interacting nuclear shell model for a variety of nuclides and interactions. Some results make intuitive sense, for example that the shell structure, as governed by single-particle and monopole energies, strongly affects the energetically available space and thus the entanglement entropy. We also find a surprising result: that the entanglement entropy at low excitation energy tends to decrease for nuclides when $N \neq Z$. While we provide evidence this arises from the physical nuclear force by contrasting with random two-body interactio…
We propose a solid-state hybrid platform based on an array of implanted nitrogen-vacancy (NV) centers in diamond magnetically coupled to a mechanical oscillator. The mechanical oscillator and the NV electronic spins both act as a quantum bus and allow us to induce an effective long-range interaction between distant nuclear spins, relaxing the requirements on their spatial distance. The coherent nuclear spin-spin interaction, having the form of an Ising model, can be maintained in the presence of mechanical damping and spin dephasing via a pulsed dynamical decoupling of the nuclear spins in add…
Entanglement properties of $^4$He and $^6$He are investigated using nuclear many-body calculations, specifically the single-nucleon entanglement entropy, and the two-nucleon mutual information and negativity. Nuclear wavefunctions are obtained by performing active-space no-core configuration-interaction calculations using a two-body nucleon-nucleon interaction derived from chiral effective field theory. Entanglement measures within single-particle bases, the harmonic oscillator (HO), Hartree-Fock (HF), natural (NAT) and variational natural (VNAT) bases, are found to exhibit different degrees o…
Scalable entanglement of nuclear spins mediated by electron exchange
Massachusetts Institute of Technology（麻省理工学院）；Quantum Machines Inc.（量子机器公司）；Intel Corporation（英特尔公司）；School of Electrical Engineering and Telecommunications, UNSW Sydney（新南威尔士大学电气与电信工程学院）；ARC Centre of Excellence for Quantum Computation and Communication Technology（ARC量子计算与通信技术卓越中心）；NNF Quantum Computing Programme, Niels Bohr Institute, University of Copenhagen（哥本哈根大学尼尔斯·玻尔研究所NNF量子计算项目）；Diraq Pty. Ltd.（Diraq有限公司）；School of Fundamental Science and Technology, Keio University（庆应义塾大学基础科学与技术学院）；School of Physics, University of Melbourne（墨尔本大学物理学院）；School of Science, RMIT University（皇家墨尔本理工大学理学院）
Relying on previous results that link entanglement entropy and parton distribution functions in deep inelastic scattering and focusing on the small Bjorken scaling region we present here indications that gluon shadowing might indeed be explained as due to a depletion of the entanglement entropy between observed and unobserved degrees of freedom per nucleon within a nucleus with respect to the free nucleon case. We apply to gluon shadowing the general Page approach to the calculation of the entanglement entropy in bipartite systems, giving physical motivations of the results.
Nuclear spins of noble-gas atoms are exceptionally isolated from the environment and can maintain their quantum properties for hours at room temperature. Here we develop a mechanism for entangling two such distant macroscopic ensembles by using coherent light input. The interaction between the light and the noble-gas spins in each ensemble is mediated by spin-exchange collisions with alkali-metal spins, which are only virtually excited. The relevant conditions for experimental realizations with ^{3}\text{He} or ^{129}\text{Xe} are outlined.
The role of electron-nuclear entanglement on the validity of the Born-Oppenheimer (BO) approximation is investigated. While nonadiabatic couplings generally lead to entanglement and to a failure of the BO approximation, surprisingly the degree of electron-nuclear entanglement is found to be uncorrelated with the degree of validity of the BO approximation. This is because while the degree of entanglement of BO states is determined by their deviation from the corresponding states in the crude BO approximation, the accuracy of the BO approximation is dictated, instead, by the deviation of the BO …
We experimentally demonstrate room-temperature storage of quantum entanglement using two nuclear spins weakly coupled to the electronic spin carried by a single nitrogen-vacancy center in diamond. We realize universal quantum gate control over the three-qubit spin system and produce entangled states encoded within the decoherence-free subspace of the two nuclear spins. By injecting arbitrary collective noise, we demonstrate that the decoherence-free entangled state has coherence time longer than that of other entangled states by an order of magnitude in our experiment.
The potential impact of future quantum networks hinges on high-quality quantum entanglement shared between network nodes. Unavoidable real-world imperfections necessitate means to improve remote entanglement by local quantum operations. Here we realize entanglement distillation on a quantum network primitive of distant electron-nuclear two-qubit nodes. We demonstrate the heralded generation of two copies of a remote entangled state through single-photon-mediated entangling of the electrons and robust storage in the nuclear spins. After applying local two-qubit gates, single-shot measurements h…
We consider the problem of correct measurement of a quantum entanglement in the two-body electron-electron scattering. An expression is derived for a spin correlation tensor of a pure two-electron state. A geometrical measure of a quantum entanglement as the distance between two forms of this tensor in entangled and separable cases is presented. We prove that this measure satisfies properties of a valid entanglement measure: nonnegativity, discriminance, normalization, non-growth under local operations and classical communication. This measure is calculated for a problem of electron-electron s…
Treating Coulomb scattering of two free electrons in a stationary approach, we explore the momentum and spin entanglement created by the interaction. We show that a particular discretisation provides an estimate of the von Neumann entropy of the one-electron reduced density matrix from the experimentally accessible Shannon entropy. For spinless distinguishable electrons the entropy is sizeable at low energies, indicating strong momentum entanglement, and drops to almost zero at energies of the order of 10 keV when the azimutal degree of freedom is integrated out, i.e. practically no entangleme…
Inspired by recent developments in the control and manipulation of quantum dot nuclear spins, which allow for the transfer of an electron spin state to the surrounding nuclear-spin ensemble for storage, we propose a quantum repeater scheme that combines individual quantum dot electron spins and nuclear-spin ensembles, which serve as spin-photon interfaces and quantum memories respectively. We consider the use of low-strain quantum dots embedded in high-cooperativity optical microcavities. Quantum dot nuclear-spin ensembles allow for the long-term storage of entangled states, and heralded entan…
A promising approach for multi-qubit quantum registers is to use optically addressable spins to control multiple dark electron-spin defects in the environment. While recent experiments have observed signatures of coherent interactions with such dark spins, it is an open challenge to realize the individual control required for quantum information processing. Here we demonstrate the initialisation, control and entanglement of individual dark spins associated to multiple P1 centers, which are part of a spin bath surrounding a nitrogen-vacancy center in diamond. We realize projective measurements …
